SearcharxivSearch

arXiv subjects

A. G. Green

Publications and source records attributed to A. G. Green.

At least 19 recordsLinked to original sources

Quench Spectroscopy of Magnetic Excitations on a Superconducting Quantum Processor

The elementary excitation spectrum of a many-body quantum system encodes many key properties, including phenomena as diverse as transport, thermalisation and ground state structure. Excitation spectra of strongly correlated systems are typically encoded in dynamical structure factors, which are demanding to measure experimentally and challenging to compute classically. Here we use quench spectroscopy on a superconducting quantum processor to extract excitation spectra of spin chains of $L=101$ spins. By tailoring the combination of quench protocol and observable, we selectively access distinct excitation sectors across several phases of the spin-$1/2$ XXZ chain, resolving free magnons, multi-magnon bound states, and two-spinon continua. Notably, we demonstrate that the protocol does not rely on ground state preparation: in the classically challenging gapless regime, we extract spectra directly from the quench dynamics of easily prepared product states, a procedure that is natural and straightforward on quantum hardware. Our work establishes quench spectroscopy as a fast and flexible probe of many-body excitation spectra on digital quantum hardware, introduces a novel quench protocol that does not require costly state preparation routines, and provides a scalable route towards regimes where classical simulation may become intractable.

quant-ph

Transition between critical antiferromagnetic phases in the $J_1$-$J_2$ spin chain

The $J_1$-$J_2$ spin chain is one of the canonical models of quantum magnetism, and has long been known to host a critical antiferromagnetic phase with power-law decay of spin correlations. We show in this Letter that there are, in fact, \textit{two} distinct critical antiferromagnetic phases, where the roles of the local dimer field and its dual field are interchanged: the `Affleck-Haldane' phase near the Heisenberg point $J_2 = 0$, where the dimer field that parametrises local singlet order is gapless and part of a joint $O(4)$ Néel-singlet order parameter; and the `Zirnbauer' phase which appears at sufficiently large ferromagnetic $J_2$, where the dimer field is gapped out and its \textit{dual} field -- the instanton density of the $O(3)$ Néel field -- is critical instead. The phases are so-named because each realises one of the competing pictures for how the $O(3)$ non-linear sigma model with a topological theta term renormalises to the $\mathfrak{\hat{su}}(2)_1$ Wess-Zumino-Witten model. We support these predictions with density matrix renormalisation group calculations.

cond-mat.stat-mech

A Generalised Haldane Map from the Matrix Product State Path Integral to the Critical Theory of the $J_1$-$J_2$ Chain

We study the $J_1$-$J_2$ spin-$1/2$ chain using a path integral constructed over matrix product states (MPS). By virtue of its non-trivial entanglement structure, the MPS ansatz captures the key phases of the model even at a semi-classical, saddle-point level, and, as a variational state, is in good agreement with the field theory obtained by abelian bosonisation. Going beyond the semi-classical level, we show that the MPS ansatz facilitates a physically-motivated derivation of the field theory of the critical phase: by carefully taking the continuum limit -- a generalisation of the Haldane map -- we recover from the MPS path integral a field theory with the correct topological term and emergent $SO(4)$ symmetry, constructively linking the microscopic states and topological field-theoretic structures. Moreover, the dimerisation transition is particularly clear in the MPS formulation -- an explicit dimerisation potential becomes relevant, gapping out the magnetic fluctuations.

cond-mat.str-el

Trajectory-Resolved Weiss Fields for Quantum Spin Dynamics

We explore the dynamics of quantum spin systems in two and three dimensions using an exact mapping to classical stochastic processes. In recent work we explored the effectiveness of sampling around the mean field evolution as determined by a stochastically averaged Weiss field. Here, we show that this approach can be significantly extended by sampling around the instantaneous Weiss field associated with each stochastic trajectory taken separately. This trajectory-resolved approach incorporates sample to sample fluctuations and allows for longer simulation times. We demonstrate the utility of this approach for quenches in the two-dimensional and three-dimensional quantum Ising model. We show that the method is particularly advantageous in situations where the average Weiss-field vanishes, but the trajectory-resolved Weiss fields are non-zero. We discuss the connection to the gauge-P phase space approach, where the trajectory-resolved Weiss field can be interpreted as a gauge degree of freedom.

