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A. M. Hurst

Publications and source records attributed to A. M. Hurst.

7 recordsLinked to original sources

Analytic calculator for determination of $γ$-ray angular distribution coefficients and tensors in aligned and partially-aligned nuclei

A program has been developed to calculate a complete set of $γ$-ray angular distribution coefficients and statistical tensors in maximally- and partially-aligned nuclei. For practical nuclear structure and reaction purposes, there is no imposed constraint on any arguments that are likely to arise in the determination of these quantities. The program can also be used as a stand-alone vector-coupling calculator for the exact evaluation of Clebsch-Gordan and Racah coefficients, the closely-related Wigner 3-$j$, 6-$j$, and 9-$j$ symbols, as well as Gaunt coefficients. These quantities, which frequently arise in quantum mechanical applications involving angular momentum coupling and recoupling schemes, provide the underlying machinery in angular distribution calculations.

nucl-th

The Online Berkeley Evaluated Alpha and Proton Radioactivity database (BE$αp$R) -- from Li to Og!

We have developed the new Berkeley Evaluated Alpha and proton Radioactivity (BE$αp$R) database detailing information on all known $β^{+}$-delayed and direct heavy-particle emitters (p, $α$, cluster, fission). The compiled data encompasses branching ratios, half lives, and all relevant $Q$-values and particle-separation energies. These are listed for all nuclei where such decays are energetically possible. In addition, for nuclei with known discrete proton and alpha transitions, the particle-emission energies, intensities, and associated initial and final states are also provided. A graphical illustration of the major decay modes and a corresponding list of experimental references is also given for each dataset. The compiled nuclides are organized by their isospin projection ($T_{z}$) and split into even and odd $Z$ datasets. Complete compilations of the database from $T_{z} = -4$ to $T_{z} = +31$ are included. We intend to maintain this database and post updates periodically as new relevant data becomes available. In its current construct, information from this database can currently be downloaded, in part or entirely, in portable document format as we are developing a more useful machine-readable format for future dissemination. Making the database publicly available in the manner described here represents the first step in the ongoing development of a fully open-source project.

nucl-ex

Westcott $g$ Factors Extended to Arbitrary Neutron Energy Spectra

Westcott $g$ factors are used in Neutron Activation Analysis (NAA) and Prompt Gamma-ray Activation Analysis (PGAA) to evaluate the impact of non-$1/v$ behavior in the neutron-capture cross sections of certain nuclei on activation product yields. This non-$1/v$ behavior arises from the presence of neutron resonances in the neutron-capture cross sections that overlap with the source neutron spectrum at low ($<5$~eV) energies. Historically, Westcott $g$ factors that have been cataloged for NAA and PGAA applications are the result of calculations that assume a Maxwellian neutron velocity distribution with a given average temperature. In this study, we use this approach with updated neutron-capture cross sections from the Evaluated Nuclear Data File, version VIII.1 (ENDF/B-VIII.1) to tabulate Westcott $g$ factor values for a broad range of Maxwellian distribution temperatures, comparing the results against currently-available $g$ factors from International Atomic Energy Agency tables and other sources. It was discovered during this analysis that the use of guided thermal and cold-neutron beams at certain facilities necessitates an approach for evaluating Westcott $g$ factors based on arbitrary non-Maxwellian spectra. In this paper, we present an approach for calculating $g$ factors with user-specified neutron spectra, and we apply these methods to obtain Westcott $g$-factors for guided- and cold-neutron beams at the Budapest Research Reactor and the Forschungsreaktor M{ü}nchen II reactor. Open-source software has been developed as part of this study that can be used to perform these calculations for applications in PGAA and NAA experiments

nucl-ex

The Baghdad Atlas: A relational database of inelastic neutron-scattering $(n,n'γ)$ data

A relational database has been developed based on the original ($n,n'γ$) work carried out by A. M. Demidov $et$ $al$., at the Nuclear Research Institute in Baghdad, Iraq [$"Atlas$ $of$ $Gamma$-$Ray$ $Spectra$ $from$ $the$ $Inelastic$ $Scattering$ $of$ $Reactor$ $Fast$ $Neutrons"$, Nuclear Research Institute, Baghdad, Iraq (Moscow, Atomizdat 1978)] for 105 independent measurements comprising 76 elemental samples of natural composition and 29 isotopically-enriched samples. The information from this Atlas includes: $γ$-ray energies and relative intensities; nuclide and level data corresponding to the residual nucleus and meta data associated with the target sample that allows for the extraction of the flux-weighted ($n,n'γ$) cross sections for a given transition relative to a defined value. The optimized angular-distribution-corrected fast-neutron flux-weighted partial $γ$-ray cross section for the production of the 846.8-keV $2^{+}_{1} \rightarrow 0^{+}_{\rm gs}$ $γ$-ray transition in $^{56}$Fe, determined to be $\langle σ_γ \rangle = 143(29)$ mb, is used for this purpose. However, different values for the adopted cross section can be readily implemented to accommodate user preference based on revised determinations of this quantity. The Atlas ($n,n'γ$) data has been compiled into a series of CSV-style ASCII data sets and a suite of Python scripts have been developed to build and install the database locally. The database can then be accessed directly through the SQLite engine, or using alternative methods such as the Jupyter Notebook Python-browser interface. Several examples exploiting different interaction methodologies are distributed with the complete software package.

