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A. Honecker

Publications and source records attributed to A. Honecker.

At least 73 records · Page 4Linked to original sources
arXiv2004

Exchange constants and spin dynamics in Mn12-acetate

We have obtained new inelastic neutron scattering (INS) data for the molecular magnet Mn12-acetate which exhibit at least six magnetic peaks in the energy range 5-35 meV. These are compared with a microscopic Heisenberg model for the 12 quantum spins localised on the Mn ions, coupled by four inequivalent magnetic exchange constants. A fit to the magnetic susceptibility under the constraint that the spin of the ground state be S=10 yields two dominant exchange constants of very similar value, J1 ~ J2 ~ 65 K (~ 5.5 meV), and two smaller exchange constants J3 and J4. We compute the low-lying excitations by exact numerical diagonalisation and demonstrate that the parameters determined from the ground state and susceptibility fit provide qualitative agreement with the excitations observed by INS.

cond-mat.str-el↗
arXiv2004

Bond-impurity induced bound states in disordered spin-1/2 ladders

We discuss the effect of weak bond-disorder in two-leg spin ladders on the dispersion relation of the elementary triplet excitations with a particular focus on the appearance of bound states in the spin gap. Both the cases of modified exchange couplings on the rungs and the legs of the ladder are analyzed. Based on a projection on the single-triplet subspace, the single-impurity and small cluster problems are treated analytically in the strong-coupling limit. Numerically, we study the problem of a single impurity in a spin ladder by exact diagonalization to obtain the low-lying excitations. At finite concentrations and to leading order in the inter-rung coupling, we compare the spectra obtained from numerical diagonalization of large systems within the single-triplet subspace with the results of diagrammatic techniques, namely low-concentration and coherent-potential approximations. The contribution of small impurity clusters to the density of states is also discussed.

cond-mat.str-el↗
arXiv2004

Magnetocaloric effect in one-dimensional antiferromagnets

An external magnetic field induces large relative changes in the entropy of one-dimensional quantum spin systems at finite temperatures. This leads to a magnetocaloric effect, i.e. a change in temperature during an adiabatic (de)magnetization process. Several examples of one-dimensional spin-1/2 models are studied by employing the Jordan-Wigner transformation and exact diagonalization. During an adiabatic (de)magnetization process temperature drops in the vicinity of a field-induced zero-temperature quantum phase transition. Comparing different levels of frustration, we find that more frustrated systems cool down to lower temperatures. For geometrically frustrated spin models a finite entropy survives down to zero temperature at certain magnetic fields. This property suggests frustrated quantum spin systems as promising alternative refrigerant materials for low-temperature magnetic refrigeration.

cond-mat.str-el↗
arXiv2004

Transport in dimerized and frustrated spin systems

We analyze the Drude weight for both spin and thermal transport of one-dimensional spin-1/2 systems by means of exact diagonalization at finite temperatures. While the Drude weights are non-zero for finite systems, we find indications of a vanishing of the Drude weights in the thermodynamic limit for non-integrable models implying normal transport behavior.

cond-mat.str-el↗
arXiv2004

Thermal conductivity of one-dimensional spin-1/2 systems

We analyze the thermal conductivity of frustrated spin-1/2 chains within linear-response theory focusing on its frequency dependence at finite temperatures. Using exact diagonalization, the low-frequency limit of the thermal conductivity is discussed in the high-temperature regime.

cond-mat.str-el↗
arXiv2004

Magnetization plateaus in frustrated antiferromagnetic quantum spin models

Plateaus can be observed in the zero-temperature magnetization curve of quantum spin systems at rational values of the magnetization. In one dimension, the appearance of a plateau is controlled by a quantization condition for the magnetization which involves the length of the local spin and the volume of a translational unit cell of the ground state. We discuss examples of geometrically frustrated quantum spin systems with large (in general unbounded) periodicities of spontaneous breaking of translational symmetry in the ground state. In two dimensions, we discuss the square, triangular and Kagome lattices using exact diagonalization (ED) for up to N=40 sites. For the spin-1/2 XXZ model on the triangular lattice we study the nature and stability region of a plateau at one third of the saturation magnetization. The Kagome lattice gives rise to particularly rich behaviour with several plateaus in the magnetization curve and a jump due to local magnon excitations just below saturation.

