arXiv subjects

A. M. Jayich

Publications and source records attributed to A. M. Jayich.

At least 19 recordsLinked to original sources

arXiv2026

Laser Cooling and Hyperfine Measurements of Radium-225 Ions

$^{225}$Ra$^+$ ions (nuclear spin $I=1/2$) have transitions that are first-order insensitive to magnetic field noise, which is advantageous for optical clocks and quantum information science. We report on laser cooling and trapping of $^{225}$Ra$^+$ ions and hyperfine splitting measurements of the ion's $\mathrm{7s}$ $^2\mathrm{S}_{1/2}$, $\mathrm{7p}$ $^2\mathrm{P}_{1/2}$, and $\mathrm{6d}$ $^2\mathrm{D}_{3/2}$ states. We measured the ground state hyperfine constant, $A(\mathrm{S}_{1/2}) =$ $-27.684511052(5)$ $\mathrm{GHz}$, and the quadratic Zeeman coefficient, $C_2 =$ $142.3(1.0)$ $\mathrm{Hz\ G}^{-2}$, of the $^2\mathrm{S}_{1/2} (F=0, m_F = 0) \leftrightarrow~^2\mathrm{S}_{1/2} (F=1, m_{F} = 0)$ transition. Our result addresses a discrepancy in the literature for the ground state hyperfine splitting. We measured the hyperfine constants of the $^2\mathrm{P}_{1/2}$ state, $A(\mathrm{P}_{1/2}) =$ $-5.447(4)$ $\mathrm{GHz}$, and the $^2\mathrm{D}_{3/2}$ state, $A(\mathrm{D}_{3/2}) =$ $-619.7(1.1)$ $\mathrm{MHz}$. We also performed state preparation and measurement using the ground state hyperfine levels and realized a fidelity of $0.9951(9)$.

physics.atom-ph↗

arXiv2026

Radioactive Molecules as Laboratories of Fundamental Physics

Radioactive molecules provide a powerful new platform in the search for new physics at energy scales complementary to high-energy particle colliders. By combining enhancements from nuclear properties with the sensitivity and control offered by molecular structure, experiments with radioactive molecules offer great reach in the search for new physics beyond the Standard Model. Rapid progress in this field is being driven by advances in the production and control of radioactive molecules, alongside the development of new experimental tools and theoretical techniques. In this Perspective, we discuss the current status and future prospects of this rapidly developing, interdisciplinary field at the intersection of nuclear physics, atomic and molecular physics, and particle physics.

physics.atom-ph↗

arXiv2024

Measurement of the Ra$^+$ $7p$ $^{2}P_{3/2}$ state lifetime

We report a measurement of the radium ion's $7p$ ${}^{2}P_{3/2}$ state lifetime, $τ=4.78(3)$ ns. The measured lifetime is in good agreement with theoretical calculations, and will enable a determination of the differential scalar polarizability of the narrow linewidth $7s$ ${}^{2}S_{1/2}\rightarrow$ $6d$ ${}^{2}D_{5/2}$ optical clock transition.

physics.atom-ph↗

arXiv2023

Laser cooling and trapping of $^{224}$Ra$^+$

We report laser cooling and trapping of $^{224}$Ra$^+$ ions. This was realized via two-step photoionization loading of radium into an ion trap. A robust source for $^{224}$Ra atoms, which have a 3.6-day half-life, was realized with an effusive oven containing $^{228}$Th, which has a 1.9-yr half-life, which continuously generates $^{224}$Ra via its $α$-decay. We characterized the efficacy of this source and found that after depleting built-up radium the thorium decay provides a continuous source of radium atoms suitable for ion trapping. The vacuum system has been sealed for more than 6 months and continues to trap ions on demand. We also report a measurement of the $^{224}$Ra $7s^2\ ^1$S$_0 \rightarrow 7s7p\ ^1$P$_1$ transition frequency: 621 043 830(60) MHz, which is helpful for efficient photoionization. With this measurement and previous isotope shift measurements we find that the frequency of the same transition in $^{226}$Ra is 621 037 830(60) MHz, which disagrees with the most precise measurement, 621 038 489(15) MHz, which is used for the recommended value in the National Institute of Standards and Technology Atomic Spectra Database.

