arXiv subjects

A. Lemaitre

Publications and source records attributed to A. Lemaitre.

At least 37 records · Page 2Linked to original sources

arXiv2018

Brillouin Scattering in Hybrid Optophononic Bragg Micropillar Resonators at 300 GHz

We introduce a monolithic Brillouin generator based on a semiconductor micropillar cavity embedding a high frequency nanoacoustic resonator operating in the hundreds of GHz range. The concept of two nested resonators allows an independent design of the ultrahigh frequency Brillouin spectrum and of the optical device. We develop an optical free-space technique to characterize spontaneous Brillouin scattering in this monolithic device and propose a measurement protocol that maximizes the Brillouin generation efficiency in the presence of optically induced thermal effects. The compact and versatile Brillouin generator studied here could be readily integrated into fibered and on-chip architectures.

physics.optics↗

arXiv2018

Topological acoustics in coupled nanocavity arrays

The Su-Schrieffer-Heeger (SSH) model is likely the simplest one-dimensional concept to study non-trivial topological phases and topological excitations. Originally developed to explain the electric conductivity of polyacetylene, it has become a platform for the study of topological effects in electronics, photonics and ultra-cold atomic systems. Here, we propose an experimentally feasible implementation of the SSH model based on coupled one-dimensional acoustic nanoresonators working in the GHz-THz range. In this simulator it is possible to implement different signs in the nearest neighbor interaction terms, showing full tunability of all parameters in the SSH model. Based on this concept we construct topological transition points generating nanophononic edge and interface states and propose an easy scheme to experimentally probe their spatial complex amplitude distribution directly by well-established optical pump-probe techniques.

cond-mat.mes-hall↗

arXiv2017

Nanomechanical resonators based on adiabatic periodicity-breaking in a superlattice

We propose a novel acoustic cavity design where we confine a mechanical mode by adiabatically changing the acoustic properties of a GaAs/AlAs superlattice. By means of high resolution Raman scattering measurements, we experimentally demonstrate the presence of a confined acoustic mode at a resonance frequency around 350 GHz. We observe an excellent agreement between the experimental data and numerical simulations based on a photoelastic model. We demonstrate that the spatial profile of the confined mode can be tuned by changing the magnitude of the adiabatic deformation, leading to strong variations of its mechanical quality factor and Raman scattering cross section. The reported alternative confinement method could lead to the development of a novel generation of nanophononic and optomechanical systems.

cond-mat.mes-hall↗

arXiv2017

BosonSampling with single-photon Fock states from a bright solid-state source

A BosonSampling device is a quantum machine expected to perform tasks intractable for a classical computer, yet requiring minimal non-classical resources as compared to full-scale quantum computers. Photonic implementations to date employed sources based on inefficient processes that only simulate heralded single-photon statistics when strongly reducing emission probabilities. BosonSampling with only single-photon input has thus never been realised. Here, we report on a BosonSampling device operated with a bright solid-state source of single-photon Fock states with high photon-number purity: the emission from an efficient and deterministic quantum dot-micropillar system is demultiplexed into three partially-indistinguishable single-photons, with a single-photon purity $1{-}g^{(2)}(0)$ of $0.990{\pm}0.001$, interfering in a linear optics network. Our demultiplexed source is between one and two orders-of-magnitude more efficient than current heralded multi-photon sources based on spontaneous parametric downconversion, allowing us to complete the BosonSampling experiment faster than previous equivalent implementations.

quant-ph↗

arXiv2017

Probing a dissipative phase transition via dynamical optical hysteresis

We experimentally explore the dynamic optical hysteresis of a semiconductor microcavity as a function of the sweep time. The hysteresis area exhibits a double power law decay due to the shot noise of the driving laser, which triggers switching between metastable states. Upon increasing the average photon number and approaching the thermodynamic limit, the double power law evolves into a single power law. This algebraic behavior characterizes a dissipative phase transition. Our findings are in good agreement with theoretical predictions, and the present experimental approach is promising for the exploration of critical phenomena in photonic lattices.

