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A. Lopez-Martens

Publications and source records attributed to A. Lopez-Martens.

At least 19 recordsLinked to original sources

The electromagnetic decay of $^{250m}$No and the stability of neutron deficient Rf isotopes

The electromagnetic decay of the $\approx$40 $μ$s isomer of $^{250}$No has been investigated using the \textsc{Geant4} toolkit for the simulations of the interaction of particles through matter. It is concluded that the decay does not follow the pattern established in the lighter isotones, where the isomer decays directly to members of the ground state rotational band. An alternative scenario is proposed. The implications on the location of the isotopic border for neutron deficient Rf isotopes are discussed.

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Direct transfer to $^{46,48}$K as a survey of the $π(s_{1/2})$$-ν(sdpf)$ interaction

The collapse of the canonical $N=28$ magic number in nuclei with $Z<20$ has drawn significant interest as it relates to the emergence of an island of inversion centered on $^{42}$Si and $^{44}$S. In particular, interactions between the $πs_{1/2}$ orbital -- empty in $^{42}$Si and full in $^{44}$S -- and the neutron orbitals just above and below the $N=28$ gap are expected to be critical in this region, but remain relatively unexplored. In this paper, we expand upon the results of our previous study of the direct transfer reaction $^{47}$K(d,p$γ$)$^{48}$K [C.\,J.~Paxman \textit{et al.}, Phys. Rev. Lett. 134, 162504 (2025)] with the results of the complementary $^{47}$K(d,t$γ$)$^{46}$K reaction. Through this study, we present a comprehensive scan of the interaction between the critical $πs_{1/2}$ orbital and a broad range of neutron orbitals spanning nearly two full shells. We identify several discrepancies between the experimental results and state-of-the-art shell model calculations, which suggest a deficiency of the shell model to fully capture the complex proton configuration mixing in this region, highlighting a significant challenge for single-particle descriptions of the island of inversion.

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Structure studies of 257Db through combined α, γ and internal-conversion-electron spectroscopy

This work reports on the study of the decay properties along the $^{257}$Db decay chain using the GABRIELA setup. The first observation of a high-K isomer in $^{257}$Db is presented. In addition, an unreported $α$-decay branch in $^{249}$Md has been evidenced, allowing to constrain the differences in energy of the $α$-decaying levels in $^{249}$Md, $^{253}$Lr and $^{257}$Db. Finally, the combination of the observed fine structure $α$-decay from the high-spin state in $^{257}$Db with the first observation the internal decay in $^{253}$Lr requires a revision of level and decay scheme. In particular, a change of parity for the high-spin state from 9/2$^{+}$ to 9/2$^{-}$ in the $^{257}$Db is suggested, and the implications of such a change are also discussed.

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Probing exotic cross-shell interactions at N=28 with single-neutron transfer on 47K

We present the first measurement of the $^{47}$K($d,pγ$)$^{48}$K transfer reaction, performed in inverse kinematics using a reaccelerated beam of $^{47}$K. The level scheme of $^{48}$K has been greatly extended with nine new bound excited states identified and spectroscopic factors deduced. Detailed comparisons with SDPF-U and SDPF-MU shell-model calculations reveal a number of discrepancies with these results, and a preference for SDPF-MU is found. Intriguingly, an apparent systematic overestimation of spectroscopic factors and a poor reproduction of the energies for 1$^-$ states suggests that the mixing between the $πs^{\,\,\,1}_{1/2} d^{\,\,\,4}_{3/2}$ and $πs^{\,\,\,2}_{1/2} d^{\,\,\,3}_{3/2}$ proton configurations in $^{48}$K is not correctly described using current interactions, challenging our descriptions of light $N=28$ nuclei.

