arXiv subjects

A. Kapitulnik

Publications and source records attributed to A. Kapitulnik.

At least 19 recordsLinked to original sources

arXiv2023

Impact of disorder in the charge-density-wave state of Pd-intercalated ErTe$_3$ revealed by the electrodynamic response

It is a general notion that disorder, introduced by either chemical substitution or intercalation as well as by electron-irradiation, is detrimental to the realisation of long-range charge-density-wave (CDW) order. We study the disorder-induced suppression of the in-plane CDW orders in the two-dimensional Pd-intercalated ErTe$_3$ compositions, by exploring the real part of the optical conductivity with light polarised along the in-plane $a$ and $c$ axes. Our findings reveal an anisotropic charge dynamics with respect to both incommensurate unidirectional CDW phases of ErTe$_3$, occurring within the $ac$-plane. The anisotropic optical response gets substantially washed out with Pd-intercalation, hand-in-hand with the suppression of both CDW orders. The spectral weight analysis though advances the scenario, for which the CDW phases evolve from a (partially) depleted Fermi surface already above their critical onset temperatures. We therefore argue that the long-range CDW orders of ErTe$_3$ tend to be progressively dwarfed by Pd-intercalation, which favours the presence of short-range CDW segments for both crystallographic directions persisting in a broad temperature ($T$) interval up to the normal state, and being suggestive of precursor effects of the CDW orders as well as possibly coexisting with superconductivity at low $T$.

cond-mat.str-el↗

arXiv2022

Direct observation of discommensurate charge density wave modulation in the quasi-1D Weyl semimetal candidate NbTe$_4$

The transition-metal tetrachalcogenides are a model system to explore the conjunction of correlated electronic states such as charge density waves (CDW), with topological phases of matter. Understanding the connection between these phases requires a thorough understanding of the individual states, which for the case of the CDW in this system, is still missing. In this paper we combine phonon-structure calculations and scanning tunneling microscopy measurements of NbTe$_4$ in order to provide a full characterization of the CDW state. We find that, at short range, the superstructure formed by the CDW is fully commensurate with the lattice parameters. Moreover, our data reveals the presence of phase-slip domain-walls separating regions of commensurate-CDW in the nanoscale, indicating that the CDW in this compound is discommensurate at long-range. Our results solve a long-standing discussion about the nature of the CDW in these materials, and provide a strong basis for the study of the interplay between this state and other novel quantum electronic states.

cond-mat.mtrl-sci↗

arXiv2021

Violation of Onsager Reciprocity in Underdoped Cuprates ?

One of the canons of condensed matter physics is the Onsager Reciprocity principle in systems in which the Hamiltonian commutes with the time-reversal operator. Recent results of measurements of the Nernst coefficient in underdoped YBa_2Cu_30_{6+x}, together with the measurements of the anisotropy of conductivity and the inferred anisotropy of the thermopower, imply that this principle is violated. The probable violation and its temperature dependence are shown to be consistent with the Loop-current phase which has been directly observed in other experiments. The violation is related directly to the magneto-electric symmetry of such a phase in which an applied electric field generates an effective magnetic field at right angle to it and to the order parameter vector, and vice versa.

cond-mat.supr-con↗

arXiv2020

Characterization of magnetic field noise in the ARIADNE source mass rotor

ARIADNE is a nuclear-magnetic-resonance-based experiment that will search for novel axion-induced spin-dependent interactions between an unpolarized source mass rotor and a nearby sample of spin-polarized $^3$He gas. To detect feeble axion signals at the sub-atto-Tesla level, the experiment relies on low magnetic background and noise. We measure and characterize the magnetic field background from a prototype tungsten rotor. We show that the requirement is met with our current level of tungsten purity and demagnetization process. We further show that the noise is dominantly caused by a few discrete dipoles, likely due to a few impurities trapped inside the rotor during manufacturing. This is done via a numerical optimization pipeline which fits for the locations and magnetic moments of each dipole. We find that under the current demagnetization, the magnetic moment of trapped impurities is bounded at $10^{-9} \mathrm{A}\mathrm{m}^2$.

