arXiv subjects

A. Iyo

Publications and source records attributed to A. Iyo.

At least 91 records · Page 5Linked to original sources

arXiv2009

Uniform mixing of antiferromagnetism and high-T_c superconductivity in multilayered copper oxides Ba_2Ca_{n-1}Cu_nO_{2n}F_2 with apical fluorines (n=2,3,4): Cu-NMR/NQR and F-NMR

We report Cu-NMR/NQR and F-NMR studies on the multilayered high-T_c copper oxides Ba_2Ca_{n-1}Cu_nO_{2n}F_2 with n=2,3,4, where n is the number of CuO_2 planes. It is revealed that bi-layered Ba_2CaCu_2O_4F_2 is an underdoped superconductor with hole carriers, which are introduced into CuO_2 planes by an unexpected deviation from the nominal content of apical fluorines. In a previous paper, we proposed a self-doping mechanism as the origin of carrier doping in n=3 and n=4; in the mechanism, electrons are transferred from the inner CuO_2 plane (IP) to the outer one (OP). However, since it has been found that the bi-layered compound is hole doped, we have reexamined the superconducting and magnetic properties in n=3 and n=4 by Cu-NMR/NQR and F-NMR. The extensive NMR studies have confirmed that the apical-fluorine compounds are not self-doped but hole-doped, and that antiferromagnetism (AFM) and superconductivity (SC) coexist in a single CuO_2 plane. In n=4, the AFM ordering occurs at T_N = 80 K, well above T_c=55 K, where the respective AFM moments are M_AFM=0.11 mu_B and 0.18 mu_B at the OP and the IP. In n=3, on the other hand, the underdoped single IP exhibits a spontaneous moment M_AFM=0.12 mu_B at low temperatures and a peak in the nuclear-spin-lattice relaxation rate 1/T_1 of F at T_N=23 K, much lower than T_c = 76 K. We note that the increase in the number of IPs from one to two leads to an increase in T_N due to strengthening the interlayer coupling, although the doping levels for both compounds are almost comparable. The present results strongly suggest that the uniform mixing of AFM and SC is a general property inherent to a single CuO_2 plane in the underdoped regime for hole-doping.

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arXiv2009

Antiferromagnetic phase transition in four-layered high-T_c superconductors Ba_2Ca_3Cu_4O_8(F_yO_{1-y})_2 with T_c=55-102 K: Cu- and F-NMR studies

We report on magnetic characteristics in four-layered high-T_c superconductors Ba_2Ca_3Cu_4O_8(F_yO_{1-y})_2 with apical fluorine through Cu- and F-NMR measurements. The substitution of oxygen for fluorine at the apical site increases the carrier density (N_h) and T_c from 55 K up to 102 K. The NMR measurements reveal that antiferromagnetic order, which can uniformly coexist with superconductivity, exists up to N_h = 0.15, which is somewhat smaller than N_h = 0.17 being the quantum critical point (QCP) for five-layered compounds. The fact that the QCP for the four-layered compounds moves to a region of lower carrier density than for five-layered ones ensures that the decrease in the number of CuO_2 layers makes an interlayer magnetic coupling weaker.

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arXiv2009

Lower Critical Fields of Superconducting PrFeAsO$_{1-y}$ Single Crystals

We have studied the lower critical fields H_{c1} of superconducting iron oxipnictide PrFeAsO_{1-y} single crystals for H parallel and perpendicular to the ab-planes. Measurements of the local magnetic induction at positions straddling the sample edge by using a miniature Hall-sensor array clearly resolve the first flux penetration from the Meissner state. The temperature dependence of H_{c1} for H || c is well scaled by the in-plane penetration depth without showing any unusual behavior, in contrast to previous reports. The anisotropy of penetration lengths at low temperatures is estimated to be ~ 2.5, which is much smaller than the anisotropy of the coherence lengths. This is indicative of multiband superconductivity in this system, in which the active band for superconductivity is more anisotropic. We also point out that the local induction measured at a position near the center of the crystal, which has been used in a number of reports for the determination of H_{c1}, might seriously overestimate the obtained H_{c1}-value.