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High-precision spectroscopy of $^{20}$O benchmarking ab-initio calculations in light nuclei

The excited states of unstable $^{20}$O were investigated via $γ$-ray spectroscopy following the $^{19}$O$(d,p)^{20}$O reaction at 8 $A$MeV. By exploiting the Doppler Shift Attenuation Method, the lifetime of the 2$^+_2$ and 3$^+_1$ states were firmly established. From the $γ$-ray branching and E2/M1 mixing ratios for transitions deexciting the 2$^+_2$ and 3$^+_1$ states, the B(E2) and B(M1) were determined. Various chiral effective field theory Hamiltonians, describing the nuclear properties beyond ground states, along with a standard USDB interaction, were compared with the experimentally obtained data. Such a comparison for a large set of $γ$-ray transition probabilities with the valence space in medium similarity renormalization group ab-initio calculations was performed for the first time in a nucleus far from stability. It was shown that the ab-initio approaches using chiral EFT forces are challenged by detailed high-precision spectroscopic properties of nuclei. The reduced transition probabilities were found to be a very constraining test of the performance of the ab-initio models.

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Fission of 215Fr studied with gamma spectroscopic methods

Background: Asymmetric fission is known to occur in two regions, the actinides and sub-lead, and is dependent on the fissioning system excitation energy. Experimental evidence in the sub-lead region show that this mode is surprisingly persistent with increasing energy and its origin is not fully understood. Purpose: To experimentally study the fusion-fission reaction of $^{215}$Fr at moderate excitation energy and determine previously unknown independent fission yields and other properties. Method: The compound nucleus was formed in the reaction $^{18}$O + $^{197}$Au. The prompt gamma-rays emitted during the reaction were measured with the high efficiency and high granularity $ν$-ball2 spectrometer. Independent fission yields of even-even nuclei were determined by detecting triple-gamma cascades in the fission fragments. Results: The observed yields, although dominated by a symmetric peak, show maxima for heavy fragment of $Z \approx 54-56$, which is consistent with the known results in the actinide region but unexpected for the nuclide of interest, and at the studied excitation energy. Conclusions: The mode of asymmetric fission is present even at relatively high excitation energies in the system studied. This observation matches experimental findings in the sub-lead region, contrary to the actinides, and so far there is no well-developed explanation of this phenomenon.

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AGATA: Performance of $γ$-ray tracking and associated algorithms

AGATA is a modern $γ$-ray spectrometer for in-beam nuclear structure studies, based on $γ$-ray tracking. Since more than a decade, it has been operated performing experimental physics campaigns in different international laboratories (LNL, GSI, GANIL). This paper reviews the obtained results concerning the performances of $γ$-ray tracking in AGATA and associated algorithms. We discuss $γ$-ray tracking and algorithms developed for AGATA. Then, we present performance results in terms of efficiency and peak-to-total for AGATA. The importance of the high effective angular resolution of $γ$-ray tracking arrays is emphasised, e.g. with respect to Doppler correction. Finally, we briefly touch upon the subject of $γ$-ray imaging and its connection to $γ$-ray tracking.

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Search for $^{22}$Na in novae supported by a novel method for measuring femtosecond nuclear lifetimes

Classical novae are thermonuclear explosions in stellar binary systems, and important sources of $^{26}$Al and $^{22}$Na. While gamma rays from the decay of the former radioisotope have been observed throughout the Galaxy, $^{22}$Na remains untraceable. The half-life of $^{22}$Na (2.6 yr) would allow the observation of its 1.275 MeV gamma-ray line from a cosmic source. However, the prediction of such an observation requires good knowledge of the nuclear reactions involved in the production and destruction of this nucleus. The $^{22}$Na($p,γ$)$^{23}$Mg reaction remains the only source of large uncertainty about the amount of $^{22}$Na ejected. Its rate is dominated by a single resonance on the short-lived state at 7785.0(7) keV in $^{23}$Mg. In the present work, a combined analysis of particle-particle correlations and velocity-difference profiles is proposed to measure femtosecond nuclear lifetimes. The application of this novel method to the study of the $^{23}$Mg states, combining magnetic and highly-segmented tracking gamma-ray spectrometers, places strong limits on the amount of $^{22}$Na produced in novae, explains its non-observation to date in gamma rays (flux < 2.5x$10^{-4}$ ph/(cm$^2$s)), and constrains its detectability with future space-borne observatories.