physics.ins-det↗

arXiv2020

Ferromagnetic order beyond the superconducting dome in a cuprate superconductor

The cuprate high-temperature superconductors (HTSC) have been the subject of intense study for more than 30 years with no consensus yet on the underlying mechanism of the superconductivity. Conventional wisdom dictates that the mysterious and extraordinary properties of the cuprates arise from doping a strongly correlated antiferromagnetic (AFM) insulator (1,2). The highly overdoped cuprates$-$those beyond the dome of superconductivity (SC)--are considered to be conventional Fermi liquid metals (3). Here, we report the emergence of itinerant ferromagnetic order (FM) below 4K for doping beyond the SC dome in electron-doped La$_{2-x} $Ce$_x$CuO$_4$ (LCCO). The existence of this FM order is evidenced by negative, anisotopic and hysteretic magnetoresistance, hysteretic magnetization, and the polar Kerr effect, all of which are standard signatures of itinerant FM in metals (4,5). This surprising new result suggests that the overdoped cuprates are also influenced by electron correlations and the physics is much richer than that of a conventional Fermi liquid metal.

cond-mat.supr-con↗

arXiv2017

A method for controlling the magnetic field near a superconducting boundary in the ARIADNE axion experiment

The QCD Axion is a particle postulated to exist since the 1970s to explain the Strong-CP problem in particle physics. It could also account for all of the observed Dark Matter in the universe. The Axion Resonant InterAction DetectioN Experiment (ARIADNE) experiment intends to detect the QCD axion by sensing the fictitious "magnetic field" created by its coupling to spin. The experiment must be sensitive to magnetic fields below the $10^{-19}$ T level to achieve its design sensitivity, necessitating tight control of the experiment's magnetic environment. We describe a method for controlling three aspects of that environment which would otherwise limit the experimental sensitivity. Firstly, a system of superconducting magnetic shielding is described to screen ordinary magnetic noise from the sample volume at the $10^8$ level. Secondly, a method for reducing magnetic field gradients within the sample up to $10^2$ times is described, using a simple and cost-effective design geometry. Thirdly, a novel coil design is introduced which allows the generation of fields similar to those produced by Helmholtz coils in regions directly abutting superconducting boundaries. The methods may be generally useful for magnetic field control near superconducting boundaries in other experiments where similar considerations apply.

physics.ins-det↗

arXiv2017

Progress on the ARIADNE axion experiment

The Axion Resonant InterAction Detection Experiment (ARIADNE) is a collaborative effort to search for the QCD axion using techniques based on nuclear magnetic resonance. In the experiment, axions or axion-like particles would mediate short-range spin-dependent interactions between a laser-polarized 3He gas and a rotating (unpolarized) tungsten source mass, acting as a tiny, fictitious "magnetic field". The experiment has the potential to probe deep within the theoretically interesting regime for the QCD axion in the mass range of 0.1-10 meV, independently of cosmological assumptions. The experiment relies on a stable rotary mechanism and superconducting magnetic shielding, required to screen the 3He sample from ordinary magnetic noise. Progress on testing the stability of the rotary mechanism is reported, and the design for the superconducting shielding is discussed.

astro-ph.IM↗

arXiv2017

Anomalous Thermal Diffusivity in Underdoped YBa$_2$Cu$_3$O$_{6+x}$

We present local optical measurements of thermal diffusivity in the $ab$ plane of underdoped YBCO crystals. We find that the diffusivity anisotropy is comparable to reported values of the electrical resistivity anisotropy, suggesting that the anisotropies have the same origin. The anisotropy drops sharply below the charge order transition. We interpret our results through a strong electron-phonon scattering picture and find that both electronic and phononic contributions to the diffusivity saturate a proposed bound. Our results suggest that neither well-defined electron nor phonon quasiparticles are present in this material.

