arXiv subjects

A. Fuente

Publications and source records attributed to A. Fuente.

At least 55 records · Page 3Linked to original sources

arXiv2022

H2CS deuteration maps towards the pre-stellar core L1544

Deuteration is a crucial tool to understand the complexity of interstellar chemical processes, especially when they involve the interplay of gas-phase and grain-surface chemistry. In the case of multiple deuteration, comparing observation with the results of chemical modelling is particularly effective to study how molecules are inherited in the different stages within the process of star and planet formation. We aim to study the the D/ H ratio in H2CS across the prototypical pre-stellar core L1544. This study allows us to test current gas-dust chemical models involving sulfur in dense cores. We present here single-dish observations of H2CS, HDCS and D2CS with the IRAM 30m telescope. We analyse their column densities and distributions, and compare these observations with gas-grain chemical models. The deuteration maps of H2CS in L1544 are compared with the deuteration maps of methanol, H2CO, N2H+ and HCO+ towards the same source. Furthermore, the single and double deuteration of H2CS towards the dust peak of L1544 is compared with H2CO and c-C3H2. The difference between the deuteration of these molecules in L1544 is discussed and compared with the prediction of chemical models. The maximum deuterium fractionation for the first deuteration of H2CS is N(HDCS)/N(H2CS)$\sim$30$\%$ and is located towards the north-east at a distance of about 10000 AU from the dust peak. While for c-C3H2 the first and second deuteration have a similar efficiency, for H2CS and H2CO the second deuteration is more efficient, leading to D2CX/HDCX$\sim$100$\%$ (with X= O or S). Our results imply that the large deuteration of H2CO and H2CS observed in protostellar cores as well as in comets is likely inherited from the pre-stellar phase. However, the comparison with state-of-the-art chemical models suggests that the reaction network for the formation of the doubly deuterated H2CS and H2CO it is not complete yet.

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arXiv2022

The chemical footprint of AGN feedback in the outflowing circumnuclear disk of NGC 1068

In the nearby (D=14 Mpc) AGN-starburst composite galaxy NGC 1068, it has been found that the molecular gas in the Circum-nuclear Disk (CND) is outflowing, which is a manifestation of ongoing AGN feedback. The outflowing gas has a large spread of velocities, which likely drive different shock chemistry signatures at different locations in the CND. We perform a multi-line molecular study using two shock tracers, SiO and HNCO, with the aim to determine the gas properties traced by these two species, and explore the possibility of reconstructing the shock history in the CND. Five SiO transitions and three HNCO transitions were imaged at high resolution $0''.5-0''.8$ with the Atacama Large Millimeter/submillimeter Array (ALMA). We performed both LTE and non-LTE radiative transfer analysis coupled with Bayesian inference process in order to characterize the gas properties, such as molecular gas density and gas temperature. We found clear evidence of chemical differentiation between SiO and HNCO, with the SiO/HNCO ratio ranging from greater than one on the east of CND to lower than one on the west side. The non-LTE radiative transfer analysis coupled with Bayesian inference confirms that the gas traced by SiO has different densities - and possibly temperatures - than that traced by HNCO. We find that SiO traces gas affected by fast shocks while the gas traced by HNCO is either just affected by slow shocks or not shocked at all. A distinct differentiation between SiO and HNCO has been revealed in our observations and the further analysis of the gas properties traced by both species, which confirms the results from previous chemical modelings.

