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A. J. Millis

Publications and source records attributed to A. J. Millis.

At least 55 records · Page 3Linked to original sources

Optical and Hall conductivities of a thermally disordered two-dimensional spin-density wave: two-particle response in the pseudogap regime of electron-doped high-$T_c$ superconductors

We calculate the longitudinal ($σ_{xx}$) and Hall ($σ_{xy}$) optical conductivities for two-dimensional metals with thermally disordered antiferromagnetism using a generalization of an approximation introduced by Lee, Rice and Anderson for the self energy. The conductivities are calculated from the Kubo formula, with current vertex function treated in a conserving approximation satisfying the Ward identity. In order to obtain a finite DC limit, we introduce phenomenologically impurity scattering, with relaxation time $τ$. $σ_{xx}(Ω)$ satisfies the $f$-sum rule. For the infinitely peaked spin correlation function, $χ(\mathbf{q})\propto δ(\mathbf{q}-\mathbf{Q})$, we recover the expressions for the conductivities in the mean-field theory of the ordered state. When the spin correlation length $ξ$ is large but finite, both $σ_{xx}$ and $σ_{xy}$ show behaviors characteristic of the state with long-range order. The calculation runs into difficulty for $Ω\lesssim 1/τ$. The difficulties are traced to an inaccurate treatment of the very low energy density of states within the Lee-Rice-Anderson approximation. The results for $σ_{xx}(Ω)$ and $σ_{xy}(Ω)$ are qualitatively consistent with data on electron-doped cuprates when $Ω>1/τ$.

cond-mat.str-el↗

Experimental determination of the Weiss temperature of Mn$_{12}$-ac and Mn$_{12}$-ac-MeOH

We report measurements of the susceptibility in the temperature range from $3.5$ K to $6.0$ K of a series of Mn$_{12}$-ac and Mn$_{12}$-ac-MeOH samples in the shape of rectangular prisms of length $l_c$ and square cross-section of side $l_a$. The susceptibility obeys a Curie-Weiss Law, $χ=C/(T-θ)$, where $θ$ varies systematically with sample aspect ratio. Using published demagnetization factors, we obtain $θ$ for an infinitely long sample corresponding to intrinsic ordering temperatures $T_c \approx 0.85$ K and $\approx 0.74$ K for Mn$_{12}$-ac and Mn$_{12}$-ac-MeOH, respectively. The difference in $T_c$ for two materials that have nearly identical unit cell volumes and lattice constant ratios suggests that, in addition to dipolar interactions, there is a non-dipolar (exchange) contribution to the Weiss temperature that differs in the two materials because of the difference in ligand molecules.

cond-mat.mtrl-sci↗

Lifshitz Transition in Underdoped Cuprates

Recent studies show that quantum oscillations thought to be associated with a density wave reconstructed Fermi surface disappear at a critical value of the doping for YBa2Cu3O6+y, and the cyclotron mass diverges as the critical value is approached from the high doping side. We argue that the phenomenon is due to a Lifshitz transition where the pockets giving rise to the quantum oscillations connect to form an open (quasi-1d) Fermi surface. The estimated critical doping is close to that found by experiment, and the theory predicts a logarithmic divergence of the cyclotron mass with a coefficient comparable to that observed in experiment.

cond-mat.supr-con↗

Theory of oxygen K-edge x-ray absorption spectra of cuprates

The dynamical mean-field theory of the three-band model of copper-oxide superconductors is used to calculate the doping dependence of the intensity of the oxygen K-edge x-ray absorption spectra of high-$T_c$ copper oxide superconductors. The model is found not to reproduce the results of a recent experiment, suggesting that at sufficiently high doping the physics beyond the conventional three-band model becomes important.

cond-mat.supr-con↗

Fluctuation-driven first order behavior near the T=0 two dimensional stripe to fermi liquid transition

The possibility is investigated that competition between fluctuations at different symmetry-related ordering wave vectors may affect the quantum phase transition between a fermi liquid and a longitudinal spin density wave state, in particular giving rise to an intermediate 'nematic' state with broken rotational symmetry but unbroken translational symmetry. At the marginal dimension the nematic transition is found to be preempted by a first order transition but a weak symmetry breaking field restores a second order magnetic transition with an intermediate regime in which correlations substantially enhance the broken rotational symmetry. Comparison to recent experiments is made.

