arXiv subjects

A. Müller

Publications and source records attributed to A. Müller.

87 records · Page 5Linked to original sources

arXiv2012

Decoherence window and electron-nuclear cross-relaxation in the molecular magnet V 15

Rabi oscillations in the V_15 Single Molecule Magnet (SMM) embedded in the surfactant DODA have been studied at different microwave powers. An intense damping peak is observed when the Rabi frequency Omega_R falls in the vicinity of the Larmor frequency of protons w_N, while the damping time t_R of oscillations reaches values 10 times shorter than the phase coherence time t_2 measured at the same temperature. The experiments are interpreted by the N-spin model showing that t_R is directly associated with the decoherence via electronic/nuclear spin cross-relaxation in the rotating reference frame. It is shown that this decoherence is accompanied with energy dissipation in the range of the Rabi frequencies w_N - sigma_e < Omega_R < w_N, where sigma_e is the mean super-hyperfine field (in frequency units) induced by protons at SMMs. Weaker damping without dissipation takes place outside this dissipation window. Simple local field estimations suggest that this rapid cross-relaxation in resonant microwave field observed for the first time in SMMV_15 should take place in other SMMs like Fe_8 and Mn_12 containing protons, too.

cond-mat.str-el↗

arXiv2012

Electron-ion Recombination of Fe XII forming Fe XI: Laboratory Measurements and Theoretical Calculations

We have measured electron-ion recombination for Fe XII forming Fe XI using a merged beams configuration at the heavy-ion storage ring TSR located at the Max Planck Institute for Nuclear Physics in Heidelberg, Germany. The measured merged beams recombination rate coefficient (MBRRC) for collision energies from 0 to 1500 eV is presented. This work uses a new method for determining the absolute MBRRC based on a comparison of the ion beam decay rate with and without the electron beam on. For energies below 75 eV, the spectrum is dominated by dielectronic recombination (DR) resonances associated with 3s-3p and 3p-3d core excitations. At higher energies we observe contributions from 3-N' and 2-N' core excitations DR. We compare our experimental results to state-of-the-art multi-configuration Breit-Pauli (MCBP) calculations and find significant differences, both in resonance energies and strengths. We have extracted the DR contributions from the measured MBRRC data and transformed them into a plasma recombination rate coefficient (PRRC) for temperatures in the range of 10^3 to 10^7 K. We show that the previously recommended DR data for Fe XII significantly underestimate the PRRC at temperatures relevant for both photoionized plasmas (PPs) and collisionaly ionized plasmas (CPs). This is to be contrasted with our MCBP PRRC results which agree with the experiment to within 30% at PP temperatures and even better at CP temperatures. We find this agreement despite the disagreement shown by the detailed comparison between our MCBP and experimental MBRRC results. Lastly, we present a simple parameterized form of the experimentally derived PRRC for easy use in astrophysical modelling codes.

astro-ph.IM↗

arXiv2012

K-shell photoionization of ground-state Li-like boron ions [B$^{2+}$]: Experiment and Theory

Absolute cross sections for the K-shell photoionization of ground-state Li-like boron [B$^{2+}$(1s$^2$2s $^2$S)] ions were measured by employing the ion-photon merged-beams technique at the Advanced Light Source synchrotron radiation facility. The energy ranges 197.5--200.5 eV, 201.9--202.1 eV of the [1s(2s\,2p)$^3$P]$^2$P${\rm ^o}$ and [1s(2s\,2p)$^1$P] $^2$P${\rm ^o}$ resonances, respectively, were investigated using resolving powers of up to 17\,600. The energy range of the experiments was extended to about 238.2 eV yielding energies of the most prominent [1s(2$\ell$\,n$\ell^{\prime}$)]$^2$P$^o$ resonances with an absolute accuracy of the order of 130 ppm. The natural linewidths of the [1s(2s\,2p)$^3$P] $^2$P${\rm ^o}$ and [1s(2s\,2p)$^1$P] $^2$P${\rm ^o}$ resonances were measured to be $4.8 \pm 0.6$ meV and $29.7 \pm 2.5$ meV, respectively, which compare favourably with theoretical results of 4.40 meV and 30.53 meV determined using an intermediate coupling R-matrix method.

astro-ph.EP↗

arXiv2011

Storage-ring measurement of the hyperfine-induced 2s 2p 3P0 -> 2s2 1S0 transition rate in beryllium-like sulfur

