arXiv subjects

A. J. Liu

Publications and source records attributed to A. J. Liu.

12 recordsLinked to original sources

arXiv2020

Predicting plasticity in disordered solids from structural indicators

Amorphous solids lack long-range order. Therefore identifying structural defects -- akin to dislocations in crystalline solids -- that carry plastic flow in these systems remains a daunting challenge. By comparing many different structural indicators in computational models of glasses, under a variety of conditions we carefully assess which of these indicators are able to robustly identify the structural defects responsible for plastic flow in amorphous solids. We further demonstrate that the density of defects changes as a function of material preparation and strain in a manner that is highly correlated with the macroscopic material response. Our work represents an important step towards predicting how and when an amorphous solid will fail from its microscopic structure.

cond-mat.soft↗

arXiv2018

The Spectrum of Structure for Jammed and Unjammed Soft Disks

We investigate the short, medium, and long-range structure of soft disk configurations for a wide range of area fractions and simulation protocols by converting the real-space spectrum of volume fraction fluctuations for windows of width $L$ to the distance $h(L)$ from the window boundary over which fluctuations occur. Rapidly quenched unjammed configurations exhibit size-dependent super-Poissonian long-range features that, surprisingly, approach the totally-random limit even close to jamming. Above and just below jamming, the spectra exhibit a plateau, $h(L)=h_e$, for $L$ larger than particle size and smaller than a cutoff $L_c$ beyond which there are long-range fluctuations. The value of $h_e$ is independent of protocol and characterizes the putative hyperuniform limit. This behavior is compared with that for Einstein solids, with and without hyperuniformity-destroying defects. We find that key structural features of the particle configurations are more evident, as well as easier and more intuitive to quantify, using the real-space spectrum of hyperuniformity lengths rather than the spectral density.

cond-mat.soft↗

arXiv2011

Temperature-pressure scaling for air-fluidized grains on approaches to Point J

We present experiments on a monolayer of air-fluidized beads in which a jamming transition is approached by increasing pressure, increasing packing fraction, and decreasing kinetic energy. This is accomplished, along with a noninvasive measurement of pressure, by tilting the system and examining behavior vs depth. We construct an equation of state and analyze relaxation time vs effective temperature. By making time and effective temperature dimensionless using factors of pressure, bead size, and bead mass, we obtain a good collapse of the data but to a functional form that differs from that of thermal hard-sphere systems. The relaxation time appears to diverge only as the effective temperature to pressure ratio goes to zero.

cond-mat.soft↗

arXiv2010

Kinetic Heterogeneities at Dynamical Crossovers

We perform molecular dynamics simulations of a model glass-forming liquid to measure the size of kinetic heterogeneities, using a dynamic susceptibility $χ_{\rm ss}(a, t)$ that quantifies the number of particles whose dynamics are correlated on the length scale $a$ and time scale $t$. By measuring $χ_{\rm ss}(a, t)$ as a function of both $a$ and $t$, we locate local maxima $χ^\star$ at distances $a^\star$ and times $t^\star$. Near the dynamical glass transition, we find two types of maxima, both correlated with crossovers in the dynamical behavior: a smaller maximum corresponding to the crossover from ballistic to sub-diffusive motion, and a larger maximum corresponding to the crossover from sub-diffusive to diffusive motion. Our results indicate that kinetic heterogeneities are not necessarily signatures of an impending glass or jamming transition.

cond-mat.soft↗

arXiv2009

Excitations of Ellipsoid Packings near Jamming

We study the vibrational modes of three-dimensional jammed packings of soft ellipsoids of revolution as a function of particle aspect ratio $ε$ and packing fraction. At the jamming transition for ellipsoids, as distinct from the idealized case using spheres where $ε= 1$, there are many unconstrained and non-trivial rotational degrees of freedom. These constitute a set of zero-frequency modes that are gradually mobilized into a new rotational band as $|ε- 1|$ increases. Quite surprisingly, as this new band is separated from zero frequency by a gap, and lies below the onset frequency for translational vibrations, $ω^*$, the presence of these new degrees of freedom leaves unaltered the basic scenario that the translational spectrum is determined only by the average contact number. Indeed, $ω^*$ depends solely on coordination as it does for compressed packings of spheres. We also discuss the regime of large $|ε- 1|$, where the two bands merge.

cond-mat.soft↗

arXiv2005

The onset of jamming as the sudden emergence of an infinite $k$-core cluster

A theory is constructed to describe the zero-temperature jamming transition as the density of repulsive soft spheres is increased. Local mechanical stability imposes a constraint on the minimum number of bonds per particle; we argue that this constraint suggests an analogy to $k$-core percolation. The latter model can be solved exactly on the Bethe lattice, and the resulting transition has a mixed first-order/continuous character. The exponents characterizing the continuous part appear to be the same as for the jamming transition. Finally, numerical simulations suggest that in finite dimensions the $k$-core transition can be discontinuous with a nontrivial diverging correlation length.

