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A. Alvermann

Publications and source records attributed to A. Alvermann.

At least 19 recordsLinked to original sources

Efficient computation of the $W_3$ topological invariant and application to Floquet-Bloch systems

We introduce an efficient algorithm for the computation of the $W_3$ invariant of general unitary maps, which converges rapidly even on coarse discretization grids. The algorithm does not require extensive manipulation of the unitary maps, identification of the precise positions of degeneracy points, or fixing the gauge of eigenvectors. After construction of the general algorithm, we explain its application to the $2+1$ dimensional maps that arise in the Floquet-Bloch theory of periodically driven two-dimensional quantum systems. We demonstrate this application by computing the $W_3$ invariant for an irradiated graphene model with a continuously modulated Hamilton operator, where it predicts the number of anomalous edge states in each gap.

quant-ph

Dynamic Stark effect, light emission, and entanglement generation in a laser-driven quantum optical system

We calculate the emission spectra, the Glauber $g^{(2)}$ function, and the entanglement of formation for a few two-level emitters coupled to a single cavity mode and subject to an external laser-excitation. To evaluate these quantities we couple the system to environmental degrees of freedom which leads to dissipative dynamics. Because of the periodic time-dependence of the system Hamiltonian, the coefficients of the (Markovian) master equation are constant if Floquet states are used as the computational basis. Studying the emission spectra we show that the dynamic Stark effect, i.e., the shift of spectral lines, first appears in the second order of the laser intensity. For the Glauber function, we find clearly distinguished parameter regimes of super- and sub-Poissonian light emission and explain the additional features appearing for finite laser intensity in terms of the quasienergy spectrum of the driven emitter-cavity system. Finally, we analyze the temperature and emitter-cavity coupling regimes where entanglement among the emitters is generated, and show that the laser-excitation leads to a decrease of entanglement.

quant-ph

Symmetry-breaking oscillations in membrane optomechanics

We study the classical dynamics of a membrane inside a cavity in the situation where this optomechanical system possesses a reflection symmetry. Symmetry breaking occurs through supercritical and subcritical pitchfork bifurcations of the static fixed point solutions. Both bifurcations can be observed through variation of the laser-cavity detuning, which gives rise to a boomerang-like fixed point pattern with hysteresis. The symmetry-breaking fixed points evolve into self-sustained oscillations when the laser intensity is increased. In addition to the analysis of the accompanying Hopf bifurcations we describe these oscillations at finite amplitudes with an ansatz that fully accounts for the frequency shift relative to the natural membrane frequency. We complete our study by following the route to chaos for the membrane dynamics.

quant-ph

Optomechanical multistability in the quantum regime

Classical optomechanical systems feature self-sustained oscillations, where multiple periodic orbits at different amplitudes coexist. We study how this multistability is realized in the quantum regime, where new dynamical patterns appear because quantum trajectories can move between different classical orbits. We explain the resulting quantum dynamics from the phase space point of view, and provide a quantitative description in terms of autocorrelation functions. In this way we can identify clear dynamical signatures of the crossover from classical to quantum mechanics in experimentally accessible quantities. Finally, we discuss a possible interpretation of our results in the sense that quantum mechanics protects optomechanical systems against the chaotic dynamics realized in the classical limit.

quant-ph

Nonclassical light from few emitters in a cavity

We study the characteristics of the light generated by few emitters in a cavity at strong light-matter coupling. By means of the Glauber $g^{(2)}$-function we can identify clearly distinguished parameter regimes with super-Poissonian and sub-Poissonian photon statistics. We establish a relation between the emission characteristics for one and multiple emitters, and explain its origin in terms of the photon-dressed emitter states. Cooperative effects lead to the generation of nonclassical light already at reduced light-matter coupling if the number of emitters is increased. Our results are obtained with a full input-output formalism and master equation valid also at strong light-matter coupling. We compare the behavior obtained with and without counter-rotating light-matter interaction terms in the Hamiltonian, and find that the generation of nonclassical light is robust against such modifications. Finally, we contrast our findings with the predictions of the quantum optical master equation and find that it fails entirely at predicting regimes with different photon statistics.

quant-ph

Route to chaos in optomechanics

We establish the emergence of chaotic motion in optomechanical systems. Chaos appears at negative detuning for experimentally accessible values of the pump power and other system parameters. We describe the sequence of period doubling bifurcations that leads to chaos, and state the experimentally observable signatures in the optical spectrum. In addition to the semi-classical dynamics we analyze the possibility of chaotic motion in the quantum regime. We find that quantum mechanics protects the optomechanical system against irregular dynamics, such that simple periodic orbits reappear and replace the classically chaotic motion. In this way observation of the dynamical signatures makes it possible to pin down the crossover from quantum to classical mechanics.