physics.optics↗

arXiv2016

Active demultiplexing of single-photons from a solid-state source

A scheme for active temporal-to-spatial demultiplexing of single-photons generated by a solid-state source is introduced. The scheme scales quasi-polynomially with photon number, providing a viable technological path for routing n photons in the one temporal stream from a single emitter to n different spatial modes. The active demultiplexing is demonstrated using a state-of-the-art photon source---a quantum-dot deterministically coupled to a micropillar cavity---and a custom-built demultiplexer---a network of electro-optically reconfigurable waveguides monolithically integrated in a lithium niobate chip. The measured demultiplexer performance can enable a six-photon rate three orders of magnitude higher than the equivalent heralded SPDC source, providing a platform for intermediate quantum computation protocols.

quant-ph↗

arXiv2016

Controlling the optical spin Hall effect with light

The optical spin Hall effect (OSHE) is a transport phenomenon of exciton polaritons in semiconductor microcavities, caused by the polaritonic spin-orbit interaction, that leads to the formation of spin textures. In the semiconductor cavity, the physical basis of the spin orbit coupling is an effective magnetic field caused by the splitting of transverse-electric and transverse-magnetic (TE-TM) modes. The spin textures can be observed in the near field (local spin distribution of polaritons), and as light polarization patterns in the more readily observable far field. For future applications in spinoptronic devices, a simple and robust control mechanism, which establishes a one-to-one correspondence between stationary incident light intensity and far-field polarization pattern, is needed. We present such a control scheme, which is made possible by a specific double-microcavity design.

physics.optics↗

arXiv2016

Scalable performance in solid-state single-photon sources

The desiderata for an ideal photon source are high brightness, high single-photon purity, and high indistinguishability. Defining brightness at the first collection lens, these properties have been simultaneously demonstrated with solid-state sources, however absolute source efficiencies remain close to the 1% level, and indistinguishability only demonstrated for photons emitted consecutively on the few nanosecond scale. Here we employ deterministic quantum dot-micropillar devices to demonstrate solid-state single-photon sources with scalable performance. In one device, an absolute brightness at the output of a single-mode fibre of 14% and purities of 97.1-99.0% are demonstrated. When non-resontantly excited, it emits a long stream of photons that exhibit indistinguishability up to 70%---above the classical limit of 50%---even after 33 consecutively emitted photons, a 400 ns separation between them. Resonant excitation in other devices results in near-optimal indistinguishability values: 96% at short timescales, remaining at 88% in timescales as large as 463 ns, after 39 emitted photons. The performance attained by our devices brings solid-state sources into a regime suitable for scalable implementations.

quant-ph↗

arXiv2016

Interaction-induced hopping phase in driven-dissipative coupled photonic microcavities

Bosons hopping across sites and interacting on-site are the essence of the Bose-Hubbard model (BHM). Inspired by the success of BHM simulators with atoms in optical lattices, proposals for implementing the BHM with photons in coupled nonlinear cavities have emerged. Two coupled semiconductor microcavities constitute a model system where the hopping, interaction, and decay of exciton polaritons --- mixed light-matter quasiparticles --- can be engineered in combination with site-selective coherent driving to implement the driven-dissipative two-site optical BHM. Here we explore the interplay of interference and nonlinearity in this system, in a regime where three distinct density profiles can be observed under identical driving conditions. We demonstrate how the phase acquired by polaritons hopping between cavities can be controlled through effective polariton-polariton interactions. Our results open new perspectives for synthesizing density-dependent gauge fields for polaritons in two-dimensional multicavity systems.

physics.optics↗

arXiv2015

Coherent control of a solid-state quantum bit with few-photon pulses

Single photons are the natural link between the nodes of a quantum network: they coherently propagate and interact with many types of quantum bits including natural and artificial atoms. Ideally, one atom should deterministically control the state of a photon and vice-versa. The interaction between free space photons and an atom is however intrinsically weak and many efforts have been dedicated to develop an efficient interface. Recently, it was shown that the propagation of light can be controlled by an atomic resonance coupled to a cavity or a single mode waveguide. Here we demonstrate that the state of a single artificial atom in a cavity can be efficiently controlled by a few-photon pulse. We study a quantum dot optimally coupled to an electrically-controlled cavity device, acting as a near optimal one-dimensional atom. By monitoring the exciton population through resonant fluorescence, we demonstrate Rabi oscillations with a $π$-pulse of only 3.8 photons on average. The probability to flip the exciton quantum bit with a single photon Fock state is calculated to reach 55% in the same device.

