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A. H. MacDonald

Publications and source records attributed to A. H. MacDonald.

At least 73 records · Page 4Linked to original sources

Theory of t2g electron-gas Rashba interactions

The spin-degeneracy of Bloch bands in a crystal can be lifted when spin-orbit (SO) coupling is present and inversion symmetry is absent. In two-dimensional electron systems (2DES) spin-degeneracy is lifted by Rashba interaction terms - symmetry invariants that are scalar products of spin and orbital axial vectors. Rashba interactions are symmetry allowed whenever a 2DES is not invariant under reflections through the plane it occupies. In this paper, we use a tight-binding model informed by ab initio electronic structure calculations to develop a theory of Rashba splitting in the t2g bands of the two- dimensional electron systems formed at cubic perovskite crystal surfaces and interfaces. We find that Rashba splitting in these systems is due to atomic-like on-site SO interactions combined with processes in which t2g electrons change orbital character when they hop between metal sites. These processes are absent in a cubic environment and are due primarily to polar lattice distortions which alter the metal-oxygen-metal bond angle.

cond-mat.str-el↗

Photoemission spectra of massless Dirac fermions on the verge of exciton condensation

Angle-resolved photoemission spectroscopy (ARPES) is a powerful probe of electron correlations in two-dimensional layered materials. In this Letter we demonstrate that ARPES can be used to probe the onset of exciton condensation in spatially-separated systems of electrons and holes created by gating techniques in either double-layer graphene or topological-insulator thin films.

cond-mat.str-el↗

Quantized Casimir Force

We investigate the Casimir effect between two-dimensional electron systems driven to the quantum Hall regime by a strong perpendicular magnetic field. In the large separation (d) limit where retardation effects are essential we find i) that the Casimir force is quantized in units of 3\hbar c α^2/(8π^2 d^4), and ii) that the force is repulsive for mirrors with same type of carrier, and attractive for mirrors with opposite types of carrier. The sign of the Casimir force is therefore electrically tunable in ambipolar materials like graphene. The Casimir force is suppressed when one mirror is a charge-neutral graphene system in a filling factor ν=0 quantum Hall state.

cond-mat.mes-hall↗

Topological Magneto-Electric Effect Decay

We address the influence of realistic disorder on the effective magnetic monopole that is induced near the surface of an ideal topological insulator (TI) by azimuthal currents which flow in response to a suddenly introduced external electric charge. We show that when the longitudinal conductivity $σ_{xx} = g (e^2/h)$ is accounted for, the apparent position of a magnetic monopole initially retreats from the TI surface at speed $v_{M} = αc g$, where $α$ is the fine structure constant and $c$ is the speed of light. For the particular case of TI surface states described by a massive Dirac model, we further find that the temperature T=0 Hall currents vanish once the surface charge has been redistributed to screen the external potential.

cond-mat.mes-hall↗

Strong Coulomb drag and broken symmetry in double-layer graphene

Spatially separated electron systems remain strongly coupled by electron-electron interactions even when they cannot exchange particles, provided that the layer separation d is comparable to a characteristic distance l between charge carriers within layers. One of the consequences of this remote coupling is a phenomenon called Coulomb drag, in which an electric current passed through one of the layers causes frictional charge flow in the other layer. Previously, only the regime of weak (d>>l) to intermediate (d ~ l) coupling could be studied experimentally. Here we use graphene-BN heterostructures with d down to 1 nm to probe interlayer interactions and Coulomb drag in the limit d<<l where the two Dirac liquids effectively nest within the same plane, but still can be tuned and measured independently. The strongly interacting regime reveals many unpredicted features that are qualitatively different from those observed previously. In particular, although drag vanishes because of electron-hole symmetry when either layer is neutral, we find that drag is at its strongest when /both/ layers are neutral. Under this circumstance, drag is positive in zero magnetic field but changes its sign and rapidly grows in strength with field. The drag remains strong at room temperature. The broken electron-hole symmetry is attributed to mutual polarization of closely-spaced interacting layers. The two-fluid Dirac system offers a large parameter space for further investigation of strong interlayer interaction phenomena.

cond-mat.mes-hall↗

Competing Ordered States in Bilayer Graphene

We use a perturbative renormalization group approach with short-range continuum model interactions to analyze the competition between isotropic gapped and anisotropic gapless ordered states in bilayer graphene, commenting specifically on the role of exchange and on the importance of spin and valley flavor degeneracy. By comparing the divergences of the corresponding susceptibilities, we conclude that this approach predicts gapped states for flavor numbers N=1,2,4. We also comment briefly on the related gapped states expected in chiral (ABC) trilayer graphene.

