arXiv subjects

A. Caciolli

Publications and source records attributed to A. Caciolli.

At least 37 records · Page 2Linked to original sources

arXiv2020

Setup commissioning for an improved measurement of the D(p,gamma)3He cross section at Big Bang Nucleosynthesis energies

Among the reactions involved in the production and destruction of deuterium during Big Bang Nucleosynthesis, the deuterium-burning D(p,gamma)3He reaction has the largest uncertainty and limits the precision of theoretical estimates of primordial deuterium abundance. Here we report the results of a careful commissioning of the experimental setup used to measure the cross-section of the D(p,gamma)3He reaction at the Laboratory for Underground Nuclear Astrophysics of the Gran Sasso Laboratory (Italy). The commissioning was aimed at minimising all sources of systematic uncertainty in the measured cross sections. The overall systematic error achieved (< 3 %) will enable improved predictions of BBN deuterium abundance.

physics.ins-det↗

arXiv2020

A new approach to monitor 13C-targets degradation in situ for 13C(alpha,n)16O cross-section measurements at LUNA

Direct measurements of reaction cross-sections at astrophysical energies often require the use of solid targets able to withstand high ion beam currents for extended periods of time. Thus, monitoring target thickness, isotopic composition, and target stoichiometry during data taking is critical to account for possible target modifications and to reduce uncertainties in the final cross-section results. A common technique used for these purposes is the Nuclear Resonant Reaction Analysis (NRRA), which however requires that a narrow resonance be available inside the dynamic range of the accelerator used. In cases when this is not possible, as for example the 13C(alpha,n)16O reaction recently studied at low energies at the Laboratory for Underground Nuclear Astrophysics (LUNA) in Italy, alternative approaches must be found. Here, we present a new application of the shape analysis of primary gamma rays emitted by the 13C(p,g)14N radiative capture reaction. This approach was used to monitor 13C target degradation {\em in situ} during the 13C(alpha,n)16O data taking campaign. The results obtained are in agreement with evaluations subsequently performed at Atomki (Hungary) using the NRRA method. A preliminary application for the extraction of the 13C(alpha,n)16O reaction cross-section at one beam energy is also reported.

physics.ins-det↗

arXiv2019

A new study of the $^{10}$B(p,$α_1 γ$)$^{7}$Be reaction from 0.35 to 1.8 MeV

The quantification of isotopes content in materials is extremely important in many research and industrial fields. Accurate determination of boron concentration is very critical in semiconductor, superconductor and steel industry, in environmental and medical applications as well as in nuclear and astrophysics research. The detection of B isotopes and of their ratio in synthetic and natural materials may be accomplished by gamma spectroscopy using the $^{10}$B(p,$α_1 γ$)$^7$Be and $^{11}$B(p,$γ$)$^{12}$C reactions at low proton energy. Here, the $^{10}$B(p,$α_1 γ$)$^7$Be cross section is reported in the center of mass energy range 0.35 to 1.8 MeV. The $E_γ$= 429 keV $γ$ rays were detected at 45$^\circ$ and 90$^\circ$ using a NaI(Tl) and an HPGe detectors, respectively. In the presented energy range, previous cross sections data revealed discrepancies and normalisation issues. Existing data are compared to the new absolute measurement and discussed. The present data have been subtracted from a previous measurement of the total cross section to derive the contribution of the $α_0$ channel.

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arXiv2018

Direct capture cross section and the $E_p$ = 71 and 105 keV resonances in the $^{22}$Ne($p,γ$)$^{23}$Na reaction

The $^{22}$Ne($p,γ$)$^{23}$Na reaction, part of the neon-sodium cycle of hydrogen burning, may explain the observed anticorrelation between sodium and oxygen abundances in globular cluster stars. Its rate is controlled by a number of low-energy resonances and a slowly varying non-resonant component. Three new resonances at $E_p$ = 156.2, 189.5, and 259.7 keV have recently been observed and confirmed. However, significant uncertainty on the reaction rate remains due to the non-resonant process and to two suggested resonances at $E_p$ = 71 and 105 keV. Here, new $^{22}$Ne($p,γ$)$^{23}$Na data with high statistics and low background are reported. Stringent upper limits of 6$\times$10$^{-11}$ and 7$\times$10$^{-11}$\,eV (90\% confidence level), respectively, are placed on the two suggested resonances. In addition, the off-resonant S-factor has been measured at unprecedented low energy, constraining the contributions from a subthreshold resonance and the direct capture process. As a result, at a temperature of 0.1 GK the error bar of the $^{22}$Ne($p,γ$)$^{23}$Na rate is now reduced by three orders of magnitude.