quant-ph↗

arXiv2015

Near optimal single photon sources in the solid state

Single-photons are key elements of many future quantum technologies, be it for the realisation of large-scale quantum communication networks for quantum simulation of chemical and physical processes or for connecting quantum memories in a quantum computer. Scaling quantum technologies will thus require efficient, on-demand, sources of highly indistinguishable single-photons. Semiconductor quantum dots inserted in photonic structures are ultrabright single photon sources, but the photon indistinguishability is limited by charge noise induced by nearby surfaces. The current state of the art for indistinguishability are parametric down conversion single-photon sources, but they intrinsically generate multiphoton events and hence must be operated at very low brightness to maintain high single photon purity. To date, no technology has proven to be capable of providing a source that simultaneously generates near-unity indistinguishability and pure single photons with high brightness. Here, we report on such devices made of quantum dots in electrically controlled cavity structures. We demonstrate on-demand, bright and ultra-pure single photon generation. Application of an electrical bias on deterministically fabricated devices is shown to fully cancel charge noise effects. Under resonant excitation, an indistinguishability of $0.9956\pm0.0045$ is evidenced with a $g^{2}(0)=0.0028\pm0.0012$. The photon extraction of $65%$ and measured brightness of $0.154\pm0.015$ make this source $20$ times brighter than any source of equal quality. This new generation of sources open the way to a new level of complexity and scalability in optical quantum manipulation.

quant-ph↗

arXiv2015

Polariton resonances for ultra-strong coupling cavity optomechanics in GaAs/AlAs multiple quantum wells

Polariton-mediated light-sound interaction is investigated through resonant Brillouin experiments in GaAs/AlAs multiple-quantum wells. Photoelastic coupling enhancement at exciton-polariton resonance reaches 105 at 30 K as compared to a typical bulk solid room temperature transparency value. When applied to GaAs based cavity optomechanical nanodevices, this result opens the path to huge displacement sensitivities and to novel ultrastrong-coupling cavity phenomena with optomechanical couplings g0 in the range of 100 THz.

cond-mat.mes-hall↗

arXiv2014

Resonant Brillouin scattering of excitonic polaritons in multiple-quantum-well structures

We present theoretical and experimental study of resonant Brillouin scattering of excitonic polaritons in one-dimensional multiple-quantum-well structure. We obtain general analytical results for the scattering light spectra, valid for arbitrary quantum well arrangement. Application of our theory to the specific case of short-period superlattice shows a perfect quantitative agreement with experimental results for the height, width and position of the Brillouin scattering peaks and allows us to determine the energy, radiative and nonradiative decay rates of quantum well excitons. We reveal the signatures of excitonic polariton formation in the scattering spectra and show, that the spectral width and height are strongly sensitive to the number of wells in the sample.

cond-mat.mes-hall↗

arXiv2013

Vortex stability and permanent flow in nonequilibrium polariton condensates

We study the effects of imprinting a single-quantized vortex on the steady state of a microcavity exciton-polariton condensate generated via parametric scattering. Interestingly we observe two distinct regimes: In the first case, at low polariton densities, the effect of the pulsed probe, containing the vortex state, is to generate a gain response in the condensate lasting for tens of picoseconds during which no dissipation of the circulating currents is detected. In the second regime, at higher densities, the gain lasts much less and the circulation is imprinted directly into the steady state, which acquires permanent rotation for as long as the vortex remains within the condensate. We use two different ways of measuring the circulation of the condensate and demonstrate that in both cases, polariton condensation in the parametric scattering regime can sustain permanent supercurrents.

cond-mat.mes-hall↗

arXiv2013

Dynamic nuclear polarization in InGaAs/GaAs and GaAs/AlGaAs quantum dots under non-resonant ultra-low power optical excitation