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Study of the production and decay properties of neutron-deficient nobelium isotopes

The new neutron-deficient isotope $^{249}$No was synthesized for the first time in the fusion-evaporation reaction $^{204}$Pb($^{48}$Ca,3n)$^{249}$No. After separation, using the kinematic separator SHELS, the new isotope was identified with the GABRIELA detection system through genetic correlations with the known daughter and granddaughter nuclei $^{245}$Fm and $^{241}$Cf. The alpha-decay activity of $^{249}$No has an energy of 9129(22)$~$keV and half-life 38.3(2.8) ms. An upper limit of 0.2\% was measured for the fission branch of $^{249}$No. Based on the present data and recent information on the decay properties of $^{253}$Rf and aided by Geant4 simulations, the ground state of $^{249}$No is assigned the 5/2$^+$[622] neutron configuration and a partial decay scheme from $^{253}$Rf to $^{245}$Fm could be established. The production cross-section was found to be $σ$(3n)=0.47(4) nb at a mid-target beam energy of 225.4 MeV, which corresponds to the maximum of the calculated excitation function. Correlations of the $^{249}$No alpha activity with subsequent alpha decays of energy 7728(20) keV and half-life $1.2_{-0.4}^{+1.0}$ min provided a firm measurement of the electron-capture or $β^{+}$ branch of $^{245}$Fm to $^{245}$Es. The excitation function for the 1n, 2n and 3n evaporation channels was measured. In the case of the 2n-evaporation channel $^{250}$No, a strong variation of the ground state and isomeric state populations as a function of bombarding energy could be evidenced.

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Spontaneous fission of 246Fm

An experiment on the study of the $^{246}$Fm spontaneous fission was conducted using the SHELS separator. The isotope was synthesized in the complete fusion reaction of $^{40}$Ar beam ions and $^{208}$Pb target nuclei. The neutron yields of $^{246}$Fm spontaneous fission ($\overlineν = 3.79\pm0.30$, $σ^{2}_ν = 2.1$) were obtained using the SFiNx detector system. The multiplicity distribution of emitted prompt neutrons was restored using the Tikhonov method of statistical regularisation ($\overlineν_{r} = 3.79\pm0.20$, $σ^{2}_{νr} = 2.8$). The spontaneous fission branching ratio ($b_{SF} = 0.061\pm0.005$) and the half-life ($T_{1/2} = 1.50^{+0.08}_{-0.07}$ s) of the isotope were determined. The experimental data were compared with scission point model predictions. Excellent convergence was observed in the average number of neutrons per spontaneous fission process. However, the forms of the experimental and model prompt neutron multiplicity distributions differ significantly.

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Fission properties of $^{253}$Rf and the stability of neutron-deficient Rf isotopes

An analysis of recent experimental data [J. Khuyagbaatar et al., Phys. Rev. C 104, L031303 (2021)] has established the existence of two fissioning states in $^{253}$Rf: the ground state and a low-lying isomeric state, most likely involving the same neutron single-particle configurations as in the lighter isotone $^{251}$No. The ratio of fission half-lives measured in $^{253}$Rf was used to predict the fission properties of the 1/2$^{+}$ isomeric state in $^{251}$No and draw conclusions as to the stability against fission of even lighter Rf systems. This paper focusses again on the fission properties of $^{253}$Rf and their impact on the stability of other neutron deficient isotopes, using new and improved data collected from two experiments performed at the Flerov Laboratory of Nuclear Reactions in Dubna, Russia. Two fission activities with half-lives of 52.8(4.4)$~μ$s and 9.9(1.2) ms were measured in the case of $^{253}$Rf, confirming the results of J. Kkuyagbaatar et al. A third state, at much higher excitation energy, was also observed through the detection of its electromagnetic decay to the 52.8$~μ$s state. This observation leads to the opposite quantum-configuration assignments for the fissioning states as compared to the ones established by J. Khuyagbaatar et al., namely that the higher-spin state has the shortest fission half-life. This inversion of the ratio of fission hindrances between the low and high-spin states is corroborated in the isotone $^{251}$No by the non observation of any substantial fission branch from the low-spin isomer.

