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A. Kimura

Publications and source records attributed to A. Kimura.

At least 37 records · Page 2Linked to original sources
arXiv2022

Angular distribution of $γ$-rays from a neutron-induced $p$-wave resonance of $^{132}$Xe

A neutron-energy dependent angular distribution was measured for individual $γ$-rays from the 3.2 eV $p$-wave resonance of $^{131}$Xe+$n$, that shows enhanced parity violation owing to a mixing between $s$- and $p$-wave amplitudes. The $γ$-ray transitions from the $p$-wave resonance were identified, and the angular distribution with respect to the neutron momentum was evaluated as a function of the neutron energy for 7132 keV $γ$-rays, which correspond to a transition to the 1807 keV excited state of $^{132}$Xe. The angular distribution is considered to originate from the interference between $s$- and $p$-wave amplitudes, and will provide a basis for a quantitative understanding of the enhancement mechanism of the fundamental parity violation in compound nuclei.

nucl-ex↗
arXiv2022

Ultrafast electron dynamics in a topological surface state observed in two-dimensional momentum space

We study ultrafast population dynamics in the topological surface state of Sb$_2$Te$_3$ in two-dimensional momentum space with time- and angle-resolved two-photon photoemission. Linear polarized mid-infrared pump pulses are used to permit a direct optical excitation across the Dirac point. We show that this resonant excitation is strongly enhanced within the Dirac cone along three of the six $\barΓ$-$\bar{M}$ directions and results in a macroscopic photocurrent when the plane of incidence is aligned along a $\barΓ$-$\bar{K}$ direction. Our experimental approach makes it possible to disentangle the decay of transiently excited population and photocurent by elastic and inelastic electron scattering within the full Dirac cone in unprecedented detail. This is utilized to show that doping of Sb$_2$Te$_3$ by vanadium atoms strongly enhances inelastic electron scattering to lower energies, but only scarcely affects elastic scattering around the Dirac cone.

cond-mat.mes-hall↗
arXiv2022

Measurement of the $^{14}$N(n,p)$^{14}$C cross section at the CERN n_TOF facility from sub-thermal energy to 800 keV

Background: The $^{14}$N(n,p)$^{14}$C reaction is of interest in neutron capture therapy, where nitrogen-related dose is the main component due to low-energy neutrons, and in astrophysics, where 14N acts as a neutron poison in the s-process. Several discrepancies remain between the existing data obtained in partial energy ranges: thermal energy, keV region and resonance region. Purpose: Measuring the 14N(n,p)14C cross section from thermal to the resonance region in a single measurement for the first time, including characterization of the first resonances, and providing calculations of Maxwellian averaged cross sections (MACS). Method: Time-of-flight technique. Experimental Area 2 (EAR-2) of the neutron time-of-flight (n_TOF) facility at CERN. $^{10}$B(n,$α$)$^7$Li and $^{235}$U(n,f) reactions as references. Two detection systems running simultaneously, one on-beam and another off-beam. Description of the resonances with the R-matrix code sammy. Results: The cross section has been measured from sub-thermal energy to 800 keV resolving the two first resonances (at 492.7 and 644 keV). A thermal cross-section (1.809$\pm$0.045 b) lower than the two most recent measurements by slightly more than one standard deviation, but in line with the ENDF/B-VIII.0 and JEFF-3.3 evaluations has been obtained. A 1/v energy dependence of the cross section has been confirmed up to tens of keV neutron energy. The low energy tail of the first resonance at 492.7 keV is lower than suggested by evaluated values, while the overall resonance strength agrees with evaluations. Conclusions: Our measurement has allowed to determine the $^{14}$N(n,p) cross-section over a wide energy range for the first time. We have obtained cross-sections with high accuracy (2.5 %) from sub-thermal energy to 800 keV and used these data to calculate the MACS for kT = 5 to kT = 100 keV.

nucl-ex↗
arXiv2022

Measurement of the transverse asymmetry of $γ$-rays in the $^{117}$Sn(n,$γ$)$^{118}$Sn reaction

