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A. Kanigel

Publications and source records attributed to A. Kanigel.

At least 19 recordsLinked to original sources

Thermal transport and low-temperature specific heat in 4Hb-TaS$_2$

We investigate the low-energy excitation spectrum of the van der Waals heterostructure superconductor 4Hb-TaS$_2$ using ultra-low-temperature specific-heat and thermal-conductivity measurements with magnetic fields applied parallel and perpendicular to the crystallographic $c$ axis. The specific heat is broadly consistent with a nodeless superconducting gap, but retains a finite residual linear contribution, indicating a small residual low-energy density of states in the superconducting state. In addition, a pronounced upturn appears below approximately 0.3K. Its weak magnetic-field dependence, together with the absence of a corresponding feature in thermal transport, supports an interpretation in terms of localized degrees of freedom, most likely a nuclear Schottky contribution. In contrast to the finite residual thermodynamic density of states, the thermal conductivity extrapolates to a vanishing zero-field electronic linear term within experimental uncertainty for both field orientations. Thus, the residual low-energy states do not form a detectable itinerant heat-conduction channel. In finite magnetic field, the electronic heat transport grows rapidly. For out-of-plane fields, this response is broadly consistent with previous thermal-conductivity measurements and with the behavior commonly associated with multigap nodeless superconductivity. The even steeper increase observed for in-plane fields suggests that the field-induced quasiparticle response of 4Hb-TaS$_2$ is more complicated than the standard multigap picture alone.

cond-mat.supr-con

Conventional superconductivity in single-crystalline BiPt

Binary Bi-Pd/Pt systems have attracted a lot of interest because of their topologically non-trivial nature along with superconductivity. We report the structural and superconducting properties of high-quality single-crystalline BiPt using a comprehensive range of experimental techniques, including X-ray diffraction, electron microscopy, muon spin rotation/relaxation ({\mu}SR), magnetization, resistivity, and heat capacity. Our findings establish that BiPt is a weak type-II superconductor with a transition temperature (Tc) of 1.2 K which exhibits pronounced anisotropic superconducting characteristics attributed to its hexagonal crystal structure. Magnetization and electronic transport studies reveal that BiPt lies within the dirty limit, while {\mu}SR and heat capacity data indicate conventional s-wave superconductivity that maintains time-reversal symmetry. This work provides valuable insights into the pairing symmetry and superconducting mechanism of topologically trivial BiPt, a sound comparison system for other Bi-based topologically nontrivial superconductors.

cond-mat.supr-con

Ground-states of the Shastry-Sutherland Lattice Materials Gd$_2$Be$_2$GeO$_7$ and Dy$_2$Be$_2$GeO$_7$

The recent realization that the rare-earth melilites RE$_2$Be$_2$GeO$_7$ host the Shastry-Sutherland lattice within planes of RE$^{3+}$ ions has sparked a number of studies. This family of materials lacks appreciable site mixing and conductivity, making them promising candidates for the Shastry-Sutherland model. Herein, we present the magnetic ground states of two of these rare-earth melilites: RE = Gd and Dy. We find, through measurements of magnetic susceptibility, magnetization, and specific heat capacity (RE = Dy only), that these two melilites are antiferromagnets (T$_N$ $\sim$~1~K). Gd$_2$Be$_2$GeO$_7$, in accordance with its electronic configuration, has isotropic single-ion anisotropy but shows a quadratic contribution to its magnetization. Dy$_2$Be$_2$GeO$_7$ has Ising-like single-ion ansiotropy and is likely an effective spin-$1/2$ system. Both materials exhibit metamagnetic transitions. We identify this transition in Dy$_2$Be$_2$GeO$_7$, occurring at 86(1)~mT for T=500~mK, to likely be a spin-flip transition.

cond-mat.str-el

Fractionalized Magnetization Plateaus in the Shastry-Sutherland Lattice Material Er$_2$Be$_2$GeO$_7$

The experimental study of magnetism on the Shastry-Sutherland lattice has been ongoing for more than two decades, following the discovery of the first Shastry-Sutherland lattice materials SrCu$_2$(BO$_3$)$_2$. However, the study of Shastry-Sutherland systems is often complicated by the requirements of high magnetic fields ($>$~20~T SrCu$_2$(BO$_3$)$_2$) or the presence of itinerate electrons (e.g. REB$_4$). In this paper, we present the magnetic properties of the Shastry-Sutherland lattice material Er$_2$Be$_2$GeO$_7$. Like SrCu$_2$(BO$_3$)$_2$, Er$_2$Be$_2$GeO$_7$ exhibits fractionalized magnetization plateaus. Unlike SrCu$_2$(BO$_3$)$_2$, Er$_2$Be$_2$GeO$_7$ exhibits long-range order below $\sim1~$K, and the plateaus are accessible using commercial laboratory equipment, occurring for fields <~1~T. The fractions of magnetization present are closest to $\frac{1}{4}$ and $\frac{1}{2}$ of the full powder moment; we show that the $\frac{1}{4}$ magnetization plateau in Er$_2$Be$_2$GeO$_7$ has a classical analog, well represented by the magnetic structure (canted antiferromagnetic) observed in powder neutron diffraction. The lack of itinerate electrons, chemical disorder, and the low fields required to access the fractionalized magnetization plateaus promises Er$_2$Be$_2$GeO$_7$ to be a prime candidate for the study of frustrated magnetism on the Shastry-Sutherland lattice.

