arXiv subjects

A. C. Andersen

Publications and source records attributed to A. C. Andersen.

26 records · Page 2Linked to original sources

arXiv2002

Extinction calculations of multi-sphere polycrystalline graphitic clusters - A comparison with the 2175 AA peak and between a rigorous solution and discrete-dipole approximations

Certain dust particles in space are expected to appear as clusters of individual grains. The morphology of these clusters could be fractal or compact. In this paper we study the light scattering by compact and fractal polycrystalline graphitic clusters consisting of touching identical spheres. We compare three general methods for computing the extinction of the clusters in the wavelength range 0.1 - 100 micron, namely, a rigorous solution (Gerardy & Ausloos 1982) and two different discrete-dipole approximation methods -- MarCODES (Markel 1998) and DDSCAT (Draine & Flatau 1994). We consider clusters of N = 4, 7, 8, 27,32, 49, 108 and 343 particles of radii either 10 nm or 50 nm, arranged in three different geometries: open fractal (dimension D = 1.77), simple cubic and face-centred cubic. The rigorous solution shows that the extinction of the fractal clusters, with N < 50 and particle radii 10 nm, displays a peak within 2% of the location of the observed interstellar extinction peak at ~4.6 inverse micron; the smaller the cluster, the closer its peak gets to this value. By contrast, the peak in the extinction of the more compact clusters lie more than 4% from 4.6 inverse micron. At short wavelengths (0.1 - 0.5 micron), all the methods show that fractal clusters have markedly different extinction from those of non-fractal clusters. At wavelengths > 5 micron, the rigorous solution indicates that the extinction from fractal and compact clusters are of the same order of magnitude. It was only possible to compute fully converged results of the rigorous solution for the smaller clusters, due to computational limitations, however, we find that both discrete-dipole approximation methods overestimate the computed extinction of the smaller fractal clusters.

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arXiv2001

Effects of Grain Morphology and Impurities on the Infrared Spectra of Silicon Carbide Particles

In this paper we demonstrate that distinguishing between the polytypes of silicon carbide by means of infrared features in small-grain spectra is impossible. Therefore, the infrared spectra of carbon stars, unfortunately, do not provide a means for drawing comparisons between the crystal structures of grains condensed in these environments and found in meteorites. This is proven first by comparing theoretical band profiles calculated for ellipsoidal particles, which show clearly a strong dependence on the axis ratio of the ellipsoids but negligible differences for the two most common polytypes. Second, spectra measured on submicron particle samples in the laboratory do not show any obvious correlation of band position or shape to the polytype. However, we demonstrate by measurements on SiC whiskers that grain shape is able to determine the spectrum completely. A further strong systematic influence on the band profile can be exerted by plasmon-phonon coupling due to conductivity of the SiC material. The latter fact probably is responsible for the confusion in the astronomical literature about spectral properties of SiC grains. We show that, although the conductivity seems to be a common property of many SiC laboratory samples, it is, however, independent of the polytype.

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arXiv2001

Carbon Star Dust from Meteorites

Inside carbonaceous chondrite meteorites are tiny dust particles which, when heated, release noble gases with an isotopic composition different from what is found anywhere else in the solar system. For this reason it is believed that these grains are (inter)stellar dust which survived the collapse of the interstellar cloud that became the solar system. We will describe here why we believe that the most abundant of these grains, nano-diamonds, were formed in the atmospheres of carbon stars, and explain how this theory can be tested observationally.

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arXiv2001

The influence of dust properties on the mass loss in pulsating AGB stars

We are currently studying carbon based dust types of relevance for carbon-rich AGB stars, to obtain a better understanding of the influence of the optical and chemical properties of the grains on the mass loss of the star. An investigation of the complex interplay between hydrodynamics,radiative transfer and chemistry has to be based on a better knowledge of the micro-physics of the relevant dust species.

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arXiv2001

Interstellar extinction by fractal polycrystalline graphite clusters?

