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A. Amato

Publications and source records attributed to A. Amato.

At least 253 records · Page 14Linked to original sources

Surface and Bulk Electronic Structure of the Strongly Correlated System SmB$_{6}$ and Implications for a Topological Kondo Insulator

Recent theoretical calculations and experimental results suggest that the strongly correlated material SmB$_{6}$ may be a realization of a topological Kondo insulator. We have performed an angle-resolved photoemission spectroscopy study on SmB$_{6}$ in order to elucidate elements of the electronic structure relevant to the possible occurrence of a topological Kondo insulator state. The obtained electronic structure in the whole three-dimensional momentum space reveals one electron-like 5d bulk band centred at the X point of the bulk Brillouin zone that is hybridized with strongly correlated f electrons, as well as the opening of a Kondo bandgap ($Δ_B$ $\sim$ 20 meV) at low temperature. In addition, we observe electron-like bands forming three Fermi surfaces at the center $\barΓ$ point and boundary $\bar{X}$ point of the surface Brillouin zone. These bands are not expected from calculations of the bulk electronic structure, and their observed dispersion characteristics are consistent with surface states. Our results suggest that the unusual low-temperature transport behavior of SmB$_{6}$ is likely to be related to the pronounced surface states sitting inside the band hybridisation gap and/or the presence of a topological Kondo insulating state.

cond-mat.str-el↗

Evidence for Time-Reversal-Symmetry-Broken Superconductivity in Locally Noncentrosymmetric SrPtAs

We report the magnetic and superconducting properties of locally noncentrosymmetric SrPtAs obtained by muon-spin-rotation/relaxation (muSR) measurements. Zero-field muSR reveals the occurrence of small spontaneous static magnetic fields with the onset of superconductivity. This finding suggests that the superconducting state of SrPtAs breaks time-reversal symmetry. The superfluid density as determined by transverse field muSR is nearly flat approaching T = 0 K proving the absence of extended nodes in the gap function. By symmetry, several superconducting states supporting time-reversal symmetry breaking in SrPtAs are allowed. Out of these, a dominantly d + id (chiral d-wave) order parameter is most consistent with our experimental data.

cond-mat.supr-con↗

Superconducting parameters of BaPt(4-x)Au(x)Ge12 filled skutterudite

We report on a study of the superconducting properties for a series of polycrystalline BaPt(4-x)Au(x)Ge12 filled skutterudite compounds for x = 0, 0.5, 0.75, and 1. Muon spin rotation (muSR) spectroscopy as well as magnetization, specific heat, and electrical resistivity measurements were performed. The magnetic penetration depth λ, the coherence length ξ, and the Ginzburg-Landau parameter κare evaluated. The temperature dependence of the superfluid density is well described by an s-wave superconducting gap and this classical scenario is supported by the field-independent λ. The gap-to-Tc ratio Δ/kTc increases with the Au content from 1.70 for x = 0 to 2.1(1) for x = 1. By combining muSR, magnetization, and specific heat data, we find that BaPt(4-x)Au(x)Ge12 compounds are in between the dirty and clean limits with mean free paths of the carriers l ~ ξ. Interestingly, resistivity data for BaPt4Ge12 indicate a much higher upper critical field, which is probably due to defects or impurities close to the surface of the crystallites.

cond-mat.supr-con↗

Structural and magnetic phase transitions in triclinic Ca10(FeAs)10(Pt3As8)

We report the structural and magnetic phase transitions of triclinic Ca10(FeAs)10(Pt3As8). High-resolution X-ray powder diffraction reveals splitting of the in-plane (a,b) lattice parameters at Ts ~ 120 K. Platinum-doping weakens the distortion and shifts the transition temperature to 80 K in Ca10(Fe1-xPt_xAs)10(Pt3As8) with x = 0.03. muSR experiments show the onset of magnetic order near Ts and a broad magnetic phase transition. No symmetry breaking is associated to the structural transition in Ca10(FeAs)10(Pt3As8) in contrast to the other parent compounds of iron arsenide superconductors.

cond-mat.supr-con↗

Superconductivity and magnetism in RbxFe2-ySe2: Impact of thermal treatment on mesoscopic phase separation