cond-mat.supr-con↗

arXiv2017

Disorder enabled band structure engineering of a topological insulator surface

Three dimensional topological insulators are bulk insulators with $\mathbf{Z}_2$ topological electronic order that gives rise to conducting light-like surface states. These surface electrons are exceptionally resistant to localization by non-magnetic disorder, and have been adopted as the basis for a wide range of proposals to achieve new quasiparticle species and device functionality. Recent studies have yielded a surprise by showing that in spite of resisting localization, topological insulator surface electrons can be reshaped by defects into distinctive resonance states. Here we use numerical simulations and scanning tunneling microscopy data to show that these resonance states have significance well beyond the localized regime usually associated with impurity bands. At native densities in the model Bi$_2$X$_3$ (X=Bi, Te) compounds, defect resonance states are predicted to generate a new quantum basis for an emergent electron gas that supports diffusive electrical transport.

cond-mat.mes-hall↗

arXiv2015

Evidence for broken time-reversal symmetry in the superconducting phase of URu$_2$Si$_2$

Recent experimental and theoretical interest in the superconducting phase of the heavy fermion material URu$_2$Si$_2$ has led to a number of proposals in which the superconducting order parameter breaks time-reversal symmetry (TRS). In this study we measured polar Kerr effect (PKE) as a function of temperature for several high-quality single crystals of URu$_2$Si$_2$. We find an onset of PKE below the superconducting transition that is consistent with a TRS-breaking order parameter. This effect appears to be independent of an additional, possibly extrinsic, PKE generated above the hidden order transition at $T_{HO}=17.5$ K, and contains structure below $T_c$ suggestive of additional physics within the superconducting state.

cond-mat.supr-con↗

arXiv2014

Observation of broken time-reversal symmetry in the heavy fermion superconductor UPt$_3$

The symmetry properties of the order parameter characterize different phases of unconventional superconductors. In the case of the heavy-fermion superconductor UPt$_3$, a key question is whether its multiple superconducting phases preserve or break time-reversal symmetry (TRS). We tested for asymmetry in the phase shift between left and right circularly polarized light reflected from a single crystal of UPt$_3$ at normal incidence, finding that this so-called polar Kerr effect appears only below the lower of the two zero-field superconducting transition temperatures. Our results provide evidence for broken TRS in the low-temperature superconducting phase of UPt$_3$, implying a complex two-component order parameter for superconductivity in this system.

cond-mat.supr-con↗

arXiv2014

Kerr effect as evidence of gyrotropic order in the cuprates - revisited

Recent analysis has confirmed earlier general arguments that the Kerr response vanishes in any time-reversal invariant system which satisfies the Onsager relations. Thus, the widely cited relation between natural optical activity (gyrotropy) and the Kerr response, employed in Hosur \textit{et al}, Phys. Rev. B \textbf{87}, 115116 (2013), is incorrect. However, there is increasingly clear experimental evidence that, as argued in our paper, the onset of an observable Kerr-signal in the cuprates reflects point-group symmetry rather than time-reversal symmetry breaking.

cond-mat.supr-con↗

arXiv2014

Evidence of Chiral Order in the Charge-Ordered Phase of Superconducting La1.875Ba0.125Cuo4 Single Crystals Using Polar Kerr-Effect Measurements

High resolution polar Kerr effect (PKE) measurements were performed on La1.875Ba0.125Cuo4 single crystals revealing that a finite Kerr signal is measured below an onset temperature-T_K that coincides with charge ordering transition temperature T_{CO}. We further show that the sign of the Kerr signal cannot be trained with magnetic field, is found to be the same of opposite sides of the same crystal, and is odd with respect to strain in the diagonal direction of the unit cell. These observations are consistent with a chiral "gyrotropic" order above T_c for La1.875Ba0.125Cuo4; similarities to other cuprates suggest that it is a universal property in the pseudogap regime.

