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A. Douglas Stone

Publications and source records attributed to A. Douglas Stone.

At least 37 records · Page 2Linked to original sources

Electromagnetically induced transparency at a chiral exceptional point

Electromagnetically induced transparency, as a quantum interference effect to eliminate optical absorption in an opaque medium, has found extensive applications in slow light generation, optical storage, frequency conversion, optical quantum memory as well as enhanced nonlinear interactions at the few-photon level in all kinds of systems. Recently, there have been great interests in exceptional points, a spectral singularity that could be reached by tuning various parameters in open systems, to render unusual features to the physical systems, such as optical states with chirality. Here we theoretically and experimentally study transparency and absorption modulated by chiral optical states at exceptional points in an indirectly-coupled resonator system. By tuning one resonator to an exceptional point, transparency or absorption occurs depending on the chirality of the eigenstate. Our results demonstrate a new strategy to manipulate the light flow and the spectra of a photonic resonator system by exploiting a discrete optical state associated with specific chirality at an exceptional point as a unique control bit, which opens up a new horizon of controlling slow light using optical states. Compatible with the idea of state control in quantum gate operation, this strategy hence bridges optical computing and storage.

physics.optics↗

Theory of reflectionless scattering modes

We develop the theory of a special type of scattering state in which a set of asymptotic channels are chosen as inputs and the complementary set as outputs, and there is zero reflection back into the input channels. In general an infinite number of such solutions exist at discrete complex frequencies. Our results apply to linear electromagnetic and acoustic wave scattering and also to quantum scattering, in all dimensions, for arbitrary geometries including scatterers in free space, and for any choice of the input/output sets. We refer to such a state as reflection-zero (R-zero) when it occurs off the real-frequency axis and as an Reflectionless Scattering Mode (RSM) when it is tuned to a real frequency as a steady-state solution. Such reflectionless behavior requires a specific monochromatic input wavefront, given by the eigenvector of a filtered scattering matrix with eigenvalue zero. Steady-state RSMs may be realized by index tuning which do not break flux conservation or by gain-loss tuning. RSMs of flux-conserving cavities are bidirectional while those of non-flux-conserving cavities are generically unidirectional. Cavities with ${\cal PT}$-symmetry have unidirectional R-zeros in complex-conjugate pairs, implying that reflectionless states naturally arise at real frequencies for small gain-loss parameter but move into the complex-frequency plane after a spontaneous ${\cal PT}$-breaking transition. Numerical examples of RSMs are given for one-dimensional cavities with and without gain/loss, a ${\cal PT}$ cavity, a two-dimensional multiwaveguide junction, and a two-dimensional deformed dielectric cavity in free space. We outline and implement a general technique for solving such problems, which shows promise for designing photonic structures which are perfectly impedance-matched for specific inputs, or can perfectly convert inputs from one set of modes to a complementary set.

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Multimode Lasing in Wave-Chaotic Semiconductor Microlasers

We investigate experimentally and theoretically the lasing behavior of dielectric microcavity lasers with chaotic ray dynamics. Experiments show multimode lasing for both D-shaped and stadium-shaped wave-chaotic cavities. Theoretical calculations also find multimode lasing for different shapes, sizes and refractive indices. While there are quantitative differences between the theoretical lasing spectra of the stadium and D-cavity, due to the presence of scarred modes with anomalously high quality factors, these differences decrease as the system size increases, and are also substantially reduced when the effects of surface roughness are taken into account. Lasing spectra calculations are based on Steady-State Ab Initio Laser Theory, and indicate that gain competition is not sufficient to result in single-mode lasing in these systems.

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Perfectly absorbing exceptional points and chiral absorbers

We identify a new kind of physically realizable exceptional point (EP) corresponding to degenerate coherent perfect absorption, in which two purely incoming solutions of the wave operator for electromagnetic or acoustic waves coalesce to a single state. Such non-hermitian degeneracies can occur at a real-valued frequency without any associated noise or non-linearity, in contrast to EPs in lasers. The absorption lineshape for the eigenchannel near the EP is quartic in frequency around its maximum in any dimension. In general, for the parameters at which an operator EP occurs, the associated scattering matrix does not have an EP. However, in one dimension, when the $S$-matrix does have a perfectly absorbing EP, it takes on a universal one-parameter form with degenerate values for all scattering coefficients. For absorbing disk resonators, these EPs give rise to chiral absorption: perfect absorption for only one sense of rotation of the input wave.