An extended study of the superconducting and normal-state properties of various as-grown and post-annealed RbxFe2-ySe2 single crystals is presented. Magnetization experiments evidence that annealing of RbxFe2-ySe2 at 413 K, well below the onset of phase separation Tp=489 K, neither changes the magnetic nor the superconducting properties of the crystals. In addition, annealing at 563 K, well above Tp, suppresses the superconducting transition temperature Tc and leads to an increase of the antiferromagnetic susceptibility accompanied by the creation of ferromagnetic impurity phases, which are developing with annealing time. However, annealing at T=488K=Tp increases Tc up to 33.3 K, sharpens the superconducting transition, increases the lower critical field, and strengthens the screening efficiency of the applied magnetic field. Resistivity measurements of the as-grown and optimally annealed samples reveal an increase of the upper critical field along both crystallographic directions as well as its anisotropy. Muon spin rotation and scanning transmission electron microscopy experiments suggest the coexistence of two phases below Tp: a magnetic majority phase of Rb2Fe4Se5 and a non-magnetic minority phase of Rb0.5Fe2Se2. Both microscopic techniques indicate that annealing the specimens just at Tp does not affect the volume fraction of the two phases, although the magnetic field distribution in the samples changes substantially. This suggests that the microstructure of the sample, caused by mesoscopic phase separation, is modified by annealing just at Tp, leading to an improvement of the superconducting properties of RbxFe2-ySe2 and an enhancement of Tc.

cond-mat.supr-con↗

Quantum Tunneling in Half-Integer-Spin Kagome-Lattice Langasites

Employing the muon spin relaxation technique we evidence temperature independent magnetic fluctuations persisting down to the lowest temperatures in the samarium-based ($J=5/2$) kagome-lattice Langasite. A detailed bulk-magnetization characterization and comparison to the neodymium-based ($J=9/2$) compound allow us to assign the persistent spin dynamics to a quantum tunneling process. This is facilitated by pairwise anisotropic magnetic interactions, leading to a universal scaling of the muon relaxation. Our study reveals a remarkable analogy between weakly interacting half-integer-spin rare-earth magnets and molecular nanomagnets.

cond-mat.str-el↗

Avoided ferromagnetic quantum critical point: Unusual short-range ordered state in CeFePO

Cerium 4f electronic spin dynamics in single crystals of the heavy-fermion system CeFePO is studied by means of ac-susceptibility, specific heat and muon-spin relaxation ($μ$SR). Short-range static magnetism occurs below the freezing temperature Tg ~ 0.7 K, which prevents the system from accessing the putative ferromagnetic quantum critical point. In the $μ$SR, the sample-averaged muon asymmetry function is dominated by strongly inhomogeneous spin fluctuations below 10 K and exhibits a characteristic time-field scaling relation expected from glassy spin dynamics, strongly evidencing cooperative and critical spin fluctuations. The overall behavior can be ascribed neither to canonical spin glasses nor other disorder-driven mechanisms.

cond-mat.str-el↗

Superfluid density and superconducting gaps of RbFe_{2}As_{2} as a function of hydrostatic pressure

The superfluid density and superconducting gaps of superconducting RbFe_{2}As_{2} have been determined as a function of temperature, magnetic field and hydrostatic pressure by susceptibility and muon-spin spectroscopy measurements. From the data, fundamental microscopic parameters of the superconducting state like the London penetration depth λ, the gap values Δ, the upper critical field B_{c2}, and the Ginzburg-Landau parameter κhave been obtained. In accordance with earlier measurements the ratio of the superfluid density n_{s} \propto λ^{-2} to the superconducting transition temperature T_{c}=2.52(2) K at ambient pressure is found to be much larger in the strongly hole-overdoped RbFe_{2}As_2 than in high-T_{c} Fe-based and other unconventional superconductors. As a function of pressure T_{c} strongly decreases with a rate of dT_{c}/dp = -1.32 K/GPa, i.e. it is reduced by 52 % at p = 1 GPa. The temperature dependence of n_{s} is best described by a two gap s-wave model with both superconducting gaps being decreased by hydrostatic pressure until smaller gap completely disappears at p = 1 GPa.

cond-mat.supr-con↗

Magnetic phase separation and superfluid density measurements in alkali metal-organic solvent intercalated iron selenide superconductor Lix(C5H5N)yFe2-zSe2

