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A. Gade

Publications and source records attributed to A. Gade.

At least 37 records · Page 2Linked to original sources

The Core of $^{25}$F studied by the $^{25}$F(-1p)$^{24}$O reaction

The $^{25}$F($5/2^+) (-1p) ^{24}$O reaction was studied at the NSCL using the S800 spectrometer. The experimental spectroscopic factor for the ground-state to ground-state transition indicates a substantial depletion of the proton $d_{5/2}$ strength compared to shell-model expectations. Our result supports the findings reported by Tang \textit{et al.}, from their study of the $(p,2p)$ reaction at RIBF. The overlap between the $^{25}$F and $^{24}$O ground-states is considerably less than anticipated if $^{24}$O acted as a robust and rigid doubly-magic core in $^{25}$F. We interpret the results within the framework of the Particle-Vibration Coupling (PVC) of a $d_{5/2}$ proton coupled to a quadrupole phonon of an effective core. This approach provides a good description of the experimental data by requiring an effective $^{24}$O* core with a phonon energy of $\hbarω_2$= 3.2 MeV, and a $B(E2) ~ 2.7$ W.u., softer and more collective than a bare $^{24}$O. Both the Nilsson deformed mean field and the PVC models appear to capture the properties of the effective core of $^{25}$F, suggesting that the additional proton tends to polarize the free, doubly magic $^{24}$O in such a way that it becomes either slightly deformed or a quadrupole vibrator.

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In-beam $γ$-ray spectroscopy of $^{32}$Mg via direct reactions

Background: The nucleus $^{32}$Mg ($N=20$ and $Z=12$) plays a central role in the so-called "island of inversion" where in the ground states $sd$-shell neutrons are promoted to the $fp$-shell orbitals across the shell gap, resulting in the disappearance of the canonical neutron magic number $N=20$. Purpose: The primary goals of this work are to extend the level scheme of $^{32}$Mg, provide spin-parity assignments to excited states, and discuss the microscopic structure of each state through comparisons with theoretical calculations. Method: In-beam $γ$-ray spectroscopy of $^{32}$Mg was performed using two direct-reaction probes, one-neutron (two-proton) knockout reactions on $^{33}$Mg ($^{34}$Si). Final-state exclusive cross sections and parallel momentum distributions were extracted from the experimental data and compared with eikonal-based reaction model calculations combined with shell-model overlap functions. Results: Owing to the remarkable selectivity of the one-neutron and two-proton knockout reactions, a significantly updated level scheme for $^{32}$Mg, which exhibits negative-parity intruder and positive-parity normal states, was constructed. The experimental results were confronted with four different nuclear structure models. Conclusions: In some of these models, different aspects of $^{32}$Mg and the transition into the island of inversion are well described. However, unexplained discrepancies remain, and even with the help of these state-of-the-art theoretical approaches, the structure of this key nucleus is not yet fully captured.

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Coexisting normal and intruder configurations in $^{32}$Mg

Situated in the so-called "island of inversion," the nucleus $^{32}$Mg is considered as an archetypal example of the disappearance of magicity at $N=20$. We report on high statistics in-beam spectroscopy of $^{32}$Mg with a unique approach, in that two direct reaction probes with different sensitivities to the underlying nuclear structure are employed at the same time. More specifically, states in $^{32}$Mg were populated by knockout reactions starting from $^{33}$Mg and $^{34}$Si, lying inside and outside the island of inversion, respectively. The momentum distributions of the reaction residues and the cross sections leading to the individual final states were confronted with eikonal-based reaction calculations, yielding a significantly updated level scheme for $^{32}$Mg and spin-parity assignments. By fully exploiting observables obtained in this measurement, a variety of structures coexisting in 32Mg was unraveled. Comparisons with theoretical predictions based on shell-model overlaps allowed for clear discrimination between different structural models, revealing that the complete theoretical description of this key nucleus is yet to be achieved.

