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A. Gutiérrez-Llorente

Publications and source records attributed to A. Gutiérrez-Llorente.

2 recordsLinked to original sources

Dimensionality of vortex matter in superconducting infinite-layer nickelates

Characterizing the dimensionality of the superconducting state in infinite-layer (IL) nickelates is essential for understanding its nature. Most studies have addressed this by examining the anisotropy of the upper critical fields. However, the dominance of Pauli paramagnetic effects over orbital effects complicates the interpretation of these experiments in terms of dimensionality. Here, we approach the question from a different perspective by mapping the vortex phase diagram. We show that superconducting Pr0.8Sr0.2NiO2 thin films with low disorder exhibit a vortex liquid-to-glass transition of a quasi-two-dimensional (2D) nature. In contrast, increasing disorder drives a crossover into a pure 2D state. This demonstrates that pure bidimensionality is an extrinsic property, resulting from the decoupling of NiO2 planes due to enhanced disorder. Our findings establish disorder as a key control parameter of superconductivity in IL nickelates and suggest that it resides within the NiO2 planes, providing two fundamental insights for understanding these materials.

cond-mat.supr-con↗

Epitaxial stabilization of pulsed laser deposited Sr$_{n+1}$Ir$_n$O$_{3n+1}$ thin films: entangled effect of growth dynamics and strain

The subtle balance of electronic correlations, crystal field splitting and spin--orbit coupling in layered Ir$^{4+}$ oxides can give rise to novel electronic and magnetic phases. Experimental progress in this field relies on the synthesis of epitaxial films of these oxides. However, the growth of layered iridates with excellent structural quality is a great experimental challenge. Here we selectively grow high quality single--phase films of Sr$_2$IrO$_4$, Sr$_3$Ir$_2$O$_7$, and SrIrO$_3$ on various substrates from a single Sr$_3$Ir$_2$O$_7$ target by tuning background oxygen pressure and epitaxial strain. We demonstrate a complex interplay between growth dynamics and strain during thin film deposition. Such interplay leads to the stabilization of different phases in films grown on different substrates under identical growth conditions, which cannot be explained by a simple kinetic model. We further investigate the thermoelectric properties of the three phases and propose that weak localization is responsible for the low temperature activated resistivity observed in SrIrO$_3$ under compressive strain.

cond-mat.mtrl-sci↗