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arXiv2022

Spatially resolved star-formation relations of dense molecular gas in NGC 1068

We analyse the influence of the dynamical environment on the star formation (SF) relations of the dense molecular gas in the starburst (SB) ring of the Seyfert 2 galaxy NGC 1068. We used ALMA to image the emission of the 1-0 transitions of HCN and HCO+ with a resolution of 56 pc. We also used ancillary data of CO(1-0) at a resolution of ~100 pc, and CO(3-2) and its underlying continuum emission at ~40 pc. These observations allow us to probe a range of molecular gas densities (n(H2)~10$^{3-5}cm^{-3}$). The SF rate (SFR) is derived from Pa$α$ line emission imaged by HST/NICMOS. We analysed how SF relations change depending on the choice of aperture sizes and molecular gas tracer. The scatter in the Kennicutt-Schmidt relation is about a factor of two to three lower for the HCN and HCO+ lines compared to CO(1-0) for a common aperture. Correlations lose statistical significance below a critical spatial scale $\approx$300-400 pc. The SF efficiency of the dense molecular gas (SFEdense) shows a scattered distribution as a function of the HCN luminosity (L'(HCN)) around a mean value of $\simeq0.01$Myr$^{-1}$. An alternative prescription for SF relations, linking the SFEdense and the boundedness of the gas measured by the parameter b$\equivΣ$dense/$σ^2$, where $Σ$dense is the dense molecular gas surface density and $σ$ the velocity dispersion, resolves the degeneracy associated with the SFEdense-L'(HCN) plot. We identify two branches in the SFEdense-b plot that correspond to two dynamical environments in the SB ring, which are defined by their proximity to the bar-ring interface region. This region corresponds to the crossing of two density wave resonances, where an increased rate of cloud-cloud collisions would favour an enhanced compression of molecular gas. Our results suggest that galactic dynamics plays a major role in the efficiency of the gas conversion into stars.

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arXiv2021

Photoprocessing of H2S on dust grains: building S chains in translucent clouds and comets

Context. Sulfur is used as a tracer of the evolution from interstellar clouds to stellar systems. However, most of the expected sulfur in molecular clouds remains undetected. Sulfur disappears from the gas phase in two steps. One first depletion occurs during the translucent phase, reducing the gas phase sulfur by 7-40 times, while the following freeze-out step occurs in molecular clouds, reducing it by another order of magnitude. This long-standing dilemma awaits an explanation. Aims. The aim of this study is to understand under which form the missing sulfur is hiding in molecular clouds. Depletion onto dust grains is considered. Methods. Experimental simulations mimicking H2S ice UV-photoprocessing in molecular clouds were conducted. The ice was monitored using infrared spectroscopy and the desorbing molecules were measured by quadrupole mass spectrometry. Theoretical Monte Carlo simulations were performed for interpretation of the experimental results and extrapolation to astrophysical conditions. Results. H2S2 formation was observed during irradiation at 8 K. Molecules H2Sx with x > 2 were also identified and found to desorb during warm-up, along with S2 to S4 species. Larger Sx molecules up to S8 are refractory at room temperature and remained on the substrate forming a residue. Monte Carlo simulations were able to reproduce the molecules desorbing during warming up, and found that residues are chains or sulfur consisting of 6-7 atoms. Conclusions. We propose that S+ in translucent clouds contributes notoriously to S depletion in denser regions by forming long S-chains on dust in few times 10^4 years. We suggest that the S2 to S4 molecules observed in comets are not produced by fragmentation of these large chains. Instead, they probably come either from UV-photoprocessing of H2S-bearing ice produced in molecular clouds or from short S chains formed during the translucent cloud phase

