arXiv subjects

A. De Wit

Publications and source records attributed to A. De Wit.

5 recordsLinked to original sources

arXiv2019

Influence of mineralization and injection flow rate on flow patterns in three-dimensional porous media

Reactive flows inside porous media play an important role in a number of geophysical and industrial processes. Here we present three-dimensional experimental measurements on how precipitation and flow patterns change with the flow rate inside a model porous medium consisting of monodisperse glass beads. The sample is initially filled with an aqueous solution of sodium carbonate into which a solution of barium chloride is injected at a constant flow rate. Upon contact and reaction, the two reactants produce water-insoluble barium carbonate which precipitates onto the glass beads. This precipitate then modifies the flow morphology which in turn changes the spatial distribution of the precipitate. We discuss the influence of the flow rate on the morphology of the flow pattern and demonstrate that neither viscous fingering nor the Rayleigh-Taylor instability have any significant influence in our model system.

cond-mat.soft↗

arXiv2019

Higgs Physics at the HL-LHC and HE-LHC

The discovery of the Higgs boson in 2012, by the ATLAS and CMS experiments, was a success achieved with only a percent of the entire dataset foreseen for the LHC. It opened a landscape of possibilities in the study of Higgs boson properties, Electroweak Symmetry breaking and the Standard Model in general, as well as new avenues in probing new physics beyond the Standard Model. Six years after the discovery, with a conspicuously larger dataset collected during LHC Run 2 at a 13 TeV centre-of-mass energy, the theory and experimental particle physics communities have started a meticulous exploration of the potential for precision measurements of its properties. This includes studies of Higgs boson production and decays processes, the search for rare decays and production modes, high energy observables, and searches for an extended electroweak symmetry breaking sector. This report summarises the potential reach and opportunities in Higgs physics during the High Luminosity phase of the LHC, with an expected dataset of pp collisions at 14 TeV, corresponding to an integrated luminosity of 3 ab$^{-1}$. These studies are performed in light of the most recent analyses from LHC collaborations and the latest theoretical developments. The potential of an LHC upgrade, colliding protons at a centre-of-mass energy of 27 TeV and producing a dataset corresponding to an integrated luminosity of 15 ab$^{-1}$, is also discussed.

hep-ph↗

arXiv2018

Influence of a chemical reaction on viscous fingering: Effect of the injection flow rate

The hydrodynamic viscous fingering instability can be influenced by a simple viscosity changing chemical reaction of type A+B --> C, when a solution of reactant A is injected into a solution of B and a product C of different viscosity is formed. We investigate here numerically such reactive viscous fingering in the case of a reaction decreasing the viscosity to define the optimal conditions on the chemical and hydrodynamic parameters for controlling fingering. In particular, we analyze the influence of the injection flow rate or equivalently of the Peclet number (Pe) of the problem on the efficiency of the chemical control of fingering. We show that the viscosity decreasing reaction has an increased stabilizing effect when Pe is decreased. On the contrary, fingering is more intense and the system more unstable when Pe is increased. The related reactive fingering patterns cover then respectively a smaller (larger) area than in the non-reactive equivalent. Depending on the value of the flow rate, a given chemical reaction may thus either enhance or suppress a fingering instability. This stabilization and destabilization at low and high Pe are shown to be related to the Pe-dependent characteristics of a minimum in the viscosity profile that develops around the miscible interface thanks to the effect of the chemical reaction.

physics.flu-dyn↗

arXiv2017

Enhanced steady-state dissolution flux in reactive convective dissolution

Chemical reactions can accelerate, slow down or even be at the very origin of the development of dissolution-driven convection in partially miscible stratifications, when they impact the density profile in the host fluid phase. We numerically analyze the dynamics of this reactive convective dissolution in the fully developed non-linear regime for a phase A dissolving into a host layer containing a dissolved reactant B. We show that for a general A+B$\rightarrow$C reaction in solution, the dynamics vary with the Rayleigh numbers of the chemical species, i.e. with the nature of the chemicals in the host phase. Depending on whether the reaction slows down, accelerates or is at the origin of the development of convection, the spatial distributions of species A, B or C, the dissolution flux and the reaction rate are different. We show that chemical reactions enhance the steady-state flux as they consume A and can induce more intense convection than in the absence of reactions. This result is important in the context of CO$_2$ geological sequestration where quantifying the storage rate of CO$_2$ dissolving into the host oil or aqueous phase is crucial to assess the efficiency and the safety of the project.

physics.chem-ph↗

arXiv2014

Spiral precipitation patterns in confined chemical gardens

Chemical gardens are mineral aggregates that grow in three dimensions with plant-like forms and share properties with self-assembled structures like nano-scale tubes, brinicles or chimneys at hydrothermal vents. The analysis of their shapes remains a challenge, as their growth is influenced by osmosis, buoyancy and reaction-diffusion processes. Here we show that chemical gardens grown by injection of one reactant into the other in confined conditions feature a wealth of new patterns including spirals, flowers, and filaments. The confinement decreases the influence of buoyancy, reduces the spatial degrees of freedom and allows analysis of the patterns by tools classically used to analyze two-dimensional patterns. Injection moreover allows the study in controlled conditions of the effects of variable concentrations on the selected morphology. We illustrate these innovative aspects by characterizing quantitatively, with a simple geometrical model, a new class of self-similar logarithmic spirals observed in a large zone of the parameter space.

cond-mat.soft↗