arXiv subjects

A. K. Zvezdin

Publications and source records attributed to A. K. Zvezdin.

At least 37 records · Page 2Linked to original sources

arXiv2021

Excitation and Detection of THz Coherent Spin Waves in Antiferromagnetic $\mathrm{α-Fe_2O_3}$

The efficiency of ultrafast excitation of spins in antiferromagnetic $\mathrm{α-Fe_{2}O_{3}}$ using nearly single-cycle THz pulse is studied as a function of the polarization of the THz pulse and the sample temperature. Above the Morin point the most efficient excitation is achieved when the magnetic field of the THz pulse is perpendicular to the antiferromagnetically coupled spins. Using the experimental results and equations of motion for spins, we show that the mechanism of the spin excitation above and below the Morin point relies on magnetic-dipole interaction of the THz magnetic field with spins and the efficiency of the coupling is proportional to the time derivative of the magnetic field.

cond-mat.str-el↗

arXiv2021

Anomalies in the dynamics of ferrimagnets near the angular momentum compensation point

In this paper, we elaborate analytical theory of domain wall dynamics close to the angular momentum compensation point based on non-linear dynamic equations derived from the effective Lagrangian of a ferrimagnet. Analysis of the precession angle and domain wall velocity oscillations in post Walker regime in a ferrimagnet is performed. In the framework of the proposed model, we explore dynamic processes in the Walker and post Walker regimes. We show that although spin oscillations quench the dynamics of domain walls near the Walker breakdown field, a further increase of the driving magnetic field increases domain wall speed and mobility. An anomalous behavior of domain wall dynamic properties near the angular momentum compensation point in ferrimagnets is discussed.

cond-mat.mtrl-sci↗

arXiv2021

THz Field-induced Spin Dynamics in Ferrimagnetic Iron Garnets

THz magnetization dynamics is excited in ferrimagnetic thulium iron garnet with a picosecond, single-cycle magnetic field pulse and seen as a high-frequency modulation of the magneto-optical Faraday effect. Data analysis combined with numerical modelling and evaluation of the effective Lagrangian allow us to conclude that the dynamics corresponds to the exchange mode excited by Zeeman interaction of the THz field with the antiferromagnetically coupled spins. We argue that THz-pump IR-probe experiments on ferrimagnets offer a unique tool for quantitative studies of dynamics and mechanisms to control antiferromagnetically coupled spins.

cond-mat.mtrl-sci↗

arXiv2021

Multiferroic order parameters in rhombic antiferromagnets. RCrO$_3$

In this paper, we explore magneteoelectricity of rare earth orthochromites from the symmetry point of view. We determine the principal structural order parameters and find their couplings with ferroelectric and magnetic orderings. Our calculations showed that electric dipole moments emerge in the vicinity of Cr3+ ions in the unit cell of RCrO3 due to the displacements of oxygen ions from their highly symmetric positions in the parent perovskite phase (structural instability). We find that the electric dipole moments are arranged in an antiferroelectric mode, so, in essence, RCrO3 are antiferroelectric materials. By classifying the order parameters according to the irreducible representations of the RCrO3 symmetry group (D2h16), we determine the possible couplings between distortive, ferroelectric and magnetic orderings and explore the emerging magnetoelectric structures in these terms. Our analysis makes it possible to explain experimentally observed polarization reversal and the concomitant reorientation of spins in a series of RCrO3 compounds and to predict the possible scenarios of phase transitions in RCrO3.

cond-mat.mtrl-sci↗

arXiv2021

Learning phase transitions in ferrimagnetic GdFeCo alloys

We present results on the identification of phase transitions in ferrimagnetic GdFeCo alloys using machine learning. The approach for finding phase transitions in the system is based on the `learning by confusion' scheme, which allows one to characterize phase transitions using a universal $W$-shape. By applying the `learning by confusion' scheme, we obtain 2D $W$-a shaped surface that characterizes a triple phase transition point of the GdFeCo alloy. We demonstrate that our results are in the perfect agreement with the procedure of the numerical minimization of the thermodynamical potential, yet our machine-learning-based scheme has the potential to provide a speedup in the task of the phase transition identification.

cond-mat.mtrl-sci↗

arXiv2020

Nanophotonic structures with optical surface modes for tunable spin current generation