We report the low-temperature electronic and magnetic properties of the alkali metal-organic solvent intercalated iron selenide superconductor Lix(C5H5N)yFe2-zSe using muon-spin-spectroscopy measurements. The zero-field \muSR results indicate that nearly half of the sample is magnetically ordered and there is a spatial phase separation between the superconducting and the magnetic fraction. The transverse-field \muSR results show that the temperature dependence of the penetration depth λ(T) in the mixed state of Lix(C5H5N)yFe2-zSe can be explained using a two-gap s+s-wave model with gap values of 6.82(92) and 0.93(7) meV. This implies that the symmetry of the superconducting gap in this system remains unaltered to the parent compound FeSe even after the intercalation with the molecular spacer layer. We obtain λ(0) = 485(21) nm at T = 0 K.

cond-mat.supr-con↗

Kapellasite: a kagome quantum spin liquid

Magnetic susceptibility, NMR, muSR, and inelastic neutron scattering measurements show that kapellasite, Cu3Zn(OH)6Cl2, a geometrically frustrated spin-1/2 kagome antiferromagnet polymorphous with the herbertsmithite mineral, is a gapless spin liquid with frustrated interactions showing unusual dynamic short-range correlations of non-coplanar cuboc2 type which persist down to 20 mK. The Hamiltonian is determined from a fit of a high-temperature series expansion to thermodynamical data. The experimental data are compared to theoretical calculations using the Schwinger-boson approach.

cond-mat.str-el↗

Evolution of spin relaxation processes in LiY$_{1-x}$Ho$_x$F$_4$ with increasing x studied via AC-susceptibility and muon spin relaxation

We present measurements of magnetic field and frequency dependences of the low temperature (T = 1.8 K) AC-susceptibility, and temperature and field dependences of the longitudinal field positive muon spin relaxation (μSR) for LiY$_{1-x}$Ho$_x$F$_4$ with x = 0.0017, 0.0085, 0.0408, and 0.0855. The fits of numerical simulations to the susceptibility data for the x = 0.0017, 0.0085 and 0.0408 show that Ho-Ho cross-relaxation processes become more important at higher concentrations, signaling the crossover from single-ion to correlated behavior. We simulate the muon spin depolarization using the parameters extracted from the susceptibility, and the simulations agree well with our data for samples with x = 0.0017 and 0.0085. The μSR data for samples with x = 0.0408 and 0.0855 at low temperatures (T < 10 K) cannot be described within a single-ion picture of magnetic field fluctuations and give evidence for additional mechanisms of depolarization due to Ho$^{3+}$ correlations. We also observe an unusual peak in the magnetic field dependence of the muon relaxation rate in the temperature interval 10 - 20 K that we ascribe to a modification of the Ho$^{3+}$ fluctuation rate due to a field induced shift of the energy gap between the ground and the first excited doublet crystal field states relative to a peak in the phonon density of states centered near 63 cm$^{-1}$.

cond-mat.str-el↗

The 10 Tesla muSR instrument: detector solutions

Solutions to the detector system of the High-Field muSR instrument at the Paul Scherrer Institut (PSI) in Switzerland are presented. The strict technical requirements are fulfilled through the application of Geiger-mode Avalanche Photodiodes.

physics.ins-det↗

Evidence for an exotic magnetic transition in the triangular spin system FeGa2S4

We report positive muon spin relaxation measurements on the triangular lattice magnetic system FeGa2S4. A magnetic transition not previously detected by specific heat and magnetic susceptibility measurements is found in zero field at T^* \simeq 30 K. It is observed through the temperature dependencies of the signal amplitude and the spin-lattice relaxation rate. This transition is therefore not a conventional magnetic phase transition. Since persistent spin dynamics is observed down to 0.1 K, the ground state cannot be of the canonical spin-glass type, which could be suggested from hysteresis effects in the bulk susceptibility below T_f \simeq 16 K. These results are compared to those found for the isomorph NiGa2S4. It is argued that the fate of the transition, which has been interpreted in terms of the Z_2 topological transition in this latter system, is probably different in FeGa2S4.

cond-mat.str-el↗

"Cigar" Fermi surface as a possible requisite for superconductivity in iron-based superconductors

