arXiv subjects

A. Arsenault

Publications and source records attributed to A. Arsenault.

6 recordsLinked to original sources

arXiv2022

$^{139}$La NMR investigation of the interplay between the lattice, charge, and spin dynamics in charge ordered high $T_c$ cuprate La$_{1.875}$Ba$_{0.125}$CuO$_{4}$

We investigate the interplay between the lattice, charge, and spin dynamics in charge ordered high $T_c$ cuprate La$_{1.875}$Ba$_{0.125}$CuO$_{4}$ ($T_{c} =4$~K) based on the inverse Laplace transform (ILT) analysis of the $^{139}$La nuclear spin-lattice relaxation rate $1/T_1$ (dubbed ILTT$_{1}$ analysis here after). A major thrust of the ILTT$_{1}$ analysis is that one can deduce the probability density function $P(1/T_1)$ of distributed $1/T_1$. We demonstrate that $1/T_{1}^{lm}$, defined as the log-mean (i.e. the center of gravity on a logarithmic scale) of $P(1/T_1)$, can be well approximated by $1/T_{1}^{str}$ deduced from the phenomenological stretched fit, however, $P(1/T_1)$ can provide much richer insight into how the lattice, charge, and spin fluctuations and their distribution develop near and below the long range charge order at $T_{charge} \sim 54$~K. Upon entering the charge ordered state, a divergent increase of $1/T_{1}^{lm}$ toward the spin ordering at $T_{spin}^{μSR} \simeq 35$~K is accompanied by an asymmetric broadening of $P(1/T_1)$. Even deep inside the charge ordered state, $1/T_{1}$ at a gradually diminishing fraction of $^{139}$La sites continues to slow down as temperature is lowered, as expected for canonical superconducting CuO$_2$ planes without enhanced spin fluctuations. The fraction of such canonical $^{139}$La sites almost disappears by $\simeq 40$~K. In contrast, nearly a half of the $^{139}$La sites in La$_{1.885}$Sr$_{0.115}$CuO$_{4}$ ($T_{charge} \simeq 80$~K) still exhibits the canonical behavior without enhanced spin fluctuations even near its $T_{c} = 31$~K. These contrasting behaviors explain why superconductivity in La$_{1.875}$Ba$_{0.125}$CuO$_{4}$ is more strongly suppressed than in La$_{1.885}$Sr$_{0.115}$CuO$_{4}$ despite the lower onset temperature of the charge order.

cond-mat.str-el↗

arXiv2022

Revisiting the $^{63}$Cu NMR signature of charge order in La$_{1.875}$Ba$_{0.125}$CuO$_{4}$

We use single crystal $^{63}$Cu NMR techniques to revisit the early $^{63}$Cu NQR signature of charge order observed for La$_{1.875}$Ba$_{0.125}$CuO$_{4}$ ($T_{\text{c}} =4$~K) [A. W. Hunt et al., Phys. Rev. Lett. {\bf 82}, 4300 (1999)]. We show that the growth of spin correlations is accelerated below $\sim 80$~K, where the inverse Laplace transform (ILT) T$_{1}$ analysis of the $^{139}$La NMR spin-lattice relaxation curve recently uncovered emergence of the slow components in the lattice and/or charge fluctuations [P. M. Singer et al., {\bf 101}, 174508 (2020)]. From the accurate measurements of the $^{63}$Cu NMR signal intensity, spin echo decay $M(2τ)$, spin-lattice relaxation rate $^{63}1/T_1$, and its density distribution function $P(^{63}1/T_{1})$, we also demonstrate that charge order at $T_{\text{charge}}\simeq 54$~K turns on strong enhancement of spin fluctuations {\it within charge ordered domains}, thereby making the CuO$_2$ planes extremely inhomogeneous. The charge ordered domains grow quickly below $T_{\text{charge}}$, and the volume fraction $F_{\text{CA}}$ of the canonical domains unaffected by charge order gradually diminishes by $\sim 35$~K. This finding agrees with our independent estimations of $F_{\text{CA}}$ based entirely on the $^{139}$La ILTT$_{1}$ analyses, but is in a stark contrast with much slower growth of charge ordered domains observed for La$_{1.885}$Sr$_{0.115}$CuO$_{4}$ from its $T_{\text{charge}}\simeq 80$~K to $T_{\text{c}}\simeq 30$~K.

cond-mat.supr-con↗

arXiv2019

Distribution of the magnetic environment in charge ordered La$_{1.885}$Sr$_{0.115}$CuO$_{4}$