cond-mat.str-el↗

Optical conductivity in cluster dynamical mean field theory: formalism and application to high temperature superconductors

The optical conductivity of the one-band Hubbard model is calculated using the 'Dynamical Cluster Approximation' implementation of dynamical mean field theory for parameters appropriate to high temperature copper-oxide superconductors. The calculation includes vertex corrections and the result demonstrates their importance. At densities of one electron per site, an insulating state is found with gap value and above-gap absorption consistent with measurements. As carriers are added the above gap conductivity rapidly weakens and a three component structure emerges, with a low frequency 'Drude' peak, a mid-infrared absorption, and a remnant of the insulating gap. The mid-infrared feature obtained at intermediate dopings is shown to arise from a pseudogap structure in the density of states. On further doping the conductivity evolves to the Drude peak plus weakly frequency dependent tail structure expected for less strongly correlated metals.

cond-mat.str-el↗

Addendum: Theory of low-temperature Hall effect in stripe-ordered cuprates

We supplement a previously published calculation of the Hall effect in stripe ordered cuprates by presenting results for the physically relevant sign of the potential arising from charge ordering. The new results are more consistent with data, underscoring the importance of charge ordering in cuprates.

cond-mat.str-el↗

Local Order and the gapped phase of the Hubbard model: a plaquette dynamical mean field investigation

The four-site DCA method of including intersite correlations in the dynamical mean field theory is used to investigate the metal-insulator transition in the Hubbard model. At half filling a gap-opening transition is found to occur as the interaction strength is increased beyond a critical value. The gapped behavior found in the 4-site DCA approximation is shown to be associated with the onset of strong antiferromagnetic and singlet correlations and the transition is found to be potential energy driven. It is thus more accurately described as a Slater phenomenon (induced by strong short ranged order) than as a Mott phenomenon. Doping the gapped phase leads to a non-Fermi-liquid state with a Fermi surface only in the nodal regions and a pseudogap in the antinodal regions at lower dopings $x \lesssim 0.15$ and to a Fermi liquid phase at higher dopings.

cond-mat.str-el↗

Theory of Low-Temperature Hall Effect in Stripe--Ordered Cuprates

We investigate the effect of static anti-phase stripe order on the weak-field Hall effect of electrons on a two-dimensional square lattice with electron dispersion appropriate to the high T$_c$ cuprates. We first consider the cases where the magnitudes of the spin and charge stripe potentials are smaller than or of the same order as the bandwidth of the two-dimensional electrons, so that the electronic properties are not too strongly one-dimensional. In a model with only spin stripe potential, and at carrier concentrations appropriate to hole-doped cuprates, increasing the stripe scattering potential from zero leads to an increase in $R_H$, followed by a sign change. If the scattering amplitude is yet further increased, a second sign change occurs. The results are in semiquantitative agreement with data. In a charge-stripe-potential-only model, $R_H$ increases as the charge stripe scattering strength increases, with no sign change occurring. In a model with both spin and charge stripe potentials, $R_H$ may be enhanced or may change sign, depending on the strengths of the two scattering potentials. We also consider the case in which the magnitudes of the stripe potentials are much larger than the bandwidth, where analytical results can be obtained. In this limit, the system is quasi-one-dimensional, while $R_H$ remains finite and its sign is determined by the carrier density and the electron band parameters.

cond-mat.str-el↗

Optical conductivity and the correlation strength of high temperature copper-oxide superconductors

High temperature copper-oxide-based superconductivity is obtained by adding carriers to insulating "parent compounds". It is widely believed the parent compounds are "Mott" insulators, in which the lack of conduction arises from anomalously strong electron-electron repulsion, and that the unusual properties of Mott insulators are responsible for high temperature superconductivity. This paper presents a comparison of optical conductivity measurements and theoretical calculations which challenges this belief. The analysis indicates that the correlation strength in the cuprates is not as strong as previously believed, that the materials are not properly regarded as Mott insulators, that antiferromagnetism is essential to obtain the insulating state and, by implication, that antiferromagnetism is essential to the properties of the doped metallic and superconducting state as well.

cond-mat.str-el↗

Gapless superconductivity and the Fermi arc in the cuprates

We argue that the Fermi arc observed in angle resolved photoemission measurements in underdoped cuprates can be understood as a consequence of inelastic scattering in a d-wave superconductor. We analyze this phenomenon in the context of strong coupling Eliashberg theory, deriving a `single lifetime' model for describing the temperature evolution of the spectral gap as measured by single particle probes such as photoemission and tunneling.