cond-mat.str-el

A Candidate for the Quantum Spin Liquid Ground-State in the Shastry-Sutherland Lattice Material Yb$_2$Be$_2$GeO$_7$

The quasi-2D Shastry-Sutherland model has remained topical in the field of condensed matter physics for the last two decades, following the experimental realization of the model in the material SrCu$_2$(BO$_3$)$_2$. Since then, research into the Shastry-Sutherland system has revealed more nuanced physics than initially predicted; recent theoretical works have even predicted a quantum spin liquid phase may exist. Herein, we report on a new Shastry-Sutherland lattice material, Yb$_2$Be$_2$GeO$_7$, of the rare-earth melilite family RE$_2$Be$_2$GeO$_7$. We find, through SQUID magnetometry, powder neutron diffraction, specific heat capacity, and muon spin relaxation, that Yb$_2$Be$_2$GeO$_7$ lacks magnetic order and exhibits persistent spin dynamics to at least 17 mK. We propose the Shastry-Sutherland lattice material Yb$_2$Be$_2$GeO$_7$ as a candidate to host a quantum spin liquid ground-state.

cond-mat.str-el

Evidence for conventional superconductivity in Bi$_2$PdPt and prediction of topological superconductivity in disorder-free $\gamma$-BiPd

We present comprehensive investigations into the structural, superconducting, and topological properties of Bi$_2$PdPt. Magnetization and heat capacity measurements performed on polycrystalline Bi$_2$PdPt demonstrate a superconducting transition at $\approx$ 0.8 K. Moreover, muon spin relaxation/rotation ($\mu$SR) measurements present evidence for a time reversal symmetry preserving, isotropically gapped superconducting state in Bi$_2$PdPt. We have also performed density-functional theory (DFT) calculations on Bi$_2$PdPt alongside the more general isostructural systems, BiPd$_{x}$Pt$_{1-x}$, of which Bi$_2$PdPt and $\gamma$-BiPd are special cases for $x=0.5$ and $x=1$ respectively. We have calculated the $Z_2$ topological index from our DFT calculations for a range of substitution fractions, $x$, between $x=0$ and $x=1$ characterizing the topology of the band structure. We find a non-trivial topological state when $x>0.75$ and a trivial topological state when $x<0.75$. Therefore our results indicate that BiPd$_{x}$Pt$_{1-x}$ could be a topological superconductor for $x>0.75$.

cond-mat.supr-con

Chiral to Nematic Crossover in the Superconducting State of 4Hb-TaS$_2$

Most superconductors have an isotropic, single component order parameter, and are well described by the BCS theory for superconductivity. Unconventional, multiple components superconductors are exceptionally rare and are much less understood. Here, we combine scanning tunneling microscopy and angle-resolved macroscopic transport to study the candidate chiral superconductor, 4Hb-TaS$_2$. We reveal quasi-periodic one-dimensional modulations in the tunneling conductance accompanied by two-fold symmetric superconducting critical field. The strong modulation of the in-plane critical field, points to a nematic, unconventional order parameter. However, the imaged vortex core is nearly circular symmetric, suggesting an isotropic order parameter. We reconcile this apparent discrepancy by modeling a competition between a dominating chiral superconducting order parameter and a nematic one, the latter emerges close to the normal phase. Our results strongly support the existence of two-component superconductivity in 4Hb-TaS$_2$ and can provide useful insights to other systems with coexistent charge order and superconductivity.

cond-mat.supr-con

Link between superconductivity and a Lifshitz transition in intercalated Bi$_2$Se$_3$

Topological superconductivity is an exotic phase of matter in which the fully gapped superconducting bulk hosts gapless Majorana surface states protected by topology. Intercalation of copper, strontium or niobium between the quintuple layers of the topological insulator Bi$_2$Se$_3$ increases the carrier density and leads to superconductivity that is suggested to be topological. Here we study the electronic structure of strontium-intercalated Bi$_2$Se$_3$ using angle resolved photoemission spectroscopy (ARPES) and Shubnikov-de Haas (SdH) oscillations. Despite the apparent low Hall number of $\sim2 \times 10 ^{19}$cm$^{-3}$, we show that the Fermi surface is shaped as an open cylinder with a larger carrier density of $\sim 10 ^{20}$cm$^{-3}$. We suggest that superconductivity in intercalated Bi$_2$Se$_3$ emerges with the appearance of a quasi-2D open Fermi surface.