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Structure of $^{43}$P and $^{42}$Si in a two-level shape-coexistence model

Exclusive cross sections for the $^{43}$P$(-1p)^{42}$Si reaction to the lowest $0^+$ and $2^+$ states, measured at NSCL with GRETINA and the S800, are interpreted in terms of a two-level mixing (collective) model of oblate and prolate co-existing shapes. Using the formalism developed for deformed nuclei we calculate the spectroscopic amplitudes and exclusive cross-sections in the strong coupling limit, where for $^{43}$P the schematic wavefunction includes the coupling of the Nilsson [211]$\frac{1}{2}$ proton orbit. Good agreement with the experimental data is obtained when the amplitude of the oblate configuration is $\gtrsim$ 80\%, suggesting that both nuclei are predominantly oblate, in line with theoretical expectations.

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Updated systematics of intermediate-energy single-nucleon removal cross sections

The body of experimental measurements of intermediate-energy reactions that remove a single nucleon from a secondary beam of neutron- or proton-rich nuclei continues to grow. These data have been analysed consistently using an approximate, eikonal-model treatment of the reaction dynamics combined with appropriate shell-model descriptions of the projectile initial state, the bound final states spectrum of the reaction residue and single-particle removal strengths computed from their wave-function overlaps. The systematics of the ratio $R_s$ of the measured inclusive cross-section to all bound final states and the calculated cross-section to bound shell-model states -- in different regions of the nuclear chart and involving both very weakly-bound and strongly-bound valence nucleons -- is important in relating the empirically deduced orbital occupancies to those from the best available shell-model predictions. Importantly, several new higher-energy measurements, for which the sudden-approximation aspect of the dynamical description is placed on an even stronger footing, now supplement the previously-analysed measurements. These additional data sets are discussed. Their $R_s$ values are shown to conform to and reinforce the earlier-observed systematics, with no indication that the approximately linear reduction in $R_s$ with increasing nucleon separation energy is a consequence of a breakdown of the sudden approximation.

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UCGretina GEANT4 Simulation of the GRETINA Gamma-Ray Energy Tracking Array

UCGretina, a GEANT4 simulation of the GRETINA gamma-ray tracking array of highly-segmented high-purity germanium detectors is described. We have developed a model of the array, in particular of the Quad Module and the capsules, that gives good agreement between simulated and measured photopeak efficiencies over a broad range of gamma-ray energies and reproduces the shape of the measured Compton continuum. Both of these features are needed in order to accurately extract gamma-ray yields from spectra collected in in-beam gamma-ray spectroscopy measurements with beams traveling at $v/c \gtrsim 0.3$ at the National Superconducting Cyclotron Laboratory and the Facility for Rare Isotope Beams. In the process of developing the model, we determined that millimeter-scale layers of passive germanium surrounding the active volumes of the simulated crystals must be included in order to reproduce measured photopeak efficiencies. We adopted a simple model of effective passive layers and developed heuristic methods of determining passive-layer thicknesses by comparison of simulations and measurements for a single crystal and for the full array. Prospects for future development of the model are discussed.

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Quenching of single-particle strength from direct reactions with stable and rare-isotope beams

In this review article we discuss the present status of direct nuclear reactions and the nuclear structure aspects one can study with them. We discuss the spectroscopic information we can assess in experiments involving transfer reactions, heavy-ion-induced knockout reactions and quasifree scattering with (p,2p), (p,pn), and (e,e'p) reactions. In particular, we focus on the proton-to-neutron asymmetry of the quenching of the spectroscopic strength.