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arXiv2018

Effect of beam energy straggling on resonant yield in thin gas targets: The cases $^{22}$Ne(p,γ)$^{23}$Na and $^{14}$N(p,γ)$^{15}$O

When deriving resonance strengths using the thick-target yield approximation, for very narrow resonances it may be necessary to take beam energy straggling into account. This applies to gas targets of a few keV width, especially if there is some additional structure in target stoichiometry or detection efficiency. The correction for this effect is shown and tested on recent studies of narrow resonances in the $^{22}$Ne(p,γ)$^{23}$Na and $^{14}$N(p,γ)$^{15}$O reactions.

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arXiv2018

A high-efficiency gas target setup for underground experiments, and redetermination of the branching ratio of the 189.5 keV $\mathbf{^{22}Ne(p,γ)^{23}Na}$ resonance

The experimental study of nuclear reactions of astrophysical interest is greatly facilitated by a low-background, high-luminosity setup. The Laboratory for Underground Nuclear Astrophysics (LUNA) 400 kV accelerator offers ultra-low cosmic-ray induced background due to its location deep underground in the Gran Sasso National Laboratory (INFN-LNGS), Italy, and high intensity, 250-500 $μ$A, proton and $α$ ion beams. In order to fully exploit these features, a high-purity, recirculating gas target system for isotopically enriched gases is coupled to a high-efficiency, six-fold optically segmented bismuth germanate (BGO) $γ$-ray detector. The beam intensity is measured with a beam calorimeter with constant temperature gradient. Pressure and temperature measurements have been carried out at several positions along the beam path, and the resultant gas density profile has been determined. Calibrated $γ$-intensity standards and the well-known $E_p$ = 278 keV $\mathrm{^{14}N(p,γ)^{15}O}$ resonance were used to determine the $γ$-ray detection efficiency and to validate the simulation of the target and detector setup. As an example, the recently measured resonance at $E_p$ = 189.5 keV in the $^{22}$Ne(p,$γ$)$^{23}$Na reaction has been investigated with high statistics, and the $γ$-decay branching ratios of the resonance have been determined.

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arXiv2017

LUNA: Status and Prospects

The essential ingredients of nuclear astrophysics are the thermonuclear reactions which shape the life and death of stars and which are responsible for the synthesis of the chemical elements in the Universe. Deep underground in the Gran Sasso Laboratory the cross sections of the key reactions responsible for the hydrogen burning in stars have been measured with two accelerators of 50 and 400 kV voltage right down to the energies of astrophysical interest. As a matter of fact, the main advantage of the underground laboratory is the reduction of the background. Such a reduction has allowed, for the first time, to measure relevant cross sections at the Gamow energy. The qualifying features of underground nuclear astrophysics are exhaustively reviewed before discussing the current LUNA program which is mainly devoted to the study of the Big-Bang nucleosynthesis and of the synthesis of the light elements in AGB stars and classical novae. The main results obtained during the study of reactions relevant to the Sun are also reviewed and their influence on our understanding of the properties of the neutrino, of the Sun and of the Universe itself is discussed. Finally, the future of LUNA during the next decade is outlined. It will be mainly focused on the study of the nuclear burning stages after hydrogen burning: helium and carbon burning. All this will be accomplished thanks to a new 3.5 MV accelerator able to deliver high current beams of proton, helium and carbon which will start running under Gran Sasso in 2019. In particular, we will discuss the first phase of the scientific case of the 3.5 MV accelerator focused on the study of $^{12}$C+$^{12}$C and of the two reactions which generate free neutrons inside stars: $^{13}$C($α$,n)$^{16}$O and $^{22}$Ne($α$,n)$^{25}$Mg.

