arXiv subjects

A. Junod

Publications and source records attributed to A. Junod.

15 recordsLinked to original sources

arXiv2006

Thermodynamic origin of the peak effect in the superconductor Nb3Sn

We report a pronounced peak effect in the magnetization and the magnetocaloric coefficient in a single crystal of the superconductor Nb3Sn. As the origin of the magnetization peak effect in classical type-II superconductors is still strongly debated, we performed an investigation of its underlying thermodynamics. Calorimetric experiments performed during field sweeps at constant temperatures reveal that the sharp increase in the current density occurs concurrently with additional degrees of freedom in the specific heat due to thermal fluctuations and a liquid vortex phase. No latent heat due to a direct first-order melting of a Bragg glass phase into the liquid phase is found which we take as evidence for an intermediate glass phase with enhanced flux pinning. The Bragg glass phase can however be restored by a small AC field. In this case a first-order vortex melting transition with a clear hysteresis is found. In the absence of an AC field the intermediate glass phase is located within the field range of this hysteresis. This indicates that the peak effect is associated with the metastability of an underlying first-order vortex melting transition.

cond-mat.supr-con↗

arXiv2006

Thermal fluctuations and vortex melting in the classical superconductor Nb3Sn from high-resolution specific-heat measurements

The range of critical thermal fluctuations in classical bulk superconductors is extremely small and especially in low fields hardly experimentally inaccessible. With a new type of calorimeter we have been able to resolve a small lambda anomaly within a narrow temperature range around the Hc2 line. We show that the evolution of the anomaly as a function of magnetic field follows scaling laws expected in the presence of critical fluctuations. The lower onset of the fluctuation regime shows many characteristics of a continuous solid-to-liquid transition in the vortex matter. It can be driven into a first-order vortex melting transition by a small AC field which helps the vortex matter to reach equilibrium.

cond-mat.supr-con↗

arXiv2005

Superconductivity mediated by a soft phonon mode: specific heat, resistivity, thermal expansion and magnetization of YB6

The superconductor YB6 has the second highest critical temperature Tc among the boride family MBn. We report measurements of the specific heat, resistivity, magnetic susceptibility and thermal expansion from 2 to 300 K, using a single crystal with Tc = 7.2 K. The superconducting gap is characteristic of medium-strong coupling. The specific heat, resistivity and expansivity curves are deconvolved to yield approximations of the phonon density of states, the spectral electron-phonon scattering function and the phonon density of states weighted by the frequency-dependent Grueneisen parameter respectively. Lattice vibrations extend to high frequencies >100 meV, but a dominant Einstein-like mode at ~8 meV, associated with the vibrations of yttrium ions in oversized boron cages, appears to provide most of the superconducting coupling and gives rise to an unusual temperature behavior of several observable quantities. A surface critical field Hc3 is also observed.

cond-mat.supr-con↗

arXiv2005

On the Origin of the Double Superconducting Transition in Overdoped YBa2Cu3Ox

The superconducting transition in a single overdoped, detwinned YBa2Cu3Ox (YBCO) crystal is studied using four different probes. Whereas the AC and DC magnetic susceptibilities find a dominant transition at 88 K with a smaller effect near 92 K, the specific heat and electrical resistivity reveal only a single transition at 88 K and 92 K, respectively. Under hydrostatic pressures to 0.60 GPa these two transitions shift in opposite directions, their separation increasing. The present experiments clearly show that the bulk transition lies at 88 K and originates from fully oxygenated YBCO; the 92 K transition likely arises from filamentary superconductivity in a minority optimally doped phase (< 1 %) of YBCO located at or near the crystal surface.

cond-mat.supr-con↗

arXiv2005

Specific heat, magnetic susceptibility, resistivity and thermal expansion of the superconductor ZrB12

In an attempt to clarify conflicting published data, we report new measurements of specific heat, resistivity, magnetic susceptibility, and thermal expansivity up to room temperature for the 6 K superconductor ZrB12, using well-characterized single crystals with a residual resistivity ratio >9. The specific heat gives the bulk result 2*delta(0)/(k_B*Tc)=3.7 for the superconducting gap ratio, and excludes multiple gaps and d-wave symmetry for the Cooper pairs. The Sommerfeld constant gamma_n = 0.34 mJ K-2 gat-1 and the magnetic susceptibility xsi = -2.1 x 10^-5 indicate a low density of states at the Fermi level. The Debye temperature theta_D is in the range 1000-1200 K near zero and room temperature, but decreases by a factor of ~2 at ~35 K. The specific heat and resistivity curves are inverted to yield approximations of the phonon density of states F(omega) and the spectral electron-phonon scattering function alpha_tr^2 F(omega), respectively. Both unveil a 15 meV mode, attributed to Zr vibrations in oversized B cages, which gives rise to electron-phonon coupling. The thermal expansivity further shows that this mode is anharmonic, while the vanishingly small discontinuity at Tc establishes that the cell volume is nearly optimal with respect to Tc.