cond-mat.str-el↗

Theory of the SrTiO3 Surface State Two-Dimensional Electron Gas

We present a theory of the quasi two-dimensional electron gas (2DEG) systems which appear near the surface of SrTiO$_3$ when a large external electric field attracts carriers to the surface. We find that non-linear and non-local screening by the strongly polarizable SrTiO$_3$ lattice plays an essential role in determining 2DEG properties. The electronic structure always includes weakly bound bulk-like bands that extend over many SrTiO$_3$ layers. At 2D carrier-densities exceeding $\sim 10^{14} {\rm cm}^{-2}$ tightly bound bands emerge that are confined within a few layers of the surface.

cond-mat.str-el↗

Interaction-Enhanced Coherence Between Two-Dimensional Dirac Layers

We estimate the strength of interaction-enhanced coherence between two graphene or topological insulator surface-state layers by solving imaginary-axis gap equations in the random phase approximation. Using a self-consistent treatment of dynamic screening of Coulomb interactions in the gapped phase, we show that the excitonic gap can reach values on the order of the Fermi energy at strong interactions. The gap is discontinuous as a function of interlayer separation and effective fine structure constant, revealing a first order phase transition between effectively incoherent and interlayer coherent phases. To achieve the regime of strong coherence the interlayer separation must be smaller than the Fermi wavelength, and the extrinsic screening of the medium embedding the Dirac layers must be negligible. In the case of a graphene double-layer we comment on the supportive role of the remote $π$-bands neglected in the two-band Dirac model.

cond-mat.mes-hall↗

Visualizing landscapes of the superconducting gap in heterogeneous superconductor thin films: geometric influences on proximity effects

The proximity effect is a central feature of superconducting junctions as it underlies many important applications in devices and can be exploited in the design of new systems with novel quantum functionality. Recently, exotic proximity effects have been observed in various systems, such as superconductor-metallic nanowires and graphene-superconductor structures. However, it is still not clear how superconducting order propagates spatially in a heterogeneous superconductor system. Here we report intriguing influences of junction geometry on the proximity effect for a 2D heterogeneous superconductor system comprised of 2D superconducting islands on top of a surface metal. Depending on the local geometry, the superconducting gap induced in the surface metal region can either be confined to the boundary of the superconductor, in which the gap decays within a short distance (~ 15 nm), or can be observed nearly uniformly over a distance of many coherence lengths due to non-local proximity effects.

cond-mat.supr-con↗

Density, spin, and pairing instabilities in polarized ultracold Fermi gases

We study the influence of population imbalance on the pairing, spin, and density instabilities of a two component ideal Fermi gas after a sudden quench of interactions near a Feshbach resonance. Over a large region of parameters the pairing instability is dominated by finite momentum pairing, suggesting the possibility of observing FFLO-like states in the unstable initial dynamics. Long-wavelength density instabilities are found on the BCS side of the resonance, and are interpreted as a precursor of the phase separation expected at equilibrium. On the BEC side of the resonance, the pairing instability is present for scattering lengths that are larger than a critical value that is only weakly dependent on population imbalance and always smaller than the scattering length at which the Stoner-like spin instability occurs.

cond-mat.quant-gas↗

Quantum Kinetic Theory of Current-Induced Torques in Rashba Ferromagnets

Motivated by recent experimental studies of thin-film devices containing a single ferromagnetic layer, we develop a quantum kinetic theory of current-induced magnetic torques in Rashba-model ferromagnets. We find that current-induced spin-densities that are responsible for the switching behavior are due most essentially to spin-dependent quasiparticle lifetimes and derive analytic expressions for relevant limits of a simple model. Quantitative model parameter estimates suggest that spin-orbit coupling in the adjacent metal normal magnetic layer plays an essential role in the strength of the switching effect.

cond-mat.mes-hall↗

Double-layer graphene and topological insulator thin-film plasmons

We present numerical and analytical results for the optical and acoustic plasmon collective modes of coupled massless-Dirac two-dimensional electron systems. Our results apply to topological insulator (TI) thin films and to two graphene sheets separated by a thin dielectric barrier layer. We find that because of strong bulk dielectric screening TI acoustic modes are locked to the top of the particle-hole continuum and therefore probably unobservable.

cond-mat.mes-hall↗

Josephson current in a four terminal superconductor - exciton condensate - superconductor system