Recently discovered A-Fe-Se (A - alkali metal) materials have questioned the most popular theories of iron-based superconductors because of their unusual electronic structure [1]. Controversial photoemission data taken in the superconducting state [2-7] are in conflict with highly magnetic state seen by neutron-, muSR-spectroscopies and transport/thermodynamic probes [8-10]. These results lead to suggestions to consider all iron-based materials as originating from Mott-insulators or semiconductors, thus once again raising the question of close relation between the cuprates and Fe-based superconductors [e.g. 2]. Here we study electronic and magnetic properties of Rb0.77Fe1.61Se2 (Tc = 32.6 K) in normal and superconducting states by means of photoemission and muSR spectroscopies as well as band structure calculations. We demonstrate that the puzzling behavior of these novel materials is the result of separation into metallic (~12%) and insulating (~ 88%) phases. Only the former becomes superconducting and has a usual electronic structure of electron-doped FeSe-slabs. Our results thus imply that the antiferromagnetic insulating phase is just a byproduct of Rb-intercalation and its magnetic properties have hardly any relation to the superconductivity. Instead, we find that also in this, already third class of iron-based compounds, the key ingredient for superconductivity is a certain proximity of a van Hove singularity to the Fermi level. These findings set the direction for effective search of new superconducting materials.

cond-mat.supr-con↗

Magnetic Order in the Pyrochlore Iridates A2Ir2O7 (A = Y, Yb)

We present results from muon spin relaxation/rotation, magnetization, neutron scattering and transport measurements on polycrystalline samples of the pyrochlore iridates Y2Ir2O7 (Y-227) and Yb2Ir2O7 (Yb-227). Well-defined spontaneous oscillations of the muon asymmetry are observed together with hysteretic behavior in magnetization below 130 K in Yb-227, indicative of commensurate long-range magnetic order. Similar oscillations are observed in Y-227 below 150 K; however the onset of hysteretic magnetization at T = 190 K indicates a transition to an intermediate state lacking long-range order as observed in Nd-227. Our results also show that insulating members of the iridate family have nearly identical magnetic ground states, and that the presence of magnetic A-site species does not play any significant role in altering the ground state properties.

cond-mat.str-el↗

Superconducting properties of single-crystalline A_{x}Fe_{2-y}Se_{2} (A=Rb, K) studied using muon spin spectroscopy

We report on the superconducting properties of A_{x}Fe_{2-y}Se_{2} (A = Rb, K) single crystals studied with the muon spin relaxation or rotation (\muSR) technique. At low temperatures, close to 90% of the sample volumes exhibit large-moment magnetic order which impedes the investigation of their superconducting properties by \muSR. On the other hand, about 10% of the sample volumes remain paramagnetic and clearly show a superconducting response. The temperature dependence of the superconducting carrier density was analyzed within the framework of a single s-wave gap scenario. The zero-temperature values of the in-plane magnetic penetration depths λ_{ab}(0) = 258(2) and 225(2) nm and the superconducting gaps Δ(0) = 7.7(2) and 6.3(2) meV have been determined for A = Rb and K, respectively. The microscopic coexistence and/or phase separation of superconductivity and magnetism is discussed.

cond-mat.supr-con↗

Magnetic order and the electronic ground state in the pyrochlore iridate Nd2Ir2O7

We report a combined muon spin relaxation/rotation, bulk magnetization, neutron scattering, and transport study of the electronic properties of the pyrochlore iridate Nd2Ir2O7. We observe the onset of strongly hysteretic behavior in the temperature dependent magnetization below 120 K, and an abrupt increase in the temperature dependent resistivity below 8 K. Zero field muon spin relaxation measurements show that the hysteretic magnetization is driven by a transition to a magnetically disordered state, and that below 8 K a complex magnetically ordered ground state sets in, as evidenced by the onset of heavily damped spontaneous muon precession. Our measurements point toward the absence of a true metal-to-insulator phase transition in this material and suggest that Nd2Ir2O7 lies either within or on the metallic side of the boundary of the Dirac semimetal regime within its topological phase diagram.

cond-mat.str-el↗

Muon diffusion in diluted paramagnetic systems

Muon Spin Rotation/Relaxation (μSR) is a powerful probe to study diffusion of hydrogen-like particles. One of the most common model to analyze μSR signals from materials where diffusion occurs, is by using functions derived from the stochastic theory of Kubo and Toyabe along with the strong collision model. Unfortunately the current formalism can not be used to analyze data from systems where not only muons diffuse, but also the magnetic moments of the material are dynamic. In this article we introduce a new model which accounts for both dynamical effects, and use this model to analyze μSR signals from Dy0.4Y1.6Ti2O7.

cond-mat.dis-nn↗