quant-ph

Dynamics of the Dicke model close to the classical limit

We study the dynamical properties of the Dicke model for increasing spin length, as the system approaches the limit of a classical spin. First, we describe the emergence of collective excitations above the groundstate that converge to the coupled spin-oscillator oscillations found in the classical limit. The corresponding Green functions reveal quantum dynamical signatures close to the superradiant quantum phase transition. Second, we identify signatures of classical quasi-periodic orbits in the quantum time evolution using numerical time-propagation of the wave function. The resulting phase space plots are compared to the classical trajectories. We complete our study with the analysis of individual eigenstates close to the quasi-periodic orbits.

quant-ph

Nonequilibrium quantum fluctuation relations for harmonic systems in nonthermal environments

We formulate exact generalized nonequilibrium fluctuation relations for the quantum mechanical harmonic oscillator coupled to multiple harmonic baths. Each of the different baths is prepared in its own individual (in general nonthermal) state. Starting from the exact solution for the oscillator dynamics we study fluctuations of the oscillator position as well as of the energy current through the oscillator under general nonequilibrium conditions. In particular, we formulate a fluctuation-dissipation relation for the oscillator position autocorrelation function that generalizes the standard result for the case of a single bath at thermal equilibrium. Moreover, we show that the generating function for the position operator fullfills a generalized Gallavotti-Cohen-like relation. For the energy transfer through the oscillator, we determine the average energy current together with the current fluctuations. Finally, we discuss the generalization of the cumulant generating function for the energy transfer to nonthermal bath preparations.

quant-ph

Equilibration and thermalization of the dissipative quantum harmonic oscillator in a non-thermal environment

We study the dissipative quantum harmonic oscillator with general non-thermal preparations of the harmonic oscillator bath. The focus is on equilibration of the oscillator in the long-time limit and the additional requirements for thermalization. Our study is based on the exact solution of the microscopic model obtained by means of operator equations of motion, which provides us with the time evolution of the central oscillator density matrix in terms of the propagating function. We find a hierarchy of conditions for thermalization, together with the relation of the asymptotic temperature to the energy distribution in the initial bath state. We discuss the presence and absence of equilibration for the example of an inhomogeneous chain of harmonic oscillators, and illustrate the general findings about thermalization for the non-thermal environment that results from a quench.

quant-ph

Numerical time propagation of quantum systems in radiation fields

Atoms, molecules or excitonic quasiparticles, for which excitations are induced by external radiation fields and energy is dissipated through radiative decay, are examples of driven open quantum systems. We explain the use of commutator-free exponential time-propagators for the numerical solution of the associated Schrödinger or master equations with a time-dependent Hamilton operator. These time-propagators are based on the Magnus series but avoid the computation of commutators, which makes them suitable for the efficient propagation of systems with a large number of degrees of freedom. We present an optimized fourth order propagator and demonstrate its efficiency in comparison to the direct Runge-Kutta computation. As an illustrative example we consider the parametrically driven dissipative Dicke model, for which we calculate the periodic steady state and the optical emission spectrum.

quant-ph

Quantum phase transition in the Dicke model with critical and non-critical entanglement

We study the quantum phase transition of the Dicke model in the classical oscillator limit, where it occurs already for finite spin length. In contrast to the classical spin limit, for which spin-oscillator entanglement diverges at the transition, entanglement in the classical oscillator limit remains small. We derive the quantum phase transition with identical critical behavior in the two classical limits and explain the differences with respect to quantum fluctuations around the mean-field ground state through an effective model for the oscillator degrees of freedom. With numerical data for the full quantum model we study convergence to the classical limits. We contrast the classical oscillator limit with the dual limit of a high frequency oscillator, where the spin degrees of freedom are described by the Lipkin-Meshkov-Glick model. An alternative limit can be defined for the Rabi case of spin length one-half, in which spin frequency renormalization replaces the quantum phase transition.

quant-ph

Collapse-revival dynamics and atom-field entanglement in the non-resonant Dicke model

We consider the dynamics of atomic and field coherent states in the non-resonant Dicke model. At weak coupling an initial product state evolves into a superposition of multiple field coherent states that are correlated with the atomic configuration. This process is accompanied by the buildup and decay of atom-field entanglement and leads to the periodic collapse and revival of Rabi oscillations. We provide a perturbative derivation of the underlying dynamical mechanism that complements the rotating wave approximation at resonance. The identification of two different time scales explains how the dynamical signatures depend on the sign of detuning between the atomic and field frequency, and predicts the generation of either atomic or field cat states in the two opposite cases. We finally discuss the restrictions that the buildup of atom-field entanglement during the collapse of Rabi oscillations imposes on the validity of semi-classical approximations that neglect entanglement.