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Polarization state of radiation from a photonic crystal slab

We point out that the polarization state of radiation from a photonic crystal slab is strongly constrained by the direct non-resonant scattering process. The phase difference between the two linearly-polarized components in the far field can be predicted analytically and is largely independent of the periodic pattern. We verify the prediction with full-field electromagnetic simulations.

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Correlation-enhanced control of wave focusing in disordered media

A fundamental challenge in physics is controlling the propagation of waves in disordered media despite strong scattering from inhomogeneities. Spatial light modulators enable one to synthesize (shape) the incident wavefront, optimizing the multipath interference to achieve a specific behavior such as focusing light to a target region. However, the extent of achievable control was not known when the target region is much larger than the wavelength and contains many speckles. Here we show that for targets containing more than $g$ speckles, where $g$ is the dimensionless conductance, the extent of transmission control is substantially enhanced by the long-range mesoscopic correlations among the speckles. Using a filtered random matrix ensemble appropriate for coherent diffusion in open geometries, we predict the full distributions of transmission eigenvalues as well as universal scaling laws for statistical properties, in excellent agreement with our experiment. This work provides a general framework for describing wavefront-shaping experiments in disordered systems.

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Controlling mode competition by tailoring the spatial pump distribution in a laser: A resonance-based approach

We introduce a simplified version of the steady-state ab initio laser theory for calculating the effects of mode competition in continuous wave lasers using the passive cavity resonances. This new theory harnesses widely available numerical methods that can efficiently calculate the passive cavity resonances, with negligible additional computational overhead. Using this theory, we demonstrate that the pump profile of the laser cavity can be optimized both for highly multi-mode and single-mode emission. An open source implementation of this method has been made available.

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Condensation of Thresholds in Multimode Microlasers

We show from ab initio laser theory that by choosing an appropriate spatial pump profile, many different spatial modes of a typical microlaser can be turned on at the same pump energy, substantially increasing the number, N, of simultaneous lasing modes. The optimal pump profile can be obtained simply from knowledge of the space-dependent saturated gain profile when the system is uniformly pumped up to the Nth modal threshold. We test this general result by applying it to a two-dimensional diffusive random laser and a microdisk laser. Achieving highly multimode lasing at reasonable pump powers is useful for reducing the spatial coherence of laser sources, making them suitable for use in speckle-free imaging and other applications.

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Concurrent Remote Entanglement with Quantum Error Correction

Remote entanglement of distant, non-interacting quantum entities is a key primitive for quantum information processing. We present a new protocol to remotely entangle two stationary qubits by first entangling them with propagating ancilla qubits and then performing a joint two-qubit measurement on the ancillas. Subsequently, single-qubit measurements are performed on each of the ancillas. We describe two continuous variable implementations of the protocol using propagating microwave modes. The first implementation uses propagating Schr$\rm{\ddot{o}}$dinger cat-states as the flying ancilla qubits, a joint-photon-number-modulo-2 measurement of the propagating modes for the two-qubit measurement and homodyne detections as the final single-qubit measurements. The presence of inefficiencies in realistic quantum systems limit the success-rate of generating high fidelity Bell-states. This motivates us to propose a second continuous variable implementation, where we use quantum error correction to suppress the decoherence due to photon loss to first order. To that end, we encode the ancilla qubits in superpositions of Schrödinger cat states of a given photon-number-parity, use a joint-photon-number-modulo-4 measurement as the two-qubit measurement and homodyne detections as the final single-qubit measurements. We demonstrate the resilience of our quantum-error-correcting remote entanglement scheme to imperfections. Further, we describe a modification of our error-correcting scheme by incorporating additional individual photon-number-modulo-2 measurements of the ancilla modes to improve the success-rate of generating high-fidelity Bell-states. Our protocols can be straightforwardly implemented in state-of-the-art superconducting circuit-QED systems.