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Narrow resonances in the continuum of the unbound nucleus $^{15}$F

The structure of the unbound $^{15}$F nucleus is investigated using the inverse kinematics resonant scattering of a radioactive $^{14}$O beam impinging on a CH$_2$ target. The analysis of $^{1}$H($^{14}$O,p)$^{14}$O and $^{1}$H($^{14}$O,2p)$^{13}$N reactions allowed the confirmation of the previously observed narrow $1/2^{-}$ resonance, near the two-proton decay threshold, and the identification of two new narrow 5/2$^{-}$ and 3/2$^{-}$ resonances. The newly observed levels decay by 1p emission to the ground of $^{14}$O, and by sequential 2p emission to the ground state (g.s.) of $^{13}$N via the $1^-$ resonance of $^{14}$O. Gamow shell model (GSM) analysis of the experimental data suggests that the wave functions of the 5/2$^{-}$ and 3/2$^{-}$ resonances may be collectivized by the continuum coupling to nearby 2p- and 1p- decay channels. The observed excitation function $^{1}$H($^{14}$O,p)$^{14}$O and resonance spectrum in $^{15}$F are well reproduced in the unified framework of the GSM.

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First observation of high-$K$ isomeric states in $^{249}$Md and $^{251}$Md

Decay spectroscopy of the odd-proton nuclei $^{249}$Md and $^{251}$Md has been performed. High-$K$ isomeric states were identified for the first time in these two nuclei through the measurement of their electromagnetic decay. An isomeric state with a half-life of $2.8(5)$ ms and an excitation energy $\geq 910$ keV was found in $^{249}$Md. In $^{251}$Md, an isomeric state with a half-life of $1.4(3)$ s and an excitation energy $\geq 844$ keV was found. Similarly to the neighbouring $^{255}$Lr, these two isomeric states are interpreted as 3 quasi-particle high-$K$ states and compared to new theoretical calculations. Excited nuclear configurations were calculated within two scenarios: via blocking nuclear states located in proximity to the Fermi surface or/and using the quasiparticle Bardeen-Cooper-Schrieffer method. Relevant states were selected on the basis of the microscopic-macroscopic model with a deformed Woods-Saxon potential. The most probable candidates for the configurations of $K$-isomeric states in Md nuclei are proposed.

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Lifetime Measurements in the Even-Even $^{102-108}$Cd Isotopes

The heaviest N=Z doubly-magic nucleus, $^{100}$Sn, and the neighboring nuclei offer unique opportunities to investigate the properties of nuclear interaction in extreme conditions. In particular, the Cd isotopes are expected to present features similar to those found in the Sn isotopic chain, since they have only two proton holes in the Z=50 shell. In this manuscript, the lifetime measurements of low-lying states in the even-mass $^{102-108}$Cd is presented. Thanks to the powerful detection capabilities of AGATA array and VAMOS++ spectrometer, the unusual employment of multi-nucleon transfer reactions permitted to investigate the first 2$^+$ and 4$^+$ states in all these nuclei, together with various deformed bands in $^{106}$Cd. The results were interpreted in the context of new state-of-the-art beyond-mean-field calculations, using the symmetry-conserving configuration-mixing approach. Despite the similarities in the electromagnetic properties of the low-lying states, there is a fundamental structural difference between the ground-state bands in the Z=48 and Z=50 isotopes. The comparison between experimental and theoretical results revealed a rotational character of the Cd nuclei, which have prolate-deformed ground states with $β_2 \approx 0.2$. At this deformation Z=48 becomes a closed-shell configuration, which is favored with respect to the spherical one.