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arXiv2021

Gas phase Elemental abundances in Molecular cloudS (GEMS) V. Methanol in Taurus

Methanol, one of the simplest complex organic molecules in the Interstellar Medium (ISM), has been shown to be present and extended in cold environments such as starless cores. We aim at studying methanol emission across several starless cores and investigate the physical conditions at which methanol starts to be efficiently formed, as well as how the physical structure of the cores and their surrounding environment affect its distribution. Methanol and C$^{18}$O emission lines at 3 mm have been observed with the IRAM 30m telescope within the large program "Gas phase Elemental abundances in Molecular CloudS" (GEMS) towards 66 positions across 12 starless cores in the Taurus Molecular Cloud. A non-LTE radiative transfer code was used to compute the column densities in all positions. We then used state-of-the-art chemical models to reproduce our observations. We have computed N(CH$_3$OH)/N(C$^{18}$O) column density ratios for all the observed offsets, and two different behaviours can be recognised: the cores where the ratio peaks at the dust peak, and the cores where the ratio peaks with a slight offset with respect to the dust peak ($\sim $10000 AU). We suggest that the cause of this behaviour is the irradiation on the cores due to protostars nearby which accelerate energetic particles along their outflows. The chemical models, which do not take into account irradiation variations, can reproduce fairly well the overall observed column density of methanol, but cannot reproduce the two different radial profiles observed. We confirm the substantial effect of the environment onto the distribution of methanol in starless cores. We suggest that the clumpy medium generated by protostellar outflows might cause a more efficient penetration of the interstellar radiation field in the molecular cloud and have an impact on the distribution of methanol in starless cores.

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arXiv2021

Probing the kinematics and chemistry of the hot core Mon R 2 IRS 3 using ALMA observations

We present high angular resolution 1.1mm continuum and spectroscopic ALMA observations of the well-known massive proto-cluster Mon R 2 IRS 3.The continuum image at 1.1mm shows two components, IRS 3 A and IRS 3 B, that are separated by $\sim$0.65$"$. We estimate that IRS 3 A is responsible of $\sim$80 % of the continuum flux, being the most massive component. We explore the chemistry of IRS 3 A based on the spectroscopic observations. In particular, we have detected intense lines of S-bearing species such as SO, SO$_2$, H$_2$CS and OCS, and of the Complex Organic Molecules (COMs) methyl formate (CH$_3$OCHO) and dimethyl ether (CH$_3$OCH$_3$). The integrated intensity maps of most species show a compact clump centered on IRS 3 A, except the emission of the COMs that is more intense towards the near-IR nebula located to the south of IRS 3 A, and HC$_3$N whose emission peak is located $\sim$0.5$"$ NE from IRS 3 A. The kinematical study suggests that the molecular emission is mainly coming from a rotating ring and/or an unresolved disk. Additional components are traced by the ro-vibrational HCN $ν_2$=1 3$\rightarrow$2 line which is probing the inner disk/jet region, and the weak lines of CH$_3$OCHO, more likely arising from the walls of the cavity excavated by the molecular outflow. Based on SO$_2$ we derive a gas kinetic temperature of T$_k$$\sim$ 170 K towards the IRS 3 A. The most abundant S-bearing species is SO$_2$ with an abundance of $\sim$ 1.3$\times$10$^{-7}$, and $χ$(SO/SO$_2$) $\sim$ 0.29. Assuming the solar abundance, SO$_2$ accounts for $\sim$1 % of the sulphur budget.

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arXiv2021

H$_2$S observations in young stellar disks in Taurus

Context. Studying gas chemistry in protoplanetary disks is key to understanding the process of planet formation. Sulfur chemistry in particular is poorly understood in interstellar environments, and the location of the main reservoirs remains unknown. Protoplanetary disks in Taurus are ideal targets for studying the evolution of the composition of planet forming systems. Aims. We aim to elucidate the chemical origin of sulfur-bearing molecular emission in protoplanetary disks, with a special focus on H$_2$S emission, and to identify candidate species that could become the main molecular sulfur reservoirs in protoplanetary systems. Methods. We used IRAM 30m observations of nine gas-rich young stellar objects (YSOs) in Taurus to perform a survey of sulfur-bearing and oxygen-bearing molecular species. In this paper we present our results for the CS 3-2 ($ν_0$ = 146.969 GHz), H$_2$CO 2$_{11}$-1$_{10}$ ($ν_0$ = 150.498 GHz), and H$_2$S 1$_{10}$-1$_{01}$ ($ν_0$ = 168,763 GHz) emission lines. Results. We detected H$_2$S emission in four sources out of the nine observed, significantly increasing the number of detections toward YSOs. We also detected H$_2$CO and CS in six out of the nine. We identify a tentative correlation between H$_2$S 1$_{10}$-1$_{01}$ and H$_2$CO 2$_{11}$-1$_{10}$ as well as a tentative correlation between H$_2$S 1$_{10}$-1$_{01}$ and H$_2$O 8$_{18}$-7$_{07}$. By assuming local thermodynamical equilibrium, we computed column densities for the sources in the sample, with N(o-H$_2$S) values ranging between $2.6\times10^{12}$ cm$^{-2}$ and $1.5\times10^{13}$ cm$^{-2}$.