cond-mat.str-el↗
arXiv2004

Comment on "Anomalous Thermal Conductivity of Frustrated Heisenberg Spin Chains and Ladders"

In a recent letter [Phys. Rev. Lett. 89, 156603 (2002); cond-mat/0201300], Alvarez and Gros have numerically analyzed the Drude weight for thermal transport in spin ladders and frustrated chains of up to 14 sites and have proposed that it remains finite in the thermodynamic limit. In this comment, we argue that this conclusion cannot be sustained if the finite-size analysis is taken to larger system sizes.

cond-mat.str-el↗
arXiv2004

High-field magnetization study of the S = 1/2 antiferromagnetic Heisenberg chain [PM Cu(NO$_3$)$_2$(H$_2$O)$_2$]$_n$ with a field-induced gap

We present a high-field magnetization study of the $S$ = 1/2 antiferromagnetic Heisenberg chain [PM Cu(NO$_3$)$_2$(H$_2$O)$_2$]$_n$. For this material, as result of the Dzyaloshinskii-Moriya interaction and a staggered $g$ tensor, the ground state is characterized by an anisotropic field-induced spin excitation gap and a staggered magnetization. Our data reveal the qualitatively different behavior in the directions of maximum and zero spin excitation gap. The data are analyzed via exact diagonalization of a linear spin chain with up to 20 sites and on basis of the Bethe ansatz equations, respectively. For both directions we find very good agreement between experimental data and theoretical calculations. We extract the magnetic coupling strength $J/k_B$ along the chain direction to 36.3(5) K and determine the field dependence of the staggered magnetization component $m_s$.

cond-mat.mtrl-sci↗
arXiv2003

Exact eigenstates and macroscopic magnetization jumps in strongly frustrated spin lattices

For a class of frustrated spin lattices including e.g. the 1D sawtooth chain, the 2D kagomé and checkerboard, as well as the 3D pyrochlore lattices we construct exact product eigenstates consisting of several independent, localized one-magnon states in a ferromagnetic background. Important geometrical elements of the relevant lattices are triangles being attached to polygons or lines. Then the magnons can be trapped on these polygons/lines. If the concentration of localized magnons is small they can be distributed randomly over the lattice. Increasing the number of localized magnons their distribution over the lattice becomes more and more regular and finally the magnons condensate in a crystal-like state. The physical relevance of these eigenstates emerges in high magnetic fields where they become groundstates of the system. As a result a macroscopic magnetization jump appears in the zero-temperature magnetization curve just below the saturation field. The height of the jump decreases with increasing spin quantum number and vanishes in the classical limit. Thus it is a true macroscopic quantum effect.

cond-mat.str-el↗
arXiv2002

Thermal conductivity of anisotropic and frustrated spin-1/2 chains

We analyze the thermal conductivity of anisotropic and frustrated spin-1/2 chains using analytical and numerical techniques. This includes mean-field theory based on the Jordan-Wigner transformation, bosonization, and exact diagonalization of systems with N<=18 sites. We present results for the temperature dependence of the zero-frequency weight of the conductivity for several values of the anisotropy Δ. In the gapless regime, we show that the mean-field theory compares well to known results and that the low-temperature limit is correctly described by bosonization. In the antiferromagnetic and ferromagnetic gapped regime, we analyze the temperature dependence of the thermal conductivity numerically. The convergence of the finite-size data is remarkably good in the ferromagnetic case. Finally, we apply our numerical method and mean-field theory to the frustrated chain where we find a good agreement of these two approaches on finite systems. Our numerical data do not yield evidence for a diverging thermal conductivity in the thermodynamic limit in case of the antiferromagnetic gapped regime of the frustrated chain.

cond-mat.str-el↗
arXiv2002

Macroscopic magnetization jumps due to independent magnons in frustrated quantum spin lattices

For a class of frustrated spin lattices including the kagome lattice we construct exact eigenstates consisting of several independent, localized one-magnon states and argue that they are ground states for high magnetic fields. If the maximal number of local magnons scales with the number of spins in the system, which is the case for the kagome lattice, the effect persists in the thermodynamic limit and gives rise to a macroscopic jump in the zero-temperature magnetization curve just below the saturation field. The effect decreases with increasing spin quantum number and vanishes in the classical limit. Thus it is a true macroscopic quantum effect.

cond-mat.str-el↗
arXiv2002

Spin dynamics and coherent tunnelling in the molecular magnetic rings Fe_6 and Fe_8