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Alpha-decay spectroscopy of $^{257}$Rf

The decay properties of the ground state and excited states of $^{257}$Rf have been investigated with the detector array GABRIELA at the FLNR, Dubna. The electromagnetic decay of a new excited state in $^{253}$No has been observed. The state lies 750 keV above the ground state and is favourably populated in the alpha decay of the low-lying spin isomer of $^{257}$Rf. It decays to the 9/2$^-$ ground state by an M1 transition and is assigned the 11/2$^-$[725] Nilsson configuration. The presence of this state suggests a possible reinterpretation of the decay of the high-K isomer in $^{253}$No.

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Position uncertainties of AGATA pulse-shape analysis estimated via the boostrapping method

The unprecedented capabilities of state-of-the-art segmented germanium-detector arrays, such as AGATA and GRETA, derive from the possibility of performing pulse-shape analysis. The comparison of the net- and transient-charge signals with databases via grid-search methods allows the identification of the $γ$-ray interaction points within the segment volume. Their precise determination is crucial for the subsequent reconstruction of the $γ$-ray paths within the array via tracking algorithms, and hence the performance of the spectrometer. In this paper the position uncertainty of the deduced interaction point is investigated using the bootstrapping technique applied to $^{60}$Co radioactive-source data. General features of the extracted position uncertainty are discussed as well as its dependence on various quantities, e.g. the deposited energy, the number of firing segments and the segment geometry.

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Performance of The Advanced GAmma Tracking Array at GANIL

The performance of the Advanced GAmma Tracking Array (AGATA) at GANIL is discussed, on the basis of the analysis of source and in-beam data taken with up to 30 segmented crystals. Data processing is described in detail. The performance of individual detectors are shown. The efficiency of the individual detectors as well as the efficiency after $γ$-ray tracking are discussed. Recent developments of $γ$-ray tracking are also presented. The experimentally achieved peak-to-total is compared with simulations showing the impact of back-scattered $γ$ rays on the peak-to-total in a $γ$-ray tracking array. An estimate of the achieved position resolution using the Doppler broadening of in-beam data is also given. Angular correlations from source measurements are shown together with different methods to take into account the effects of $γ$-ray tracking on the normalization of the angular correlations.

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In-beam gamma-ray and electron spectroscopy of $^{249,251}$Md

The odd-$Z$ $^{251}$Md nucleus was studied using combined $γ$-ray and conversion-electron in-beam spectroscopy. Besides the previously observed rotational band based on the $[521]1/2^-$ configuration, another rotational structure has been identified using $γ$-$γ$ coincidences. The use of electron spectroscopy allowed the rotational bands to be observed over a larger rotational frequency range. Using the transition intensities that depend on the gyromagnetic factor, a $[514]7/2^-$ single-particle configuration has been inferred for this band, i.e., the ground-state band. A physical background that dominates the electron spectrum with an intensity of $\simeq$ 60% was well reproduced by simulating a set of unresolved excited bands. Moreover, a detailed analysis of the intensity profile as a function of the angular momentum provided a method for deriving the orbital gyromagnetic factor, namely $g_K = 0.69^{+0.19}_{-0.16}$ for the ground-state band. The odd-$Z$ $^{249}$Md was studied using $γ$-ray in-beam spectroscopy. Evidence for octupole correlations resulting from the mixing of the $Δl = Δj = 3$ $[521]3/2^-$ and $[633]7/2^+$ Nilsson orbitals were found in both $^{249,251}$Md. A surprising similarity of the $^{251}$Md ground-state band transition energies with those of the excited band of $^{255}$Lr has been discussed in terms of identical bands. Skyrme-Hartree-Fock-Bogoliubov calculations were performed to investigate the origin of the similarities between these bands.

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