quant-ph

Non-equilibrium transport through molecular junctions in the quantum regime

We consider a quantum dot, affected by a local vibrational mode and contacted to macroscopic leads, in the non-equilibrium steady-state regime. We apply a variational Lang-Firsov transformation and solve the equations of motion of the Green functions in the Kadanoff-Baym formalism up to second order in the interaction coefficients. The variational determination of the transformation parameter through minimization of the thermodynamic potential allows us to calculate the electron/polaron spectral function and conductance for adiabatic to anti-adiabatic phonon frequencies and weak to strong electron-phonon couplings. We investigate the qualitative impact of the quasi-particle renormalization on the inelastic electron tunneling spectroscopy signatures and discuss the possibility of a polaron induced negative differential conductance. In the high-voltage regime we find that the polaron level follows the lead chemical potential to enhance resonant transport.

cond-mat.str-el

Variational discrete variable representation for excitons on a lattice

We construct numerical basis function sets on a lattice, whose spatial extension is scalable from single lattice sites to the continuum limit. They allow us to compute small and large bound states with comparable, moderate effort. Adopting concepts of discrete variable representations, a diagonal form of the potential term is achieved through a unitary transformation to Gaussian quadrature points. Thereby the computational effort in three dimensions scales as the fourth instead of the sixth power of the number of basis functions along each axis, such that it is reduced by two orders of magnitude in realistic examples. As an improvement over standard discrete variable representations, our construction preserves the variational principle. It allows for the calculation of binding energies, wave functions, and excitation spectra. We use this technique to study central-cell corrections for excitons beyond the continuum approximation. A discussion of the mass and spectrum of the yellow exciton series in the cuprous oxide, which does not follow the hydrogenic Rydberg series of Mott-Wannier excitons, is given on the basis of a simple lattice model.

cond-mat.other

High-order commutator-free exponential time-propagation of driven quantum systems

We discuss the numerical solution of the Schr\"odinger equation with a time-dependent Hamilton operator using commutator-free time-propagators. These propagators are constructed as products of exponentials of simple weighted sums of the Hamilton operator. Owing to their exponential form they strictly preserve the unitarity of time-propagation. The absence of commutators or other computationally involved operations allows for straightforward implementation and application also to large scale and sparse matrix problems. We explain the derivation of commutator-free exponential time-propagators in the context of the Magnus expansion, and provide optimized propagators up to order eight. An extensive theoretical error analysis is presented together with practical efficiency tests for different problems. Issues of practical implementation, in particular the use of the Krylov technique for the calculation of exponentials, are discussed. We demonstrate for two advanced examples, the hydrogen atom in an electric field and pumped systems of multiple interacting two-level systems or spins that this approach enables fast and accurate computations.

math.NA

Transport through a vibrating quantum dot: Polaronic effects

We present a Green's function based treatment of the effects of electron-phonon coupling on transport through a molecular quantum dot in the quantum limit. Thereby we combine an incomplete variational Lang-Firsov approach with a perturbative calculation of the electron-phonon self energy in the framework of generalised Matsubara Green functions and a Landauer-type transport description. Calculating the ground-state energy, the dot single-particle spectral function and the linear conductance at finite carrier density, we study the low-temperature transport properties of the vibrating quantum dot sandwiched between metallic leads in the whole electron-phonon coupling strength regime. We discuss corrections to the concept of an anti-adiabatic dot polaron and show how a deformable quantum dot can act as a molecular switch.

cond-mat.mes-hall

Non-equilibrium current and electron pumping in nanostructures

We discuss a numerical method to study electron transport in mesoscopic devices out of equilibrium. The method is based on the solution of operator equations of motion, using efficient Chebyshev time propagation techniques. Its peculiar feature is the propagation of operators backwards in time. In this way the resource consumption scales linearly with the number of states used to represent the system. This allows us to calculate the current for non-interacting electrons in large one-, two- and three-dimensional lead-device configurations with time-dependent voltages or potentials. We discuss the technical aspects of the method and present results for an electron pump device and a disordered system, where we find transient behaviour that exists for a very long time and may be accessible to experiments.

cond-mat.mes-hall

Sparse polynomial space approach to dissipative quantum systems: Application to the sub-ohmic spin-boson model

We propose a general numerical approach to open quantum systems with a coupling to bath degrees of freedom. The technique combines the methodology of polynomial expansions of spectral functions with the sparse grid concept from interpolation theory. Thereby we construct a Hilbert space of moderate dimension to represent the bath degrees of freedom, which allows us to perform highly accurate and efficient calculations of static, spectral and dynamic quantities using standard exact diagonalization algorithms. The strength of the approach is demonstrated for the phase transition, critical behaviour, and dissipative spin dynamics in the spin boson model

cond-mat.stat-mech