quant-ph↗

Coherent control of photocurrent in a strongly scattering photoelectrochemical system

A fundamental issue that limits the efficiency of many photoelectrochemical systems is that the photon absorption length is typically much longer than the electron diffusion length. Various photon management schemes have been developed to enhance light absorption; one simple approach is to use randomly scattering media to enable broadband and wide-angle enhancement. However, such systems are often opaque, making it difficult to probe photo-induced processes. Here we use wave interference effects to modify the spatial distribution of light inside a highly-scattering dye-sensitized solar cell to control photon absorption in a space-dependent manner. By shaping the incident wavefront of a laser beam, we enhance or suppress photocurrent by increasing or decreasing light concentration on the front side of the mesoporous photoanode where the collection efficiency of photoelectrons is maximal. Enhanced light absorption is achieved by reducing reflection through the open boundary of the photoanode via destructive interference, leading to a factor of two increase in photocurrent. This approach opens the door to probing and manipulating photoelectrochemical processes in specific regions inside nominally opaque media.

physics.optics↗

Interaction-induced mode switching in steady-state microlasers

We demonstrate that due to strong modal interactions through cross-gain saturation, the onset of a new lasing mode can switch off an existing mode via a negative power slope. In this process of interaction-induced mode switching (IMS) the two involved modes maintain their identities, i.e. they do not change their spatial field patterns or lasing frequencies. For a fixed pump profile, a simple analytic criterion for the occurrence of IMS is given in terms of their self- and cross-interaction coefficients and non-interacting thresholds, which is verified for the example of a two-dimensional microdisk laser. When the spatial pump profile is varied as the pump power is increased, IMS can be induced even when it would not occur with a fixed pump profile, as we show for two coupled laser cavities. Our findings apply to steady-state lasing and are hence different from dynamical mode switching or hopping. IMS may have potential applications in robust and flexible all-optical switching.

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Remote Entanglement by Coherent Multiplication of Concurrent Quantum Signals

Concurrent remote entanglement of distant, non-interacting quantum entities is a crucial function for quantum information processing. In contrast with the existing protocols which employ addition of signals to generate entanglement between two remote qubits, the protocol we present is based on multiplication of signals. This protocol can be straightforwardly implemented by a novel Josephson junction mixing circuit. Our scheme would be able to generate provable entanglement even in presence of practical imperfections: finite quantum efficiency of detectors and undesired photon loss in current state-of-the-art devices.

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Broadband Coherent Enhancement of Transmission and Absorption in Disordered Media

We study the optimal diffusive transmission and absorption of broadband or polychromatic light in a disordered medium. By introducing matrices describing broadband transmission and reflection, we formulate an extremal eigenvalue problem where the optimal input wavefront is given by the corresponding eigenvector. We show analytically that a single wavefront can exhibit strongly enhanced total transmission or total absorption across a bandwidth that is orders of magnitude broader than the spectral correlation width of the medium, due to long-range correlations in coherent diffusion. We find excellent agreement between the analytic theory and numerical simulations.

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Why the laser linewidth is so narrow: A modern perspective

We review and interpret a modern approach to laser theory, steady-state ab initio laser theory (SALT), which treats lasing and amplification in a unified manner as a non-unitary scattering problem described by a non-linear scattering matrix. Within the semiclassical version of the theory the laser line has zero width as the lasing mode corresponds to the existence of an eigenvector of the S-matrix with diverging eigenvalue due to the occurrence of a pole of the scattering matrix on the real axis. In this approach the system is infinite from the outset and no distinction is made between cavity modes and modes of the universe; lasing modes exist both in the cavity and in the external region as solutions satisfying Sommerfeld radiation boundary conditions. We discuss how such solutions can be obtained by a limiting procedure in a finite box with damping according to the limiting absorption principle. When the electromagnetic and matter fields are treated as operators, quantum fluctuations enter the relevant correlation functions and a finite linewidth is obtained, via a generalization of SALT to include noise (N-SALT). N-SALT leads to an analytic formula for the linewidth that is more general than all previous corrected versions of the Schawlow-Townes formula, and can be evaluated simply from knowledge of the semiclassical SALT modes. We derive a simpler version of this formula which emphasizes that the noise is dominated by the fluctuations in the polarization of the gain medium and is controlled by the rate of spontaneous emission.

