arXiv subjects

A. Henderson

Publications and source records attributed to A. Henderson.

4 recordsLinked to original sources

arXiv2021

A phase diagram for light-induced superconductivity in $κ$-(ET)$_2$-X

Resonant optical excitation of certain molecular vibrations in $κ$-(BEDT-TTF)$_2$Cu[N(CN)$_2$]Br has been shown to induce transient superconducting-like optical properties at temperatures far above equilibrium $T_c$. Here, we report experiments across the bandwidth-tuned phase diagram of this class of materials, and study the Mott insulator $κ$-(BEDT-TTF)$_2$Cu[N(CN)$_2$]Cl and the metallic compound $κ$-(BEDT-TTF)$_2$Cu(NCS)$_2$. We find non-equilibrium photoinduced superconductivity only in $κ$-(BEDT-TTF)$_2$Cu[N(CN)$_2$]Br, indicating that the proximity to the Mott insulating phase and possibly the presence of preexisting superconducting fluctuations are pre-requisites for this effect.

cond-mat.supr-con↗

arXiv2020

Photo-molecular high temperature superconductivity

Superconductivity in organic conductors is often tuned by the application of chemical or external pressure. With this type of tuning, orbital overlaps and electronic bandwidths are manipulated, whilst the properties of the molecular building blocks remain virtually unperturbed.Here, we show that the excitation of local molecular vibrations in the charge-transfer salt $κ-(BEDT-TTF)_2Cu[N(CN)_2]Br$ induces a colossal increase in carrier mobility and the opening of a superconducting-like optical gap. Both features track the density of quasi-particles of the equilibrium metal, and can be achieved up to a characteristic coherence temperature $T^* \approxeq 50 K$, far higher than the equilibrium transition temperature $T_C = 12.5 K$. Notably, the large optical gap achieved by photo-excitation is not observed in the equilibrium superconductor, pointing to a light induced state that is different from that obtained by cooling. First-principle calculations and model Hamiltonian dynamics predict a transient state with long-range pairing correlations, providing a possible physical scenario for photo-molecular superconductivity.

cond-mat.supr-con↗

arXiv2018

Weak ferromagnetism and glassy state in kappa-(BEDT-TTF)2Hg(SCN)2Br

Since the first observation of weak ferromagnetism in the charge-transfer salt kappa-(BEDT-TTF)2-Cu[N(CN)2]Cl [U. Welp et al., Phys. Rev. Lett. 69, 840 (1992)], no further evidence of ferromagnetism in this class of organic materials has been reported. Here we present static and dynamic spin susceptibility measurements on kappa-(BEDT-TTF)2Hg(SCN)2Br revealing weak ferromagnetism below about TWF = 20 K. We suggest that frustrated spins in the molecular dimers suppress long-range order, forming a spin-glass ground state in the insulating phase.

cond-mat.str-el↗

arXiv2017

Measurement of the beam asymmetry $Σ$ for $π^0$ and $η$ photoproduction on the proton at $E_γ= 9$ GeV

We report measurements of the photon beam asymmetry $Σ$ for the reactions $\vecγp\to pπ^0$ and $\vecγp\to pη$ from the GlueX experiment using a 9 GeV linearly-polarized, tagged photon beam incident on a liquid hydrogen target in Jefferson Lab's Hall D. The asymmetries, measured as a function of the proton momentum transfer, possess greater precision than previous $π^0$ measurements and are the first $η$ measurements in this energy regime. The results are compared with theoretical predictions based on $t$-channel, quasi-particle exchange and constrain the axial-vector component of the neutral meson production mechanism in these models.

nucl-ex↗