We study experimentally the dependence of dynamic nuclear spin polarization on the power of non-resonant optical excitation in two types of individual neutral semiconductor quantum dots: InGaAs/GaAs and GaAs/AlGaAs. We show that the mechanism of nuclear spin pumping via second order recombination of optically forbidden (''dark'') exciton states recently reported in InP/GaInP quantum dots [Phys. Rev. B 83, 125318 (2011)] is relevant for material systems considered in this work. In the InGaAs/GaAs dots this nuclear spin polarization mechanism is particularly pronounced, resulting in Overhauser shifts up to ~80 micro-eV achieved at optical excitation power ~1000 times smaller than the power required to saturate ground state excitons. The Overhauser shifts observed at low-power optical pumping in the interface GaAs/AlGaAs dots are generally found to be smaller (up to ~40 micro-eV). Furthermore in GaAs/AlGaAs we observe dot-to-dot variation and even sign reversal of the Overhauser shift which is attributed to dark-bright exciton mixing originating from electron-hole exchange interaction in dots with reduced symmetry. Nuclear spin polarization degrees reported in this work under ultra-low power optical pumping are comparable to those achieved by techniques such as resonant optical pumping or above-gap pumping with high power circularly polarized light. Dynamic nuclear polarization via second-order recombination of ''dark'' excitons may become a useful tool in single quantum dot applications, where manipulation of the nuclear spin environment or electron spin is required.

cond-mat.mes-hall↗

arXiv2012

Macroscopic quantum self-trapping and Josephson oscillations of exciton-polaritons

A textbook example of quantum mechanical effects is the coupling of two states through a tunnel barrier. In the case of macroscopic quantum states subject to interactions, the tunnel coupling gives rise to Josephson phenomena including Rabi oscillations, the a.c. and d.c. effects, or macroscopic self-trapping depending on whether tunnelling or interactions dominate. Non-linear Josephson physics, observed in superfluid helium and atomic condensates, has remained inaccessible in photonic systems due to the required effective photon-photon interactions. We report on the observation of non-linear Josephson oscillations of two coupled polariton condensates confined in a photonic molecule etched in a semiconductor microcavity. By varying both the distance between the micropillars forming the molecule and the condensate density in each micropillar, we control the ratio of coupling to interaction energy. At low densities we observe coherent oscillations of particles tunnelling between the two micropillars. At high densities, interactions quench the transfer of particles inducing the macroscopic self-trapping of the condensate in one of the micropillars. The finite lifetime of polaritons results in a dynamical transition from self-trapping to oscillations with pi phase. Our results open the way to the experimental study of highly non-linear regimes in photonic systems, such as chaos or symmetry-breaking bifurcations.

cond-mat.mes-hall↗

arXiv2012

Isotope sensitive measurement of the hole-nuclear spin interaction in quantum dots

Decoherence caused by nuclear field fluctuations is a fundamental obstacle to the realization of quantum information processing using single electron spins. Alternative proposals have been made to use spin qubits based on valence band holes having weaker hyperfine coupling. However, it was demonstrated recently both theoretically and experimentally that the hole hyperfine interaction is not negligible, although a consistent picture of the mechanism controlling the magnitude of the hole-nuclear coupling is still lacking. Here we address this problem by performing isotope selective measurement of the valence band hyperfine coupling in InGaAs/GaAs, InP/GaInP and GaAs/AlGaAs quantum dots. Contrary to existing models we find that the hole hyperfine constant along the growth direction of the structure (normalized by the electron hyperfine constant) has opposite signs for different isotopes and ranges from -15% to +15%. We attribute such changes in hole hyperfine constants to the competing positive contributions of p-symmetry atomic orbitals and the negative contributions of d-orbitals. Furthermore, we find that the d-symmetry contribution leads to a new mechanism for hole-nuclear spin flips which may play an important role in hole spin decoherence. In addition the measured hyperfine constants enable a fundamentally new approach for verification of the computed Bloch wavefunctions in the vicinity of nuclei in semiconductor nanostructures.

cond-mat.mes-hall↗

arXiv2012

Miniature GaAs disk resonators probed by a looped fiber taper for optomechanics applications

GaAs disk resonators (typical disk size 5 \mum * 200 nm in our work) are good candidates for boosting optomechanical coupling thanks to their ability to confine both optical and mechanical energy in a sub-micron interaction volume. We present results of optomechanical characterization of GaAs disks by near-field optical coupling from a tapered silica nano-waveguide. Whispering gallery modes with optical Q factor up to a few 10^5 are observed. Critical coupling, optical resonance doublet splitting and mode identification are discussed. We eventually show an optomechanical phenomenon of optical force attraction of the silica taper to the disk. This phenomenon shows that mechanical and optical degrees of freedom naturally couple at the micro-nanoscale.

physics.optics↗