cond-mat.supr-con↗

arXiv2005

Reversible and irreversible magnetocaloric effect in the NdBa_2Cu_3O_7 superconductor in relation with specific heat and magnetization

A recently developed technique for measuring the isothermal magnetocaloric coefficient ($M_T$) is applied to the study of a superconducting NdBa$_2$Cu$_3$O$_7$ single crystal. Results are compared with magnetization ($M$) and specific heat ($C$). In the reversible region both $C$ and $M_T$ follow the scaling law of the 3D-xy universality class. The anomalies connected with flux-line lattice melting are visible on $M_T(B)$ curves as peaks and steps, similar to $C(T)$ curves yet with much smaller background. At lower temperature, in the irreversible region the $M_T(B)$ behaviour resembles more that of $M(B)$, exhibiting the "fishtail" effect. Our results confirm that the peculiarities of the phase diagram known from the high temperature superconductor YBa$_2$Cu$_3$O$_7$, e.g. vortex melting, dominance of critical fluctuations and absence of a $B_{c2}$ critical field line, are a common property of RE-123 systems.

cond-mat.supr-con↗

arXiv2004

Specific heat of Nb_3Sn: The case for a second energy gap

We present new specific heat data for Nb3Sn, a well-known technically applied superconductor with a critical temperature T_c ~ 18 K, in the temperature range from 1.2 to 200 K in zero magnetic field, and from 1.5 to 22 K in fields H <= 16 T. The particularly dense and homogeneous polycrystalline sample used for this study is characterized in detail. We determine the bulk upper critical field H_c2(T) from specific heat data, and the Sommerfeld constant Gamma from the entropy S(T). We investigate in detail a low-temperature anomaly already noticed in previous investigations in zero field, and find that this feature can be quantitatively ascribed to the presence of a second superconducting gap 2 Delta_S(0) ~ 0.8 k_B T_c, in addition to the main one 2 Delta_L(0) ~ 4.9 k_B T_c. The signature of this minor gap, which affects 7.5% of the electronic density-of-states, vanishes in fields above ~ 7 T.

cond-mat.supr-con↗

arXiv2002

Unusual effects of anisotropy on the specific heat of ceramic and single crystal MgB2

The two-gap structure in the superconducting state of MgB_2 gives rise to unusual thermodynamic properties which depart markedly from the isotropic single-band BCS model, both in their temperature- and field dependence. We report and discuss measurements of the specific heat up to 16 T on ceramic, and up to 14 T on single crystal samples, which demonstrate these effects in the bulk. The behavior in zero field is described in terms of two characteristic temperatures, a crossover temperature Tc_pi ~ 13 K, and a critical temperature Tc = Tc_sigma ~ 38 K, whereas the mixed-state specific heat requires three characteristic fields, an isotropic crossover field Hc2_pi ~ 0.35 T, and an anisotropic upper critical field with extreme values Hc2_sigma_c ~ 3.5 T and Hc2_sigma_ab ~ 19 T, where the indexes πand σrefer to the 3D and 2D sheets of the Fermi surface. Irradiation-induced interband scattering tends to move the gaps toward a common value, and increases the upper critical field up to ~ 28 T when Tc = 30 K.

cond-mat.supr-con↗

arXiv2002

Specific heat of single crystal MgB_2: a two-band superconductor with two different anisotropies

Heat-capacity measurements of a 39 microgramm MgB_2 single crystal in fields up to 14 T and below 3 K allow the determination of the low-temperature linear term of the specific heat, its field dependence and its anisotropy. Our results are compatible with two-band superconductivity, the band carrying the small gap being isotropic, that carrying the large gap having an anisotropy of ~ 5. Three different upper critical fields are thus needed to describe the superconducting state of MgB2.

cond-mat.supr-con↗

arXiv2002

Specific heat of heavy fermion CePd2Si2 in high magnetic fields

We report specific heat measurements on the heavy fermion compound CePd2Si2 in magnetic fields up to 16 T and in the temperature range 1.4-16 K. A sharp peak in the specific heat signals the antiferromagnetic transition at T_N ~ 9.3 K in zero field. The transition is found to shift to lower temperatures when a magnetic field is applied along the crystallographic a-axis, while a field applied parallel to the tetragonal c-axis does not affect the transition. The magnetic contribution to the specific heat below T_N is well described by a sum of a linear electronic term and an antiferromagnetic spin wave contribution. Just below T_N, an additional positive curvature, especially at high fields, arises most probably due to thermal fluctuations. The field dependence of the coefficient of the low temperature linear term, gamma_0, extracted from the fits shows a maximum at about 6 T, at the point where an anomaly was detected in susceptibility measurements. The relative field dependence of both T_N and the magnetic entropy at T_N scales as [1-(B/B_0)^2] for B // a, suggesting the disappearance of antiferromagnetism at B_0 ~ 42 T. The expected suppression of the antiferromagnetic transition temperature to zero makes the existence of a magnetic quantum critical point possible.