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arXiv2017

Astrophysical S-factor of the $^{14}\textrm{N(p,}γ\textrm{)}^{15}\textrm{O}$ reaction at 0.4 -- 1.3\,MeV

The $^{14}\textrm{N(p,}γ\textrm{)}^{15}\textrm{O}$ reaction is the slowest reaction of the carbon-nitrogen cycle of hydrogen burning and thus determines its rate. The precise knowledge of its rate is required to correctly model hydrogen burning in asymptotic giant branch stars. In addition, it is a necessary ingredient for a possible solution of the solar abundance problem by using the solar $^{13}$N and $^{15}$O neutrino fluxes as probes of the carbon and nitrogen abundances in the solar core. After the downward revision of its cross section due to a much lower contribution by one particular transition, capture to the ground state in $^{15}$O, the evaluated total uncertainty is still 8\%, in part due to an unsatisfactory knowledge of the excitation function over a wide energy range. The present work reports precise S-factor data at twelve energies between 0.357-1.292~MeV for the strongest transition, capture to the 6.79~MeV excited state in $^{15}$O, and at ten energies between 0.479-1.202~MeV for the second strongest transition, capture to the ground state in $^{15}$O. An R-matrix fit is performed to estimate the impact of the new data on astrophysical energies. The recently suggested slight enhancement of the 6.79~MeV transition at low energy could not be confirmed. The present extrapolated zero-energy S-factors are $S_{6.79}(0)$~=~1.24$\pm$0.11~keV~barn and $S_{\rm GS}(0)$~=~0.19$\pm$0.05~keV~barn.

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arXiv2017

Origin of meteoritic stardust unveiled by a revised proton-capture rate of $^{17}$O

Stardust grains recovered from meteorites provide high-precision snapshots of the isotopic composition of the stellar environment in which they formed. Attributing their origin to specific types of stars, however, often proves difficult. Intermediate-mass stars of 4-8 solar masses are expected to contribute a large fraction of meteoritic stardust. However, no grains have been found with characteristic isotopic compositions expected from such stars. This is a long-standing puzzle, which points to serious gaps in our understanding of the lifecycle of stars and dust in our Galaxy. Here we show that the increased proton-capture rate of $^{17}$O reported by a recent underground experiment leads to $^{17}$O/$^{16}$O isotopic ratios that match those observed in a population of stardust grains, for proton-burning temperatures of 60-80 million K. These temperatures are indeed achieved at the base of the convective envelope during the late evolution of intermediate-mass stars of 4-8 solar masses, which reveals them as the most likely site of origin of the grains. This result provides the first direct evidence that these stars contributed to the dust inventory from which the Solar System formed.

astro-ph.SR↗

arXiv2016

$^{22}$Ne and $^{23}$Na ejecta from intermediate-mass stars: The impact of the new LUNA rate for $^{22}$Ne(p,$γ$)$^{23}$Na

We investigate the impact of the new LUNA rate for the nuclear reaction $^{22}$Ne$(p,γ)^{23}$Na on the chemical ejecta of intermediate-mass stars, with particular focus on the thermally-pulsing asymptotic giant branch (TP-AGB) stars that experience hot-bottom burning. To this aim we use the PARSEC and COLIBRI codes to compute the complete evolution, from the pre-main sequence up to the termination of the TP-AGB phase, of a set of stellar models with initial masses in the range $3.0\,M_{\odot} - 6.0\,M_{\odot}$, and metallicities $Z_{\rm i}=0.0005$, $Z_{\rm i}=0.006$, and $Z_{\rm i} = 0.014$. We find that the new LUNA measures have much reduced the nuclear uncertainties of the $^{22}$Ne and $^{23}$Na AGB ejecta, which drop from factors of $\simeq 10$ to only a factor of few for the lowest metallicity models. Relying on the most recent estimations for the destruction rate of $^{23}$Na, the uncertainties that still affect the $^{22}$Ne and $^{23}$Na AGB ejecta are mainly dominated by evolutionary aspects (efficiency of mass-loss, third dredge-up, convection). Finally, we discuss how the LUNA results impact on the hypothesis that invokes massive AGB stars as the main agents of the observed O-Na anti-correlation in Galactic globular clusters. We derive quantitative indications on the efficiencies of key physical processes (mass loss, third dredge-up, sodium destruction) in order to simultaneously reproduce both the Na-rich, O-poor extreme of the anti-correlation, and the observational constraints on the CNO abundance. Results for the corresponding chemical ejecta are made publicly available.