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arXiv2021

Evolutionary view through the starless cores in Taurus: deuteration in TMC 1-C and TMC 1-CP

The chemical and physical evolution of starless and pre-stellar cores are of paramount importance to understanding the process of star formation. The Taurus Molecular Cloud cores TMC 1-C and TMC 1-CP share similar initial conditions and provide an excellent opportunity to understand the evolution of the pre-stellar core phase. We investigated the evolutionary stage of starless cores based on observations towards the prototypical dark cores TMC 1-C and TMC 1-CP, mapping them in the CS $3\rightarrow 2$, C$^{34}$S $3\rightarrow 2$, $^{13}$CS $2\rightarrow 1$, DCN $1\rightarrow 0$, DCN $2\rightarrow 1$, DNC $1\rightarrow 0$, DNC $2\rightarrow 1$, DN$^{13}$C $1\rightarrow 0$, DN$^{13}$C $2\rightarrow 1$, N$_2$H$^+$ $1\rightarrow 0$, and N$_2$D$^+$ $1\rightarrow 0$ transitions. We performed a multi-transitional study of CS and its isotopologs, DCN, and DNC lines to characterize the physical and chemical properties of these cores. We studied their chemistry using the state-of-the-art gas-grain chemical code Nautilus and pseudo time-dependent models to determine their evolutionary stage. Observational diagnostics seem to indicate that TMC 1-C is in a later evolutionary stage than TMC 1-CP, with a chemical age $\sim$1 Myr. TMC 1-C shows signs of being an evolved core at the onset of star formation, while TMC 1-CP appears to be in an earlier evolutionary stage due to a more recent formation or, alternatively, a collapse slowed down by a magnetic support.

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arXiv2021

Efficiency of non-thermal desorptions in cold-core conditions. Testing the sputtering of grain mantles induced by cosmic rays

Under cold conditions in dense cores, gas-phase molecules and atoms are depleted from the gas-phase to the surface of interstellar grains. Considering the time scales and physical conditions within these cores, a portion of these molecules has to be brought back into the gas-phase to explain their observation by milimeter telescopes. We tested the respective efficiencies of the different mechanisms commonly included in the models. We also tested the addition of sputtering of ice grain mantles via a collision with cosmic rays in the electronic stopping power regime. The ice sputtering induced by cosmic rays has been added to the Nautilus gas-grain model while the other processes were already present. Each of these processes were tested on a 1D physical structure determined by observations in TMC1 cold cores. The resulting 1D chemical structure was also compared to methanol gas-phase abundances observed in these cores. We found that all species are not sensitive in the same way to the non-thermal desorption mechanisms, and the sensitivity also depends on the physical conditions. Thus, it is mandatory to include all of them. Chemical desorption seems to be essential in reproducing the observations for H densities smaller than $4\times 10^4$~cm$^{-3}$, whereas sputtering is essential above this density. The models are, however, systematically below the observed methanol abundances. A more efficient chemical desorption and a more efficient sputtering could better reproduce the observations. In conclusion, the sputtering of ices by cosmic-rays collisions may be the most efficient desorption mechanism at high density (a few $10^4$~cm$^{-3}$ under the conditions studied here) in cold cores, whereas chemical desorption is still required at smaller densities. Additional works are needed on both mechanisms to assess their efficiency with respect to the main ice composition.