cond-mat.str-el

Strain control of a bandwidth-driven spin reorientation in Ca$_{3}$Ru$_{2}$O$_{7}$

The layered-ruthenate family of materials possess an intricate interplay of structural, electronic and magnetic degrees of freedom that yields a plethora of delicately balanced ground states. This is exemplified by Ca$_{3}$Ru$_{2}$O$_{7}$, which hosts a coupled transition in which the lattice parameters jump, the Fermi surface partially gaps and the spins undergo a $90^{\circ}$ in-plane reorientation. Here, we show how the transition is driven by a lattice strain that tunes the electronic bandwidth. We apply uniaxial stress to single crystals of Ca$_{3}$Ru$_{2}$O$_{7}$, using neutron and resonant x-ray scattering to simultaneously probe the structural and magnetic responses. These measurements demonstrate that the transition can be driven by externally induced strain, stimulating the development of a theoretical model in which an internal strain is generated self-consistently to lower the electronic energy. We understand the strain to act by modifying tilts and rotations of the RuO$_{6}$ octahedra, which directly influences the nearest-neighbour hopping. Our results offer a blueprint for uncovering the driving force behind coupled phase transitions, as well as a route to controlling them.

cond-mat.str-el

Magnetic hard-direction ordering in anisotropic Kondo systems

We present a generic mechanism that explains why many Kondo materials show magnetic ordering along directions that are not favoured by the crystal-field anisotropy. Using a renormalization-group (RG) analysis of single impurity Kondo models with single-ion anisotropy, we demonstrate that strong fluctuations above the Kondo temperature drive a moment re-orientation over a wide range of parameters, e.g. for different spin values $S$ and number of Kondo channels $N$. In tetragonal systems this can happen for both easy-plane or easy axis anisotropy. The characteristic crossing of magnetic susceptibilities is not an artefact of the weak-coupling RG treatment but can be reproduced in brute-force perturbation theory. Employing numerical renormalization group (NRG), we show that for an under-screened moment ($S=1$, $N=1$) with easy-plane anisotropy, a crossing of magnetic susceptibilities can also occur in the strong-coupling regime (below the Kondo temperature). This suggests that collective magnetic ordering of such under-screened moments would develop along the magnetic hard axis.

cond-mat.str-el

Deterministic Tensor Network Classifiers

We present tensor networks for feature extraction and refinement of classifier performance. These networks can be initialised deterministically and have the potential for implementation on near-term intermediate-scale quantum (NISQ) devices. Feature extraction proceeds through a direct combination and compression of images amplitude-encoded over just $\log N_{\text{pixels}}$ qubits. Performance is refined using `Quantum Stacking', a deterministic method that can be applied to the predictions of any classifier regardless of structure, and implemented on NISQ devices using data re-uploading. These procedures are applied to a tensor network encoding of data, and benchmarked against the 10 class MNIST and fashion MNIST datasets. Good training and test accuracy are achieved without any variational training.

quant-ph

Time-Evolving Weiss Fields in the Stochastic Approach to Quantum Spins

We investigate non-equilibrium quantum spin systems via an exact mapping to stochastic differential equations. This description is invariant under a shift in the mean of the Gaussian noise. We show that one can extend the simulation time for real-time dynamics in one and two dimensions by a judicious choice of this shift. This can be updated dynamically in order to reduce the impact of stochastic fluctuations. We discuss the connection to drift gauges in the gauge-P literature.