astro-ph.SR↗

arXiv2016

The impact of the revised $^{17}$O$(p,α)^{14}$N reaction rate on $^{17}$O stellar abundances and yields

Context. Material processed by the CNO cycle in stellar interiors is enriched in 17O. When mixing processes from the stellar surface reach these layers, as occurs when stars become red giants and undergo the first dredge up, the abundance of 17O increases. Such an occurrence explains the drop of the 16O/17O observed in RGB stars with mass larger than 1.5 M_\solar. As a consequence, the interstellar medium is continuously polluted by the wind of evolved stars enriched in 17O . Aims. Recently, the Laboratory for Underground Nuclear Astrophysics (LUNA) collaboration released an improved rate of the 17O(p,alpha)14N reaction. In this paper we discuss the impact that the revised rate has on the 16O/17O ratio at the stellar surface and on 17O stellar yields. Methods. We computed stellar models of initial mass between 1 and 20 M_\solar and compared the results obtained by adopting the revised rate of the 17O(p,alpha)14N to those obtained using previous rates. Results. The post-first dredge up 16O/17O ratios are about 20% larger than previously obtained. Negligible variations are found in the case of the second and the third dredge up. In spite of the larger 17O(p,alpha)14N rate, we confirm previous claims that an extra-mixing process on the red giant branch, commonly invoked to explain the low carbon isotopic ratio observed in bright low-mass giant stars, marginally affects the 16O/17O ratio. Possible effects on AGB extra-mixing episodes are also discussed. As a whole, a substantial reduction of 17O stellar yields is found. In particular, the net yield of stars with mass ranging between 2 and 20 M_\solar is 15 to 40% smaller than previously estimated. Conclusions. The revision of the 17O(p,alpha)14N rate has a major impact on the interpretation of the 16O/17O observed in evolved giants, in stardust grains and on the 17O stellar yields.

astro-ph.SR↗

arXiv2016

Direct measurement of low-energy $^{22}$Ne(p,$γ$)$^{23}$Na resonances

The $^{22}$Ne(p,$γ$)$^{23}$Na reaction is the most uncertain process in the neon-sodium cycle of hydrogen burning. At temperatures relevant for nucleosynthesis in asymptotic giant branch stars and classical novae, its uncertainty is mainly due to a large number of predicted but hitherto unobserved resonances at low energy. Purpose: A new direct study of low energy $^{22}$Ne(p,$γ$)$^{23}$Na resonances has been performed at the Laboratory for Underground Nuclear Astrophysics (LUNA), in the Gran Sasso National Laboratory, Italy. Method: The proton capture on $^{22}$Ne was investigated in direct kinematics, delivering an intense proton beam to a $^{22}$Ne gas target. $γ$ rays were detected with two high-purity germanium detectors enclosed in a copper and lead shielding suppressing environmental radioactivity. Results: Three resonances at 156.2 keV ($ωγ$ = (1.48\,$\pm$\,0.10)\,$\cdot$\,10$^{-7}$ eV), 189.5 keV ($ωγ$ = (1.87\,$\pm$\,0.06)\,$\cdot$\,10$^{-6}$ eV) and 259.7 keV ($ωγ$ = (6.89\,$\pm$\,0.16)\,$\cdot$\,10$^{-6}$ eV) proton beam energy, respectively, have been observed for the first time. For the levels at 8943.5, 8975.3, and 9042.4 keV excitation energy corresponding to the new resonances, the $γ$-decay branching ratios have been precisely measured. Three additional, tentative resonances at 71, 105 and 215 keV proton beam energy, respectively, were not observed here. For the strengths of these resonances, experimental upper limits have been derived that are significantly more stringent than the upper limits reported in the literature. Conclusions: Based on the present experimental data and also previous literature data, an updated thermonuclear reaction rate is provided in tabular and parametric form. The new reaction rate is significantly higher than previous evaluations at temperatures of 0.08-0.3 GK.