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Structure of $^{30}$Mg explored via in-beam $γ$-ray spectroscopy

Background: In the "island of inversion", ground states of neutron-rich $sd$-shell nuclei exhibit strong admixtures of intruder configurations from the $fp$ shell. The nucleus $^{30}$Mg, located at the boundary of the island of inversion, serves as a cornerstone to track the structural evolution as one approaches this region. Purpose: Spin-parity assignments for excited states in $^{30}$Mg, especially negative-parity levels, have yet to be established. In the present work, the nuclear structure of $^{30}$Mg was investigated by in-beam $γ$-ray spectroscopy mainly focusing on firm spin-parity determinations. Method: High-intensity rare-isotope beams of $^{31}$Mg, $^{32}$Mg, $^{34}$Si, and $^{35}$P bombarded a Be target to induce nucleon removal reactions populating states in $^{30}$Mg. $γ$ rays were detected by the state-of-the-art $γ$-ray tracking array GRETINA. For the direct one-neutron removal reaction, final-state exclusive cross sections and parallel momentum distributions were deduced. Multi-nucleon removal reactions from different projectiles were exploited to gain complementary information. Results: With the aid of the parallel momentum distributions, an updated level scheme with revised spin-parity assignments was constructed. Spectroscopic factors associated with each state were also deduced. Conclusions: Results were confronted with large-scale shell-model calculations using two different effective interactions, showing excellent agreement with the present level scheme. However, a marked difference in the spectroscopic factors indicates that the full delineation of the transition into the island of inversion remains a challenge for theoretical models.

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Shell structure of $^{43}$S and collapse of the $N=28$ shell closure

The single-particle structure of the $N=27$ isotones provides insights into the shell evolution of neutron-rich nuclei from the doubly-magic $^{48}$Ca toward the drip line. $^{43}$S was studied employing the one-neutron knockout reaction from a radioactive $^{44}$S beam. Using a combination of prompt and delayed $γ$-ray spectroscopy the level structure of $^{43}$S was clarified. Momentum distributions were analyzed and allowed for spin and parity assignments. The deduced spectroscopic factors show that the $^{44}$S ground-state configuration has a strong intruder component. The results were confronted with shell model calculations using two effective interactions. General agreement was found between the calculations, but strong population of states originating from the removal of neutrons from the $2p_{3/2}$ orbital in the experiment indicates that the breakdown of the $N=28$ magic number is more rapid than the theoretical calculations suggest.

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The Structure of $^{33}$Si and the magicity of the N=20 gap at Z=14

The structure of $^{33}$Si was studied by a one-neutron knockout reaction from a $^{34}$Si beam at 98.5 MeV/u incident on a $^{9}$Be target. The prompt $γ$-rays following the de-excitation of $^{33}$Si were detected using the GRETINA $γ$-ray tracking array while the reaction residues were identified on an event-by-event basis in the focal plane of the S800 spectrometer at NSCL (National Superconducting Cyclotron Laboratory). The presently derived spectroscopic factor values, $C^2S$, for the 3/2$^+$ and 1/2$^+$ states, corresponding to a neutron removal from the $0d_{3/2}$ and $1s_{1/2}$ orbitals, agree with shell model calculations and point to a strong $N=20$ shell closure. Three states arising from the more bound $0d_{5/2}$ orbital are proposed, one of which is unbound by about 930 keV. The sensitivity of this experiment has also confirmed a weak population of 9/2$^-$ and 11/2$_{1,2}^-$ final states, which originate from a higher-order process. This mechanism may also have populated, to some fraction, the 3/2$^-$ and 7/2$^-$ negative-parity states, which hinders a determination of the $C^2S$ values for knockout from the normally unoccupied $1p_{3/2}$ and $0f_{7/2}$ orbits.

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Shape Coexistence at Zero Spin in 64Ni Driven by the Monopole Tensor Interaction

The low-spin structure of the semimagic 64Ni nucleus has been considerably expanded: combining four experiments, several 0+ and 2+ excited states were identified below 4.5 MeV, and their properties established. The Monte Carlo shell model accounts for the results and unveils an unexpectedly complex landscape of coexisting shapes: a prolate 0+ excitation is located at a surprisingly high energy (3463 keV), with a collective 2+ state 286 keV above it, the first such observation in Ni isotopes. The evolution in excitation energy of the prolate minimum across the neutron N = 40 subshell gap highlights the impact of the monopole interaction and its variation in strength with N.

