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A. Gade

Publications and source records attributed to A. Gade.

At least 91 records · Page 5Linked to original sources

Probing elastic and inelastic breakup contributions to intermediate-energy two-proton removal reactions

The two-proton removal reaction from 28Mg projectiles has been studied at 93 MeV/u at the NSCL. First coincidence measurements of the heavy 26Ne projectile residues, the removed protons and other light charged particles enabled the relative cross sections from each of the three possible elastic and inelastic proton removal mechanisms to be determined. These more final-state-exclusive measurements are key for further interrogation of these reaction mechanisms and use of the reaction channel for quantitative spectroscopy of very neutron-rich nuclei. The relative and absolute yields of the three contributing mechanisms are compared to reaction model expectations - based on the use of eikonal dynamics and sd-shell-model structure amplitudes.

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Observation of mutually enhanced collectivity in self-conjugate $^{76}_{38}$Sr$_{38}$

The lifetimes of the first 2$^{+}$ states in the neutron-deficient $^{76,78}$Sr isotopes were measured using a unique combination of the $γ$-ray line-shape method and two-step nucleon exchange reactions at intermediate energies. The transition rates for the 2$^{+}$ states were determined to be $B$(E2;2$^{+}$$\to 0^{+}$) = 2220(270) e$^{2}$fm$^{4}$ for $^{76}$Sr and 1800(250) e$^{2}$fm$^{4}$ for $^{78}$Sr, corresponding to large deformation of $β_2$ = 0.45(3) for $^{76}$Sr and 0.40(3) for $^{78}$Sr. The present data provide experimental evidence for mutually enhanced collectivity that occurs at $N$ = $Z$ = 38. The systematic behavior of the excitation energies and $B$(E2) values indicates a signature of shape coexistence in $^{76}$Sr, characterizing $^{76}$Sr as one of most deformed nuclei with an unusually reduced $E$(4$^{+}$)/$E$(2$^{+}$) ratio.

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Quadrupole collectivity beyond N=28: Intermediate-energy Coulomb excitation of 47,48Ar

We report on the first experimental study of quadrupole collectivity in the very neutron-rich nuclei \nuc{47,48}{Ar} using intermediate-energy Coulomb excitation. These nuclei are located along the path from doubly-magic Ca to collective S and Si isotopes, a critical region of shell evolution and structural change. The deduced $B(E2)$ transition strengths are confronted with large-scale shell-model calculations in the $sdpf$ shell using the state-of-the-art SDPF-U and EPQQM effective interactions. The comparison between experiment and theory indicates that a shell-model description of Ar isotopes around N=28 remains a challenge.

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Spectroscopy of neutron-unbound $^{27,28}$F

The ground state of $^{28}$F has been observed as an unbound resonance $2\underline{2}0$ keV above the ground state of $^{27}$F. Comparison of this result with USDA/USDB shell model predictions leads to the conclusion that the $^{28}$F ground state is primarily dominated by $sd$-shell configurations. Here we present a detailed report on the experiment in which the ground state resonance of $^{28}$F was first observed. Additionally, we report the first observation of a neutron-unbound excited state in $^{27}$F at an excitation energy of $25\underline{0}0 (2\underline{2}0)$ keV.

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Intermediate-energy inverse-kinematics one-proton pickup reactions on neutron-deficient $fp$-shell nuclei