Largely enhanced parity-violating effects observed in compound resonances induced by epithermal neutrons are currently attributed to the mixing of parity-unfavored partial amplitudes in the entrance channel of the compound states. Furthermore, it is proposed that the same mechanism that enhances the parity-violation also enhances the breaking of time-reversal-invariance in the compound nucleus. The entrance-channel mixing induces energy-dependent spin-angular correlations of individual $γ$-rays emitted from the compound nuclear state. For a detailed study of the mixing model, a $γ$-ray yield in the reaction of $^{117}$Sn(n,$γ$)$^{118}$Sn was measured using the pulsed beam of polarized epithermal neutrons and Ge detectors. An angular dependence of asymmetric $γ$-ray yields for the orientation of the neutron polarization was observed.

nucl-ex↗
arXiv2022

The CERN n TOF NEAR station for astrophysics- and application-related neutron activation measurements

A new experimental area, the NEAR station, has recently been built at the CERN n TOF facility, at a short distance from the spallation target (1.5 m). The new area, characterized by a neutron beam of very high flux, has been designed with the purpose of performing activation measurements of interest for astrophysics and various applications. The beam is transported from the spallation target to the NEAR station through a hole in the shielding wall of the target, inside which a collimator is inserted. The new area is complemented with a γ-ray spectroscopy laboratory, the GEAR station, equipped with a high efficiency HPGe detector, for the measurement of the activity resulting from irradiation of a sample in the NEAR station. The use of a moderator/filter assembly is envisaged, in order to produce a neutron beam of Maxwellian shape at different thermal energies, necessary for the measurement of Maxwellian Averaged Cross Sections of astrophysical interest. A new fast-cycling activation technique is also being investigated, for measurements of reactions leading to isotopes of very short half life.

physics.ins-det↗
arXiv2022

Advances and new ideas for neutron-capture astrophysics experiments at CERN n_TOF

This article presents a few selected developments and future ideas related to the measurement of $(n,γ)$ data of astrophysical interest at CERN n_TOF. The MC-aided analysis methodology for the use of low-efficiency radiation detectors in time-of-flight neutron-capture measurements is discussed, with particular emphasis on the systematic accuracy. Several recent instrumental advances are also presented, such as the development of total-energy detectors with $γ$-ray imaging capability for background suppression, and the development of an array of small-volume organic scintillators aimed at exploiting the high instantaneous neutron-flux of EAR2. Finally, astrophysics prospects related to the intermediate $i$ neutron-capture process of nucleosynthesis are discussed in the context of the new NEAR activation area.

nucl-ex↗
arXiv2022

Angular distribution of $γ$ rays from the p-wave resonance of $^{118}$Sn

The neutron energy-dependent angular distribution of $γ$ rays from $^{117}{\rm Sn}(n,γ)$ reaction was measured with germanium detectors and a pulsed neutron beam. The angular distribution was clearly observed in $γ$-ray emissions with an energy of 9327 keV which corresponds to the transition from a neutron resonance of $^{117}{\rm Sn}+n$ to the ground state of $^{118}{\rm Sn}$. The angular distribution causes an angular-dependent asymmetric resonance shape. An asymmetry $A_{\rm LH}$ was defined as $(N_{\rm L}-N_{\rm H})/(N_{\rm L}+N_{\rm H})$, where $N_{\rm L}$ and $N_{\rm H}$ are integrated values for lower- and higher-energy regions of a neutron resonance, respectively. We found that the $A_{\rm LH}$ has the angular dependence of $(A \cos θ_γ+B)$, where $θ_γ$ is the $γ$-ray emission angle with respect to the incident neutron momentum, with $A=0.394 \pm 0.073$ and $B = 0.118 \pm 0.029$ in the 1.33 eV p-wave resonance.

nucl-ex↗
arXiv2022

High accuracy, high resolution 235U(n,f) cross section from n_TOF (CERN) in the thermal to 10 keV energy range