The hyperfine induced 2s 2p 3P0 -> 2s2 1S0 transition rate in Be-like sulfur was measured by monitoring the decay of isotopically pure beams of 32-S12+ and 33-S12+ ions in a heavy-ion storage ring. Within the 4% experimental uncertainty the experimental value of 0.096(4)/s agrees with the most recent theoretical results of Cheng et al. [Phys. Rev. A 77, 052504 (2008)] and Andersson et al. [Phys. Rev. A 79, 032501 (2009)]. Repeated experiments with different magnetic fields in the storage-ring bending magnets demonstrate that artificial quenching of the 2s 2p 3P0 state by these magnetic fields is negligible.

physics.atom-ph↗

arXiv2011

Orbit of the young very low-mass spectroscopic binary CHXR 74

The pre-main sequence star CHXR74 (M4.25) in ChaI was detected a few years ago to be a very low-mass spectroscopic binary. Determination of its mass would provide a valuable dynamical mass measurement at young ages in the poorly constrained mass regime of <0.3 Msun. We carried out follow-up radial velocity (RV) monitoring with UVES/VLT between 2008 and 2011 and high-resolution adaptive optic assisted imaging with NACO/VLT in 2008 with the aim to constrain the binary orbit. We present an orbital solution of the system based on the combined RV data set which spans more than 11 years of UVES monitoring for CHXR74. The best-fit Kepler model has an orbital period of 13.1 yrs, zero eccentricity, and a RV semi-amplitude of 2.2 km/s. A companion mass M2sini of 0.08 Msun is derived by using a model-dependent mass estimate for the primary of 0.24 Msun. The binary separation for i=90deg is 3.8 AU (23 mas). Complementary NACO images of CHXR74 were taken with the aim to directly resolve the binary. While there are marginal signs of an extended PSF, we have no convincing companion detected to CHXR74 in these images. From the non-detection of the companion together with a prediction of the binary separation at the time of the NACO observations, we derive an upper limit for the K-band brightness ratio of 0.5. This allows us to estimate an upper limit of the companion mass of 0.14 Msun by applying evolutionary models. Thus, we have confirmed that CHXR74 is a very low-mass spectroscopic binary and constrained the secondary mass to lie within the range of about 0.08 and 0.14 Msun. We predict an astrometric signal of the primary between 0.2 and 0.4 mas when taking into account the luminosity of the companion. The GAIA astrometric mission might well be able to solve the astrometric orbit of the primary and in combination with the presented RV data to determine an absolute companion mass.

astro-ph.SR↗

arXiv2011

Versatile sputtering technology for Al2O3 gate insulators on graphene

We report a novel fabrication method of graphene Al2O3 gate insulators based on sputtering. Electrical performance of dual-gated mono- and bilayer exfoliated graphene devices is presented. Sputtered Al2O3 layers possess comparable quality to oxides obtained by atomic layer deposition (ALD) with respect to a high relative dielectric constant of about 8, as well as low-hysteresis performance and high breakdown voltage. We observe a moderate carrier mobility of about 1000 cm2/Vs in graphene and 350 cm2/Vs in its bilayer due to increased resonant scattering on atomic scale defects. Most likely this originated from the thin Al precursor layer evaporated prior to sputtering the Al2O3 gate oxide.

cond-mat.mes-hall↗

arXiv2011

Classification of super domains and super domain walls in permalloy antidot lattices

We study the remanent domain configurations of rectangular permalloy antidot lattices over a range of lattice parameters. The influence of antidot diameter, antidot spacing, and the aspect ratio of the lattice on the remanent domain configuration are investigated by magnetic force microscopy and supported by micromagnetic simulations. In the remanent state, areas of cells with the same orientation of average magnetization form magnetic super domains separated by super domain walls (SDWs). Two types of SDWs are identified. The first type is characterized by low stray field energy, is linear, and expands over many lattice constants. In contrast the second type shows high stray field energy and is situated at kinks of low energy SDWs. Its width can vary from a minimum of two lattice cells up to several lattice constants, depending on the lattice parameters. The occurrence and structure of these two types of SDWs as function of lattice parameters are classified and discussed in terms of the interplay of stray field and exchange energy.