Heat generated by spin currents in spintronics-based devices is typically much less than that generated by charge current flows in conventional electronic devices. However, the conventional approaches for excitation of spin currents based on spin-pumping and spin Hall effect are limited in efficiency which restricts their application for viable spintronic devices. We propose a novel type of photonic-crystal (PC) based structures for efficient and tunable optically-induced spin current generation via the Spin Seebeck and inverse spin Hall effects. It is experimentally demonstrated that optical surface modes localized at the PC surface covered by ferromagnetic layer and materials with giant spin-orbit coupling (SOC) notably increase the efficiency of the optically-induced spin current generation and provides its tunability by modifying light wavelength or angle of incidence. Up to 100% of the incident light power can be transferred to heat within the SOC layer and, therefore, to spin current. Importantly, high efficiency becomes accessible even for ultra-thin SOC layers. Moreover, surface patterning of the PC-based spintronic nanostructure allows local generation of spin currents at the pattern scales rather than diameter of the laser beam.

cond-mat.mes-hall↗

arXiv2020

Unusual magnetoelectric effect in paramagnetic rare-earth langasite

Violation of time reversal and spatial inversion symmetries has profound consequences for elementary particles and cosmology. Spontaneous breaking of these symmetries at phase transitions gives rise to unconventional physical phenomena in condensed matter systems, such as ferroelectricity induced by magnetic spirals, electromagnons, non-reciprocal propagation of light and spin waves, and the linear magnetoelectric (ME) effect - the electric polarization proportional to the applied magnetic field and the magnetization induced by the electric field. Here, we report the experimental study of the holmium-doped langasite, Ho$_{x}$La$_{3-x}$Ga$_5$SiO$_{14}$, showing a puzzling combination of linear and highly non-linear ME responses in the disordered paramagnetic state: its electric polarization grows linearly with the magnetic field but oscillates many times upon rotation of the magnetic field vector. We propose a simple phenomenological Hamiltonian describing this unusual behavior and derive it microscopically using the coupling of magnetic multipoles of the rare-earth ions to the electric field.

cond-mat.mtrl-sci↗

arXiv2020

Temporal and spectral fingerprints of ultrafast all-coherent spin switching

Future information technology demands ultimately fast, low-loss quantum control. Intense light fields have facilitated important milestones, such as inducing novel states of matter, accelerating electrons ballistically, or coherently flipping the valley pseudospin. These dynamics leave unique signatures, such as characteristic bandgaps or high-order harmonic radiation. The fastest and least dissipative way of switching the technologically most important quantum attribute - the spin - between two states separated by a potential barrier is to trigger an all-coherent precession. Pioneering experiments and theory with picosecond electric and magnetic fields have suggested this possibility, yet observing the actual dynamics has remained out of reach. Here, we show that terahertz (1 THz = 10$^{12}$ Hz) electromagnetic pulses allow coherent navigation of spins over a potential barrier and we reveal the corresponding temporal and spectral fingerprints. This goal is achieved by coupling spins in antiferromagnetic TmFeO$_{3}$ with the locally enhanced THz electric field of custom-tailored antennas. Within their duration of 1 ps, the intense THz pulses abruptly change the magnetic anisotropy and trigger a large-amplitude ballistic spin motion. A characteristic phase flip, an asymmetric splitting of the magnon resonance, and a long-lived offset of the Faraday signal are hallmarks of coherent spin switching into adjacent potential minima, in agreement with a numerical simulation. The switchable spin states can be selected by an external magnetic bias. The low dissipation and the antenna's sub-wavelength spatial definition could facilitate scalable spin devices operating at THz rates.

cond-mat.mes-hall↗

arXiv2019

Unusual Field Dependence of Anomalous Hall Effect in Ta/TbFeCo

Experimental studies of anomalous Hall effect are performed for thin filmed Ta/TbFeCo in a wide range of temperatures and magnetic fields up to 3 T. While far from the compensation temperature (TM=277 K) the field dependence has a conventional shape of a single hysteresis loop, just below the compensation point the dependence is anomalous having the shape of a triple hysteresis. To understand this behavior, we experimentally reveal the magnetic phase diagram and theoretically analyze it in terms of spin-reorientation phase transitions. We show that one should expect anomalous hysteresis loops below the compensation point if in the vicinity of it the magnetic anisotropy is dominated by FeCo sublattice due to interaction with Ta.

cond-mat.mtrl-sci↗

arXiv2019

H-T Phase Diagram of Rare-Earth -- Transition Metal Alloy in the Vicinity of the Compensation Point

