arXiv subjects

A. Georges

Publications and source records attributed to A. Georges.

84 records · Page 5Linked to original sources

arXiv2003

Spectroscopic signatures of a bandwidth-controlled Mott transition at the surface of 1T-TaSe$_2$

High-resolution angle-resolved photoemission (ARPES) data show that a metal-insulator Mott transition occurs at the surface of the quasi-two dimensional compound TaSe$_2$. The transition is driven by the narrowing of the Ta $5d$ band induced by a temperature-dependent modulation of the atomic positions. A dynamical mean-field theory calculation of the spectral function of the half-filled Hubbard model captures the main qualitative feature of the data, namely the rapid transfer of spectral weight from the observed quasiparticle peak at the Fermi surface to the Hubbard bands, as the correlation gap opens up.

cond-mat.str-el↗

arXiv2003

Mott transition and transport crossovers in the organic compound $κ-(BEDT-TTF)_2 Cu[N(CN)_2] Cl$

We have performed in-plane transport measurements on the two-dimensional organic salt $κ$-(BEDT-TTF)$_{2}$Cu[N(CN)$_{2}$]Cl. A variable (gas) pressure technique allows for a detailed study of the changes in conductivity through the insulator-to-metal transition. We identify four different transport regimes as a function of pressure and temperature (corresponding to insulating, semi-conducting, ''bad metal'', and strongly correlated Fermi liquid behaviours). Marked hysteresis is found in the transition region, which displays complex physics that we attribute to strong spatial inhomogeneities. Away from the critical region, good agreement is found with a dynamical mean-field calculation of transport properties using the numerical renormalization group technique.

cond-mat.str-el↗

arXiv2002

First principles approach to the electronic structure of strongly correlated systems: combining GW and DMFT

We propose a dynamical mean field approach for calculating the electronic structure of strongly correlated materials from first principles. The scheme combines the GW method with dynamical mean field theory, which enables one to treat strong interaction effects. It avoids the conceptual problems inherent to conventional ``LDA+DMFT'', such as Hubbard interaction parameters and double counting terms. We apply a simplified version of the approach to the electronic structure of nickel and find encouraging results.

cond-mat.str-el↗

arXiv2002

Mott transition at large orbital degeneracy: dynamical mean-field theory

We study analytically the Mott transition of the N-orbital Hubbard model using dynamical mean-field theory and a low-energy projection onto an effective Kondo model. It is demonstrated that the critical interaction at which the insulator appears (Uc1) and the one at which the metal becomes unstable (Uc2) have different dependence on the number of orbitals as the latter becomes large: Uc1 ~ \sqrt{N} while Uc2 ~ N. An exact analytical determination of the critical coupling Uc2/N is obtained in the large-N limit. The metallic solution close to this critical coupling has many similarities at low-energy with the results of slave boson approximations, to which a comparison is made. We also discuss how the critical temperature associated with the Mott critical endpoint depends on the number of orbitals.

cond-mat.str-el↗

arXiv2002

Heavy-fermion and spin-liquid behavior in a Kondo lattice with magnetic frustration

We study the competition between the Kondo effect and frustrating exchange interactions in a Kondo-lattice model within a large-${\cal N}$ dynamical mean-field theory. We find a T=0 phase transition between a heavy Fermi-liquid and a spin-liquid for a critical value of the exchange $J_c = T_{K}^0$, the single-impurity Kondo temperature. Close to the critical point, the Fermi liquid coherence scale $T^\star$ is strongly reduced and the effective mass strongly enhanced. The regime $T>T^\star$ is characterized by spin-liquid magnetic correlations and non-Fermi-liquid properties. It is suggested that magnetic frustration is a general mechanism which is essential to explain the large effective mass of some metallic compounds such as LiV$_2$O$_4$.

cond-mat.str-el↗

arXiv2002

Quasi-one-dimensional organic conductors: dimensional crossover and some puzzles

We review some properties of quasi-one-dimensional organic conductors, such as the Bechgaard salts, with an emphasis on aspects related to the crossovers between a Mott insulating state to a metallic state, and crossovers between different metallic behaviors. We discuss why a theoretical description of these issues is a particularly challenging problem, and describe a recent non-perturbative approach designed to deal with systems of coupled chains. This method, dubbed "chain-DMFT", is a generalization of dynamical mean field theory that treats both, one-dimensional and higher dimensional physics, in a unified manner. We present numerical results for a system of coupled Hubbard chains. Chain-DMFT indeed captures the metal-insulator transition and the dimensional crossover from a high temperature Luttinger liquid to a low temperature Fermi liquid phase, and allows to access the properties of these phases. Based on these results perspectives for a theoretical understanding of the physics of the Bechgaard salts are discussed.

