arXiv subjects

A. Fang

Publications and source records attributed to A. Fang.

12 recordsLinked to original sources

arXiv2022

Direct observation of discommensurate charge density wave modulation in the quasi-1D Weyl semimetal candidate NbTe$_4$

The transition-metal tetrachalcogenides are a model system to explore the conjunction of correlated electronic states such as charge density waves (CDW), with topological phases of matter. Understanding the connection between these phases requires a thorough understanding of the individual states, which for the case of the CDW in this system, is still missing. In this paper we combine phonon-structure calculations and scanning tunneling microscopy measurements of NbTe$_4$ in order to provide a full characterization of the CDW state. We find that, at short range, the superstructure formed by the CDW is fully commensurate with the lattice parameters. Moreover, our data reveals the presence of phase-slip domain-walls separating regions of commensurate-CDW in the nanoscale, indicating that the CDW in this compound is discommensurate at long-range. Our results solve a long-standing discussion about the nature of the CDW in these materials, and provide a strong basis for the study of the interplay between this state and other novel quantum electronic states.

cond-mat.mtrl-sci↗

arXiv2020

Characterization of magnetic field noise in the ARIADNE source mass rotor

ARIADNE is a nuclear-magnetic-resonance-based experiment that will search for novel axion-induced spin-dependent interactions between an unpolarized source mass rotor and a nearby sample of spin-polarized $^3$He gas. To detect feeble axion signals at the sub-atto-Tesla level, the experiment relies on low magnetic background and noise. We measure and characterize the magnetic field background from a prototype tungsten rotor. We show that the requirement is met with our current level of tungsten purity and demagnetization process. We further show that the noise is dominantly caused by a few discrete dipoles, likely due to a few impurities trapped inside the rotor during manufacturing. This is done via a numerical optimization pipeline which fits for the locations and magnetic moments of each dipole. We find that under the current demagnetization, the magnetic moment of trapped impurities is bounded at $10^{-9} \mathrm{A}\mathrm{m}^2$.

physics.ins-det↗

arXiv2020

Ion transport across solid-state ion channels perturbed by directed strain

We combine quantum-chemical calculations and molecular dynamics simulations to consider aqueous ion flow across non-axisymmetric nanopores in monolayer graphene and MoS$_2$. When the pore-containing membrane is subject to uniaxial tensile strains applied in various directions, the corresponding permeability exhibits considerable directional dependence. This anisotropy is shown to arise from directed perturbations of the local electrostatics by the corresponding pore deformation, as enabled by the pore edge geometries and atomic compositions. By considering nanopores with ionic permeability that depends on the strain direction, we present model systems that may yield a detailed understanding of the structure-function relationship in solid-state and biological ion channels. Specifically, the observed anisotropic effects potentially enable the use of permeation measurements across strained membranes to obtain directional profiles of ion-pore energetics as contributed by groups of atoms or even individual atoms at the pore edge. The resulting insight may facilitate the development of subnanoscale pores with novel functionalities arising from locally asymmetric pore edge features.

physics.app-ph↗

arXiv2019

Non-Universal Critical Behaviors in Disordered Pseudospin-1 Systems

It is well known that for ordinary one-dimensional (1D) disordered systems, the Anderson localization length $ξ$ diverges as $λ^m$ in the long wavelength limit ($λ\rightarrow \infty$ ) with a universal exponent $m=2$, independent of the type of disorder. Here, we show rigorously that pseudospin-1 systems exhibit non-universal critical behaviors when they are subjected to 1D random potentials. In such systems, we find that $ξ\propto λ^m$ with $m$ depending on the type of disorder. For binary disorder, $m=6$ and the fast divergence is due to a super-Klein-tunneling effect (SKTE). When we add additional potential fluctuations to the binary disorder, the critical exponent $m$ crosses over from 6 to 4 as the wavelength increases. Moreover, for disordered superlattices, in which the random potential layers are separated by layers of background medium, the exponent $m$ is further reduced to 2 due to the multiple reflections inside the background layer. To obtain the above results, we developed a new analytic method based on a stack recursion equation. Our analytical results are in excellent agreements with the numerical results obtained by the transfer-matrix method (TMM). For pseudospin-1/2 systems, we find both numerically and analytically that $ξ\proptoλ^2$ for all types of disorder, same as ordinary 1D disordered systems. Our new analytical method provides a convenient way to obtain easily the critical exponent $m$ for general 1D Anderson localization problems.

cond-mat.dis-nn↗

arXiv2019

Mechanosensitive ion permeation across sub-nanoporous MoS$_2$ monolayers

We use all-atom molecular dynamics simulations informed by density functional theory calculations to investigate aqueous ion transport across sub-nanoporous monolayer molybdenum disulfide (MoS$_2$) membranes subject to varying tensile strains. Driven by a transmembrane electric field, highly mechanosensitive permeation of both anions and cations is demonstrated in membranes featuring certain pore structures. For pores that are permeable when unstrained, we demonstrate ion current modulation by a factor of over 20 in the tensile strain range of 0 - 4%. For unstrained pores that are impermeable, a clear strain-induced onset of permeability is demonstrated within the same range of strains. The underlying mechanism is shown to be a strain-induced reduction of the generally repulsive ion-pore interactions resulting from the ions' short-range interactions with the atoms in the pore interior and desolvation effects. The mechanosensitive pores considered in this work gain their electrostatic properties from the pore geometries and in principle do not require additional chemical functionalization. Here we propose the possibility of a new class of mechanosensitive nanoporous materials with permeation properties determined by the targeted engineering of vacancy defects.