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arXiv2021

Gas phase Elemental abundances in Molecular cloudS (GEMS). IV. Observational results and statistical trends

Gas phase Elemental abundances in Molecular CloudS (GEMS) is an IRAM 30m Large Program designed to estimate the S, C, N, and O depletions and gas ionization degree, X(e-), in a set of star-forming filaments of Taurus, Perseus and Orion. Our immediate goal is to build up a complete database of molecular abundances that can serve as an observational basis for estimating X(e-) and the C, O, N, and S depletions through chemical modeling. We observed and derived the abundances of 14 species (13CO, C18O, HCO+, H13CO+, HC18O+, HCN, H13CN, HNC, HCS+, CS, SO, 34SO, H2S, and OCS) in 244 positions, covering the AV 3 to 100 mag, n(H2) a few 10$^{3}$ to 10$^6$ cm$^{-3}$, and Tk 10 to 30 K ranges in these clouds, avoiding protostars, HII regions, and outflows. A statistical analysis is carried out to identify general trends between different species and with physical parameters. Relations between molecules reveal strong linear correlations which define three different families: (1) 13CO and C18O; (2) H13CO+, HC18O+, H13CN, and HNC; and (3) the S-bearing molecules. The abundances of the CO isotopologs increase with the gas kinetic temperature until TK 15 K. For higher temperatures, the abundance remains constant with a scatter of a factor of 3. The abundances of H13CO+, HC18O+, H13CN, and HNC are well correlated with each other, and all of them decrease with molecular hydrogen density, following the law n(H2)$^{-0.8\pm0.2}$. The abundances of S-bearing species also decrease with n(H2) at a rate of (S-bearing/H)gas n(H2)$^{-0.6\pm0.1}$. The abundances of molecules belonging to groups 2 and 3 do not present any clear trend with gas temperature. At scales of molecular clouds, the C18O abundance is the quantity that better correlates with the cloud mass. We discuss the utility of the 13CO/C18O, HCO+/H13CO+, and H13CO+/H13CN abundance ratios as chemical diagnostics of star formation in external galaxies.

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arXiv2021

Bottlenecks to interstellar sulfur chemistry: Sulfur-bearing hydrides in UV-illuminated gas and grains

Hydride molecules lie at the base of interstellar chemistry, but the synthesis of sulfuretted hydrides is poorly understood. Motivated by new observations of the Orion Bar PDR - 1'' resolution ALMA images of SH+; IRAM 30m detections of H2S, H2S34, and H2S33; H3S+ (upper limits); and SOFIA observations of SH - we perform a systematic study of the chemistry of S-bearing hydrides. We determine their column densities using coupled excitation, radiative transfer as well as chemical formation and destruction models. We revise some of the key gas-phase reactions that lead to their chemical synthesis. This includes ab initio quantum calculations of the vibrational-state-dependent reactions SH+ + H2 <-> H2S+ + H and S + H2 <-> SH + H. We find that reactions of UV-pumped H2 (v>1) with S+ explain the presence of SH+ in a high thermal-pressure gas component, P_th~10^8 cm^-3 K, close to the H2 dissociation front. However, subsequent hydrogen abstraction reactions of SH+, H2S+, and S with vibrationally excited H2, fail to ultimately explain the observed H2S column density (~2.5x10^14 cm^-2, with an ortho-to-para ratio of 2.9+/-0.3). To overcome these bottlenecks, we build PDR models that include a simple network of grain surface reactions leading to the formation of solid H2S (s-H2S). The higher adsorption binding energies of S and SH suggested by recent studies imply that S atoms adsorb on grains (and form s-H2S) at warmer dust temperatures and closer to the UV-illuminated edges of molecular clouds. Photodesorption and, to a lesser extent, chemical desorption, produce roughly the same H2S column density (a few 10^14 cm-^2) and abundance peak (a few 10^-8) nearly independently of n_H and G_0. This agrees with the observed H2S column density in the Orion Bar as well as at the edges of dark clouds without invoking substantial depletion of elemental sulfur abundances.