physics.atom-ph↗

arXiv2023

Ion optical clocks with three electronic states

Optical clocks are the apotheosis of precision measurement, but they require frequent maintenance by scientists. The supporting laser systems are a particularly demanding component of these instruments. To reduce complexity and increase robustness we propose an optical clock with trapped alkali-like ions that use the $S_{1/2}\rightarrow D_{3/2}$ electric quadrupole transition. Compared to traditional group-II ion clocks this reduces the number of laser wavelengths required, and uses hyperfine state preparation and readout techniques enabled by the nuclear spin $I=1/2$. We consider $^{225}$Ra$^{+}$ as a candidate system for a clock with three electronic states, and discuss the potential to help realize a transportable optical clock.

physics.atom-ph↗

arXiv2023

Fundamental Symmetries, Neutrons, and Neutrinos (FSNN): Whitepaper for the 2023 NSAC Long Range Plan

This whitepaper presents the research priorities decided on by attendees of the 2022 Town Meeting for Fundamental Symmetries, Neutrons and Neutrinos, which took place December 13-15, 2022 in Chapel Hill, NC, as part of the Nuclear Science Advisory Committee (NSAC) 2023 Long Range Planning process. A total of 275 scientists registered for the meeting. The whitepaper makes a number of explicit recommendations and justifies them in detail.

nucl-ex↗

arXiv2022

Radium Ion Optical Clock

We report the first operation of a Ra$^{+}$ optical clock, a promising high-performance clock candidate. The clock uses a single trapped $^{226}$Ra$^{+}$ ion and operates on the $7s\ ^2S_{1/2}\rightarrow$ $6d\ ^2D_{5/2}$ electric quadrupole transition. By self-referencing three pairs of symmetric Zeeman transitions, we demonstrate a frequency instability of 1.1$\times10^{-13}$/$\sqrtτ$, where $τ$ is the averaging time in seconds. The total systematic uncertainty is evaluated to be ${Δν/ ν= 9 \times 10^{-16}}$. Using the clock, we realize the first measurement of the ratio of the $D_{5/2}$ state to the $S_{1/2}$ state Landé $g$-factors: $g_{D}/g_{S}$ = 0.5988053(11). A Ra$^{+}$ optical clock could improve limits on the time variation of the fine structure constant, $\dot α/ α$, in an optical frequency comparison. The ion also has several features that make it a suitable system for a transportable optical clock.

physics.atom-ph↗

arXiv2021

Measurement of the $7p\,\, ^2\!P_{3/2}$ state branching fractions in $\mathrm{Ra}^+$

We report a measurement of the radium ion's $7p\,\, ^2\!P_{3/2}$ state branching fractions and improved theoretical calculations. With a single laser-cooled $^{226}\mathrm{Ra}^+$ ion we measure the $P_{3/2}$ branching fractions to the $7s\,\,^2\!S_{1/2}$ ground state 0.87678(20), the $6d\,\,^2\!D_{5/2}$ state 0.10759(10), and the $6d$ ${}^{2}D_{3/2}$ state 0.01563(21).

physics.atom-ph↗

arXiv2021

Optical Mass Spectrometry of Cold $\mathrm{RaOH}^+$ and ${\mathrm{RaOCH}_3}^+$

We present an all-optical mass spectrometry technique to identify trapped ions. The new method uses laser-cooled ions to determine the mass of a cotrapped dark ion with a sub-dalton resolution within a few seconds. We apply the method to identify the first controlled synthesis of cold, trapped $\mathrm{RaOH}^+$ and ${\mathrm{RaOCH}_3}^+$. These molecules are promising for their sensitivity to time and parity violations that could constrain sources of new physics beyond the standard model. The nondestructive nature of the mass spectrometry technique may help identify molecular ions or highly charged ions prior to optical spectroscopy. Unlike previous mass spectrometry techniques for small ion crystals that rely on scanning, the method uses a Fourier transform which is inherently broadband and comparatively fast. The technique's speed provides new opportunities for studying state-resolved chemical reactions in ion traps.