cond-mat.supr-con

Superconductivity and phonon self-energy effects in Fe$_{1+y}$Te$_{0.6}$Se$_{0.4}$

We study Fe$_{1+y}$Te$_{0.6}$Se$_{0.4}$ multi-band superconductor with $T_c=14$K by polarization-resolved Raman spectroscopy. Deep in the superconducting state, we detect pair-breaking excitation at 45cm$^{-1}$ ($2Δ=5.6$meV) in the $XY$($B_{2g}$) scattering geometry, consistent with twice of the superconducting gap energy (3 meV) revealed by ARPES on the hole-like Fermi pocket with $d_{xz}/d_{yz}$ character. We analyze the superconductivity induced phonon self-energy effects for the $B_{1g}$(Fe) phonon and estimate the electron-phonon coupling constant $λ^Γ\approx 0.026$, which is insufficient to explain superconductivity with $T_c=14$K.

cond-mat.supr-con

Chiral superconductivity in the alternate stacking compound 4Hb-TaS$_2$

Layered van der Waals (vdW) materials are emerging as one of the most versatile directions in the field of quantum condensed matter physics. They allow an unprecedented control of electronic properties via stacking of different types of two-dimensional (2D) materials. A fascinating frontier, largely unexplored, is the stacking of strongly-correlated phases of matter in vdW materials. Here, we study 4Hb-TaS$_2$, which naturally realizes an alternating stacking of a Mott insulator, recently reported as a gapless spin-liquid candidate(1T-TaS$_2$), and a 2D superconductor (1H-TaS$_2$). This raises the question of how these two components affect each other. We find a superconducting ground state with a transition temperature of 2.7K, which is significantly elevated compared to the 2H polytype (Tc=0.7K). Strikingly, the superconducting state exhibits signatures of time-reversal-symmetry breaking abruptly appearing at the superconducting transition, which can be naturally explained by a chiral superconducting state.

cond-mat.supr-con

Gapless excitations in the ground state of 1T-TaS$_2$

1T-TaS$_2$ is a layered transition metal dichalgeonide with a very rich phase diagram. At T=180K it undergoes a metal to Mott insulator transition. Mott insulators usually display anti-ferromagnetic ordering in the insulating phase but 1T-TaS$_2$ was never shown to order magnetically. In this letter we show that 1T-TaS$_2$ has a large paramagnetic contribution to the magnetic susceptibility but it does not show any sign of magnetic ordering or freezing down to 20mK, as probed by $μ$SR, possibly indicating a quantum spin liquid ground state. Although 1T-TaS$_2$ exhibits a strong resistive behavior both in and out-of plane at low temperatures we find a linear term in the heat capacity suggesting the existence of a Fermi-surface, which has an anomalously strong magnetic field dependence.

cond-mat.str-el

Tuning across the BCS-BEC crossover in the multiband superconductor Fe$_{1+y}$Se$_x$Te$_{1-x}$ : An angle-resolved photoemission study

The crossover from Bardeen-Cooper-Schrieffer (BCS) superconductivity to Bose-Einstein condensation (BEC) is difficult to realize in quantum materials because, unlike in ultracold atoms, one cannot tune the pairing interaction. We realize the BCS-BEC crossover in a nearly compensated semimetal Fe$_{1+y}$Se$_x$Te$_{1-x}$ by tuning the Fermi energy, $ε_F$, via chemical doping, which permits us to systematically change $Δ/ ε_F$ from 0.16 to 0.5 were $Δ$ is the superconducting (SC) gap. We use angle-resolved photoemission spectroscopy to measure the Fermi energy, the SC gap and characteristic changes in the SC state electronic dispersion as the system evolves from a BCS to a BEC regime. Our results raise important questions about the crossover in multiband superconductors which go beyond those addressed in the context of cold atoms.

cond-mat.supr-con

The electronic structure of BSCCO in the presence of a super-current: Flux-flow, Doppler shift and quasiparticle pockets