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Quantitative test of general theories of the intrinsic laser linewidth

We perform a first-principles calculation of the quantum-limited laser linewidth, testing the predictions of recently developed theories of the laser linewidth based on fluctuations about the known steady-state laser solutions against traditional forms of the Schawlow-Townes linewidth. The numerical study is based on finite-difference time-domain simulations of the semiclassical Maxwell-Bloch lasing equations, augmented with Langevin force terms, and thus includes the effects of dispersion, losses due to the open boundary of the laser cavity, and non-linear coupling between the amplitude and phase fluctuations ($α$ factor). We find quantitative agreement between the numerical results and the predictions of the noisy steady-state ab initio laser theory (N-SALT), both in the variation of the linewidth with output power, as well as the emergence of side-peaks due to relaxation oscillations.

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Ab-initio multimode linewidth theory for arbitrary inhomogeneous laser cavities

We present a multimode laser-linewidth theory for arbitrary cavity structures and geometries that contains nearly all previously known effects and also finds new nonlinear and multimode corrections, e.g. a bad-cavity correction to the Henry $α$ factor and a multimode Schawlow--Townes relation (each linewidth is proportional to a sum of inverse powers of all lasing modes). Our theory produces a quantitatively accurate formula for the linewidth, with no free parameters, including the full spatial degrees of freedom of the system. Starting with the Maxwell--Bloch equations, we handle quantum and thermal noise by introducing random currents whose correlations are given by the fluctuation--dissipation theorem. We derive coupled-mode equations for the lasing-mode amplitudes and obtain a formula for the linewidths in terms of simple integrals over the steady-state lasing modes.

physics.optics↗

Continuous Generation and Stabilization of Mesoscopic Field Superposition States in a Quantum Circuit

While dissipation is widely considered as being harmful for quantum coherence, it can, when properly engineered, lead to the stabilization of non-trivial pure quantum states. We propose a scheme for continuous generation and stabilization of Schrödinger cat states in a cavity using dissipation engineering. We first generate non-classical photon states with definite parity by means of a two-photon drive and dissipation, and then stabilize these transient states against single-photon decay. The single-photon stabilization is autonomous, and is implemented through a second engineered bath, which exploits the photon number dependent frequency-splitting due to Kerr interactions in the strongly dispersive regime of circuit QED. Starting with the Hamiltonian of the baths plus cavity, we derive an effective model of only the cavity photon states along with analytic expressions for relevant physical quantities, such as the stabilization rate. The deterministic generation of such cat states is one of the key ingredients in performing universal quantum computation.

quant-ph↗

Parity-Time Symmetry Breaking beyond One Dimension: The Role of Degeneracy

We consider the role of degeneracy in Parity-Time (PT) symmetry breaking for non-hermitian wave equations beyond one dimension. We show that if the spectrum is degenerate in the absence of T-breaking, and T is broken in a generic manner (without preserving other discrete symmetries), then the standard PT-symmetry breaking transition does not occur, meaning that the spectrum is complex even for infinitesimal strength of gain and loss. However the realness of the entire spectrum can be preserved over a finite interval if additional discrete symmetries X are imposed when T is broken, if X decouple all degenerate modes. When this is true only for a subset of the degenerate spectrum, there can be a partial PT transition in which this subset remains real over a finite interval of T-breaking. If the spectrum has odd-degeneracy, a fraction of the degenerate spectrum can remain in the symmetric phase even without imposing additional discrete symmetries, and they are analogous to dark states in atomic physics. These results are illustrated by the example of different T-breaking perturbations of a uniform dielectric disk and sphere, and a group theoretical analysis is given in the disk case. Finally, we show that multimode coupling is capable of restoring the T-symmetric phase at finite T-breaking. We also analyze these questions when the parity operator is replaced by another spatial symmetry operator and find that the behavior can be qualitatively different.

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