arXiv subjects

A. Lemaître

Publications and source records attributed to A. Lemaître.

At least 19 recordsLinked to original sources

arXiv2026

Crossing over universal scaling laws in two-dimensional driven dissipative condensates

In low dimensional systems, fluctuations are enhanced and prevent the spontaneous breaking of continuous symmetries. As a result, spatial and temporal correlation functions decay at large distances and long times. A well established example is given by two-dimensional bosonic condensates at equilibrium, which do not display long-range order of the coherence but algebraic decay belonging to the Berezinski-Kosterlitz-Thouless universality class. In contrast, the universal behaviors of non-equilibrium bosonic condensates are more diverse and many open questions remain. Here, we explore the spatio-temporal coherence properties of two-dimensional driven-dissipative polariton condensates in semiconductor optical microcavities. By tuning microscopic parameters, we observe a cross-over between two scaling laws that we attribute to the Edwards-Wilkinson (EW) and the Kardar-Parisi-Zhang (KPZ) universality classes. We demonstrate the collapse of the measured first-order correlations onto the EW and KPZ universal scaling functions and obtain critical exponents, well matching the values predicted theoretically. Our results highlight the intrinsic non-equilibrium nature of polariton condensates and establish them as a platform of choice for controlled exploration of the two-dimensional KPZ universality class.

cond-mat.quant-gas↗

arXiv2026

Dynamical decoupling of a quantum dot spin in a micropillar cavity for spin-multiphoton entanglement

Graph states of mutually entangled photons are key resources for quantum computation and communication and can be generated by leveraging the entanglement between a single resident spin and emitted photons from a charged semiconductor quantum dot (QD). This approach is intrinsically limited by the decoherence of the spin. We study how to mitigate this decoherence with dynamical decoupling of an electron spin in the weak transverse magnetic field regime using spin echo and Carr-Purcell-Meiboom-Gill (CPMG) techniques. Application of these techniques allows us to extend the coherence time of a spin by more than two orders of magnitude, extracting a $T_2^{CPMG}$ of $298\pm53$ ns. We further demonstrate that this technique is compatible with the generation of a spin-photon-photon entangled state at a high rate enabled by a micropillar cavity, with a 20% improvement in simulated state fidelity when using dynamical decoupling. These results pave the way for generating larger and more complex entangled states with QDs.

quant-ph↗

arXiv2026

Accessing which-path information in the absorption and emission of light by a quantum dot in a Ramsey sequence

We quantify which-path information in the absorption and emission of light by a quantum dot along a Ramsey-like sequence. The quantum dot is excited by two successive classical $π/2$-pulses with tunable relative phase, yielding the spontaneous release of coherent superpositions of zero- and one-photon Fock states into two successive time bins. Along the sequence, the first time bin extracts information on the quantum dot energy state, behaving as a which-path detector for the Ramsey interferometer. The which-path information increases over time, and is accessed through the reduction of contrast of the Ramsey fringes. After the second pulse, the information still present in the first time bin controls the emission of coherent light into the second time bin, which is measurable through the reduction of the contrast of self-homodyne interference fringes in a Mach-Zehnder interferometer. Both measurements are in remarkable agreement with theoretical predictions. Our results quantitatively illustrate how which-path information and more generally quantum correlations impact light-matter energy exchanges in the quantum realm.

quant-ph↗

arXiv2025

Tailoring quantum walks in integrated photonic lattices

Unlike discrete photonic circuits, which manipulate photons step-by-step using a series of optical elements, arrays of coupled waveguides enable photons to interfere continuously across the entire structure. When composed of a nonlinear material, such arrays can also directly generate quantum states of light within the circuit. To clarify the similarities and distinctions between these two approaches of quantum walks, we conduct here a systematic comparison between linear waveguide arrays, injected with photons produced externally, and nonlinear arrays, where photon pairs are continuously generated via parametric down-conversion. We experimentally validate these predictions using III-V semiconductor nonlinear waveguide lattices with varied geometries, enabling us to tune the depth of the quantum walks over an order of magnitude and reveal the gradual emergence of non-classicality in the output state. Finally, we demonstrate an inverse-design approach to engineer \textit{aperiodic} waveguide arrays, whose optimized coupling profiles generate maximally entangled states such as the biphoton W-state. These results highlight the potential of continuously-coupled photonic systems to harness high-dimensional entanglement within compact architectures.