Background: Thick-target-induced nucleon-adding transfer reactions onto energetic rare-isotope beams are an emerging spectroscopic tool. Their sensitivity to single-particle structure complements one-nucleon removal reaction capabilities in the quest to reveal the evolution of nuclear shell structure in very exotic nuclei. Purpose: To add intermediate-energy, carbon-target-induced one-proton pickup reactions to the arsenal of $γ$-ray tagged direct reactions applicable in the regime of low beam intensities and to apply these for the first time to $fp$-shell nuclei. Methods: Inclusive and partial cross sections were measured for the $\nuc{12}{C}(\nuc{48}{Cr},\nuc{49}{Mn}+γ)$X and $\nuc{12}{C}(\nuc{50}{Fe},\nuc{51}{Co}+γ)$X proton pickup reactions at 56.7 and 61.2 MeV/nucleon, respectively, using coincident particle-$γ$ spectroscopy at the NSCL. The results are compared to reaction theory calculations using $fp$-shell-model nuclear structure input. For comparison with our previous work, the same reactions were measured on \nuc{9}{Be} targets. Results: The measured partial cross sections confirm the specific population pattern predicted by theory, with pickup into high-$\ell$ orbitals being strongly favored; driven by linear and angular momentum matching. Conclusion: Carbon target-induced pickup reactions are well-suited, in the regime of modest beam intensity, to study the evolution of nuclear structure, with specific sensitivities that are well described by theory.

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Exploring the Low-$Z$ Shore of the Island of Inversion at $N = 19$

The technique of invariant mass spectroscopy has been used to measure, for the first time, the ground state energy of neutron-unbound $^{28}\textrm{F},$ determined to be a resonance in the $^{27}\textrm{F} + n$ continuum at $2\underline{2}0 (\underline{5}0)$ keV. States in $^{28}\textrm{F}$ were populated by the reactions of a 62 MeV/u $^{29}\textrm{Ne}$ beam impinging on a 288 $\textrm{mg/cm}^2$ beryllium target. The measured $^{28}\textrm{F}$ ground state energy is in good agreement with USDA/USDB shell model predictions, indicating that $pf$ shell intruder configurations play only a small role in the ground state structure of $^{28}\textrm{F}$ and establishing a low-$Z$ boundary of the island of inversion for N=19 isotones.

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Time-of-flight mass measurements for nuclear processes in neutron star crusts

The location of electron capture heat sources in the crust of accreting neutron stars depends on the masses of extremely neutron-rich nuclei. We present first results from a new implementation of the time-of-flight technique to measure nuclear masses of rare isotopes at the National Superconducting Cyclotron Laboratory. The masses of 16 neutron-rich nuclei in the scandium -- nickel range were determined simultaneously, improving the accuracy compared to previous data in 12 cases. The masses of $^{61}${V}, $^{63}${Cr}, $^{66}${Mn}, and $^{74}${Ni} were measured for the first time with mass excesses of $-30.510(890)$ MeV, $-35.280(650)$ MeV, $-36.900(790)$ MeV, and $-49.210(990)$ MeV, respectively. With the measurement of the $^{66}$Mn mass, the locations of the two dominant electron capture heat sources in the outer crust of accreting neutron stars that exhibit superbursts are now experimentally constrained. We find that the location of the $^{66}$Fe$\rightarrow^{66}$Mn electron capture transition occurs significantly closer to the surface than previously assumed because our new experimental Q-value is 2.1 MeV (2.6$σ$) smaller than predicted by the FRDM mass model.

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High-spin μs isomeric states in 96Ag

The isomeric and β decays of the N = Z +2 nucleus 96Ag were investigated at NSCL. A cascade of γ-ray transitions originating from the de-excitation of a μs isomer was observed for the first time and was found in coincidence with two previously-known transitions with energies of 470 and 667 keV. The isomeric half-life was determined as 1.45(7) μs, more precise than previously reported. The existence of a second, longer-lived μs isomer, associated with a 743-keV transition, is also proposed here. Shell model results within the (p_{3/2}p_{1/2}f_{5/2}g_{9/2}) model space, using the jj44b interaction, reproduced level energies and isomeric decay half-lives reasonably well.

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Quenching of spectroscopic factors for proton removal in oxygen isotopes

We present microscopic coupled-cluster calculations of the spectroscopic factors for proton removal from the closed-shell oxygen isotopes $^{14,16,22,24,28}$O with the chiral nucleon-nucleon interaction at next-to-next-to-next-to-leading order. We include coupling-to-continuum degrees of freedom by using a Hartree-Fock basis built from a Woods-Saxon single-particle basis. This basis treats bound and continuum states on an equal footing. We find a significant quenching of spectroscopic factors in the neutron-rich oxygen isotopes, pointing to enhanced many-body correlations induced by strong coupling to the scattering continuum above the neutron emission thresholds.