cond-mat.str-el↗

arXiv2001

Phenomenological two-gap model for the specific heat of MgB_2

We show that the specific heat of the superconductor MgB_2 (MgB2) in zero field, for which significant non-BCS features have been reported, can be fitted, essentially within experimental error, over the entire range of temperature to T_c by a phenomenological two-gap model. The resulting gap parameters agree with previous determinations from band-structure calculations, and from various spectroscopic experiments. The determination from specific heat, a bulk property, shows that the presence of two superconducting gaps in MgB_2 is a volume effect.

cond-mat.supr-con↗

arXiv2001

Specific heat in the superconducting and normal state (2-300 K, 0-16 Teslas), and magnetic susceptibility of the 38-K superconductor MgB2: evidence for a multicomponent gap

The specific heat C of a sintered polycrystalline sample of MgB2 with a bulk superconducting transition temperature Tc=36.7 K is measured as a function of the temperature (2-300 K) and magnetic field (0-16 T), together with magnetic properties (normal-state susceptibility, superconducting state magnetization, etc.). The Sommerfeld constant gamma=0.89+-0.05 mJ/K^2/gat (2.7 mJ/K^2/mol) is determined in the normal state above Hc2. The normal- and superconducting state entropies are equal at Tc. Several moments of the phonon density of states are obtained from the lattice specific heat. We report bulk values for: the thermodynamic critical field, the slope of the upper critical field, the Ginzburg-Landau parameter, the coherence length, the lower critical field, the London penetration depth. These results characterize MgB2 as a type-II superconductor. The nearly quadratic dependence of C(T) versus T at T<<Tc, its non-linear field dependence, and the discrepancy between the electron-phonon coupling constant lambda_ep as determined by the renormalization of the electron density-of-states (lambda_ep=0.6) and by McMillan's equation for isotropic superconductors (lambda_ep=1.1), are inconsistent with a single isotropic gap. In addition to high phonon frequencies, anisotropy or two-band gap structure may explain why the critical temperature of this superconductor is high in spite of its low condensation energy, which does not exceed 1/16 of that of YBa2Cu3O7 and 1/4 of that of Nb3Sn.

cond-mat.supr-con↗

arXiv1999

Calorimetric Investigation of CeRu2Ge2 up to 8 GPa

We have developed a calorimeter able to give a qualitative picture of the specific heat of a sample under high pressure up to approximately 10 GPa. The principle of ac-calorimetry was adapted to the conditions in a high pressure clamp. The performance of this technique was successfully tested with the measurement of the specific heat of CeRu2Ge2 in the temperature range 1.5 K<T<12 K. The phase diagram of its magnetic phases is consistent with previous transport measurements.

cond-mat.str-el↗

arXiv1997

Observation of d-wave scaling relations in the mixed-state specific heat of YBa2Cu3O7

The low temperature specific heat C(B,T) of an YBa2Cu3O7.00 single crystal is measured from 1.2 to 10 K in magnetic fields up to 14 T. The anisotropic component Caniso(T,B)=C(T,B//c)-C(T,B//ab) is a pure vortex quantity obtained directly from experiment. It follows a scaling relation predicted recently for line nodes characteristic of d-wave vortices. Our experimental field and temperature range corresponds to a crossover region where the limit Caniso(T,B)is proportional to T*sqrt(B) does not strictly apply. The variation of the entropy caused by the magnetic field at low T is thermodynamically compatible with measurements near Tc.

cond-mat.supr-con↗

arXiv1996

Transport Properties, Thermodynamic Properties, and Electronic Structure of SrRuO3

SrRuO$_3$ is a metallic ferromagnet. Its electrical resistivity is reported for temperatures up to 1000K; its Hall coefficient for temperatures up to 300K; its specific heat for temperatures up to 230K. The energy bands have been calculated by self-consistent spin-density functional theory, which finds a ferromagnetic ordered moment of 1.45$μ_{\rm B}$ per Ru atom. The measured linear specific heat coefficient $γ$ is 30mJ/mole, which exceeds the theoretical value by a factor of 3.7. A transport mean free path at room temperature of $\approx 10 Å$ is found. The resistivity increases nearly linearly with temperature to 1000K in spite of such a short mean free path that resistivity saturation would be expected. The Hall coefficient is small and positive above the Curie temperature, and exhibits both a low-field and a high-field anomalous behavior below the Curie temperature.

cond-mat↗