physics.app-ph

Radiative-capture cross sections for the $^{139}$La($n,γ$) reactionusing thermal neutrons and structural properties of $^{140}$La

A set of prompt partial $γ$-ray production cross sections from thermal neutron-capture were measured for the $^{139}$La($n,γ$) reaction using a guided beam of subthermal (thermal and cold) neutrons incident upon a $^{\rm nat}$La$_{2}$O$_{3}$ target at the Prompt Gamma Activation Analysis facility of the Budapest Research Reactor. Absolute $^{140}$La cross sections were determined relative to the well-known comparator $^{35}$Cl($n,γ$) cross sections from the irradiation of a stoichiometric $^{\rm nat}$LaCl$_{3}$ sample. The total cross section for radiative thermal neutron-capture on $^{139}$La from the sum of experimentally measured cross sections observed to directly feed the $^{140}$La ground state was determined to be $σ_{0}^{\rm expt} = 8.58(50)$ b. To assess completeness of the decay scheme and as a consistency check, the measured cross sections for transitions feeding the ground state from levels below a critical energy of $E_{c} = 285$ keV were combined with a modeled contribution accounting for ground-state feeding from the quasicontinuum to arrive at a total cross section of $σ_{0} = 9.36(74)$ b. In addition, a neutron-separation energy of $S_{n} = 5161.005(21)$ keV was determined from a least-squares fit of the measured primary $γ$-ray energies to the low-lying levels of the $^{140}$La decay scheme. Furthermore, several nuclear structure improvements are proposed for the decay scheme. The measured cross-section and separation-energy results are comparable to earlier measurements of these quantities.

nucl-ex

A structural evaluation of the tungsten isotopes via thermal neutron capture

Total radiative thermal neutron-capture $γ$-ray cross sections for the $^{182,183,184,186}$W isotopes were measured using guided neutron beams from the Budapest Research Reactor to induce prompt and delayed $γ$ rays from elemental and isotopically-enriched tungsten targets. These cross sections were determined from the sum of measured $γ$-ray cross sections feeding the ground state from low-lying levels below a cutoff energy, E$_{\rm crit}$, where the level scheme is completely known, and continuum $γ$ rays from levels above E$_{\rm crit}$, calculated using the Monte Carlo statistical-decay code DICEBOX. The new cross sections determined in this work for the tungsten nuclides are: $σ_{0}(^{182}{\rm W}) = 20.5(14)$ b and $σ_{11/2^{+}}(^{183}{\rm W}^{m}, 5.2 {\rm s}) = 0.177(18)$ b; $σ_{0}(^{183}{\rm W}) = 9.37(38)$ b and $σ_{5^{-}}(^{184}{\rm W}^{m}, 8.33 μ{\rm s}) = 0.0247(55)$ b; $σ_{0}(^{184}{\rm W}) = 1.43(10)$ b and $σ_{11/2^{+}}(^{185}{\rm W}^{m}, 1.67 {\rm min}) = 0.0062(16)$ b; and, $σ_{0}(^{186}{\rm W}) = 33.33(62)$ b and $σ_{9/2^{+}}(^{187}{\rm W}^{m}, 1.38 μ{\rm s}) = 0.400(16)$ b. These results are consistent with earlier measurements in the literature. The $^{186}$W cross section was also independently confirmed from an activation measurement, following the decay of $^{187}$W, yielding values for $σ_{0}(^{186}{\rm W})$ that are consistent with our prompt $γ$-ray measurement. The cross-section measurements were found to be insensitive to choice of level density or photon strength model, and only weakly dependent on E$_{\rm crit}$. Total radiative-capture widths calculated with DICEBOX showed much greater model dependence, however, the recommended values could be reproduced with selected model choices. The decay schemes for all tungsten isotopes were improved in these analyses.

nucl-ex

Reaction rate sensitivity of 44Ti production in massive stars and implications of a thick target yield measurement of 40Ca(alpha,gamma)44Ti

We evaluate two dominant nuclear reaction rates and their uncertainties that affect 44Ti production in explosive nucleosynthesis. Experimentally we develop thick-target yields for the 40Ca(alpha,gamma)44Ti reaction at E(alpha) = 4.13, 4.54, and 5.36 MeV using gamma-ray spectroscopy. At the highest beam energy, we also performed an activation measurement that agrees with the thick target result. From the measured yields a stellar reaction rate was developed that is smaller than current statistical-model calculations and recent experimental results, which would suggest lower 44Ti production in scenarios for the alpha-rich freeze out. Special attention has been paid to assessing realistic uncertainties of stellar rates produced from a combination of experimental and theoretical cross sections, which we use to develop a re-evaluation of the 44Ti(alpha,p)47V reaction rate. Using these we carry out a sensitivity survey of 44Ti synthesis in eight expansions representing peak temperature and density conditions drawn from a suite of recent supernova explosion models. Our results suggest that the current uncertainty in these two reaction rates could lead to as large an uncertainty in 44Ti synthesis as that produced by different treatments of stellar physics.

astro-ph.HE