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arXiv2008

Microwave Penetration Depth and Quasiparticle Conductivity in PrFeAsO_1-y Single Crystals : Evidence for a Full-Gap Superconductor

In-plane microwave penetration depth $λ_{ab}$ and quaiparticle conductivity at 28 GHz are measured in underdoped single crystals of the Fe-based superconductor PrFeAsO$_{1-y}$ ($T_c\approx 35$ K) by using a sensitive superconducting cavity resonator. $λ_{ab}(T)$ shows flat dependence at low temperatures, which is incompatible with the presence of nodes in the superconducting gap $Δ({\bf k})$. The temperature dependence of the superfluid density demonstrates that the gap is non-zero ($Δ/k_BT_c\gtrsim 1.6$) all over the Fermi surface. The microwave conductivity below $T_c$ exhibits an enhancement larger than the coherence peak, reminiscent of high-$T_c$ cuprate superconductors.

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arXiv2008

Spin Fluctuations and Unconventional Superconductivity in the Fe-based Oxypnictide Superconductor LaFeAsO_0.7 probed by 57Fe-NMR

We report $^{57}$Fe-NMR studies on the oxygen-deficient iron (Fe)-based oxypnictide superconductor LaFeAsO$_{0.7}$ ($T_{c}=$ 28 K) enriched by $^{57}$Fe isotope. In the superconducting state, the spin component of $^{57}$Fe-Knight shift $^{57}K$ decreases almost to zero at low temperatures and the nuclear spin-lattice relaxation rate $^{57}(1/T_{1})$ exhibits a $T^{3}$-like dependence without the coherence peak just below $T_{c}$, which give firm evidence of the unconventional superconducting state formed by spin-singlet Cooper pairing. All these events below $T_c$ are consistently argued in terms of the extended s$_{\pm}$-wave pairing with a sign reversal of the order parameter among Fermi surfaces. In the normal state, we found the remarkable decrease of $1/T_1T$ upon cooling for both the Fe and As sites, which originates from the decrease of low-energy spectral weight of spin fluctuations over whole ${\bm q}$ space upon cooling below room temperature. Such behavior has never been observed for other strongly correlated superconductors where an antiferromagnetic interaction plays a vital role in mediating the Cooper pairing.

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arXiv2008

Lattice Dynamics of LaFeAsO_{1-x}F_{x} and PrFeAsO_{1-y} via Inelastic X-Ray Scattering and First-Principles Calculation

The lattice dynamics of LaFeAsO_{1-x}F_{x} (x=0, 0.1) and PrFeAsO_{1-y} (y~0.1) are investigated using inelastic x-ray scattering and ab-initio calculation. Measurements of powder samples provide an approximation to the phonon DOS, while dispersion is measured from a single crystal of PrFeAsO_{1-y}. A model that agrees reasonably well with all of the data at room temperature is built from results of ab-initio calculations by softening the strength of the Fe-As bond by 30%.

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arXiv2008

Genuine Phase Diagram of Homogeneously Doped CuO2 Plane in High-Tc Cuprate Superconductors

We report a genuine phase diagram for a disorder-free CuO_2 plane based on the precise evaluation of the local hole density (N_h) by site-selective Cu-NMR studies on five-layered high-Tc cuprates. It has been unraveled that (1) the antiferromagnetic metallic state (AFMM) is robust up to N_h=0.17, (2) the uniformly mixed phase of superconductivity (SC) and AFMM is realized at N_h< 0.17, (3) the tetracritical point for the AFMM/(AFMM+SC)/SC/PM(Paramagnetism) phases may be present at N_h=0.15 and T=75 K, (4) Tc is maximum close to a quantum critical point (QCP) at which the AFM order collapses, suggesting the intimate relationship between the high-Tc SC and the AFM order. The results presented here strongly suggest that the AFM interaction plays the vital role as the glue for the Cooper pairs, which will lead us to a genuine understanding of why the Tc of cuprate superconductors is so high.

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arXiv2008

Suppression of Magnetic Order by Pressure in BaFe2As2

We performed the dc resistivity and the ZF 75As-NMR measurement of BaFe2As2 under high pressure. The T-P phase diagram of BaFe2As2 determined from resistivity anomalies and the ZF 75As-NMR clearly revealed that the SDW anomaly is quite robust against P.

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arXiv2008

Effect of Structural Parameters on Superconductivity in Fluorine-Free LnFeAsO1-y (Ln=La,Nd)

The crystal structure of LnFeAsO$_{1-y}$ (Ln = La, Nd) has been studied by the powder neutron diffraction technique. The superconducting phase diagram of NdFeAsO$_{1-y}$ is established as a function of oxygen content which is determined by Rietveld refinement. The small As-Fe bond length suggests that As and Fe atoms are connected covalently. FeAs$_4$-tetrahedrons transform toward a regular shape with increasing oxygen deficiency. Superconducting transition temperatures seem to attain maximum values for regular FeAs$_4$-tetrahedrons.