cond-mat.str-el↗

arXiv2001

Deconfinement transition and Luttinger to Fermi Liquid crossover in quasi one-dimensional systems

We investigate a system of one dimensional Hubbard chains of interacting fermions coupled by inter-chain hopping. Using a generalization of the Dynamical Mean Field Theory we study the deconfinement transition from a Mott insulator to a metal and the crossover between Luttinger and Fermi liquid phases. One-particle properties, local spin response and inter-chain optical conductivity are calculated. Possible applications to organic conductors are discussed.

cond-mat.str-el↗

arXiv2000

Quantum Fluctuations of a Nearly Critical Heisenberg Spin Glass

We describe the interplay of quantum and thermal fluctuations in the infinite-range Heisenberg spin glass. This model is generalized to SU(N) symmetry, and we describe the phase diagram as a function of the spin S and the temperature T. The model is solved in the large N limit and certain universal critical properties are shown to hold to all orders in 1/N. For large S, the ground state is a spin glass, but quantum effects are crucial in determining the low T thermodynamics: we find a specific heat linear in T and a local spectral density of spin excitations linear in frequency for a spin glass state which is marginally stable to fluctuations in the replicon modes. For small S, the spin-glass order is fragile, and a spin-liquid state dominates the properties over a significant range of temperatures and frequencies. We argue that the latter state may be relevant in understanding the properties of strongly-disordered transition metal and rare earth compounds.

cond-mat.str-el↗

arXiv2000

Coherence scale of the Kondo lattice

It is shown that the large-N approach yields two energy scales for the Kondo lattice model. The single-impurity Kondo temperature, $T_K$, signals the onset of local singlet formation, while Fermi liquid coherence sets in only below a lower scale, $T^{\star}$. At low conduction electron density $n_c$ ("exhaustion" limit), the ratio $T^{\star}/T_K$ is much smaller than unity, and is shown to depend only on $n_c$ and not on the Kondo coupling. The physical meaning of these two scales is demonstrated by computing several quantities as a function of $n_c$ and temperature.

cond-mat.str-el↗

arXiv1996

Reflections on the One Dimensional Realization of Odd-Frequency Pairing

We discuss the odd-frequency pairing correlations discovered by Zachar, Kivelson and Emery (ZKE) in a one dimensional Kondo lattice. A lattice model that realizes the continuum theory of ZKE is introduced and the correlations it gives rise to are identified as odd-frequency singlet pairing. The excitation spectrum is found to contain a spin gap, and a much lower energy band of spinless excitations. We discuss how the power-law correlations realized in the ZKE model evolve into true long-range order when Kondo chains are weakly coupled together and tentatively suggest a way in which the higher dimensional model can be treated using mean-field theory.

cond-mat.str-el↗

arXiv1995

The Local Impurity Self Consistent Approximation (LISA) to Strongly Correlated Fermion Systems and the Limit of Infinite Dimensions

We review the dynamical mean-field theory of strongly correlated fermion systems which is based on a mapping of lattice models onto quantum impurity models subject to a self-consistency condition. This mapping is exact in the limit of large lattice coordination (or infinite spatial dimensions). This method can be used for the determination of phase diagrams and the calculation of thermodynamic properties, one-particle Green's functions, and response functions, using analytic and numerical techniques which are described. We review the recent progress in understanding the Hubbard model and the Mott metal-insulator transition within this approach, including some comparison to experiments on three-dimensional transition-metal oxides. Some applications of this method to other models are also reviewed. The present limitations of the approach, and possible extensions of the formalism are finally discussed. Computer programs for the numerical implementation of this method are provided with this article.

cond-mat↗

arXiv1994

Solution of the two impurity, two channel Kondo Model

We solve the two-impurity two-channel Kondo model using a combination of conformal invariance and bosonisation techniques. The odd-even symmetric case is analysed in detail. The RKKY interaction turns out to be exactly marginal, resulting in a line of non-Fermi liquid fixed points. Explicit formulae are given for the critical exponents and for the finite-size spectrum, which depend continuously on a single parameter. The marginal line spans a range of values of the RKKY coupling $I$ which goes from the infinitely strong ferromagnetic point $I=-\infty$ (associated with a 4-channel spin-1 Kondo model) to a finite antiferromagnetic critical value $I_c>0$ beyond which a Fermi liquid is recovered. We also find that, when the odd-even symmetry is broken, the marginal line is unstable for ferromagnetic $I$, while for antiferromagnetic $I$ it extends into a manifold of fixed points.

cond-mat↗