We present detailed calculations of low-energy spin dynamics in the ``ferric wheel'' systems Na:Fe_6 and Cs:Fe_8 in a magnetic field. We compute by exact diagonalisation the low-energy spectra and matrix elements for total-spin and N'eel-vector components, and thus the time-dependent correlation functions of these operators. Comparison of our results with the semiclassical theory of coherent quantum tunnelling of the N'eel vector demonstrates the validity of a two-state description for the low-energy dynamics of ferric wheels. We discuss the implications of our results for mesoscopic quantum coherent phenomena, and for the experimental techniques to observe them, in molecular magnetic rings.

cond-mat.mes-hall↗
arXiv2001

Nishimori point in random-bond Ising and Potts models in 2D

We study the universality class of the fixed points of the 2D random bond q-state Potts model by means of numerical transfer matrix methods. In particular, we determine the critical exponents associated with the fixed point on the Nishimori line. Precise measurements show that the universality class of this fixed point is inconsistent with percolation on Potts clusters for q=2, corresponding to the Ising model, and q=3

cond-mat.stat-mech↗
arXiv2001

Field-Induced Order and Magnetization Plateaux in Frustrated Antiferromagnets

We argue that collinearly ordered states which exist in strongly frustrated spin systems for special rational values of the magnetization are stabilized by thermal as well as quantum fluctuations. These general predictions are tested by Monte Carlo simulations for the classical and Lanczos diagonalization for the S=1/2 frustrated square-lattice antiferromagnet.

cond-mat.str-el↗
arXiv2001

Nishimori point in the 2D +/- J random-bond Ising model

We study the universality class of the Nishimori point in the 2D +/- J random-bond Ising model by means of the numerical transfer-matrix method. Using the domain-wall free-energy, we locate the position of the fixed point along the Nishimori line at the critical concentration value p_c = 0.1094 +/- 0.0002 and estimate nu = 1.33 +/- 0.03. Then, we obtain the exponents for the moments of the spin-spin correlation functions as well as the value for the central charge c = 0.464 +/- 0.004. The main qualitative result is the fact that percolation is now excluded as a candidate for describing the universality class of this fixed point.

cond-mat.dis-nn↗
arXiv2001

Frustrated trimer chain model and Cu3Cl6(H2O)2 2H8C4SO2 in a magnetic field

Recent magnetization and susceptibility measurements on Cu3Cl6(H2O)2 2H8C4SO2 by Ishii et.al. [J. Phys. Soc. Jpn. 69, 340 (2000)] have demonstrated the existence of a spin gap. In order to explain the opening of a spin gap in this copper-trimer system, Ishii et.al. have proposed a frustrated trimer chain model. Since the exchange constants for this model have not yet been determined, we develop a twelfth-order high-temperature series for the magnetic susceptibility and fit it to the experimentally measured one. We find that some of the coupling constants are likely to be ferromagnetic. The combination of several arguments does not provide any evidence for a spin gap in the parameter region with ferromagnetic coupling constants, but further results e.g. for the magnetization process are in qualitative agreement with the experimental observations.

cond-mat.str-el↗
arXiv2001

Emergence of Irrationality: Magnetization Plateaux in Modulated Hubbard Chains

Hubbard chains with periodically modulated coupling constants in a magnetic field exhibit gaps at zero temperature in their magnetic and charge excitations in a variety of situations. In addition to fully gapped situations (plateau in the magnetization curve and charge gap), we have shown [cond-mat/9908398] that plateaux also appear in the presence of massless modes, leading to a plateau with a magnetization m whose value depends continuously on the filling n. Here we detail and extend the arguments leading to such doping-dependent magnetization plateaux. First we analyze the low-lying excitations using Abelian bosonization. We compute the susceptibility and show that due to the constraint of fixed n, it vanishes at low temperatures (thus leading to a magnetization plateau) even in the presence of one massless mode. Next we study correlation functions and show that one component of the superconducting order parameter develops quasi-long-range order on a doping-dependent magnetization plateau. We then use perturbation theory in the on-site repulsion U to compute the width of these plateaux up to first order in U. Finally, we compute groundstate phase diagrams and correlation functions by Lanczos diagonalization of finite clusters, confirming the presence of doping-dependent plateaux and their special properties.

cond-mat.str-el↗