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arXiv2021

Evidence of galaxy interaction in the Narrow-line Seyfert 1 galaxy IRAS17020+4544 seen by NOEMA

The narrow-line Seyfert 1 galaxy IRAS17020+4544 is one of the few sources where both an X-ray ultra-fast outflow and a molecular outflow were observed to be consistent with energy conservation. However, IRAS17020+4544 is less massive and has a much more modest active galactic nucleus (AGN) luminosity than the other examples. Using recent CO(1-0) observations with the NOrthern Extended Millimeter Array (NOEMA), we characterised the molecular gas content of the host galaxy for the first time. We found that the molecular gas is distributed into an apparent central disc of 1.1x10^9 Msun, and a northern extension located up to 8 kpc from the centre with a molecular gas mass M_H2~10^8 Msun. The molecular gas mass and the CO dynamics in the northern extension reveal that IRAS 17020+4544 is not a standard spiral galaxy, instead it is interacting with a dwarf object corresponding to the northern extension. This interaction possibly triggers the high accretion rate onto the super massive black hole. Within the main galaxy, which hosts the AGN, a simple analytical model predicts that the molecular gas may lie in a ring, with less molecular gas in the nuclear region. Such distribution may be the result of the AGN activity which removes or photodissociates the molecular gas in the nuclear region (AGN feedback). Finally, we have detected a molecular outflow of mass M_H2=(0.7-1.2)x10^7 Msun in projection at the location of the northern galaxy, with a similar velocity to that of the massive outflow reported in previous millimeter data obtained by the Large Millimeter Telescope.

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arXiv2020

Gas-phase Elemental abundances in Molecular cloudS (GEMS) III. Unlocking the CS chemistry: the CS+O reaction

CS is among the most abundant gas-phase S-bearing molecules in cold dark molecular clouds. It is easily observable with several transitions in the millimeter wavelength range, and has been widely used as a tracer of the gas density in the interstellar medium in our Galaxy and external galaxies. Chemical models fail to account for the observed CS abundances when assuming the cosmic value for the elemental abundance of sulfur. The CS+O -> CO + S reaction has been proposed as a relevant CS destruction mechanism at low temperatures, and could explain the discrepancy between models and observations. Its reaction rate has been experimentally measured at temperatures of 150-400 K, but the extrapolation to lower temperatures is doubtful. Here we calculate the CS+O reaction rate at temperatures <150 K which are prevailing in the interstellar medium. We performed ab initio calculations to obtain the three lowest PES of the CS+O system. These PESs are used to study the reaction dynamics, using several methods to eventually calculate the CS+O thermal reaction rates. We compare the results of our theoretical calculations for 150-400 K with those obtained in the laboratory. Our detailed theoretical study on the CS+O reaction, which is in agreement with the experimental data obtained at 150-400 K, demonstrates the reliability of our approach. After a careful analysis at lower temperatures, we find that the rate constant at 10 K is negligible, which is consistent with the extrapolation of experimental data using the Arrhenius expression. We use the updated chemical network to model the sulfur chemistry in TMC1 based on molecular abundances determined from GEMS project observations. In our model, we take into account the expected decrease of the cosmic ray ionization rate along the cloud. The abundance of CS is still overestimated when assuming the cosmic value for the sulfur abundance.