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In-beam $γ$-ray spectroscopy at the proton dripline: $^{40}$Sc

We report on the first in-beam $γ$-ray spectroscopy of the proton-dripline nucleus $^{40}$Sc using two-nucleon pickup onto an intermediate-energy rare-isotope beam of $^{38}$Ca. The $^{9}$Be($^{38}$Ca,$^{40}$Sc$+γ$)X reaction at 60.9 MeV/nucleon mid-target energy selectively populates states in $^{40}$Sc for which the transferred proton and neutron couple to high orbital angular momentum. In turn, due to angular-momentum selection rules in proton emission and the nuclear structure and energetics of $^{39}$Ca, such states in $^{40}$Sc then exhibit $γ$-decay branches although they are well above the proton separation energy. This work uniquely complements results from particle spectroscopy following charge-exchange reactions on $^{40}$Ca as well as $^{40}$Ti EC/$β^+$ decay which both display very different selectivities. The population and $γ$-ray decay of the previously known first $(5^-)$ state at 892 keV and the observation of a new level at 2744 keV are discussed in comparison to the mirror nucleus and shell-model calculations. On the experimental side, this work shows that high-resolution in-beam $γ$-ray spectroscopy is possible with new generation Ge arrays for reactions induced by rare-isotope beams on the level of a few $μ$b of cross section.

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Nuclear Mass Measurements Map the Structure of Atomic Nuclei and Accreting Neutron Stars

We present mass excesses (ME) of neutron-rich isotopes of Ar through Fe, obtained via TOF-$Bρ$ mass spectrometry at the National Superconducting Cyclotron Laboratory. Our new results have significantly reduced systematic uncertainties relative to a prior analysis, enabling the first determination of ME for $^{58,59}{\rm Ti}$, $^{62}{\rm V}$, $^{65}{\rm Cr}$, $^{67,68}{\rm Mn}$, and $^{69,70}{\rm Fe}$. Our results show the $N=34$ subshell weaken at Sc and vanish at Ti, along with the absence of an $N=40$ subshell at Mn. This leads to a cooler accreted neutron star crust, highlighting the connection between the structure of nuclei and neutron stars.

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Inverse-kinematics proton scattering from $^{42,44}$S, $^{41,43}$P and the collapse of the $N=28$ major shell closure

Excited states of the neutron-rich isotopes $^{42,44}$S and $^{41,43}$P have been studied via inverse-kinematics proton scattering from a liquid hydrogen target, using the GRETINA $γ$-ray tracking array to extract inelastic scattering cross sections. Deformation lengths of the $2^+_1$ excitations in $^{42,44}$S have been determined and, when combined with deformation lengths determined with electromagnetic probes, yield the ratio of neutron-to-proton matrix elements $M_n/M_p$ for the $2^+_1$ excitations in these nuclei. The present results for $^{41,43}$P$(p,p')$ are used to compare two shell model interactions, SDPF-U and SDPF-MU. As in a recent study of $^{42}$Si, the present results on $^{41,43}$P favor the SDPF-MU interaction.

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Experimental identification of the $T = 1$, $J^π = 6^+$ state of $^{54}$Co and isospin symmetry in $A = 54$ studied via one-nucleon knockout reactions

New experimental data obtained from $γ$-ray tagged one-neutron and one-proton knockout from $^{55}$Co is presented. A candidate for the sought-after $T=1, T_z = 0, J^π = 6^+$ state in $^{54}$Co is proposed based on a comparison to the new data on $^{54}$Fe, the corresponding observables predicted by large-scale-shell-model (LSSM) calculations in the full $fp$-model space employing charge-dependent contributions, and isospin-symmetry arguments. Furthermore, possible isospin-symmetry breaking in the $A=54$, $T=1$ triplet is studied by calculating the experimental $c$ coefficients of the isobaric mass multiplet equation (IMME) up to the maximum possible spin $J=6$ expected for the $(1f_{7/2})^{-2}$ two-hole configuration relative to the doubly-magic nucleus $^{56}$Ni. The experimental quantities are compared to the theoretically predicted $c$ coefficients from LSSM calculations using two-body matrix elements obtained from a realistic chiral effective field theory potential at next-to-next-to-next-to-leading order (N$^3$LO).