cond-mat.mes-hall↗

arXiv2011

Dielectronic recombination of xenonlike tungsten ions

Dielectronic recombination (DR) of xenonlike W20+ forming W19+ has been studied experimentally at a heavy-ion storage-ring. A merged-beams method has been employed for obtaining absolute rate coefficients for electron-ion recombination in the collision energy range 0-140 eV. The measured rate coefficient is dominated by strong DR resonances even at the lowest experimental energies. At plasma temperatures where the fractional abundance of W20+ is expected to peak in a fusion plasma, the experimentally derived plasma recombination rate coefficient is over a factor of 4 larger than the theoretically-calculated rate coefficient which is currently used in fusion plasma modeling. The largest part of this discrepancy stems most probably from the neglect in the theoretical calculations of DR associated with fine-structure excitations of the W20+([Kr] 4d10 4f8) ion core.

physics.atom-ph↗

arXiv2009

Epitaxial growth of Fe3O4 thin films on ZnO and MgO substrates

Magnetite thin fims have been grown epitaxially on ZnO and MgO substrates using molecular beam epitaxy. The film quality was found to be strongly dependent on the oxygen partial pressure during growth. Structural, electronic, and magnetic properties were analyzed utilizing Low Energy Electron Diffraction (LEED), HArd X-ray PhotoElectron Spectroscopy (HAXPES), Magneto Optical Kerr Effect (MOKE), and X-ray Magnetic Circular Dichroism (XMCD). Diffraction patterns show clear indication for growth in the (111) direction on ZnO. Vertical structure analysis by HAXPES depth profiling revealed uniform magnetite thin films on both type of substrates. Both, MOKE and XMCD measurements show in-plane easy magnetization with a reduced magnetic moment in case of the films on ZnO.

cond-mat.mtrl-sci↗

arXiv2009

Electron-ion Recombination of Fe X forming Fe IX and of Fe XI forming Fe X: Laboratory Measurements and Theoretical Calculations

We have measured electron-ion recombination for Fe$^{9+}$ forming Fe$^{8+}$ and for Fe$^{10+}$ forming Fe$^{9+}$ using merged beams at the TSR heavy-ion storage-ring in Heidelberg. The measured merged beams recombination rate coefficients (MBRRC) for relative energies from 0 to 75 eV are presented, covering all dielectronic recombination (DR) resonances associated with 3s->3p and 3p->3d core transitions in the spectroscopic species Fe X and Fe XI, respectively. We compare our experimental results to multi-configuration Breit-Pauli (MCBP) calculations and find significant differences. From the measured MBRRC we have extracted the DR contributions and transform them into plasma recombination rate coefficients (PRRC) for astrophysical plasmas with temperatures from 10^2 to 10^7 K. This spans across the regimes where each ion forms in photoionized or in collisionally ionized plasmas. For both temperature regimes the experimental uncertainties are 25% at a 90% confidence level. The formerly recommended DR data severely underestimated the rate coefficient at temperatures relevant for photoionized gas. At the temperatures relevant for photoionized gas, we find agreement between our experimental results and MCBP theory. At the higher temperatures relevant for collisionally ionized gas, the MCBP calculations yield a Fe XI DR rate coefficent which is significantly larger than the experimentally derived one. We present parameterized fits to our experimentally derived DR PRRC.

astro-ph.GA↗

arXiv2008

Isotope shift in the dielectronic recombination of three-electron ^{A}Nd^{57+}

Isotope shifts in dielectronic recombination spectra were studied for Li-like ^{A}Nd^{57+} ions with A=142 and A=150. From the displacement of resonance positions energy shifts δE^{142,150}(2s-2p_1/2)= 40.2(3)(6) meV (stat)(sys)) and δE^{142,150}(2s-2p_3/2) = 42.3(12)(20) meV of 2s-2p_j transitions were deduced. An evaluation of these values within a full QED treatment yields a change in the mean-square charge radius of ^{142,150}δ = -1.36(1)(3) fm^2. The approach is conceptually new and combines the advantage of a simple atomic structure with high sensitivity to nuclear size.

physics.atom-ph↗

arXiv2007

Dielectronic Recombination of Fe XV forming Fe XIV: Laboratory Measurements and Theoretical Calculations