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arXiv2020

ALMA observations of CS in NGC 1068: chemistry and excitation

We present results from Atacama Large Millimeter/submillimeter Array (ALMA) observations of CS from the nearby galaxy NGC 1068 ($\sim14$ Mpc). This Seyfert 2 barred galaxy possesses a circumnuclear disc (CND, $r\sim200$ pc) and a starburst ring (SB ring, $r\sim1.3$ kpc). These high-resolution maps ($\sim0.5$", $\sim35$ pc) allow us to analyse specific sub-regions in the galaxy and investigate differences in line intensity ratios and physical conditions, particularly those between the CND and SB ring. Local thermodynamic equilibrium (LTE) analysis of the gas is used to calculate CS densities in each sub-region, followed by non-LTE analysis conducted using the radiative transfer code RADEX to fit observations and constrain gas temperature, CS column density and hydrogen density. Finally, the chemical code UCLCHEM is used to reconstruct the gas, allowing an insight into its origin and chemical history. The density of hydrogen in the CND is found to be $\geq10^5$ cm$^{-2}$, although exact values vary, reaching $10^6$ cm$^{-2}$ at the AGN. The conditions in the two arms of the SB ring appear similar to one another, though the density found ($\sim10^4$ cm$^{-2}$) is lower than in the CND. The temperature in the CND increases from east to west, and is also overall greater than found in the SB ring. These modelling methods indicate the requirement for multi-phase gas components in order to fit the observed emission over the galaxy. A larger number of high resolution transitions across the SLED may allow for further constraining of the conditions, particularly in the SB ring.

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arXiv2020

Gas kinematics of key prebiotic molecules in GV Tau N revealed with an ALMA, PdBI, and Herschel synergy

A large effort has been made to detect warm gas in the planet formation zone of circumstellar discs using space and ground-based near infrared facilities. GV Tau N, the most obscured component of the GV Tau system, is an outstanding source, being one of the first targets detected in HCN and the only one detected in CH$_4$ so far. Although near infrared observations have shed light on its chemical content, the physical structure and kinematics of the circumstellar matter remained unknown. We use interferometric images of the HCN 3-2 and $^{13}$CO 3-2 lines, and far-IR observations of $^{13}$CO, HCN, CN and H$_2$O transitions to discern the morphology, kinematics, and chemistry of the dense gas close to the star. These observations constitute the first detection of H$_2$O towards GV Tau N. Moreover, ALMA high spatial resolution (~ 7 au) images of the continuum at 1.1 mm and the HCN 3-2 line resolve different gas components towards GV Tau N, a gaseous disc with R~25 au, an ionized jet, and one (or two) molecular outflows. The asymmetric morphology of the gaseous disc shows that it has been eroded by the jet. All observations can be explained if GV Tau N is binary, and the primary component has a highly inclined individual disc relative to the circumbinary disc. We discuss the origin of the water and the other molecules emission according to this scenario. In particular, we propose that the water emission would come from the disrupted gaseous disc and the molecular outflows.

astro-ph.SR↗

arXiv2020

Gas phase Elemental abundances in Molecular cloudS (GEMS). II. On the quest for the sulphur reservoir in molecular clouds: the $H_{2}S$ case

Sulphur is one of the most abundant elements in the Universe. Surprisingly, sulphuretted molecules are not as abundant as expected in the interstellar medium, and the identity of the main sulphur reservoir is still an open question. Our goal is to investigate the H$_{2}$S chemistry in dark clouds, as this stable molecule is a potential sulphur reservoir. Using millimeter observations of CS, SO, H$_{2}$S, and their isotopologues, we determine the physical conditions and H$_{2}$S abundances along the cores TMC 1-C, TMC 1-CP, and Barnard 1b. The gas-grain model Nautilus is then used to model the sulphur chemistry and explore the impact of photo-desorption and chemical desorption on the H$_2$S abundance. Our model shows that chemical desorption is the main source of gas-phase H$_2$S in dark cores. The measured H$_{2}$S abundance can only be fitted if we assume that the chemical desorption rate decreases by more than a factor of 10 when $n_{\rm H}>2\times10^{4}$. This change in the desorption rate is consistent with the formation of thick H$_2$O and CO ice mantles on grain surfaces. The observed SO and H$_2$S abundances are in good agreement with our predictions adopting an undepleted value of the sulphur abundance. However, the CS abundance is overestimated by a factor of $5-10$. Along the three cores, atomic S is predicted to be the main sulphur reservoir. We conclude that the gaseous H$_2$S abundance is well reproduced, assuming undepleted sulphur abundance and chemical desorption as the main source of H$_2$S. The behavior of the observed H$_{2}$S abundance suggests a changing desorption efficiency, which would probe the snowline in these cores. Our model, however, overestimates the observed gas-phase CS abundance. Given the uncertainty in the sulphur chemistry, our data are consistent with a cosmic elemental S abundance with an uncertainty of a factor of 10.