cond-mat.soft↗

arXiv2005

Reply to "Comment on `Jamming at zero temperature and zero applied stress: The epitome of disorder' "

We answer the questions raised by Donev, Torquato, Stillinger, and Connelly in their "Comment on "Jamming at zero temperature and zero applied stress: The epitome of disorder.' " We emphasize that we follow a fundamentally different approach than they have done to reinterpret random close packing in terms of the "maximally random jammed" framework. We define the "maximally random jammed packing fraction" to be where the largest number of initial states, chosen completely randomly, have relaxed final states at the jamming threshold in the thermodynamic limit. Thus, we focus on an ensemble of states at the jamming threshold, while DTSC are interested in determining the amount of order and degree of jamming for a particular configuration. We also argue that soft-particle systems are as "clean" as those using hard spheres for studying jammed packings and point out the benefits of using soft potentials.

cond-mat.soft↗

arXiv2005

Vibrations and diverging length scales near the unjamming transition

We numerically study the vibrations of jammed packings of particles interacting with finite-range, repulsive potentials at zero temperature. As the packing fraction $ϕ$ is lowered towards the onset of unjamming at $ϕ_{c}$, the density of vibrational states approaches a non-zero value in the limit of zero frequency. For $ϕ>ϕ_{c}$, there is a crossover frequency, $ω^{*}$ below which the density of states drops towards zero. This crossover frequency obeys power-law scaling with $ϕ-ϕ_{c}$. Characteristic length scales, determined from the dominant wavevector contributing to the eigenmode at $ω^{*}$, diverge as power-laws at the unjamming transition.

cond-mat.soft↗

arXiv2004

Effective Temperatures in Driven Systems: Static vs. Time-Dependent Relations

Using simulations of glassy systems under steady-state shear, we compare effective temperatures obtained from static linear response with those from time-dependent fluctuation-dissipation relations. Although these two definitions are not expected to agree, we show that they yield the same answer over two and a half decades of effective temperature. This suggests that a more complete conceptual framework is necessary for effective temperatures in steady-state driven systems.

cond-mat.soft↗

arXiv2003

Jamming at Zero Temperature and Zero Applied Stress: the Epitome of Disorder

We have studied how 2- and 3- dimensional systems made up of particles interacting with finite range, repulsive potentials jam (i.e., develop a yield stress in a disordered state) at zero temperature and applied stress. For each configuration, there is a unique jamming threshold, $ϕ_c$, at which particles can no longer avoid each other and the bulk and shear moduli simultaneously become non-zero. The distribution of $ϕ_c$ values becomes narrower as the system size increases, so that essentially all configurations jam at the same $ϕ$ in the thermodynamic limit. This packing fraction corresponds to the previously measured value for random close-packing. In fact, our results provide a well-defined meaning for "random close-packing" in terms of the fraction of all phase space with inherent structures that jam. The jamming threshold, Point J, occurring at zero temperature and applied stress and at the random close-packing density, has properties reminiscent of an ordinary critical point. As Point J is approached from higher packing fractions, power-law scaling is found for many quantities. Moreover, near Point J, certain quantities no longer self-average, suggesting the existence of a length scale that diverges at J. However, Point J also differs from an ordinary critical point: the scaling exponents do not depend on dimension but do depend on the interparticle potential. Finally, as Point J is approached from high packing fractions, the density of vibrational states develops a large excess of low-frequency modes. All of these results suggest that Point J may control behavior in its vicinity-perhaps even at the glass transition.

cond-mat.soft↗

arXiv2001

Random Packings of Frictionless Particles

We study random packings of frictionless particles at T=0. The packing fraction where the pressure becomes nonzero is the same as the jamming threshold, where the static shear modulus becomes nonzero. The distribution of threshold packing fractions narrows and its peak approaches random close-packing as the system size increases. For packing fractions within the peak, there is no self-averaging, leading to exponential decay of the interparticle force distribution.

cond-mat.soft↗

arXiv2001

Elastically-Driven Linker Aggregation between Two Semi-Flexible Polyelectrolytes

The behavior of mobile linkers connecting two semi-flexible charged polymers, such as polyvalent counterions connecting DNA or F-actin chains, is studied theoretically. The chain bending rigidity induces an effective repulsion between linkers at large distances while the inter-chain electrostatic repulsion leads to an effective short range inter-linker attraction. We find a rounded phase transition from a dilute linker gas where the chains form large loops between linkers to a dense disordered linker fluid connecting parallel chains. The onset of chain pairing occurs within the rounded transition.

cond-mat.soft↗