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A. Eliáš

Publications and source records attributed to A. Eliáš.

5 recordsLinked to original sources

Magnetoelastic coupling at the field-induced transition in EuAl$_{12}$O$_{19}$

Magnetoelastic coupling plays a crucial role in magnetic-field-induced transitions in anisotropic ferromagnets. Ultrasonic methods are suitable for experimental investigations of these phenomena. We investigate elastic constants in EuAl$_{12}$O$_{19}$, a quasi-two-dimensional anisotropic ferromagnet, by measuring sound velocity in magnetic fields perpendicular to spontaneous magnetization. The shear modulus $C_{44}$ exhibits dramatic softening at the field-induced transition from the ferromagnetic to a paramagnetic phase with magnetic moments forced to polarize along the applied transverse field. The softening is attributed to strong magnetic fluctuations near a second-order phase transition. Theoretical calculations based on magnetization data qualitatively reproduced the observed behavior within a strain-exchange mechanism. These results demonstrate that magnetoelastic coupling in EuAl$_{12}$O$_{19}$ arises primarily from exchange striction and provide a framework for modeling similar transitions in other anisotropic ferromagnets.

cond-mat.str-el↗

Quantum disordered ground state and relative proximity to an exactly solvable model in the frustrated magnet CeMgAl$_{11}$O$_{19}$

The magnetic properties of the triangular magnet CeMgAl$_{11}$O$_{19}$ were investigated by magnetization and specific heat measurements down to $T=0.03\,$K on single crystals grown by the floating zone method. The formation of effective spins $S_\mathrm{eff}= 1/2$ below $T < 10$\,K was confirmed both by DFT calculations and specific heat measurements. No magnetic order was found down to $T=0.03\,$K despite the formation of magnetic correlations observed in specific heat. The measured magnetization was compared with DMRG computation and their agreement supports the proposal of a strongly anisotropic magnetic interaction antiferromagnetically coupling the spin components in the $ab$ plane and ferromagnetically coupling the spin component along the $c$ axis. However, our quantitative study of the magnetization indicates a weaker proximity to quantum criticality between ferromagnetism and antiferromagnetism than the previous inelastic neutron scattering study. Finally, we propose that the absence of magnetic order in CeMgAl$_{11}$O$_{19}$ would most probably be related to the structural disorder revealed by single-crystal X-ray diffraction.

cond-mat.str-el↗

Induced quantum magnetism on a triangular lattice of non-Kramers ions in PrMgAl11O19

We report the magnetic properties of the quantum triangular lattice antiferromagnet (TLAF) PrMgAl11O19 through magnetization and specific heat measurements. Strong magnetic anisotropy indicates the realization of an Ising-like magnetism in PrMgAl11O19 single crystal while no long-range magnetic ordering is realized down to 0.4 K. The splitting of the low-lying quasi-doublet into two singlets suggested by experimental data, is consistent with an effective pseudospin-1/2 scenario. The observed gapless excitations in zero field are attributed to induced quantum magnetism, they would be induced by magnetic interactions of an energy scale comparable with the splitting between the two singlets. Based on these results, we modeled the magnetic ground state of PrMgAl11O19 by a quantum Ising magnet with an intrinsic transverse field rather than a quantum spin liquid (QSL). In addition, our data show a non-monotonous response of the low-temperature specific heat to the external fields revealing a complex interplay between intrinsic and external magnetic fields.

cond-mat.str-el↗

A frustrated antipolar phase analogous to classical spin liquids

The study of magnetic frustration in classical spin systems was motivated by the prediction and discovery of classical spin liquid states. These uncommon magnetic phases are characterized by a massive degeneracy of their ground state implying a finite magnetic entropy at zero temperature. While the classical spin liquid state was originally predicted in the Ising triangular lattice antiferromagnet in 1950, this state has never been experimentally observed in any triangular magnets. We report here the discovery of an electric analogue of classical spin liquids on a triangular lattice of uniaxial electric dipoles in EuAl12O19 . This new type of frustrated antipolar phase is characterized by a highly degenerate state at low temperature implying an absence of long-range antiferroelectric order, despite short-range antipolar correlations. Its dynamics are governed by a thermally activated process, slowing down upon cooling towards a complete freezing at zero temperature.

cond-mat.str-el↗

Quasi-two-dimensional ferromagnetism in the triangular magnet EuAl$_{12}$O$_{19}$

We report ferromagnetic ordering at $T_\mathrm {C}=1.3\,$K in the quasi-two dimensional magnet EuAl$_{12}$O$_{19}$ with large spins $S=7/2$. This ferromagnetic state was characterized by magnetization and specific heat measurements and the experimental results were compared with classical Monte Carlo simulations. They reveal a strong single ion anisotropy leading to an uniaxial spontaneous magnetization along the $c$ axis. Furthermore the application of a magnetic field in the hard magnetization plane $ab$ reduces the Curie temperature and it reaches zero temperature at a magnetic field of $μ_\mathrm{0} H_c \approx 0.5\,$T.

cond-mat.str-el↗