The 235U(n,f) cross section was measured in a wide energy range (25 meV - 170 keV) at the n_TOF facility at CERN, relative to 6Li(n,t) and 10B(n,alpha) standard reactions, with high resolution and accuracy, with a setup based on a stack of six samples and six silicon detectors placed in the neutron beam. In this paper we report on the results in the region between thermal and 10 keV neutron energy. A resonance analysis has been performed up to 200 eV, with the code SAMMY. The resulting fission kernels are compared with the ones extracted on the basis of the resonance parameters of the most recent major evaluated data libraries. A comparison of the n_TOF data with the evaluated cross sections is also performed from thermal to 10 keV neutron energy for the energy-averaged cross section in energy groups of suitably chosen width. A good agreement is found in average between the new results and the latest evaluated data files ENDF-B/VIII and JEFF-3.3, as well as with respect to the IAEA reference files. However, some discrepancies are still present in some specific energy regions. The new dataset here presented, characterized by unprecedented resolution and accuracy, can help improving the evaluations in the Resolved Resonance Region and up to 10 keV, and reduce the uncertainties that affect this region.

nucl-ex↗
arXiv2022

The $^{7}$Be(n,p)$^{7}$Li reaction and the Cosmological Lithium Problem: measurement of the cross section in a wide energy range at n_TOF (CERN)

We report on the measurement of the $^{7}$Be($n, p$)$^{7}$Li cross section from thermal to approximately 325 keV neutron energy, performed in the high-flux experimental area (EAR2) of the n_TOF facility at CERN. This reaction plays a key role in the lithium yield of the Big Bang Nucleosynthesis (BBN) for standard cosmology. The only two previous time-of-flight measurements performed on this reaction did not cover the energy window of interest for BBN, and showed a large discrepancy between each other. The measurement was performed with a Si-telescope, and a high-purity sample produced by implantation of a $^{7}$Be ion beam at the ISOLDE facility at CERN. While a significantly higher cross section is found at low-energy, relative to current evaluations, in the region of BBN interest the present results are consistent with the values inferred from the time-reversal $^{7}$Li($p, n$)$^{7}$Be reaction, thus yielding only a relatively minor improvement on the so-called Cosmological Lithium Problem (CLiP). The relevance of these results on the near-threshold neutron production in the p+$^{7}$Li reaction is also discussed.

nucl-ex↗
arXiv2021

Sample-dependent Dirac point gap in MnBi$_2$Te$_4$ and its response to the applied surface charge: a combined photoemission and ab initio study

Recently discovered intrinsic antiferromagnetic topological insulator MnBi$_2$Te$_4$ presents an exciting platform for realization of the quantum anomalous Hall effect and a number of related phenomena at elevated temperatures. An important characteristic making this material attractive for applications is its predicted large magnetic gap at the Dirac point (DP). However, while the early experimental measurements reported on large DP gaps, a number of recent studies claimed to observe a gapless dispersion of the MnBi$_2$Te$_4$ Dirac cone. Here, using micro($μ$)-laser angle-resolved photoemission spectroscopy, we study the electronic structure of 15 different MnBi$_2$Te$_4$ samples, grown by two different chemists groups. Based on the careful energy distribution curves analysis, the DP gaps between 15 and 65 meV are observed, as measured below the Néel temperature at about 10-16 K. At that, roughly half of the studied samples show the DP gap of about 30 meV, while for a quarter of the samples the gaps are in the 50 to 60 meV range. Summarizing the results of both our and other groups, in the currently available MnBi$_2$Te$_4$ samples the DP gap can acquire an arbitrary value between a few and several tens of meV. Further, based on the density functional theory, we discuss a possible factor that might contribute to the reduction of the DP gap size, which is the excess surface charge that can appear due to various defects in surface region. We demonstrate that the DP gap is influenced by the applied surface charge and even can be closed, which can be taken advantage of to tune the MnBi$_2$Te$_4$ DP gap size.

cond-mat.mtrl-sci↗
arXiv2021

Energy dependent angular distribution of individual $γ$-rays in the $^{139}$La($n$, $γ$)$^{140}$La* reaction