quant-ph↗

arXiv2025

Topological protection of photon-pair generation in nonlinear waveguide arrays

Harnessing topological effects offers a promising route to protect quantum states of light from imperfections, potentially enabling more robust platforms for quantum information processing. This capability is particularly relevant for active photonic circuits that generate quantum light directly on-chip. Here, we explore topological effects on photon-pair generation via spontaneous parametric down-conversion (SPDC) in nonlinear waveguide arrays, both theoretically and experimentally. A systematic comparison of homogeneous, trivial, and topological Su-Schrieffer-Heeger arrays reveals that only the topological configuration preserves a stable SPDC resonance spectrum under disorder in the tunnel couplings, with fluctuations in the resonance position reduced by more than one order of magnitude. An analytical model supports our experimental observations by linking this robustness to the band-structure properties of the interacting modes. These findings establish quadratic nonlinear waveguide arrays as a promising platform to explore the interplay of nonlinearity, topology, and disorder in quantum photonic circuits.

quant-ph↗

arXiv2025

The impact of hole $g$-factor anisotropy on spin-photon entanglement generation with InGaAs quantum dots

Self-assembled InGaAs/GaAs quantum dots (QDs) are of particular importance for the deterministic generation of spin-photon entanglement. One promising scheme relies on the Larmor precession of a spin in a transverse magnetic field, which is governed by the in-plane $g$-factors of the electron and valence band heavy-hole. We probe the origin of heavy-hole $g$-factor anisotropy with respect to the in-plane magnetic field direction and uncover how it impacts the entanglement generated between the spin and the photon polarization. First, using polarization-resolved photoluminescence measurements on a single QD, we determine that the impact of valence-band mixing dominates over effects due to a confinement-renormalized cubic Luttinger $q$ parameter. From this, we construct a comprehensive hole $g$-tensor model. We then use this model to simulate the concurrence and fidelity of spin-photon entanglement generation with anisotropic hole $g$-factors, which can be tuned via magnetic field angle and excitation polarization. The results demonstrate that post-growth control of the hole $g$-factor can be used to improve spin-photon cluster state generation.

cond-mat.mes-hall↗

arXiv2025

Deterministic and reconfigurable graph state generation with a single solid-state quantum emitter

Measurement-based quantum computing offers a promising route towards scalable, universal photonic quantum computation. This approach relies on the deterministic and efficient generation of photonic graph states in which many photons are mutually entangled with various topologies. Recently, deterministic sources of graph states have been demonstrated with quantum emitters in both the optical and microwave domains. In this work, we demonstrate deterministic and reconfigurable graph state generation with optical solid-state integrated quantum emitters. Specifically, we use a single semiconductor quantum dot in a cavity to generate caterpillar graph states, the most general type of graph state that can be produced with a single emitter. By using fast detuned optical pulses, we achieve full control over the spin state, enabling us to vary the entanglement topology at will. We perform quantum state tomography of two successive photons, measuring Bell state fidelities up to 0.80$\pm$0.04 and concurrences up to 0.69$\pm$0.09, while maintaining high photon indistinguishability. This simple optical scheme, compatible with commercially available quantum dot-based single photon sources, brings us a step closer to fault-tolerant quantum computing with spins and photons.

quant-ph↗

arXiv2024

Tunable Generation of Spatial Entanglement in Nonlinear Waveguide Arrays

Harnessing high-dimensional entangled states of light presents a frontier for advancing quantum information technologies, from fundamental tests of quantum mechanics to enhanced computation and communication protocols. In this context, the spatial degree of freedom stands out as particularly suited for on-chip integration. But while traditional demonstrations produce and manipulate path-entangled states sequentially with discrete optical elements, continuously-coupled nonlinear waveguide systems offer a promising alternative where photons can be generated and interfere along the entire propagation length, unveiling novel capabilities within a reduced footprint. Here we exploit this concept to implement a compact and reconfigurable source of path-entangled photon pairs based on parametric down-conversion in semiconductor nonlinear waveguides arrays. We use a double-pump configuration to engineer the output quantum state and implement various types of spatial correlations, exploiting a quantum interference effect between the biphoton state generated in each pumped waveguide. This demonstration, at room temperature and telecom wavelength, illustrates the potential of continuously-coupled systems as a promising alternative to discrete multi-component quantum circuits for leveraging the high-dimensional spatial degree of freedom of photons.