Certain dust particles in space are expected to appear as clusters of individual grains. The morphology of these clusters could be fractal or compact. To determine how these structural features would affect the interpretation of the observed interstellar extinction peak at $\sim 4.6 μ$m, we have calculated the extinction by compact and fractal polycrystalline graphite clusters consisting of touching identical spheres. We compare three general methods for computing the extinction of the clusters, namely, a rigorous solution and two different discrete-dipole approximation methods.

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arXiv1999

Infrared properties of SiC particles

We present basic laboratory infrared data on a large number of SiC particulate samples, which should be of great value for the interpretation of the 11.3 micron feature observed in the spectra of carbon-rich stars. The laboratory spectra show a wide variety of the SiC phonon features in the 10-13 micron wavelength range, both in peak wavelength and band shape. The main parameters determining the band profile are morphological factors as grain size and shape and, in many cases, impurities in the material. We discovered the interesting fact that free charge carriers, generated e.g. by nitrogen doping, are a very common characteristics of many SiC particle samples. These free charge carriers produce very strong plasmon absorption in the near and middle infrared, which may also heavily influence the 10-13 micron feature profile via plasmon-phonon coupling. We also found that there is no systematic dependence of the band profile on the crystal type (alpha- vs. beta-SiC). This is proven both experimentally and by theoretical calculations based on a study of the SiC phonon frequencies. Further, we give optical constants of amorphous SiC. We discuss the implications of the new laboratory results for the interpretation of the spectra of carbon stars.

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arXiv1998

Infrared Spectra of Meteoritic SiC Grains

We present here the first infrared spectra of meteoritic SiC grains. The mid-infrared transmission spectra of meteoritic SiC grains isolated from the Murchison meteorite were measured in the wavelength range 2.5--16.5 micron, in order to make available the optical properties of presolar SiC grains. These grains are most likely stellar condensates with an origin predominately in carbon stars. Measurements were performed on two different extractions of presolar SiC from the Murchison meteorite. The two samples show very different spectral appearance due to different grain size distributions. The spectral feature of the smaller meteoritic SiC grains is a relatively broad absorption band found between the longitudinal and transverse lattice vibration modes around 11.3 micron, supporting the current interpretation about the presence of SiC grains in carbon stars. In contrast to this, the spectral feature of the large (> 5 micron) grains has an extinction minimum around 10 micron. The obtained spectra are compared with commercially available SiC grains and the differences are discussed. This comparison shows that the crystal structure (e.g., beta-SiC versus alpha-SiC) of SiC grains plays a minor role on the optical signature of SiC grains compared to e.g. grain size.

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arXiv1997

Spectral features of presolar diamonds in the laboratory and in carbon star atmospheres

Laboratory analyses on fine-grained diamond residues from primitive meteorites have shown that nano-diamonds represent the most abundant form of presolar dust preserved in meteoritic samples. The presolar diamonds carry isotopic anomalies which indicate a very complex formation history. Several groups of diamonds may exist with origin in different types of stars. In order to identify the sites of formation observationally, we have extracted presolar diamonds from the Allende meteorite and measured the monochromatic absorption coefficient in a form which is useful for stellar atmosphere calculations. The monochromatic absorption coefficient was measured in the wavelength ranges 400--4000 cm-1 (2.5--25 micron) and 12200--52600 cm-1 (190--820 nm). We have made identical laboratory measurements on CVD diamonds as on the meteoritic diamonds, in order to get a more solid basis for the interpretation of the diamond spectrum. The monochromatic absorption coefficient for the presolar diamonds was incorporated in self-consistent carbon star photospheric models. The main influence of the diamond dust in our photospheric models is a heating of the upper photospheric layers and a reduction of the C2H2 abundance. Due to the relatively small absorption coefficient of the diamonds compared to other stellar dust grains, their spectral appearance is weak. However, the weak interaction of the diamonds with the radiation field may give them an important role in the dust nucleation process. The gas pressure will stay high and the gas will be much closer to hydrostatic equilibrium during possible diamond nucleation than is normally the case in dust forming stellar regions, and therefore allow ample time for the nucleation process.

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