Neutron energy-dependent angular distributions were observed for individual $γ$-rays from the 0.74 eV p-wave resonance of $^{139}$La+$n$ to several lower excited states of $^{140}$La. The $γ$-ray signals were analyzed in a two dimensional histogram of the $γ$-ray energy, measured with distributed germanium detectors, and neutron energy, determined with the time-of-flight of pulsed neutrons, to identify the neutron energy dependence of the angular distribution for each individual $γ$-rays. The angular distribution was also found for a photopeak accompanied with a faint p-wave resonance component in the neutron energy spectrum. Our results can be interpreted as interference between s- and p-wave amplitudes which may be used to study discrete symmetries of fundamental interactions.

nucl-ex↗
arXiv2020

Imaging neutron capture cross sections: i-TED proof-of-concept and future prospects based on Machine-Learning techniques

i-TED is an innovative detection system which exploits Compton imaging techniques to achieve a superior signal-to-background ratio in ($n,γ$) cross-section measurements using time-of-flight technique. This work presents the first experimental validation of the i-TED apparatus for high-resolution time-of-flight experiments and demonstrates for the first time the concept proposed for background rejection. To this aim both $^{197}$Au($n,γ$) and $^{56}$Fe($n, γ$) reactions were measured at CERN n\_TOF using an i-TED demonstrator based on only three position-sensitive detectors. Two \cds detectors were also used to benchmark the performance of i-TED. The i-TED prototype built for this study shows a factor of $\sim$3 higher detection sensitivity than state-of-the-art \cds detectors in the $\sim$10~keV neutron energy range of astrophysical interest. This paper explores also the perspectives of further enhancement in performance attainable with the final i-TED array consisting of twenty position-sensitive detectors and new analysis methodologies based on Machine-Learning techniques.

physics.ins-det↗
arXiv2020

Measurement of $γ$ rays from $^6$LiF tile as an inner wall of a neutron-decay detector

A neutron lifetime measurement conducted at the Japan Proton Accelerator Research Complex (J-PARC) is counting the number of electrons from neutron decays with a time projection chamber (TPC). The $γ$ rays produced in the TPC cause irreducible background events. To achieve the precise measurement, the inner walls of the TPC consist of $^6$Li-enriched lithium-fluoride ($^6$LiF) tiles to suppress the amount of $γ$ rays. In order to estimate the amount of $γ$ rays from the $^{6}{\rm LiF}$ tile, prompt gamma ray analysis (PGA) measurements were performed using germanium detectors. We reconstructed the measured $γ$-ray energy spectrum using a Monte Carlo simulation with the stripping method. Comparing the measured spectrum with a simulated one, the number of $γ$ rays emitted from the$^{6}{\rm LiF}$ tile was $(2.3^{+0.7}_{-0.3}) \times 10^{-4}$ per incident neutron. This is $1.4^{+0.5}_{-0.2}$ times the value assumed for a mole fraction of the $^{6}{\rm LiF}$ tile. We concluded that the amount of $γ$ rays produced from the $^{6}{\rm LiF}$ tile is not more twice the originally assumed value.

physics.ins-det↗
arXiv2020

HPRL -- International cooperation to identify and monitor priority nuclear data needs for nuclear applications

The OECD-NEA High Priority Request List (HPRL) is a point of reference to guide and stimulate the improvement of nuclear data for nuclear energy and other applications, and a tool to bridge the gap between data users and producers. The HPRL is application-driven and the requests are submitted by nuclear data users or representatives of the user's communities. A panel of international experts reviews and monitors the requests in the framework of an Expert Group mandated by the NEA Nuclear Science Committee Working Party on International Nuclear Data Evaluation Cooperation (WPEC). After approval, individual requests are classified to three categories: high priority requests, general requests, and special purpose requests (e.g., dosimetry, standards). The HPRL is hosted by the NEA in the form of a relational database publicly available on the web. This paper provides an overview of HPRL entries, status and outlook. Examples of requests successfully completed are given and new requests are described with emphasis on updated nuclear data needs in the fields of nuclear energy, neutron standards and dosimetry.