quant-ph↗

arXiv2024

Quantum interferences and gates with emitter-based coherent photon sources

Quantum emitters such as quantum dots, defects in diamond or in silicon have emerged as efficient single photon sources that are progressively exploited in quantum technologies. In 2019, it was shown that the emitted single photon states often include coherence with the vacuum component. Here we investigate how such photon-number coherence alters quantum interference experiments that are routinely implemented both for characterising or exploiting the generated photons. We show that it strongly modifies intensity correlation measurements in a Hong-Ou-Mandel experiment and leads to errors in indistinguishability estimations. It also results in additional entanglement when performing partial measurements. We illustrate the impact on quantum protocols by evidencing modifications in heralding efficiency and fidelity of two-qubit gates.

quant-ph↗

arXiv2024

Simultaneous measurements of nuclear spin heat capacity, temperature and relaxation in GaAs microstructures

Heat capacity of the nuclear spin system (NSS) in GaAs-based microstructures has been shown to be much greater than expected from dipolar coupling between nuclei, thus limiting the efficiency of NSS cooling by adiabatic demagnetization. It was suggested that quadrupole interaction induced by some small residual strain could provide this additional reservoir for the heat storage. We check and validate this hypothesis by combining nuclear spin relaxation measurements with adiabatic remagnetization and nuclear magnetic resonance experiments, using electron spin noise spectroscopy as a unique tool for detection of nuclear magnetization. Our results confirm and quantify the role of the quadrupole splitting in the heat storage within NSS and provide additional insight into fundamental, but still actively debated relation between a mechanical strain and the resulting electric field gradients in GaAs.

cond-mat.mes-hall↗

arXiv2023

Experimental analysis of energy transfers between a quantum emitter and light fields

Energy transfer between quantum systems can either be achieved through an effective unitary interaction or through the generation of entanglement. This observation defines two types of energy exchange: unitary and correlation energy. Here we propose and implement experimental protocols to access these energy transfers in interactions between a quantum emitter and light fields. Upon spontaneous emission, we measure the unitary energy transfer from the emitter to the optical field and show that it never exceeds half of the total energy and is reduced when introducing decoherence. We then study the interference of the emitted field and a laser field at a beam splitter and show that the energy transfers quantitatively depend on the quantum purity of the emitted field.

quant-ph↗

arXiv2022

Giant optomechanical coupling and dephasing protection with cavity exciton-polaritons

Electronic resonances can significantly enhance the photon-phonon coupling in cavity optomechanics, but are normally avoided due to absorption losses and dephasing by inhomogeneous broadening. We experimentally demonstrate that exciton-polaritons in semiconductor microcavities enable GHz optomechanics with single-particle resonant couplings reaching record values in the 10s of MHz range. Moreover, this resonant enhancement is protected from inhomogeneous broadening by the Rabi gap. Single-polariton non-linearities and the optomechanical strong-coupling regime become accessible in this platform.

cond-mat.mes-hall↗

arXiv2022

On-chip generation of hybrid polarization-frequency entangled biphoton states

We demonstrate a chip-integrated semiconductor source that combines polarization and frequency entanglement, allowing the generation of entangled biphoton states in a hybrid degree of freedom without postmanipulation. Our AlGaAs device is based on type-II spontaneous parametric down-conversion (SPDC) in a counterpropagating phase-matching scheme, in which the modal birefringence lifts the degeneracy between the two possible nonlinear interactions. This allows the direct generation of polarization-frequency entangled photons, at room temperature and telecom wavelength, and in two distinct spatial modes, offering enhanced flexibility for quantum information protocols. The state entanglement is quantified by a combined measurement of the joint spectrum and Hong-ou-Mandel interference of the biphotons, allowing to reconstruct a restricted density matrix in the hybrid polarization-frequency space.

quant-ph↗

arXiv2022

High-rate entanglement between a semiconductor spin and indistinguishable photons