nucl-ex↗

arXiv2016

Improved Direct Measurement of the 64.5 keV Resonance Strength in the 17O(p,a)14N Reaction at LUNA

The $^{17}$O(p,$α$)$^{14}$N reaction plays a key role in various astrophysical scenarios, from asymptotic giant branch stars to classical novae. It affects the synthesis of rare isotopes such as $^{17}$O and $^{18}$F, which can provide constraints on astrophysical models. A new direct determination of the $E_{\rm R}~=~64.5$~keV resonance strength performed at the Laboratory for Underground Nuclear Astrophysics accelerator has led to the most accurate value to date, $ωγ= 10.0 \pm 1.4_{\rm stat} \pm 0.7_{\rm syst}$~neV, thanks to a significant background reduction underground and generally improved experimental conditions. The (bare) proton partial width of the corresponding state at $E_{\rm x} = 5672$~keV in $^{18}$F is $Γ_{\rm p} = 35 \pm 5_{\rm stat} \pm 3_{\rm syst}$~neV. This width is about a factor of 2 higher than previously estimated thus leading to a factor of 2 increase in the $^{17}$O(p,$α$)$^{14}$N reaction rate at astrophysical temperatures relevant to shell hydrogen-burning in red giant and asymptotic giant branch stars. The new rate implies lower $^{17}$O/$^{16}$O ratios, with important implications on the interpretation of astrophysical observables from these stars.

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arXiv2016

A new study of $^{10}$B(p,$α$)$^{7}$Be reaction at low energies

The $^{10}$B(p,$α$)$^{7}$Be reaction is of great interest since it has many applications in different fields of research such as nuclear astrophysics, nuclear physics, and models of new reactors for clean energy generation. This reaction has been studied at the AN2000 accelerator of the INFN National Laboratories of Legnaro (LNL). The total cross section has been measured in a wide energy range (250 $-$ 1182 keV) by using the activation method. The decays of the $^7$Be nuclei produced by the reaction were measured at the low counting facility of LNL by using two fully shielded high-purity germanium detectors. The present dataset shows a large discrepancy with respect to one of the previous data at the same energies and reduces the total uncertainty to the level of 6\%. An R-matrix calculation has been performed on the present data using the parameters from previous Trojan Horse measurements for the 10 and 500 keV resonances. The present data do not lay on the R-matrix fit in one point suggesting the existence of a $^{11}$C level not observed yet. Further nuclear investigations are needed to confirm this hypothesis.

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arXiv2016

Underground nuclear astrophysics: why and how

The goal of nuclear astrophysics is to measure cross sections of nuclear physics reactions of interest in astrophysics. At stars temperatures, these cross sections are very low due to the suppression of the Coulomb barrier. Cosmic ray induced background can seriously limit the determination of reaction cross sections at energies relevant to astrophysical processes and experimental setups should be arranged in order to improve the signal-to-noise ratio. Placing experiments in underground sites, however, reduces this background opening the way towards ultra low cross section determination. LUNA (Laboratory for Underground Nuclear Astrophysics) was pioneer in this sense. Two accelerators were mounted at the INFN National Laboratories of Gran Sasso (LNGS) allowing to study nuclear reactions close to stellar energies. A summary of the relevant technology used, including accelerators, target production and characterisation, and background treatment is given.