cond-mat.str-el↗

Antiphase Stripe Order as the Origin of Electron Pockets Observed in 1/8-Hole-Doped Cuprates

Recent quantum oscillation measurements on underdoped cuprates are shown to be consistent with the predictions of a mean field theory of the 1/8 magnetic antiphase stripe order proposed to occur in high-$T_c$ cuprates. In particular, for intermediate values of the stripe order parameter, the magneto-transport is found to be dominated by an electron pocket.

cond-mat.supr-con↗

Nonequilibrium quantum criticality in open electronic systems

A theory is presented of quantum criticality in open (coupled to reservoirs) itinerant electron magnets, with nonequilibrium drive provided by current flow across the system. Both departures from equilibrium at conventional (equilibrium) quantum critical points and the physics of phase transitions induced by the nonequilibrium drive are treated. Nonequilibrium-induced phase transitions are found to have the same leading critical behavior as conventional thermal phase transitions.

cond-mat.mes-hall↗

Interference as a Probe of Spin Incoherence in Strongly Interacting Quantum Wires

We show that interference experiments can be used to identify the spin-incoherent regime of strongly interacting one-dimensional conductors. Two qualitative signatures of spin-incoherence are found: a strong magnetic field dependence of the interference contrast and an anomalous scaling of the interference contrast with the applied voltage, with a temperature and magnetic field dependent scaling exponent. The experiments distinguish the spin-incoherent from the spin-polarized regime, and so may be useful in deciding between alternative explanations proposed for the anomalous conductance quantization observed in quantum point contacts and quantum wires at low density.

cond-mat.mes-hall↗

Photoemission from buried interfaces in SrTiO3/LaTiO3 superlattices

We have measured photoemission spectra of SrTiO3/LaTiO3 superlattices with a topmost SrTiO3 layer of variable thickness. Finite coherent spectral weight with a clear Fermi cut-off was observed at chemically abrupt SrTiO3/LaTiO3 interfaces, indicating that an ``electronic reconstruction'' occurs at the interface between the Mott insulator LaTiO3 and the band insulator SrTiO3. For SrTiO3/LaTiO3 interfaces annealed at high temperatures (~ 1000 C), which leads to Sr/La atomic interdiffusion and hence to the formation of La1-xSrxTiO3-like material, the intensity of the incoherent part was found to be dramatically reduced whereas the coherent part with a sharp Fermi cut-off is enhanced due to the spread of charge. These important experimental features are well reproduced by layer dynamical-mean-field-theory calculation.

cond-mat.mtrl-sci↗

Nonanalytic corrections to the specific heat of a three-dimensional Fermi liquid

We revisit the issue of the leading nonanalytic corrections to the temperature dependence of the specific heat coefficient, $γ(T)=C(T)/T,$ for a system of interacting fermions in three dimensions. We show that the leading temperature dependence of the specific heat coefficient $γ(T)-γ(0) \propto T^3 \ln T$ comes from two physically distinct processes. The first process involves a thermal excitation of a single particle-hole pair, whose components interact via a nonanalytic dynamic vertex. The second process involves an excitation of three particle-hole pairs which interact via the analytic static fixed-point vertex. We show that the single-pair contribution is expressed via the backscattering amplitude of quasiparticles at the Fermi surface. The three-pair contribution does not have a simple expression in terms of scattering in particular directions. We clarify the relation between these results and previous literature on both 3D and 2D systems, and discuss the relation between the nonanalyticities in $γ$ and those in spin susceptibilities.

cond-mat.str-el↗

Spin dynamics and violation of the fluctuation dissipation theorem in a non-equilibrium ohmic spin boson model

We present results for the dynamics of an impurity spin coupled to a magnetic field and to two ohmic baths which are out-of equilibrium due to the application of a bias voltage. Both the non-equilibrium steady state and the rate constants describing the approach to steady state are found to depend sensitively on the relative strengths of a magnetic field and a voltage dependent decoherence rate. Computation of physical quantities including the frequency dependent ratio of response to correlation functions and the probabilities of the two spin states allows the extraction of voltage dependent effective temperatures. The temperatures extracted from different quantities differ from one another in magnitude and their dependence on parameters, and in general are non-monotonic.

cond-mat.mes-hall↗