nucl-ex↗
arXiv2020

Nature of the Dirac gap modulation and surface magnetic interaction in axion antiferromagnetic topological insulator MnBi$_2$Te$_4$

Modification of the gap at the Dirac point (DP) in antiferromagnetic (AFM) axion topological insulator MnBi$_2$Te$_4$ and its electronic and spin structure has been studied by angle- and spin-resolved photoemission spectroscopy (ARPES) under laser excitation with variation of temperature (9-35~K), light polarization and photon energy. We have distinguished both a large (62-67~meV) and a reduced (15-18~meV) gap at the DP in the ARPES dispersions, which remains open above the Néel temperature ($T_\mathrm{N}=24.5$~K). We propose that the gap above $T_\mathrm{N}$ remains open due to short-range magnetic field generated by chiral spin fluctuations. Spin-resolved ARPES, XMCD and circular dichroism ARPES measurements show a surface ferromagnetic ordering for large-gap sample and significantly reduced effective magnetic moment for the reduced-gap sample. These effects can be associated with a shift of the topological DC state towards the second Mn layer due to structural defects and mechanical disturbance, where it is influenced by a compensated effect of opposite magnetic moments.

cond-mat.mtrl-sci↗
arXiv2019

Review and new concepts for neutron-capture measurements of astrophysical interest

The idea of slow-neutron capture nucleosynthesis formulated in 1957 triggered a tremendous experimental effort in different laboratories worldwide to measure the relevant nuclear physics input quantities, namely ($n,γ$) cross sections over the stellar temperature range (from few eV up to several hundred keV) for most of the isotopes involved from Fe up to Bi. A brief historical review focused on total energy detectors will be presented to illustrate how, advances in instrumentation have led, over the years, to the assessment and discovery of many new aspects of $s$-process nucleosynthesis and to the progressive refinement of theoretical models of stellar evolution. A summary will be presented on current efforts to develop new detection concepts, such as the Total-Energy Detector with $γ$-ray imaging capability (i-TED). The latter is based on the simultaneous combination of Compton imaging with neutron time-of-flight (TOF) techniques, in order to achieve a superior level of sensitivity and selectivity in the measurement of stellar neutron capture rates.

physics.ins-det↗
arXiv2019

Variety of magnetic topological phases in the (MnBi$_2$Te$_4$)(Bi$_2$Te$_3$)$_m$ family

Quantum states of matter combining non-trivial topology and magnetism attract a lot of attention nowadays; the special focus is on magnetic topological insulators (MTIs) featuring quantum anomalous Hall and axion insulator phases. Feasibility of many novel phenomena that \emph{intrinsic} magnetic TIs may host depends crucially on our ability to engineer and efficiently tune their electronic and magnetic structures. Here, using angle- and spin-resolved photoemission spectroscopy along with \emph{ab initio} calculations we report on a large family of intrinsic magnetic TIs in the homologous series of the van der Waals compounds (MnBi$_2$Te$_4$)(Bi$_2$Te$_3$)$_m$ with $m=0, ..., 6$. Magnetic, electronic and, consequently, topological properties of these materials depend strongly on the $m$ value and are thus highly tunable. The antiferromagnetic (AFM) coupling between the neighboring Mn layers strongly weakens on moving from MnBi2Te4 (m=0) to MnBi4Te7 (m=1), changes to ferromagnetic (FM) one in MnBi6Te10 (m=2) and disappears with further increase in m. In this way, the AFM and FM TI states are respectively realized in the $m=0,1$ and $m=2$ cases, while for $m \ge 3$ a novel and hitherto-unknown topologically-nontrivial phase arises, in which below the corresponding critical temperature the magnetizations of the non-interacting 2D ferromagnets, formed by the \MBT\, building blocks, are disordered along the third direction. The variety of intrinsic magnetic TI phases in (MnBi$_2$Te$_4$)(Bi$_2$Te$_3$)$_m$ allows efficient engineering of functional van der Waals heterostructures for topological quantum computation, as well as antiferromagnetic and 2D spintronics.

cond-mat.mtrl-sci↗