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arXiv2015

Three new low-energy resonances in the $^{22}$Ne(p,$γ$)$^{23}$Na reaction

The $^{22}$Ne(p,$γ$)$^{23}$Na reaction takes part in the neon-sodium cycle of hydrogen burning. This cycle affects the synthesis of the elements between $^{20}$Ne and $^{27}$Al in asymptotic giant branch stars and novae. The $^{22}$Ne(p,$γ$)$^{23}$Na reaction rate is very uncertain because of a large number of unobserved resonances lying in the Gamow window. At proton energies below 400\,keV, only upper limits exist in the literature for the resonance strengths. Previous reaction rate evaluations differ by large factors. In the present work, the first direct observations of the $^{22}$Ne(p,$γ$)$^{23}$Na resonances at 156.2, 189.5, and 259.7\,keV are reported. Their resonance strengths have been derived with 2-7\% uncertainty. In addition, upper limits for three other resonances have been greatly reduced. Data were taken using a windowless $^{22}$Ne gas target and high-purity germanium detectors at the Laboratory for Underground Nuclear Astrophysics in the Gran Sasso laboratory of the National Institute for Nuclear Physics, Italy, taking advantage of the ultra-low background observed deep underground. The new reaction rate is a factor of 5 higher than the recent evaluation at temperatures relevant to novae and asymptotic giant branch stars nucleosynthesis.

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arXiv2015

Determination of gamma-ray widths in $^{15}$N using nuclear resonance fluorescence

The stable nucleus $^{15}$N is the mirror of $^{15}$O, the bottleneck in the hydrogen burning CNO cycle. Most of the $^{15}$N level widths below the proton emission threshold are known from just one nuclear resonance fluorescence (NRF) measurement, with limited precision in some cases. A recent experiment with the AGATA demonstrator array determined level lifetimes using the Doppler Shift Attenuation Method (DSAM) in $^{15}$O. As a reference and for testing the method, level lifetimes in $^{15}$N have also been determined in the same experiment. The latest compilation of $^{15}$N level properties dates back to 1991. The limited precision in some cases in the compilation calls for a new measurement in order to enable a comparison to the AGATA demonstrator data. The widths of several $^{15}$N levels have been studied with the NRF method. The solid nitrogen compounds enriched in $^{15}$N have been irradiated with bremsstrahlung. The $γ$-rays following the deexcitation of the excited nuclear levels were detected with four HPGe detectors. Integrated photon-scattering cross sections of ten levels below the proton emission threshold have been measured. Partial gamma-ray widths of ground-state transitions were deduced and compared to the literature. The photon scattering cross sections of two levels above the proton emission threshold, but still below other particle emission energies have also been measured, and proton resonance strengths and proton widths were deduced. Gamma and proton widths consistent with the literature values were obtained, but with greatly improved precision.

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arXiv2014

A new study of the $^{22}$Ne(p,$γ$)$^{23}$Na reaction deep underground: Feasibility, setup, and first observation of the 186 keV resonance

The $^{22}$Ne(p,$γ$)$^{23}$Na reaction takes part in the neon-sodium cycle of hydrogen burning. This cycle is active in asymptotic giant branch stars as well as in novae and contributes to the nucleosythesis of neon and sodium isotopes. In order to reduce the uncertainties in the predicted nucleosynthesis yields, new experimental efforts to measure the $^{22}$Ne(p,$γ$)$^{23}$Na cross section directly at the astrophysically relevant energies are needed. In the present work, a feasibility study for a $^{22}$Ne(p,$γ$)$^{23}$Na experiment at the Laboratory for Underground Nuclear Astrophysics (LUNA) 400\,kV accelerator deep underground in the Gran Sasso laboratory, Italy, is reported. The ion beam induced $γ$-ray background has been studied. The feasibility study led to the first observation of the $E_{\rm p}$ = 186\,keV resonance in a direct experiment. An experimental lower limit of 0.12\,$\times$\,10$^{-6}$\,eV has been obtained for the resonance strength. Informed by the feasibility study, a dedicated experimental setup for the $^{22}$Ne(p,$γ$)$^{23}$Na experiment has been developed. The new setup has been characterized by a study of the temperature and pressure profiles. The beam heating effect that reduces the effective neon gas density due to the heating by the incident proton beam has been studied using the resonance scan technique, and the size of this effect has been determined for a neon gas target.

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