cond-mat.str-el

Phase Transitions in the Classical Simulability of Open Quantum Systems

We study the evolution of an open quantum system using a Langevin unravelling of the density matrix evolution over matrix product states. As the strength of coupling to and temperature of the environment is increased, we find a transition where the entanglement of the individual trajectories saturates, permitting a classical simulation of the system for all times. This is the Hamiltonian open system counterpart of the saturation in entanglement found in random circuits with projective or weak measurements. If a system is open, there is a limit to the advantage in simulating its behaviour on a quantum computer, even when that evolution harbours important quantum effects.

quant-ph

Fluctuations and Non-Hermiticity in the Stochastic Approach to Quantum Spins

We investigate the non-equilibrium dynamics of isolated quantum spin systems via an exact mapping to classical stochastic differential equations. We show that one can address significantly larger system sizes than recently obtained, including two-dimensional systems with up to 49 spins. We demonstrate that the results for physical observables are in excellent agreement with exact results and alternative numerical techniques where available. We further develop a hybrid stochastic approach involving matrix product states. In the presence of finite numerical sampling, we show that the non-Hermitian character of the stochastic representation leads to the growth of the norm of the time-evolving quantum state and to departures for physical observables at late times. We demonstrate approaches that correct for this and discuss the prospects for further development.

cond-mat.str-el

Feynman Path Integrals Over Entangled States

The saddle points of a conventional Feynman path integral are not entangled, since they comprise a sequence of classical field configurations. We combine insights from field theory and tensor networks by constructing a Feynman path integral over a sequence of matrix product states. The paths that dominate this path integral include some degree of entanglement. This new feature allows several insights and applications: i. A Ginzburg-Landau description of deconfined phase transitions. ii. The emergence of new classical collective variables in states that are not adiabatically continuous with product states. iii. Features that are captured in product-state field theories by proliferation of instantons are encoded in perturbative fluctuations about entangled saddles. We develop a general formalism for such path integrals and a couple of simple examples to illustrate their utility.

cond-mat.str-el

Electronic spin-triplet nematic with a twist

We analyze a model of itinerant electrons interacting through a quadrupole density-density repulsion in three dimensions. At the mean field level, the interaction drives a continuous Pomeranchuk instability towards $d$-wave, spin-triplet nematic order, which simultaneously breaks the SU(2) spin-rotation and spatial rotational symmetries. This order results in spin antisymmetric, elliptical deformations of the Fermi surfaces of up and down spins. We show that the effects of quantum fluctuations are similar to those in metallic ferromagnets, rendering the nematic transition first-order at low temperatures. Using the fermionic quantum order-by-disorder approach to self-consistently calculate fluctuations around possible modulated states, we show that the first-order transition is pre-empted by the formation of a nematic state that is intertwined with a helical modulation in spin space. Such a state is closely related to $d$-wave bond density wave order in square-lattice systems. Moreover, we show that it may coexist with a modulated, $p$-wave superconducting state.

cond-mat.str-el

Magnetic hard-axis ordering near ferromagnetic quantum criticality

We investigate the interplay of quantum fluctuations and magnetic anisotropies in metallic ferromagnets. Our central result is that fluctuations close to a quantum critical point can drive the moments to point along a magnetic hard axis. As a proof of concept, we show this behavior explicitly for a generic two-band model with local Coulomb and Hund's interactions, and a spin-orbit-induced easy plane anisotropy. The phase diagram is calculated within the fermionic quantum order-by-disorder approach, which is based on a self-consistent free energy expansion around a magnetically ordered state with unspecified orientation. Quantum fluctuations render the transition of the easy-plane ferromagnet first-order below a tricritical point. At even lower temperatures, directionally dependent transverse fluctuations dominate the magnetic anisotropy and the moments flip to lie along the magnetic hard axis. We discuss our findings in the context of recent experiments that show this unusual ordering along the magnetic hard direction.