We have measured resonance strengths and energies for dielectronic recombination (DR) of Mg-like Fe XV forming Al-like Fe XIV via N=3 -> N' = 3 core excitations in the electron-ion collision energy range 0-45 eV. All measurements were carried out using the heavy-ion Test Storage Ring at the Max Planck Institute for Nuclear Physics in Heidelberg, Germany. We have also carried out new multiconfiguration Breit-Pauli (MCBP) calculations using the AUTOSTRUCTURE code. For electron-ion collision energies < 25 eV we find poor agreement between our experimental and theoretical resonance energies and strengths. From 25 to 42 eV we find good agreement between the two for resonance energies. But in this energy range the theoretical resonance strengths are ~ 31% larger than the experimental results. This is larger than our estimated total experimental uncertainty in this energy range of +/- 26% (at a 90% confidence level). Above 42 eV the difference in the shape between the calculated and measured 3s3p(^1P_1)nl DR series limit we attribute partly to the nl dependence of the detection probabilities of high Rydberg states in the experiment. We have used our measurements, supplemented by our AUTOSTRUCTURE calculations, to produce a Maxwellian-averaged 3 -> 3 DR rate coefficient for Fe XV forming Fe XIV. The resulting rate coefficient is estimated to be accurate to better than +/- 29% (at a 90% confidence level) for k_BT_e > 1 eV. At temperatures of k_BT_e ~ 2.5-15 eV, where Fe XV is predicted to form in photoionized plasmas, significant discrepancies are found between our experimentally-derived rate coefficient and previously published theoretical results. Our new MCBP plasma rate coefficient is 19-28% smaller than our experimental results over this temperature range.

astro-ph↗

arXiv2007

Evidence for a planetary companion around a nearby young star

We report evidence for a planetary companion around the nearby young star HD 70573. The star is a G type dwarf located at a distance of 46 pc with age estimation between 20 and 300 Myrs. We carried out spectroscopic observations of this star with FEROS at the 2.2 m MPG/ESO telescope at La Silla. Our spectroscopic analysis yields a spectral type of G1-1.5V and an age of about 100 Myrs. Variations in stellar radial velocity of HD 70573 have been monitored since December 2003 until January 2007. The velocity accuracy of FEROS within this period is about 10 m/s. HD 70573 shows a radial velocity variation with a period of 852 +/- 12 days and a semi-amplitude of 149 +/- 6 m/s. The period of this variation is significantly longer than its rotational period, which is 3.3 days. Based on the analysis of the Ca II K emission line, Halpha and Teff variation as stellar activity indicators as well as the lack of a correlation between the bisector velocity span and the radial velocity, we can exclude the rotational modulation and non-radial pulsations as the source of the long-period radial velocity variation. Thus, the presence of a low-mass companion around the star provides the best explanation for the observed radial velocity variation. Assuming a primary mass m1=1.0 +/- 0.1 Msun for the host star, we calculated a minimum mass of the companion m2sini of 6.1 Mjup, which lies in the planetary mass regime, and an orbital semi-major axis of 1.76 AU. The orbit of the planet has an eccentricity of e=0.4. The planet discovery around the young star HD 70573 gives an important input for the study of debris disks around young stars and their relation to the presence of planets.

astro-ph↗

arXiv2000

Butterfly hysteresis loop and dissipative spin reversal in the S=1/2, V15 molecular complex

Time resolved magnetization measurements have been performed on a spin 1/2 molecular complex, so called V$_{15}$. Despite the absence of a barrier, magnetic hysteresis is observed over a timescale of several seconds. A detailed analysis in terms of a dissipative two level model is given, in which fluctuations and splittings are of same energy. Spin-phonon coupling leads to long relaxation times and to a particular "butterfly" hysteresis loop.

cond-mat.mes-hall↗

arXiv2000

Non-adiabatic Landau-Zener transitions in low spin molecular magnet V15

The V_{15} polyoxovanadate molecule is made of 15 spins 1/2 with antiferromagnetic couplings. It belongs to the class of molecules with very large Hilbert space dimension (2^{15} in V_{15}, 10^8 in Mn_{12}-ac). It is a low-spin/big-molecule with spin S=1/2. Contrary large-spins/big-molecules of the Mn_{12}-ac type, V_{15} has no energy barrier against spin rotation. Magnetization measurements have been performed and despite the absence of a barrier, magnetic hysteresis is observed over a timescale of several seconds. This new phenomenon characterized by a "butterfly" hysteresis loop is due to the effect of the environment on the quantum rotation of the entangled 15 spins of the molecule, in which the phonon density of states is not at its equilibrium (phonon bottleneck).

cond-mat.mes-hall↗