Anomalous hysteresis loops of ferrimagnetic amorphous alloys in high magnetic field and in the vicinity of the compensation temperature have so far been explained by sample inhomogeneities. We obtain H-T magnetic phase diagram for ferrimagnetic GdFeCo alloy using a two-sublattice model in the paramagnetic rare-earth ion approximation and taking into account rare-earth (Gd) magnetic anisotropy. It is shown that if the magnetic anisotropy of the $f$-sublattice is larger than that of the $d$-sublattice, the tricritical point can be at higher temperature than the compensation point. The obtained phase diagram explains the observed anomalous hysteresis loops as a result of high-field magnetic phase transition, the order of which changes with temperature. It also implies that in the vicinity of the magnetic compensation point the shape of magnetic hysteresis loop is strongly temperature dependent.

cond-mat.mtrl-sci↗

arXiv2019

High Field Anomalies of Equilibrium and Ultrafast Magnetism in Rare-Earth-Transition Metal Ferrimagnets

Magneto-optical spectroscopy in fields up to 30 Tesla reveals anomalies in the equilibrium and ultrafast magnetic properties of the ferrimagnetic rare-earth-transition metal alloy TbFeCo. In particular, in the vicinity of the magnetization compensation temperature, each of the magnetizations of the antiferromagnetically coupled Tb and FeCo sublattices show triple hysteresis loops. Contrary to state-of-the-art theory, which explains such loops by sample inhomogeneities, here we show that they are an intrinsic property of the rare-earth ferrimagnets. Assuming that the rare-earth ions are paramagnetic and have a non-zero orbital momentum in the ground state and, therefore, a large magnetic anisotropy, we are able to reproduce the experimentally observed behavior in equilibrium. The same theory is also able to describe the experimentally observed critical slowdown of the spin dynamics in the vicinity of the magnetization compensation temperature, emphasizing the role played by the orbital momentum in static and ultrafast magnetism of ferrimagnets.

cond-mat.mtrl-sci↗

arXiv2019

Ultrafast magnetization dynamics in uniaxial ferrimagnets with compensation point. GdFeCo

We derive an effective Lagrangian in the quasi-antiferromagnetic approximation that allows to describe the magnetization dynamics for uniaxial f-d (rare-earth - transition metal) ferrimagnet near the magnetization compensation point in the presence of external magnetic field. We perform calculations for the parameters of GdFeCo, a metallic ferrimagnet with compensation point that is one of the most promising materials in ultrafast magnetism. Using the developed approach, we find the torque that acts on the magnetization due to ultrafast demagnetization pulse that can be caused either by ultrashort laser or electrical current pulse. We show that the torque is non-zero only in the non-collinear magnetic phase that can be acquired by applying external magnetic field to the material. The coherent response of magnetization dynamics amplitude and its timescale exhibits critical behavior near certain values of the magnetic field corresponding to a spin-flop like phase transition. Understanding the underlying mechanisms for these effects opens the way to efficient control of the amplitude and the timescales of the spin dynamics, which is one of the central problems in the field of ultrafast magnetism.

cond-mat.mtrl-sci↗

arXiv2018

Transverse Magneto-Optical Kerr Effect at Narrow Optical Resonances

Magneto-optical spectroscopy based on the transverse magneto-optical Kerr effect (TMOKE) is a sensitive method for investigation of magnetically-ordered media. However, in magnetic materials the optical transitions are usually characterized by spectrally broad resonances with widths considerably exceeding the Zeeman splitting in the magnetic field. Here we investigate experimentally and theoretically the TMOKE in the vicinity of relatively narrow optical resonances provided by confined quantum systems. For experimental demonstration we use the exciton resonance in a (Cd,Mn)Te diluted magnetic semiconductor quantum well, where the strong exchange interaction with magnetic ions enables the giant Zeeman splitting of exciton spin states $Δ$ in magnetic fields of a few Tesla. In the weak coupling regime, when the splitting $Δ$ is smaller than the spectral broadening of the optical transitions $Γ$, the TMOKE magnitude grows linearly with the increase of the Zeeman splitting and its spectrum has an S-shape, which remains virtually unchanged in this range. In the strong coupling regime ($Δ>Γ$) the TMOKE magnitude saturates, while its spectrum is strongly modified resulting in the appearance of two separate peaks. The TMOKE is sensitive not only to the sample surface but can be used to probe the confined electronic states in depth if the upper layer is sufficiently transparent. Our results demonstrate that TMOKE of spectrally narrow resonances serves as a versatile tool for probing the charge and spin structure of electronic states in various confined quantum systems and can be used for spin tomography in combination with the conventional polar Kerr effect.