cond-mat.str-el

Quantum and Classical in Adiabatic Computation

Adiabatic transport provides a powerful way to manipulate quantum states. By preparing a system in a readily initialised state and then slowly changing its Hamiltonian, one may achieve quantum states that would otherwise be inaccessible. Moreover, a judicious choice of final Hamiltonian whose groundstate encodes the solution to a problem allows adiabatic transport to be used for universal quantum computation. However, the dephasing effects of the environment limit the quantum correlations that an open system can support and degrade the power of such adiabatic computation. We quantify this effect by allowing the system to evolve over a restricted set of quantum states, providing a link between physically inspired classical optimisation algorithms and quantum adiabatic optimisation. This new perspective allows us to develop benchmarks to bound the quantum correlations harnessed by an adiabatic computation. We apply these to the D-Wave Vesuvius machine with revealing - though inconclusive - results.

quant-ph

Non-equilibrium conductivity at quantum critical points

Quantum criticality provides an important route to revealing universal non-equilibrium behaviour. A canonical example of a quantum critical point is the Bose-Hubbard model, which we study under the application of an electric field. A Boltzmann transport formalism and $ε$-expansion are used to obtain the non-equilibrium conductivity and current noise. This approach allows us to explicitly identify how a universal non-equilibrium steady state is maintained, by identifying the rate-limiting step in balancing Joule heating and dissipation to a heat bath. It also reveals that the non-equilibrium distribution function is very far from a thermal distribution.

cond-mat.str-el

Resummation of fluctuations near ferromagnetic quantum critical points

We present a detailed analysis of the non-analytic structure of the free energy for the itinerant ferromagnet near the quantum critical point in two and three dimensions. We analyze a model of electrons with an isotropic dispersion interacting through a contact repulsion. A fermionic version of the quantum order-by-disorder mechanism allows us to calculate the free energy as a functional of the dispersion in the presence of homogeneous and spiralling magnetic order. We re-sum the leading divergent contributions, to derive an algebraic expression for the non-analytic contribution to free energy from quantum fluctuations. Using a recursion which relates sub-leading divergences to the leading term, we calculate the full T=0 contribution in $d=3$. We propose an interpolating functional form, which allows us to track phase transition lines at temperatures far below the tricritical point and down to T=0. In $d=2$, quantum fluctuations are stronger and non-analyticities more severe. Using a similar re-summation approach, we find that despite the different non-analytic structures, the phase diagrams in two and three dimensions are remarkably similar, exhibiting an incommensurate spiral phase near to the avoided quantum critical point.

cond-mat.str-el

Helical glasses near ferromagnetic quantum criticality

We study the effects of quenched charge disorder on the phase reconstruction near itinerant ferromagnetic quantum critical points in three spatial dimensions. Combining a replica disorder average with a fermionic version of the quantum order-by-disorder mechanism, we show that weak disorder destabilizes the ferromagnetic state and enhances the susceptibility towards incommensurate, spiral magnetic ordering. The Goldstone modes of the spiral phase are governed by a 3d-XY model. The induced disorder in the pitch of the spiral generates a random anisotropy for the Goldstone modes, inducing vortex lines in the phase of the helical order and rendering the magnetic correlations short ranged with a strongly anisotropic correlation length.

cond-mat.str-el

Fluctuation-induced pair density wave in itinerant ferromagnets

Magnetic fluctuations near to quantum criticality can have profound effects. They lead to characteristic scaling at high temperature which may ultimately give way to a reconstruction of the phase diagram and the formation of new phases at low temperatures. The ferromagnet UGe2 is unstable to p-wave superconducting order -- an effect presaged by the superfluidity in He3 -- whereas in CeFePO fluctuations drive the formation of spiral magnetic order. Here we develop a general quantum order-by-disorder description of these systems that encompasses both of these instabilities within a unified framework. This allows us to demonstrate that in fact these instabilities intertwine to form a new phase, a pair density wave.

cond-mat.str-el