We report the inverse Laplace transform (ILT) analysis of the $^{139}$La nuclear spin-lattice relaxation rate $1/T_1$ in charge ordered La$_{1.885}$Sr$_{0.115}$CuO$_4$ ($T_{charge} \sim 80$K, $T_{c} \simeq T_{spin}^{neutron}=30$K), and shed new light on its magnetic inhomogeneity. We deduce the probability density function $P(1/T_{1})$ of the distributed $1/T_1$ (i.e. the histogram of distributed $1/T_1$) by taking the inverse Laplace transform of the experimentally observed nuclear magnetization recovery curve $M(t)$. We demonstrate that spin freezing sets in in some domains precisely below the onset of charge order at $T_{charge}$, but their volume fraction grows only gradually toward $T_{c}$. Nearly a half of the sample volume exhibits properties expected for canonical high $T_c$ cuprates without charge order even near $T_c$. Our findings explain why charge order does not suppress $T_c$ of La$_{1.885}$Sr$_{0.115}$CuO$_4$ as significantly as in La$_{1.875}$Ba$_{0.125}$CuO$_4$.

cond-mat.supr-con↗

arXiv2018

Dirac cones, Floquet side bands and theory of time resolved ARPES

Pump-probe techniques with high temporal resolution allow one to drive a system of interest out of equilibrium and at the same time, probe its properties. Recent advances in these techniques open the door to studying new, non-equilibrium phenomena such as Floquet topological insulators and superconductors. These advances also necessitate the development of theoretical tools for understanding the experimental findings and predicting new ones. In the present work, we provide a theoretical foundation to understand the non-equilibrium behavior of a Dirac system. We present detailed numerical calculations and simple analytic results for the evolution of a Dirac system irradiated by light. These results are framed intuitively by appealing to the recently revitalized notion of side-bands. We find that, under the application of circularly polarized light, a Dirac point only ever splits into two copies of sidebands. Meanwhile, the application of linearly polarized light leaves the Dirac point intact while producing side bands. Our immediate interest in this work is in connection to time and angle resolved photoemission experiments, where we find excellent qualitative agreement between our results and those in the literature. However, our results are general and may prove useful beyond this particular application and should be relevant to other pump-probe experiments.

cond-mat.str-el↗

arXiv2018

Low frequency spin dynamics in XY quantum spin ice Yb$_2$Pt$_2$O$_7$

The XY pyrochlore Yb$_2$Ti$_2$O$_7$, with pseudo spin 1/2 at the Yb$^{3+}$ site, has been celebrated as potential host for the quantum spin ice state. The substitution of non-magnetic Ti with Pt gives Yb$_2$Pt$_2$O$_7$, a system with remarkably similar magnetic properties. The large nuclear gyromagnetic ratio ($γ_{n}/2 π= 9.15$~MHz/T) of $^{195}$Pt makes Yb$_2$Pt$_2$O$_7$ an ideal material for NMR investigation of its unconventional magnetic properties. Based on the $^{195}$Pt nuclear spin-lattice relaxation rate $1/T_1$ and the magnetic specific heat $C_{p}$ measured in a broad range of magnetic field $B_{ext}$, we demonstrate that the field-induced magnon gap linearly decreases with $B_{ext}$ but additional low energy mode of spin excitations emerge below $\sim 0.5$~T.

cond-mat.str-el↗

arXiv2017

Revisiting $^{63}$Cu NMR evidence for charge order in superconducting La$_{1.885}$Sr$_{0.115}$CuO$_4$

The presence of charge and spin stripe order in the La2CuO4-based family of superconductors continues to lead to new insight on the unusual ground state properties of high Tc cuprates. Soon after the discovery of charge stripe order at T(charge)=65K in Nd3+ co-doped LSCO ($T_{c}\simeq6$~K) [Tranquada et al., Nature {\bf 375} (1995) 561], Hunt et al. demonstrated that La$_{1.48}$Nd$_{0.4}$Sr$_{0.12}$CuO$_4$ and superconducting LSCO with x~1/8 (Tc ~ 30K) share nearly identical NMR anomalies near $T_{charge}$ of the former [Phys. Rev. Lett. {\bf 82} (1999) 4300]. Their inevitable conclusion that LSCO also undergoes charge order at a comparable temperature became controversial, because diffraction measurements at the time were unable to detect Bragg peaks associated with charge order. Recent advances in x-ray diffraction techniques finally led to definitive confirmations of the charge order Bragg peaks in LSCO with an onset at as high as T(charge)=80K. Meanwhile, improved instrumental technology has enabled routine NMR measurements that were not feasible two decades ago. Motivated by these new developments, we revisit the charge order transition of a LSCO single crystal based on 63Cu NMR techniques. We demonstrate that 63Cu NMR properties of the nuclear spin $I_{z}$ = -1/2 to +1/2 central transition below T(charge) exhibit unprecedentedly strong dependence on the measurement time scale set by the NMR pulse separation time $τ$; a new kind of anomalous, very broad wing-like 63Cu NMR signals gradually emerge below T(charge) only for extremely short $τ\lesssim 4~μ$s, while the spectral weight of the normal NMR signals is progressively wiped out. The NMR linewidth and relaxation rates depend strongly on $τ$ below T(charge), and their enhancement in the charge ordered state indicates that charge order turns on strong but inhomogeneous growth of Cu spin-spin correlations.

cond-mat.supr-con↗