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Two-neutron knockout as a probe of the composition of states in $^{22}$Mg, $^{23}$Al, and $^{24}$Si

Simpson and Tostevin proposed that the width and shape of exclusive parallel momentum distributions of the A-2 residue in direct two-nucleon knockout reactions carry a measurable sensitivity to the nucleon single-particle configurations and their couplings within the wave functions of exotic nuclei. We report here on the first benchmarks and use of this new spectroscopic tool. Exclusive parallel momentum distributions for states in the neutron-deficient nuclei $^{22}$Mg, $^{23}$Al, and $^{24}$Si populated in such direct two-neutron removal reactions were extracted and compared to predictions combining eikonal reaction theory and shell-model calculations. For the well-known $^{22}$Mg and $^{23}$Al nuclei, measurements and calculations were found to agree, supporting the dependence of the parallel momentum distribution width on the angular momentum composition of the shell-model two-neutron amplitudes. In $^{24}$Si, a level at 3439(9) keV, of relevance for the important $^{23}$Al(p,$γ$)$^{24}$Si astrophysical reaction rate, was confirmed to be the $2^+_2$ state, while the $4^+_1$ state, expected to be strongly populated in two-neutron knockout, was not observed. This puzzle is resolved by theoretical considerations of the Thomas-Ehrman shift, which also suggest that a previously reported 3471-keV state in $^{24}$Si is in fact the ($0^+_2$) level with one of the largest experimental mirror-energy shifts ever observed.

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Electromagnetic properties of $^{21}$O for benchmarking nuclear Hamiltonians

The structure of exotic nuclei provides valuable tests for state-of-the-art nuclear theory. In particular electromagnetic transition rates are more sensitive to aspects of nuclear forces and many-body physics than excitation energies alone. We report the first lifetime measurement of excited states in $^{21}$O, finding $τ_{1/2^+}=420^{+35}_{-32}\text{(stat)}^{+34}_{-12}\text{(sys)}$\,ps. This result together with the deduced level scheme and branching ratio of several $γ$-ray decays are compared to both phenomenological shell-model and ab initio calculations based on two- and three-nucleon forces derived from chiral effective field theory. We find that the electric quadrupole reduced transition probability of $\rm B(E2;1/2^+ \rightarrow 5/2^+_{g.s.}) = 0.71^{+0.07\ +0.02}_{-0.06\ -0.06}$~e$^2$fm$^4$, derived from the lifetime of the $1/2^+$ state, is smaller than the phenomenological result where standard effective charges are employed, suggesting the need for modifications of the latter in neutron-rich oxygen isotopes. We compare this result to both large-space and valence-space ab initio calculations, and by using multiple input interactions we explore the sensitivity of this observable to underlying details of nuclear forces.

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Probing the role of proton cross-shell excitations in 70Ni using nucleon knockout reactions

The neutron-rich Ni isotopes have attracted attention in recent years due to the occurrence of shape or configuration coexistence. We report on the difference in population of excited final states in 70Ni following gamma-ray tagged one-proton, one-neutron, and two-proton knockout from 71Cu, 71Ni, and 72Zn rare-isotope beams, respectively. Using variations observed in the relative transition intensities, signaling the changed population of specific final states in the different reactions, the role of neutron and proton configurations in excited states of 70Ni is probed schematically, with the goal of identifying those that carry, as leading configuration, proton excitations across the Z = 28 shell closure. Such states are suggested in the literature to form a collective structure associated with prolate deformation. Adding to the body of knowledge for 70Ni, 29 new transitions are reported, of which 15 are placed in its level scheme.

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