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Inverse-kinematics one-neutron pickup with fast rare-isotope beams

New measurements and reaction model calculations are reported for single neutron pickup reactions onto a fast \nuc{22}{Mg} secondary beam at 84 MeV per nucleon. Measurements were made on both carbon and beryllium targets, having very different structures, allowing a first investigation of the likely nature of the pickup reaction mechanism. The measurements involve thick reaction targets and $γ$-ray spectroscopy of the projectile-like reaction residue for final-state resolution, that permit experiments with low incident beam rates compared to traditional low-energy transfer reactions. From measured longitudinal momentum distributions we show that the $\nuc{12}{C} (\nuc{22}{Mg},\nuc{23}{Mg}+γ)X$ reaction largely proceeds as a direct two-body reaction, the neutron transfer producing bound \nuc{11}{C} target residues. The corresponding reaction on the \nuc{9}{Be} target seems to largely leave the \nuc{8}{Be} residual nucleus unbound at excitation energies high in the continuum. We discuss the possible use of such fast-beam one-neutron pickup reactions to track single-particle strength in exotic nuclei, and also their expected sensitivity to neutron high-$\ell$ (intruder) states which are often direct indicators of shell evolution and the disappearance of magic numbers in the exotic regime.

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In-beam gamma-ray spectroscopy of 35Mg and 33Na

Excited states in the very neutron-rich nuclei 35Mg and 33Na were populated in the fragmentation of a 38Si projectile beam on a Be target at 83 MeV/u beam energy. We report on the first observation of gamma-ray transitions in 35Mg, the odd-N neighbor of 34Mg and 36Mg, which are known to be part of the "Island of Inversion" around N = 20. The results are discussed in the framework of large- scale shell-model calculations. For the A = 3Z nucleus 33Na, a new gamma-ray transition was observed that is suggested to complete the gamma-ray cascade 7/2+ --> 5/2+ --> 3/2+ gs connecting three neutron 2p-2h intruder states that are predicted to form a close-to-ideal K = 3/2 rotational band in the strong-coupling limit.

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Gamow-Teller Unit Cross Sections for (t,3He) and (3He,t) Reactions

The proportionality between differential cross sections at vanishing linear momentum transfer and Gamow-Teller transition strength, expressed in terms of the \textit{unit cross section} ($\hatσ_{GT}$) was studied as a function of target mass number for ($t$,$^{3}$He) and ($^{3}$He,$t$) reactions at 115 $A$MeV and 140 $A$MeV, respectively. Existing ($^{3}$He,$t$) and ($t$,$^{3}$He) data on targets with mass number $12\leq A\leq 120$ were complemented with new and reevaluated ($t$,$^{3}$He) data on proton, deuteron, $^{6}$Li and $^{12}$C targets. It was found that in spite of the small difference in beam energies between the two probes, the unit cross sections have a nearly identical and simple dependence on target mass number $A$, for $A\geq 12$: $\hatσ_{GT}=109/A^{0.65}$. The factorization of the unit cross sections in terms of a kinematical factor, a distortion factor and the strength of the effective spin-isospin transfer nucleus-nucleus interaction was investigated. Simple phenomenological functions depending on mass number $A$ were extracted for the latter two. By comparison with plane and distorted-wave Born approximation calculations, it was found that the use of a short-range approximation for knock-on exchange contributions to the transition amplitude results in overestimated cross sections for reactions involving the composite ($^{3}$He,$t$) and ($t$,$^{3}$He) probes.