We investigate the transport properties of a bilayer exciton condensate that is contacted by four superconducting leads. We focus on the equilibrium regime and investigate how the Josephson currents induced in the bilayer by phase biases applied to the superconducting electrodes are affected by the presence of an exciton condensate in the bulk of the system. As long as the distance between the superconducting electrodes is much larger than the exciton coherence length, the Josephson current depends only on the difference between the phase biases in the two layers. This result holds true in both short- and long-junction limits. We relate it to a novel correlated four-particle Andreev process which occurs at the superconductor - exciton condensate interface. The system we investigate provides an implementation of the supercurrent mirror proposed by Kitaev as a viable way to realize topologically protected qubits.

cond-mat.supr-con↗

The tunneling density-of-states of interacting massless Dirac fermions

We calculate the tunneling density-of-states (DOS) of a disorder-free two-dimensional interacting electron system with a massless-Dirac band Hamiltonian. The DOS exhibits two main features: i) linear growth at large energies with a slope that is suppressed by quasiparticle velocity enhancement, and ii) a rich structure of plasmaron peaks which appear at negative bias voltages in an n-doped sample and at positive bias voltages in a p-doped sample. We predict that the DOS at the Dirac point is non-zero even in the absence of disorder because of electron-electron interactions, and that it is then accurately proportional to the Fermi energy. The finite background DOS observed at the Dirac point of graphene sheets and topological insulator surfaces can therefore be an interaction effect rather than a disorder effect.

cond-mat.mes-hall↗

Quantum Hall Effects in Graphene-Based Two-Dimensional Electron Systems

In this article we review the quantum Hall physics of graphene based two-dimensional electron systems, with a special focus on recent experimental and theoretical developments. We explain why graphene and bilayer graphene can be viewed respectively as J=1 and J=2 chiral two-dimensional electron gases (C2DEGs), and why this property frames their quantum Hall physics. The current status of experimental and theoretical work on the role of electron-electron interactions is reviewed at length with an emphasis on unresolved issues in the field, including assessing the role of disorder in current experimental results. Special attention is given to the interesting low magnetic field limit and to the relationship between quantum Hall effects and the spontaneous anomalous Hall effects that might occur in bilayer graphene systems in the absence of a magnetic field.

cond-mat.mes-hall↗

Magneto-Optical Faraday and Kerr Effects in Topological Insulator Films and in Other Layered Quantized Hall Systems

We present a theory of the magneto-optical Faraday and Kerr effects of topological insulator (TI) films. For film thicknesses short compared to wavelength, we find that the low-frequency Faraday effect in ideal systems is quantized at integer multiples of the fine structure constant, and that the Kerr effect exhibits a giant $π/2$ rotation for either normal or oblique incidence. For thick films that contain an integer number of half wavelengths, we find that the Faraday and Kerr effects are both quantized at integer multiples of the fine structure constant. For TI films with bulk parallel conduction, we obtain a criterion for the observability of surface-dominated magneto-optical effects. For thin samples supported by a substrate, we find that the universal Faraday and Kerr effects are present when the substrate is thin compared to the optical wavelength or when the frequency matches a thick-substrate cavity resonance. Our theory applies equally well to any system with two conducting layers that exhibit quantum Hall effects.

cond-mat.mes-hall↗

Transport Spectroscopy of Symmetry-Broken Insulating States in Bilayer Graphene

The flat bands in bilayer graphene(BLG) are sensitive to electric fields E\bot directed between the layers, and magnify the electron-electron interaction effects, thus making BLG an attractive platform for new two-dimensional (2D) electron physics[1-5]. Theories[6-16] have suggested the possibility of a variety of interesting broken symmetry states, some characterized by spontaneous mass gaps, when the electron-density is at the carrier neutrality point (CNP). The theoretically proposed gaps[6,7,10] in bilayer graphene are analogous[17,18] to the masses generated by broken symmetries in particle physics and give rise to large momentum-space Berry curvatures[8,19] accompanied by spontaneous quantum Hall effects[7-9]. Though recent experiments[20-23] have provided convincing evidence of strong electronic correlations near the CNP in BLG, the presence of gaps is difficult to establish because of the lack of direct spectroscopic measurements. Here we present transport measurements in ultra-clean double-gated BLG, using source-drain bias as a spectroscopic tool to resolve a gap of ~2 meV at the CNP. The gap can be closed by an electric field E\bot \sim13 mV/nm but increases monotonically with a magnetic field B, with an apparent particle-hole asymmetry above the gap, thus providing the first mapping of the ground states in BLG.

cond-mat.mes-hall↗

The Influence of Remote Bands on Exciton Condensation in Double-Layer Graphene

We examine the influence of remote bands on the tendency toward exciton condensation in a system consisting of two parallel graphene layers with negligible interlayer tunneling. We find that the remote bands can play a crucial supporting role, especially at low carrier densities, and comment on some challenges that arise in attempting quantitative estimates of condensation temperatures.

cond-mat.mes-hall↗