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A. I. Smirnov

Publications and source records attributed to A. I. Smirnov.

42 records · Page 3Linked to original sources

The magnetic ordering in the mixed valence compound beta-Na0.33V2O5

The low-temperature electron spin resonance (ESR) spectra and the static magnetization data obtained for the stoichiometric single crystals of $β$-Na$_{0.33}$V$_2$O$_5$ indicate that this quasi-one-dimensional mixed valence (V4+/V5+) compound demonstrates at $T_N=22$ K the phase transition into the canted antiferromagnetically ordered state. The spontaneous magnetization of $3.4\times 10^{-3}$ $μ_B$ per V$^{4+}$ ion was found to be oriented along the two-fold $b$ axis of the monoclinic structure, the vector of antiferromagnetism is aligned with the $a$ axis and the Dzyaloshinsky vector is parallel to the $c$-axis. The experimental data were successfully described in the frame of the macroscopic spin dynamics and the following values for the macroscopic parameters of the spin system were obtained: the Dzyaloshinsky field $H_D=6$ kOe, the energy gaps of two branches of the spin wave spectrum $Δ_1=48$ GHz and $Δ_2=24$ GHz.

cond-mat.str-el↗

Space-VLBI observations of OH maser OH34.26+0.15: low interstellar scattering

We report on the first space-VLBI observations of the OH34.26+0.15 maser in two main line OH transitions at 1665 and 1667 MHz. The observations involved the space radiotelescope on board the Japanese satellite HALCA and an array of ground radio telescopes. The map of the maser region and images of individual maser spots were produced with an angular resolution of 1 milliarcsec which is several times higher than the angular resolution available on the ground. The maser spots were only partly resolved and a lower limit to the brightness temperature 6x10^{12} K was obtained. The maser seems to be located in the direction of low interstellar scattering, an order of magnitude lower than the scattering of a nearby extragalactic source and pulsar.

astro-ph↗

Investigation of thermal and magnetic properties of defects in a spin-gap compound NaV2O5

The specific heat, magnetic susceptibility and ESR signals of a Na-deficient vanadate Na_xV_2O_5 (x=1.00 - 0.90) were studied in the temperature range 0.07 - 10 K, well below the transition point to a spin-gap state. The contribution of defects provided by sodium vacancies to the specific heat was observed. It has a low temperature part which does not tend to zero till at least 0.3 K and a high temperature power-like tail appears above 2 K. Such dependence may correspond to the existence of local modes and correlations between defects in V-O layers. The magnetic measurements and ESR data reveal S=1/2 degrees of freedom for the defects, with their effective number increasing in temperature and under magnetic field. The latter results in the nonsaturating magnetization at low temperature. No long-range magnetic ordering in the system of defects was found. A model for the defects based on electron jumps near vacancies is proposed to explain the observed effects. The concept of a frustrated two-dimensional correlated magnet induced by the defects is considered to be responsible for the absence of magnetic ordering.

cond-mat.str-el↗

High frequency dielectric and magnetic anomaly at the phase transition in NaV2O5

We found anomalies in the temperature dependence of the dielectric and the magnetic susceptibiliy of NaV_2O_5 in the microwave and far infrared frequency ranges. The anomalies occur at the phase transition temperature T_c, at which the spin gap opens. The real parts of the dielectric constants epsilon_a and epsilon_c decrease below T_c. The decrease of epsilon_a (except for the narrow region close to T_c) is proportional to the intensity of the x-ray reflection appearing at T_c. The dielectric constant anomaly can be explained by the zigzag charge ordering in the ab-plane appearing below T_c. The anomaly of the microwave magnetic losses is probably related to the coupling between the spin and charge degrees of freedom in vanadium ladders.

cond-mat.str-el↗

Magnetic Resonance of the Intrinsic Defects of the Spin-Peierls Magnet CuGeO3

ESR of the pure monocrystals of CuGeO3 is studied in the frequency range 9-75 GHz and in the temperature interval 1.2-25 K. The splitting of the ESR line into several spectral components is observed below 5 K, in the temperature range where the magnetic susceptibility is suppressed by the spin-Peierls dimerization. The analysis of the magnetic resonance signals allows one to separate the signals of the S=1/2- and S=1 defects of the spin-Peierls phase. The value of g-factor of these signals is close to that of the Cu-ion. The additional line of the magnetic resonance is characterized by an anomalous value of the g-factor and by the threshold-like increase of the microwave susceptibility when the microwave power is increasing. The ESR signals are supposingly attributed to two types of the planar magnetic defects, arising at the boundaries of the domains of the spin-Peierls state with the different values of the phase of the dimerization.

cond-mat.str-el↗

Electron-spin-resonance in the doped spin-Peierls compound Cu(1-x)Ni(x)GeO3

ESR-study of the Ni-doped spin-Peierls compound CuGeO3 has been performed in the frequency range 9-75 GHz. At low temperatures the g-factor is smaller than the value expected for Cu- and Ni-ions. This anomaly is explained by the formation of magnetic clusters around the Ni-ions within a nonmagnetic spin-Peierls matrix. The transition into the AFM-state detected earlier by neutron scattering for doped samples was studied by means of ESR. For x=0.032 a gap in the magnetic resonance spectrum is found below the Neel temperature and the spectrum is well described by the theory of antiferromagnetic resonance based on the molecular field approximation. For x=0.017 the spectrum below the Neel point remained gapless. The gapless spectrum of the antiferromagnetic state in weekly doped samples is attributed to the small value of the Neel order parameter and to the magnetically disordered spin-Peierls background.

cond-mat.str-el↗