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arXiv2008

75As NMR study of the ternary iron arsenide BaFe2As2

We report 75As-NMR measurements of the ternary iron arsenide BaFe2As2. 75As-NMR spectra clearly revealed that magnetic transition occurs at around 131 K in our samples, which corresponds to the emergence of spin density wave. Temperature dependence of the internal magnetic field suggests that the transition is likely of the first order. The critical-slowing-down phenomenon in the spin-lattice relaxation rate 1/T1 is not pronounced in this material.

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arXiv2008

75As NQR/NMR Studies on Oxygen-deficient Iron-based Oxypnictide Superconductors LaFeAsO_{1-y} (y=0,0.25,0.4) and NdFeAsO_{0.6}

We report 75As-NQR/NMR studies on the oxygen-deficient iron(Fe)-based oxypnictide superconductors LaFeAsO_{0.6} (T_c=28 K) along with the results on LaFeAsO, LaFeAsO_{0.75}(T_c=20 K) and NdFeAsO_{0.6}(T_c=53 K). Nuclear spin-lattice relaxation rate 1/T_1 of 75As NQR at zero field on LaFeAsO_{0.6} has revealed a T^3 dependence below T_c upon cooling without the coherence peak just below T_c, evidencing the unconventional superconducting state with the line-node gap. We have found an intimate relationship between the nuclear quadrupole frequencyof 75As and T_c for four samples used in this study. It implies microscopically that the local configuration of Fe and As atoms is significantly related to the T_c of the Fe-oxypnictide superconductors, namely, the T_c can be enhanced up to 50 K when the local configuration of Fe and As atoms is optimal, in which the band structure may be also optimized through the variation of hybridization between As 4p orbitals and Fe 3d orbitals.

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arXiv2007

Superconducting gap of overdoped Tl2Ba2CuO6+d observed by Raman scattering

We report Raman scattering spectra for single crystals of overdoped Tl2Ba2CuO6+d (Tl-2201) at low temperatures. It was observed that the pair-breaking peaks in A1g and B1g spectra radically shift to lower energy with carrier doping. We interpret it as s-wave component mixing into d-wave, although the crystal structure is tetragonal. Since similar phenomena were observed also in YBa2Cu3Oy and Bi2Sr2CaCu2Oz, we conclude that s-wave mixing is a common property for overdoped high-Tc superconductors.

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arXiv2007

Uniform Mixing of Antiferromagnetism and High-Tc Superconductivity in Electron-doped Layers in Four-layered Ba2Ca3Cu4O8F2 : A New Phenomenon in an Electron Underdoped RegimePhenomenon in an Electron Underdoped Regime

We report Cu- and F-NMR studies on a four-layered high-temperature superconductor Ba2Ca3Cu4O8F2(0234F(2.0)) with apical fluorine (F-1), an undoped 55 K-superconductor with a nominal Cu2+ valence on average. We reveal that this compound exhibits the antiferromagnetism (AFM) with a Neel temperature TN=100 K despite being a Tc= 55 K-superconductor. Through a comparison with a related tri-layered cuprate Ba2Ca2Cu3O6F2 (0223F(2.0)), it is demonstrated that electrons are transferred from the inner plane (IP) to the outer plane (OP) in 0234F(2.0) and 0223F(2.0), confirming the self-doped high-temperature superconductivity (HTSC) having electron and hole doping in a single compound. Remarlably, uniform mixing of AFM and HTSC takes place in both the electron-doped OPs and the hole-doped IPs in 0234F(2.0).

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arXiv2006

Uniform Mixing of High-Tc Superconductivity and Antiferromagnetism on a Single CuO2 Plane in Hg-based Five-layered Cuprate

We report a site selective Cu-NMR study on under-doped Hg-based five-layered high-$T_{\rm c}$ cuprate HgBa2Ca4Cu5Oy with a Tc=72 K. Antiferromagnetism (AF) has been found to take place at TN=290 K, exhibiting a large antiferromagnetic moment of 0.67-0.69uB at three inner planes (IP's). This value is comparable to the values reported for non-doped cuprates, suggesting that the IP may be in a nearly non-doped regime. Most surprisingly, the AF order is also detected with M(OP)=0.1uB even at two outer planes (OP's) that are responsible for the onset of superconductivity (SC). The high-Tc SC at Tc = 72 K can uniformly coexist on a microscopic level with the AF at OP's. This is the first microscopic evidence for the uniform mixed phase of AF and SC on a single CuO2 plane in a simple environment without any vortex lattice and/or stripe order.