cond-mat.mtrl-sci↗

arXiv2018

Optically Pumped Floquet States of Magnetization in Ferromagnets

Floquet states have been subject of great research interest since Zel'dovich's pioneering work on the quasienergy of a quantum system subject to a temporally periodic action. Nowadays periodic modulation of the system Hamiltonian is mostly achieved by microwaves leading to novel exciting phenomena in condensed matter physics: Floquet topological insulators, chiral edge states etc. On the other hand, nonthermal optical control of magnetization at picosecond time scales is currently a highly appealing research topic for potential applications in magnetic data storage. Here we combine these two concepts to investigate Floquet states in the system of exchange-coupled spins in a ferromagnet. We periodically perturb the magnetization of an iron-garnet film by a train of circularly-polarized femtosecond laser pulses hitting the sample at 1 GHz repetition rate and monitor the magnetization dynamics behaving like a Floquet state. An external magnetic field allows tuning of the Floquet states leading to a pronounced increase of the precession amplitude by one order of magnitude at the center of the Brillouin zone, i.e. when the precession frequency is a multiple of the laser pulse repetition rate. Floquet states might potentially allow for parametric generation of magnetic oscillations. The observed phenomena expand the capabilities of coherent ultrafast optical control of magnetization and pave a way for their application in quantum computation or data processing.

cond-mat.mes-hall↗

arXiv2018

Selection Rules for All-Optical Magnetic Recording in Iron Garnet

Finding an electronic transition a subtle excitation of which can launch dramatic changes of electric, optical or magnetic properties of media is one of the long-standing dreams in the field of photo-induced phase transitions [1-5]. Therefore the discovery of the magnetization switching only by a femtosecond laser pulse [6-10] triggered intense discussions about mechanisms responsible for these laser-induced changes. Here we report the experimentally revealed selection rules on polarization and wavelengths of ultrafast photo-magnetic recording in Co-doped garnet film and identify the workspace of the parameters (magnetic damping, wavelength and polarization of light) allowing this effect. The all-optical magnetic switching under both single pulse and multiple-pulse sequences can be achieved at room temperature, in narrow spectral ranges with light polarized either along <110> or <100> crystallographic axes of the garnet. The revealed selection rules indicate that the excitations responsible for the coupling of light to spins are d-electron transitions in octahedral and tetrahedral Co-sublattices, respectively.

cond-mat.mtrl-sci↗

arXiv2017

Strain and Magnetic Field Induced Spin-Structure Transitions in Multiferroic BiFeO3

The magnetic-field-dependent spin ordering of strained BiFeO3 films is determined using nuclear resonant scattering and Raman spectroscopy. The critical field required to destroy the cycloidal modulation of the Fe spins is found to be significantly lower than in the bulk, with appealing implications for field-controlled spintronic and magnonic devices.

cond-mat.mtrl-sci↗

arXiv2017

Synchrotron radiation induced magnetization in magnetically-doped and pristine topological insulators

Quantum mechanics postulates that any measurement influences the state of the investigated system. Here, by means of angle-, spin-, and time-resolved photoemission experiments and ab initio calculations we demonstrate how non-equal depopulation of the Dirac cone (DC) states with opposite momenta in V-doped and pristine topological insulators (TIs) created by a photoexcitation by linearly polarized synchrotron radiation (SR) is followed by the hole-generated uncompensated spin accumulation and the SR-induced magnetization via the spin-torque effect. We show that the photoexcitation of the DC is asymmetric, that it varies with the photon energy, and that it practically does not change during the relaxation. We find a relation between the photoexcitation asymmetry, the generated spin accumulation and the induced spin polarization of the DC and V 3d states. Experimentally the SR-generated in-plane and out-of-plane magnetization is confirmed by the $k_{\parallel}$-shift of the DC position and by the splitting of the states at the Dirac point even above the Curie temperature. Theoretical predictions and estimations of the measurable physical quantities substantiate the experimental results.

cond-mat.mtrl-sci↗

arXiv2017

Dynamics of domain walls in weak ferromagnets

It is shown that the total set of equations, which determines the dynamics of the domain bounds (DB) in a weak ferromagnet, has the same type of specific solution as the well-known Walker's solution for ferromagnets. We calculated the functional dependence of the velocity of the DB on the magnetic field, which is described by the obtained solution. This function has a maximum at a finite field and a section of the negative differential mobility of the DB. According to the calculation, the maximum velocity $ c \approx 2 \times 10^6$ cm/sec in YFeO$_3$ is reached at $H_m \approx 4 \times 10^3$ Oe.

cond-mat.stat-mech↗