arXiv subjects

A. B. Voitkiv

Publications and source records attributed to A. B. Voitkiv.

At least 37 records · Page 2Linked to original sources

arXiv2021

Formation of $\bar{\rm{H}}^+$ via three body attachment of $\rm{e}^+$ to $\bar{\rm{H}}$

The formation of positive ions of antihydrogen $\bar{\rm{H}}^+$ via the three body reaction (i) $\rm{e}^+ + \rm{e}^- + \bar{\rm{H}} \rightarrow \rm{e}^- + \bar{\rm{H}}^+$ is considered. In reaction (i), free positrons $\rm{e}^+$ are incident on antihydrogen $\bar{\rm{H}}$ embedded in a gas of low-energy ($\sim $ meV) electrons and, due to the positron-electron interaction, a positron is attached to $\bar{\rm{H}}$ whereas an electron carries away the energy excess. We compare reaction (i) with two radiative attachment mechanisms. One of them is (ii) spontaneous radiative attachment, in which the ion is formed due to spontaneous emission of a photon by a positron incident on $\bar{\rm{H}}$. The other is (iii) two-center dileptonic attachment which takes place in the presence of a neighboring atom B and in which an incident positron is attached to $\bar{\rm{H}}$ via resonant transfer of energy to B with its subsequent relaxation through spontaneous radiative decay. It is shown that reaction (i) can strongly dominate over mechanisms (ii) and (iii) for positron energies below $0.1$ eV. It is also shown that at the energies considered reaction (i) will not be influenced by annihilation and that the reaction $\rm{e}^+ + \rm{e}^+ + \bar{\rm{H}} \rightarrow \rm{e}^+ + \bar{\rm{H}}^+$ has a vanishingly small rate compared to reaction (i).

physics.atom-ph↗

arXiv2021

Probing the helium dimer by relativistic highly-charged projectiles

We study the fragmentation of He$_2$ dimers into He$^+$ ions by relativistic highly-charged projectiles. It is demonstrated that the interaction between an ultrafast projectile with an extremely extended object -- the helium dimer -- possesses interesting features which are absent in collisions with "normal" molecules. It is also shown that such projectiles, due to their enormous interaction range, can accurately probe the ground state of the dimer and even be used for a precise determination of its binding energy.

physics.atom-ph↗

arXiv2021

Resonant elastic scattering of polarized electrons on H-like ions

The polarization properties of the elastic electron scattering on H-like ions are investigated within the framework of the relativistic QED theory. The polarization properties are determined by a combination of relativistic effects and spin exchange between the incident and bound electrons. The scattering of a polarized electron on an initially unpolarized ion is fully described by five parameters. We study these parameters for non-resonant scattering, as well as in the vicinity of LL resonances, where scattering occurs through the formation and subsequent decay of intermediate autoionizing states. The study was carried out for ions from $\txt{B}^{4+}$ to $\txt{Xe}^{53+}$. Special attention was paid to the study of asymmetry in electron scattering.

physics.atom-ph↗

arXiv2020

Influence of nuclear motion on resonant two-center photoionization

Photoionization of an atom in the presence of a neighboring atom of different species is studied. The latter first undergoes resonant photoexcitation, leading to an autoionizing state of the diatomic system. Afterwards, the excitation energy is transferred radiationlessly via a two-center Auger process to the other atom, causing its ionization. Assuming a fixed internuclear distance, it has been predicted theoretically that this indirect ionization pathway can strongly dominate over the direct photoionization. Here, we extend the theory of resonant two-center photoionization by including the nuclear motion in van-der-Waals molecules. An analytical formula is derived reflecting the influence of molecular vibrational dynamics on the relative strength of the two-center channel. For the specific example of Li-He dimers we show that the two-center autoionizing resonances are split by the nuclear motion into multiplets, with the resonance lines reaching a comparable level of enhancement over direct photoionization as is obtained in a model based on spatially fixed nuclei.

physics.atom-ph↗

arXiv2020

Photo ionization of an atom passed through a diffraction grating

We consider photo ionization of an atom which, due to passing through a diffraction grating, is prepared in a multi-site state possessing a periodic space structure with alternating maxima and minima. It has been found that this process qualitatively differs from photo ionization of a 'normal' atom. In particular, the spectra of emitted electrons and recoil ions in this process display clear one- and two-particle interference effects. Moreover, there are also striking differences between the momentum distributions of these particles, which no longer mirror each other. The origin of all these features is discussed in detail. It is also shown that the information about the diffraction grating, which is encoded in the multi-site state of the atom, can be fully decoded by exploring the spectra of recoil ions whereas the photo-electron spectra contain this information only partially.