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arXiv2005

The Influence of Neutron Irradiation on (B0.65C0.35)Ba1.4Sr0.6Ca2Cu3Oz Superconducting Phase: the Role of the Grain Edge

Using the transport and magnetization measurements the influence of neutron irradiation at a fluence of 5x10$^{17}$ n cm$^{-2}$ on (B0.65C0.35)Ba1.4Sr0.6Ca2Cu3Oz has been investigated. The neutron irradiation was found to decrease critical temperature and transport critical current density, increase the residual and normal state resistivity, and improve the intragranular critical current density with 1.6x10$^{57}$ A/cm$^{2}$ (at 77.3K and in the applied field up to 160 kA m) and ΔMirr/ΔMnonirr ratio (up to factor of 3) at highest field used for investigation. The field dependence of this ratio, which is below the unity at very low field but higher than 1 at high fields, correlated with the shape of the hystertic loops as well as with the change of the transport parameters after irradiation suggests the role of the irradiation induced effects on the grain edges. We discuss these effects in the framework of the Bean-Livingstone surface barriers and geometrical barriers.

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arXiv2005

Fish-tail Effect and Irreversibility Field of (Cu,C)Ba$_{2}$Ca$_{3}$Cu$_{4}$O$_{x}$-(LiF)$_{y}$ superconductor

Addition of (LiF)$_{y<0.15}$, and of proper amount of (AgO)$_{z=0.45-0.8}$ as oxidizing agent, to (Cu,C)Ba$_{2}$Ca$_{3}$Cu$_{4}$O$_{10+d}$ superconductor is useful to control and shift the doping characteristics (hole density and distribution, and level of disorder) into the region where the irreversible properties, i.e. fish-tail effect (FTE) and irreversibility field H$_{irr}$, are improved. Among notable effects are the development of the second magnetization peak with a higher amplitude J$_{c}$, max and the enhancement of H$_{irr}$ at high temperatures, above a certain value T* which depends on both y$_{LiF}$ and z$_{AgO}$. The best results are obtained for the sample with y$_{LiF}$=0.1 and z$_{AgO}$=0.73. This sample preserves its single phase Cu,C-1234 composition. The influence on the FTE and H$_{irr}$ of the interplay between doping characteristics, controlled by LiF and AgO content, is discussed.

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arXiv2004

Coexistence of Superconductivity and Antiferromagnetism in Multilayered High-$T_c$ Superconductor HgBa$_2$Ca$_4$Cu$_5$O$_y$: A Cu-NMR Study

We report a coexistence of superconductivity and antiferromagnetism in five-layered compound HgBa$_2$Ca$_4$Cu$_5$O$_y$ (Hg-1245) with $T_c=108$ K, which is composed of two types of CuO$_2$ planes in a unit cell; three inner planes (IP's) and two outer planes (OP's). The Cu-NMR study has revealed that the optimallydoped OP undergoes a superconducting (SC) transition at $T_c=108$ K, whereas the three underdoped IP's do an antiferromagnetic (AF) transition below $T_N\sim$ 60 K with the Cu moments of $\sim (0.3-0.4)μ_B$. Thus bulk superconductivity with a high value of $T_c=108$ K and a static AF ordering at $T_N=60$ K are realized in the alternating AF and SC layers. The AF-spin polarization at the IP is found to induce the Cu moments of $\sim0.02μ_B$ at the SC OP, which is the AF proximity effect into the SC OP.

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arXiv2003

Simple test for high Jc and low Rs superconducting thin films

A simple method, fishing high-Tc superconductor thin films out of liquid nitrogen bath by a permanent magnet (field > Hc1) due to the effect of high flux pinning, has been suggested to identify films having high critical current density (Jc > 106 A/cm2 at 77 K) and thus a low microwave surface resistance (Rs). We have demonstrated that a Nd-Fe-B magnet, having a maximum field of ~ 0.5 T, could fish out Tl-1223 superconducting thin films on LSAT substrate with a thickness of ~ 5000 Angstrong having Jc > 1 MA/cm2 (at 77 K) whereas it could not fish out other films with Jc < 0.1 MA/cm2 at 77 K. The fished out films exhibit Rs values 237 - 245 ((at 77 K and 10 GHz, which is lower than that (Rs = 317 (() of the best YBCO film at the same temperature and frequency. On the other hand, the non-fishable films show very high Rs values. This method is a very simple tool to test for high Jc and good microwave properties of superconducting films of large area which otherwise require a special and expensive tool.

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