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arXiv2020

On The Photodesorption of CO$_2$ Ice Analogues: The Formation of Atomic C in The Ice and the Effect of The VUV Emission Spectrume

CO$_2$ ice has a phase transition at 35 K when its structure changes from amorphous to crystalline. Using Reflection absorption Infrared Spectroscopy (RAIRS), Öberg et al. observed that the photodesorption yield of CO$_2$ ice deposited at 60 K and irradiated at 18 K is 40% lower than that of CO$_2$ ice deposited and irradiated at 18 K. In this work, CO$_2$ ices were deposited at 16-60 K and UV-irradiated at 16 K to rule out the temperature effect and figure out the relationship between photodesorption yield and ice structure. IR spectroscopy is a common method used for measurement of the photodesorption yield in ices. We found that undetectable C atoms produced in irradiated CO$_2$ ice can account for 33% of the amount of depleted CO$_2$ molecules in the ice. A quantitative calibration of QMS was therefore performed to convert the measured ion current into photodesorption yield. During various irradiation periods, the dominant photodesorbing species were CO, O$_2$, and CO$_2$, and their photodesorption yields in CO$_2$ ices deposited at different temperature configurations were almost the same, indicating that ice morphology has no effect on the photodesorption yield of CO$_2$ ice. In addition, we found that the lower desorption yield reported by Martín-Doménech et al. is due to a linear relationship between the photodesorption yield and the combination of energy distribution of Microwave-Discharge Hydrogen-flow Lamp (MDHL) and UV absorption cross section of ices.

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arXiv2019

ALMA images the many faces of the NGC1068 torus and its surroundings

We investigate the fueling and the feedback of nuclear activity in the Seyfert 2 galaxy NGC1068, by studying the distribution and kinematics of molecular gas in the torus and its connections. We use ALMA to image the emission of a set of molecular gas tracers in the circumnuclear disk (CND) and the torus of the galaxy using the CO(2-1), CO(3-2) and HCO+(4-3) lines with spatial resolutions ~0.03"-0.09"(2-6pc). ALMA resolves the CND as an asymmetric ringed disk of D~400pc-size and mass of ~1.4x10^8 Msun. The inner edge of the ring is associated with edge-brightened arcs of NIR polarized emission identified with the working surface of the AGN ionized wind. ALMA proves the existence of a molecular torus of M_torus ~ 3x10^5Msun, which extends over a large range of spatial scales D=10-30pc around the central engine. The new observations evidence the density radial stratification of the torus: the HCO+(4-3) torus, with a full size D=11pc, is a factor of 2-3 smaller than its CO(2-1) and CO(3-2) counterparts, which have full-sizes D=26pc and D=28pc, respectively. The torus is connected to the CND through a network of gas streamers. The kinematics of molecular gas show strong departures from circular motions in the torus, the gas streamers, and the CND. These velocity distortions are interconnected and are part of a 3D outflow that reflects the effects of AGN feedback on the kinematics of molecular gas across a wide range of spatial scales. We conclude that a wide-angle AGN wind launched from the accretion disk is impacting a sizeable fraction of the gas inside the torus (~0.4-0.6 x M_torus). However, a large gas reservoir (~1.2-1.8 x 10^5Msun) close to the equatorial plane of the torus remains unaffected by the AGN wind and can continue fueling the AGN for ~1-4Myr. AGN fueling seems nevertheless thwarted on intermediate scales (15pc < r < 50pc).

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