physics.atom-ph↗

arXiv2020

Interatomic distance dependence of resonant energy-transfer phenomena

It is well known that interatomic or intermolecular interactions driven by two-center electronic dipole-dipole correlations fall off rapidly with the inter-site distance. We show, however, that the effective strength of interatomic reaction channels, which are triggered by a resonant field, can exhibit a nonmonotonous distance dependence, being strongly reduced when the atoms come closer. This surprising result is demonstrated by considering resonant two-center photoionization as an example. Our findings are supported by available experimental data.

physics.atom-ph↗

arXiv2020

Probing atomic 'quantum grating' by collisions with charged projectiles

The wave function of an atom passed through a diffraction grating acquires a regular space structure and the interaction of another particle with this atom can be thought of as scattering on a 'quantum grating' composed of a single atom. Probing this 'grating' by collisions with charged projectiles reveals interference effects due to coherent contributions of its 'slits' to the transition amplitude. In particular, the spectra of electrons emitted from the atom in collisions with swift ions exhibit a pronounced interference pattern whose shape can be extremely sensitive to the collision velocity.

quant-ph↗

arXiv2019

Two-center electron-impact ionization via collisional excitation-autoionization

Electron-impact ionization of an atom or ion in the presence of a neighboring atom is studied. The latter is first collisionally excited by the incident electron, whose energy is assumed to be high but nonrelativistic. Afterwards, the excitation energy is transferred radiationlessly via a two-center Auger process to the other atom or ion, leading to its ionization. We show that the participation of the neighboring atom manifests in a very pronounced resonance peak in the energy-differential cross section and can substantially enhance the total cross section of electron-impact ionization. We also discuss the influence of the neighbouring atom on the angular distribution of the ejected electron.

physics.atom-ph↗

arXiv2019

QED theory of elastic electron scattering on hydrogen-like ions involving formation and decay of autoionizing states

We develop {\it ab initio} relativistic QED theory for elastic electron scattering on hydrogen-like highly charged ions for impact energies where, in addition to direct (Coulomb) scattering, the process can also proceed via formation and consequent Auger decay of autoionizing states of the corresponding helium-like ions. Even so the primary goal of the theory is to treat electron scattering on highly charged ions, a comparison with experiment shows that it can also be applied for relatively light ions covering thus a very broad range of the scattering systems. Using the theory we performed calculations for elastic electron scattering on B$^{4+}$, Ca$^{19+}$, Fe$^{25+}$, Kr$^{35+}$, and Xe$^{53+}$. The theory was also generalized for collisions of hydrogen-like highly charged ions with atoms considering the latter as a source of (quasi-) free electrons.

physics.atom-ph↗

arXiv2019

Resonant single-photon double ionization driven by combined intra- and interatomic electron correlations

Double ionization of an atom by single-photon absorption in the presence of a neighbouring atom is studied. The latter is, first, resonantly photoexcited and, afterwards, transfers the excitation energy radiationlessly to the other atom, leading to its double ionization. The process relies on the combined effect of interatomic and intraatomic electron correlations. It can dominate over the direct double photoionization by several orders of magnitude at interatomic distances up to few nanometers. The relative position of the neighbouring atom is shown to exert a characteristic influence on the angular distribution of emitted electrons.

physics.atom-ph↗

arXiv2019

Two-center dielectronic recombination in slow atomic collisions

A free electron can form a bound state with an atomic center $A$ upon photo emission (radiative recombination). In the presence of a neighboring atom $B$, such a bound state can, under certain conditions, be also formed via resonant transfer of energy to $B$, with its subsequent relaxation through radiative decay (two-center dielectronic recombination). This two-center process is very efficient in the 'static' case where $A$ and $B$ form a weakly bound system, dominating over single-center radiative recombination up to internuclear distances as large as several nanometers. Here we study its dynamic variant in which recombination occurs when a beam of species $A$ collides with a gas of atoms $B$ and show that, even though the average distance between $A$ and $B$ in collisions is orders of magnitude larger than the typical size of a bound system, the two-center recombination can still outperform the single-center radiative recombination.

physics.atom-ph↗

arXiv2018

Dynamic two-center resonant photoionization in slow atomic collisions

An additional channel opens for photoionization of atom $A$ by an electromagnetic field if it traverses a gas of atoms $B$ resonantly coupled to this field. We show that this channel, in which $A$ is ionized via resonant photoexcitation of $B$ with subsequent energy transfer to $A$ through two-center electron correlations and which is very efficient when $A$ and $B$ constitute a bound system, can strongly dominate the ionization of $A$ also in collisions where the average distance between $A$ and $B$ exceeds the typical size of a bound system by orders of magnitude.