physics.app-ph↗

arXiv2016

Klein tunneling and supercollimation of pseudospin-1 electromagnetic waves

Pseudospin plays a central role in many novel physical properties of graphene and other artificial systems which have pseudospins of 1/2. Here we show that in certain photonic crystals (PCs) exhibiting conical dispersions at k = 0, the eigenmodes near the "Dirac-like point" can be described by an effective spin-orbit Hamiltonian with a pseudospin of 1, treating wave propagations in the upper cone, the lower cone and a flat band (corresponding to zero refractive index) within a unified framework. The 3-component spinor gives rise to boundary conditions distinct from those of pseudospin-1/2, leading to new wave transport behaviors as manifested in Klein tunneling and supercollimation. For example, collimation can be realized more easily with pseudospin-1 than pseudospin-1/2. The special wave scattering properties of pseudospin-1 photons, coupled with the discovery that the effective photonic "potential" can be varied by a simple change of length scale, may offer new ways to control photon transport.

physics.optics↗

arXiv2009

STM imaging of electronic waves on the surface of Bi$_2$Te$_3$: topologically protected surface states and hexagonal warping effects

Scanning tunneling spectroscopy studies on high-quality Bi$_2$Te$_3$ crystals exhibit perfect correspondence to ARPES data, hence enabling identification of different regimes measured in the local density of states (LDOS). Oscillations of LDOS near a step are analyzed. Within the main part of the surface band oscillations are strongly damped, supporting the hypothesis of topological protection. At higher energies, as the surface band becomes concave, oscillations appear which disperse with a particular wave-vector that may result from an unconventional hexagonal warping term.

cond-mat.str-el↗

arXiv2009

Self-consistent calculation of metamaterials with gain

We present a computational scheme allowing for a self-consistent treatment of a dispersive metallic photonic metamaterial coupled to a gain material incorporated into the nanostructure. The gain is described by a generic four-level system. A critical pumping rate exists for compensating the loss of the metamaterial. Nonlinearities arise due to gain depletion beyond a certain critical strength of a test field. Transmission, reflection, and absorption data as well as the retrieved effective parameters are presented for a lattice of resonant square cylinders embedded in layers of gain material and split ring resonators with gain material embedded into the gaps.

physics.optics↗

arXiv2007

STM Studies of TbTe3: Evidence for a fully Incommensurate Charge Density Wave

We observe unidirectional charge density wave ordering on the cleaved surface of TbTe3 with a Scanning Tunneling Microscope at ~6 K. The modulation wave-vector q_{CDW} as determined by Fourier analysis is 0.71 +/- 0.02 * 2 pi/c. (Where c is one edge of the in-plane 3D unit cell.) Images at different tip-sample voltages show the unit cell doubling effects of dimerization and the layer below. Our results agree with bulk X-ray measurements, with the addition of ~(1/3) * 2 pi/a ordering perpendicular to the CDW. Our analysis indicates that the CDW is incommensurate.

cond-mat.other↗

arXiv2006

Inferring effective interactions from the local density of states: application to STM data from Bi$_2$Sr$_2$CaCu$_2$O$_{8+δ}$

While the influence of impurities on the local density of states (LDOS) in a metal is notoriously non-local due to interference effects, low order moments of the LDOS in general can be shown to depend only on the local structure of the Hamiltonian. Specifically, we show that an analysis of the spatial variations of these moments permits one to ``work backwards'' from scanning tunneling microscopy (STM) data to infer the local structure of the underlying effective Hamiltonian. Applying this analysis to STM data from the high temperature superconductor, Bi$_2$Sr$_2$CaCu$_2$O$_{8+δ}$, we find that the variations of the electro-chemical potential are remarkably small (i.e., the disorder is, in a sense, weak) but that there are large variations in the local magnitude of the d-wave gap parameter.

cond-mat.supr-con↗

arXiv2004

STM Studies of Near-Optimal Doped Bi$_2$Sr$_2$CaCu$_2$O$_{8+δ}$

In this paper we summarize our STM studies of the density of electronic states in nearly optimally doped Bi$_2$Sr$_2$CaCu$_2$O$_{8+δ}$ in zero field. We report on the inhomogeneity of the gap structure, density of states modulations with four-lattice constant period, and coherence peak modulation.

cond-mat.supr-con↗

arXiv2004

Periodic Coherence Peak Height Modulations in Superconducting BSCCO

In this paper we analyze, using scanning tunneling spectroscopy (STS), the local density of electronic states (LDOS) in nearly optimally doped BSCCO in zero field. We see both dispersive and non-dispersive spatial LDOS modulations as a function of energy in our samples. Moreover, a spatial map of the superconducting coherence peak heights shows the same structure as the low energy LDOS. This suggests that these non-dispersive LDOS modulations originate from an underlying charge-density modulation which interacts with superconductivity.

cond-mat.supr-con↗