There are several ways to turn a superconductor into a normal conductor: increase the temperature, apply a high magnetic field, or run a large current. High-T$_c$ cuprate superconductors are unusual in the sense that experiments suggest that destroying superconductivity by heating the sample to temperatures above T$_c$ or by applying a high magnetic field result in different 'normal' states. Spectroscopic probes show that above T$_c$, in the pseudogap regime, the Fermi surface is partly gapped and there are no well-defined quasiparticles. Transport measurements, on the contrary, reveal quantum oscillations in high magnetic fields and at low temperatures, suggesting a more usual Fermi liquid state. Studying the electronic structure while suppressing superconductivity by using current, will hopefully shed new light on this problem. In type II superconductors, such as the cuprates, the resistive state created by the current is a result of vortex motion. The large dissipation in the flux-flow regime makes spectroscopic measurements in the presence of current challenging. We performed angle-resolved photoemission experiments in thin films of Bi$_2$Sr$_2$CaCu$_2$O$_y$ while running high-density current through the samples. Clear evidence was found for non-uniform flux flow, leaving most of the sample volume free of mobile vortices and dissipation. The super-current changes the electronic spectrum, creating quasiparticle and quasihole pockets. The size of these pockets as a function of the current is found to be doping dependent; it depends both on the superfluid stiffness and on the strength of interactions.

cond-mat.supr-con

ARPES sensitivity to short-range antiferromagnetic correlations

Angle-resolved photoemission spectroscopy (ARPES) is one of most powerful techniques to unravel the electronic properties of layered materials and in the last decades it has lead to a significant progress in the understanding of the band structures of cuprates, pnictides and other materials of current interest. On the other hand, its application to Mott-Hubbard insulating materials where a Fermi surface is absent has been more limited. Here we show that in these latter materials, where electron spins are localized, ARPES may provide significant information on the spin correlations which can be complementary to the one derived from neutron scattering experiments. Sr$_2$Cu$_{1-x}$Zn$_x$O$_2$Cl$_2$, a prototype of diluted spin $S=1/2$ antiferromagnet (AF) on a square lattice, was chosen as a test case and a direct correspondence between the amplitude of the spectral weight beyond the AF zone boundary derived from ARPES and the spin correlation length $ξ$ estimated from $^{35}$Cl NMR established. It was found even for correlation lengths of a few lattice constants a significant spectral weight in the back-bended band is present which depends markedly on $ξ$. Moreover the temperature dependence of that spectral weight is found to scale with the $x$ dependent spin-stiffness. These findings prove that ARPES technique is very sensitive to short-range correlations and its relevance in the understanding of the electronic correlations in cuprates is discussed.

cond-mat.str-el

Anisotropic scattering rate in Fe substituted Bi2212

We measured the electronic structure of Fe substituted Bi2212 using Angle Resolved Photoemission Spectroscopy (ARPES). We find that the substitution does not change the momentum dependence of the superconducting gap but induces a very anisotropic enhancement of the scattering rate. A comparison of the effect of Fe substitution to that of Zn substitution suggests that the Fe reduces T$_c$ so effectively because it supresses very strongly the coherence weight around the anti-nodes.

cond-mat.supr-con

Evolution of the fermi surface of a doped topological insulator with carrier concentration

In an ideal bulk topological-insulator (TI) conducting surface states protected by time reversal symmetry enfold an insulating crystal. However, the archetypical TI, Bi2Se3, is actually never insulating; it is in fact a relatively good metal. Nevertheless, it is the most studied system among all the TIs, mainly due to its simple band-structure and large spin-orbit gap. Recently it was shown that copper intercalated Bi2Se3 becomes superconducting and it was suggested as a realization of a topological superconductor (TSC). Here we use a combination of techniques that are sensitive to the shape of the Fermi surface (FS): the Shubnikov-de Haas (SdH) effect and angle resolved photoemission spectroscopy (ARPES) to study the evolution of the FS shape with carrier concentration, n. We find that as n increases, the FS becomes 2D-like. These results are of crucial importance for understanding the superconducting properties of CuxBi2Se3.

cond-mat.mes-hall

Unconventional superconductivity in CuxBi2Se3

We report point contact measurements in high quality single crystals of Cu0.2Bi2Se3. We observe three different kinds of spectra: (1) Andreev-reflection spectra, from which we infer a superconducting gap size of 0.6mV; (2) spectra with a large gap which closes above Tc at about 10K; and (3) tunneling-like spectra with zero-bias conductance peaks. These tunneling spectra show a very large gap of ~2meV (2Delta/KTc ~ 14).

cond-mat.supr-con

Probing the surface states in Bi2Se3 using the Shubnikov-de Haas effect

Shubnikov-de Haas (SdH) oscillations are observed in Bi2Se3 flakes with high carrier concentration and low bulk mobility. These oscillations probe the protected surface states and enable us to extract their carrier concentration, effective mass and Dingle temperature. The Fermi momentum obtained is in agreement with angle resolved photoemission spectroscopy (ARPES) measurements performed on crystals from the same batch. We study the behavior of the Berry phase as a function of magnetic field. The standard theoretical considerations fail to explain the observed behavior.

cond-mat.mes-hall