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Enhanced collectivity in 74Ni

The neutron-rich nucleus 74Ni was studied with inverse-kinematics inelastic proton scattering using a 74Ni radioactive beam incident on a liquid hydrogen targetat a center-of-mass energy of 80 MeV. From the measured de-excitation gamma-rays, the population of the first 2+ state was quantified. The angle-integrated excitation cross section was determined to be 14(4) mb. A deformation length of delta = 1.04(16) fm was extracted in comparison with distorted wave theory, which suggests that the enhancement of collectivity established for 70Ni continues up to 74Ni. A comparison with results of shell model and quasi-particle random phase approximation calculations indicates that the magic character of Z = 28 or N = 50 is weakened in 74Ni.

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Observation of isotonic symmetry for enhanced quadrupole collectivity in neutron-rich 62,64,66Fe isotopes at N=40

The transition rates for the 2_{1}^{+} states in 62,64,66Fe were studied using the Recoil Distance Doppler-Shift technique applied to projectile Coulomb excitation reactions. The deduced E2 strengths illustrate the enhanced collectivity of the neutron-rich Fe isotopes up to N=40. The results are interpreted by the generalized concept of valence proton symmetry which describes the evolution of nuclear structure around N=40 as governed by the number of valence protons with respect to Z~30. The deformation suggested by the experimental data is reproduced by state-of-the-art shell calculations with a new effective interaction developed for the fpgd valence space.

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Collectivity at N=50: 82Ge and 84Se

The neutron-rich N=50 isotones 82Ge and 84Se were investigated using intermediate-energy Coulomb excitation on a 197Au target and inelastic scattering on 9Be. As typical for intermediate-energy Coulomb excitation with projectile energies exceeding 70 MeV/nucleon, only the first 2^+ states were excited in 82Ge and 84Se. However, in the inelastic scattering on a 9Be target, a strong population of the first 4^+ state was observed for 84Se, while there is no indication of a similarly strong excitation of the corresponding state in the neighboring even-even isotone 82Ge. The results are discussed in the framework of systematics and shell-model calculations using three different effective interactions.

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Nuclear Astrophysics with Radioactive Beams

The quest to comprehend how nuclear processes influence astrophysical phenomena is driving experimental and theoretical research programs worldwide. One of the main goals in nuclear astrophysics is to understand how energy is generated in stars, how elements are synthesized in stellar events and what the nature of neutron stars is. New experimental capabilities, the availability of radioactive beams and increased computational power paired with new astronomical observations have advanced the present knowledge. This review summarizes the progress in the field of nuclear astrophysics with a focus on the role of indirect methods and reactions involving beams of rare isotopes.

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Production of very neutron-rich nuclei with a 76Ge beam

Production cross sections for neutron-rich nuclei from the fragmentation of a 76Ge beam at 132 MeV/u were measured. The longitudinal momentum distributions of 34 neutron-rich isotopes of elements 13 <= Z <= 27 were scanned using a novel experimental approach of varying the target thickness. Production cross sections with beryllium and tungsten targets were determined for a large number of nuclei including 15 isotopes first observed in this work. These are the most neutron-rich nuclides of the elements 17 <= Z <= 25 (50Cl, 53Ar, 55,56K, 57,58Ca, 59,60,61Sc, 62,63Ti, 65,66V, 68Cr,70Mn). A one-body Qg systematics is used to describe the production cross sections based on thermal evaporation from excited prefragments. Some of the fragments near 58Ca show anomalously large production cross sections.

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Gamow-Teller transitions to 64-Cu measured using the 64-Zn(t,3-He) reaction

The 64-Zn(t,3-He) reaction has been studied using a secondary triton beam of 115 MeV/nucleon to extract the Gamow-Teller transition-strength distribution to 64-Cu. The results were compared with shell-model calculations using the pf-shell effective interactions KB3G and GXPF1A and with existing data from the 64-Zn(d,2-He) reaction. Whereas the experimental results exhibited good consistency, neither of the theoretical predictions managed to reproduce the data. The implications for electron-capture rates during late stellar evolution were investigated. The rates based on the theoretical strength distributions are lower by factors of 3.5-5 compared to the rates based on experimental strength distributions.

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