Photonic graph states, quantum light states where multiple photons are mutually entangled, are key resources for optical quantum technologies. They are notably at the core of error-corrected measurement-based optical quantum computing and all-optical quantum networks. In the discrete variable framework, these applications require high efficiency generation of cluster-states whose nodes are indistinguishable photons. Such photonic cluster states can be generated with heralded single photon sources and probabilistic quantum gates, yet with challenging efficiency and scalability. Spin-photon entanglement has been proposed to deterministically generate linear cluster states. First demonstrations have been obtained with semiconductor spins achieving high photon indistinguishablity, and most recently with atomic systems at high collection efficiency and record length. Here we report on the efficient generation of three partite cluster states made of one semiconductor spin and two indistinguishable photons. We harness a semiconductor quantum dot inserted in an optical cavity for efficient photon collection and electrically controlled for high indistinguishability. We demonstrate two and three particle entanglement with fidelities of 80 % and 63 % respectively, with photon indistinguishability of 88%. The spin-photon and spin-photon-photon entanglement rates exceed by three and two orders of magnitude respectively the previous state of the art. Our system and experimental scheme, a monolithic solid-state device controlled with a resource efficient simple experimental configuration, are very promising for future scalable applications.

quant-ph↗

arXiv2022

Photon-number entanglement generated by sequential excitation of a two-level atom

Entanglement and spontaneous emission are fundamental quantum phenomena that drive many applications of quantum physics. During the spontaneous emission of light from an excited two-level atom, the atom briefly becomes entangled with the photonic field. Here, we show that this natural process can be used to produce photon-number entangled states of light distributed in time. By exciting a quantum dot -- an artificial two-level atom -- with two sequential $π$ pulses, we generate a photon-number Bell state. We characterise this state using time-resolved intensity and phase correlation measurements. Furthermore, we theoretically show that applying longer sequences of pulses to a two-level atom can produce a series of multi-temporal mode entangled states with properties intrinsically related to the Fibonacci sequence. Our results on photon-number entanglement can be further exploited to generate new states of quantum light with applications in quantum technologies.

quant-ph↗

arXiv2021

Three-dimensional electrical control of the excitonic fine structure for a quantum dot in a cavity

The excitonic fine structure plays a key role for the quantum light generated by semiconductor quantum dots, both for entangled photon pairs and single photons. Controlling the excitonic fine structure has been demonstrated using electric, magnetic, or strain fields, but not for quantum dots in optical cavities, a key requirement to obtain high source efficiency and near-unity photon indistinguishability. Here, we demonstrate the control of the fine structure splitting for quantum dots embedded in micropillar cavities. We propose a scheme based on remote electrical contacts connected to the pillar cavity through narrow ridges. Numerical simulations show that such a geometry allows for a three-dimensional control of the electrical field. We experimentally demonstrate tuning and reproducible canceling of the fine structure, a crucial step for the reproducibility of quantum light source technology.

quant-ph↗

arXiv2021

Chiral emission induced by optical Zeeman effect in polariton micropillars

The low sensitivity of photons to external magnetic fields is one of the major challenges for the engineering of photonic lattices with broken time-reversal symmetry. Here we show that time-reversal symmetry can be broken for microcavity polaritons in the absence of any external magnetic field thanks to polarization dependent polariton interactions. Circularly polarized excitation of carriers in a micropillar induces a Zeeman-like energy splitting between polaritons of opposite polarizations. In combination with optical spin-orbit coupling inherent to semiconductor microstructures, the interaction induced Zeeman splitting results in emission of vortical beams with a well-defined chirality. Our experimental findings can be extended to lattices of coupled micropillars opening the possibility of controling optically the topological properties of polariton Chern insulators.

cond-mat.mes-hall↗

arXiv2021

Flexible entanglement-distribution network with an AlGaAs chip for secure communications

Quantum communication networks enable applications ranging from highly secure communication to clock synchronization and distributed quantum computing. Miniaturized, flexible, and cost-efficient resources will be key elements for ensuring the scalability of such networks as they progress towards large-scale deployed infrastructures. Here, we bring these elements together by combining an on-chip, telecom-wavelength, broadband entangled photon source with industry-grade flexible-grid wavelength division multiplexing techniques, to demonstrate reconfigurable entanglement distribution between up to 8 users in a resource-optimized quantum network topology. As a benchmark application we use quantum key distribution, and show low error and high secret key generation rates across several frequency channels, over both symmetric and asymmetric metropolitan-distance optical fibered links and including finite-size effects. By adapting the bandwidth allocation to specific network constraints, we also illustrate the flexible networking capability of our configuration. Together with the potential of our semiconductor source for distributing secret keys over a 60 nm bandwidth with commercial multiplexing technology, these results offer a promising route to the deployment of scalable quantum network architectures.

quant-ph↗