cond-mat.str-el↗

arXiv2012

Kerr effect as evidence of gyrotropic order in the cuprates

The Kerr effect can arise in a time-reversal invariant dissipative medium that is "gyrotropic", i.e. one that breaks inversion ($\mathcal I$) and all mirror symmetries. Examples of such systems include electron analogs of cholesteric liquid crystals, and their descendants, such as systems with chiral charge ordering. We present arguments that the striking Kerr onset seen in the pseudogap phase of a large number of cuprate high temperature superconductors is evidence of chiral charge ordering. We discuss additional experimental consequences of a phase transition to a gyrotropic state, including the appearance of a zero field Nernst effect.

cond-mat.str-el↗

arXiv2012

Magneto-optical signatures of a cascade of transitions in La$_2-x$Ba$_x$CuO$_4$

Recent experiments in the original cuprate high temperature superconductor, La$_2-x$Ba$_x$CuO$_4$, have revealed a remarkable sequence of transitions [1]. Here we investigate such crystals with Kerr effect which is sensitive to time-reversal-symmetry breaking (TRSB). Concurrent birefringence measurements accurately locate the structural phase transitions from high-temperature tetragonal to low temperature orthorhombic, and then to lower temperature tetragonal, at which temperature a strong Kerr signal onsets. Hysteretic behavior of the Kerr signal suggests that TRSB occurs well above room temperature, an effect that was previously observed in high quality YBa$_2$Cu$_3$O$_{6+x} crystals [2].

cond-mat.supr-con↗

arXiv2011

STM imaging of a bound state along a step on the surface of the topological insulator Bi$_2$Te$_3$

Detailed study of the LDOS associated with the surface-state-band near a step-edge of the strong topological-insulator Bi2Te3, reveal a one-dimensional bound state that runs parallel to the stepedge and is bound to it at some characteristic distance. This bound state is clearly observed in the bulk gap region, while it becomes entangled with the oscillations of the warped surface band at high energy, and with the valence band states near the Dirac point. Using the full effective Hamiltonian proposed by Zhang et al., we obtain a closed formula for this bound state that fits the data and provide further insight into the general topological properties of the electronic structure of the surface band near strong structural defects.

cond-mat.str-el↗

arXiv2011

From a single-band metal to a high-temperature superconductor via two thermal phase transitions

The nature of the pseudogap phase of cuprate high-temperature superconductors is a major unsolved problem in condensed matter physics. We studied the commencement of the pseudogap state at temperature T* using three different techniques (angle-resolved photoemission spectroscopy, polar Kerr effect, and time-resolved reflectivity) on the same optimally-doped Bi2201 crystals. We observed the coincident, abrupt onset at T* of a particle-hole asymmetric antinodal gap in the electronic spectrum, a Kerr rotation in the reflected light polarization, and a change in the ultrafast relaxational dynamics, consistent with a phase transition. Upon further cooling, spectroscopic signatures of superconductivity begin to grow close to the superconducting transition temperature (Tc), entangled in an energy-momentum-dependent fashion with the pre-existing pseudogap features, ushering in a ground state with coexisting orders.

cond-mat.supr-con↗

arXiv2010

Hidden quasi one-dimensional superconductivity in Sr$_2$RuO$_4$

Using an asymptotically exact weak coupling analysis of a multi-orbital Hubbard model of the electronic structure of \SRO, we show that the interplay between spin and charge fluctuations leads unequivocally to triplet pairing which originates in the quasi-one dimensional bands. The resulting superconducting state spontaneously breaks time-reversal symmetry and is of the form $Δ\sim p_x + i p_y \hat{z}$ with sharp gap minima and a d-vector that is only {\it weakly} pinned. The supercondutor is topologically {\it trivial} and hence lacks robust chiral Majorana fermion modes along the boundary. The absence of topologically protected edge modes could explain the surprising absence of experimentally detectable edge currents in this system.

cond-mat.supr-con↗