physics.atom-ph↗

arXiv2018

Strong-field photoionization in two-center atomic systems

Photoionization of an atom $A$ by a strong laser field in the presence of a spatially well-separated neighboring atom $B$ is considered. The laser field frequency is assumed to lie below the ionization potential of atom $A$ and be resonant with a dipole-allowed transition in atom $B$. In this situation, the ionization may occur either directly by multiphoton absorption from the laser field at the first atomic center. Or via an indirect pathway involving two-center electron-electron correlations, where the neighbor atom $B$ is first photoexcited and, afterwards, transfers its energy upon deexcitation radiationlessly to atom $A$. Considering monochromatic as well as bichromatic laser fields, we study various coupling regimes of the photoionization process and identify experimentally accessible parameter domains where the two-center channel is dominant.

physics.atom-ph↗

arXiv2018

Resonant electron scattering and dielectronic recombination in two-center atomic systems

Electron scattering and dielectronic recombination with an ion in the presence of a neighboring atom is studied. The incident electron is assumed to be captured by the ion, leading to resonant excitation of the atom which afterwards may stabilize either by electron re-emission or radiative decay. We show that the participation of the atom can strongly affect, both quantitatively and qualitatively, the corresponding processes of electron scattering and recombination. Various ion-atom systems and electronic transitions are considered. In particular we show that electron scattering under backward angles may be strongly enhanced and derive the scaling behavior of two-center dielectronic recombination with the principal quantum numbers of the participating atomic states.

physics.atom-ph↗

arXiv2017

Electron loss from hydrogen-like highly charged ions in collisions with electrons, protons and light atoms

We study electron loss from a hydrogen-like highly charged ion by the impact of equivelocity electrons and protons and also in collisions with hydrogen and helium. The collision velocity $v$ varies between $v_{min}$ and $v_{max}$, where $v_{min}$ and $v_{max}$ correspond to the energy threshold $\varepsilon_{th}$ for electron loss in collisions with a free electron and to $\approx 5 \, \varepsilon_{th}$, respectively. Our results show that in this range of $v$: i) compared to equivelocity electrons protons are more effective in inducing electron loss (due to a substantially larger volume of the effectively available final-state electron momentum space), ii) the relative (compared to protons) effectiveness of electron projectiles grows with increase in the atomic number of a highly charged ion, iii) a substantial part of the volume of the final-state-electron momentum space, kinematically available in collisions with electrons, is weaker populated in collisions with protons than with electrons, iv) even when the total loss cross sections in collisions with electrons and protons become already equal the spectra of the outgoing electrons still remain quite different in almost the entire volume of the final-state-electron momentum space. The points i) and iii), in particular, mean that in collisions with hydrogen target the contributions to the loss process from the interactions with the nucleus and the electron(s) of the atom would be to a large extent separated in the final-state-electron momentum space.

physics.atom-ph↗

arXiv2016

Effects of autoionization in electron loss from helium-like highly charged ions in collisions with photons and fast atomic particles

We study theoretically single electron loss from helium-like highly charged ions involving excitation and decay of autoionizing states of the ion. Electron loss is caused by either photo absorption or the interaction with a fast atomic particle (a bare nucleus, a neutral atom, an electron). The interactions with the photon field and the fast particles are taken into account in the first order of perturbation theory. Two initial states of the ion are considered: $1s^2$ and $(1s2s)_{J=0}$. We analyze in detail how the shape of the emission pattern depends on the atomic number $Z_{I}$ of the ion discussing, in particular, the inter-relation between electron loss via photo absorption and due to the impact of atomic particles in collisions at modest relativistic and extreme relativistic energies. According to our results, in electron loss from the $1s^2$ state autoionization may substantially influence the shape of the emission spectra only up to $Z_{I} \approx 35-40$. A much more prominent role is played by autoionization in electron loss from $(1s2s)_{J=0}$ where it not only strongly affect the shape of the emission pattern but also may substantially increase the total loss cross section.

physics.atom-ph↗

arXiv2014

Relativistic transfer ionization and the Breit interaction

We consider correlated transfer ionization in relativistic collisions between a highly charged ion and a light atom. In this process two quasi-free electrons of the atom interact with each other during the short collision time that results in capture of one of them by the ion and emission of the other. We show that this process is strongly influenced by the generalized Breit interaction already at modest relativistic impact energies.

physics.atom-ph↗

arXiv2013

Mutual ionization in atomic collisions near the electronic threshold

We study mutual ionization in collisions between atomic hydrogen and helium at impact velocities near the electronic threshold for this process (determined by the condition that kinetic energy of an equivelocity free electron is approximately equal to the sum of binding energies of active electrons in the projectile and target). We show that this process is substantially influenced by the Coulomb repulsion between the emitted electrons and that the atomic nuclei are very strongly involved in the momentum balance along the collision velocity.

physics.atom-ph↗