physics.atom-ph↗

arXiv2020

Direct measurement of the $7s\ ^2S_{1/2}\rightarrow$ $7p\ ^2P_{3/2}$ transition frequency in $^{226}$Ra$^{+}$

We report a direct measurement of the $7s\ ^2S_{1/2}\rightarrow$ $7p\ ^2P_{3/2}$ electric dipole transition frequency in $^{226}$Ra$^{+}$. With a single laser-cooled radium ion we determine the transition frequency to be 785722.11(3) GHz by directly driving the transition with frequency-doubled light and measuring the frequency of the undoubled light with an iodine reference. This measurement addresses a discrepancy of five combined standard deviations between previously reported values.

physics.atom-ph↗

arXiv2020

Searches for new sources of CP violation using molecules as quantum sensors

We discuss how molecule-based searches offer complementary probes to study the violation of fundamental symmetries. These experiments have the potential to probe not only the electron EDM, but also hadronic CPV phenomena. Future experimental developments will offer generic sensitivity to probe flavor neutral sources of both leptonic and hadronic CPV at scales of $\geq$ 100 TeV, and flavor changing CPV at scales of $\geq$ 1000 TeV.

hep-ph↗

arXiv2020

Measurements of electric quadrupole transition frequencies in $^{226}$Ra$^{+}$

We report the first driving of the $7s\ ^2S_{1/2}\rightarrow 6d\ ^2D_{3/2}$ and $7s\ ^2S_{1/2}\rightarrow 6d\ ^2D_{5/2}$ electric quadrupole (E2) transitions in Ra$^{+}$. We measure the frequencies of both E2 transitions, and two other low-lying transitions in $^{226}$Ra$^{+}$ that are important for controlling the radium ion's motional and internal states: $6d\ ^2D_{3/2}\rightarrow 7p\ ^2P_{3/2}^{0}$ and $6d\ ^2D_{5/2}\rightarrow 7p\ ^2P_{3/2}^{0}$.

physics.atom-ph↗

arXiv2019

Laser Cooling of Radium Ions

The unstable radium nucleus is appealing for probing new physics due to its high mass, octupole deformation and energy level structure. Ion traps, with long hold times and low particle numbers, are excellent for work with radioactive species, such as radium and radium-based molecular ions, where low activity, and hence low total numbers, is desirable. We address the challenges associated with the lack of stable isotopes in a tabletop experiment with a low-activity ($\sim 10 \ μ\mathrm{Ci}$) source where we laser-cool trapped radium ions. With a laser-cooled radium ion we measured the $7p\ ^2P_{1/2}^o$ state's branching fractions to the ground state, $7s\ ^2S_{1/2}$, and a metastable excited state, $6d\ ^2D_{3/2}$, to be $p=0.9104(7)$ and $0.0896(7)$, respectively. With a nearby tellurium reference line we measured the $7s\ ^2S_{1/2} \rightarrow 7p\ ^2P_{1/2}^o$ transition frequency, 640.09663(6) THz.

physics.atom-ph↗

arXiv2016

Direct frequency comb laser cooling and trapping

Continuous wave (CW) lasers are the enabling technology for producing ultracold atoms and molecules through laser cooling and trapping. The resulting pristine samples of slow moving particles are the de facto starting point for both fundamental and applied science when a highly-controlled quantum system is required. Laser cooled atoms have recently led to major advances in quantum information, the search to understand dark energy, quantum chemistry, and quantum sensors. However, CW laser technology currently limits laser cooling and trapping to special types of elements that do not include highly abundant and chemically relevant atoms such as hydrogen, carbon, oxygen, and nitrogen. Here, we demonstrate that Doppler cooling and trapping by optical frequency combs may provide a route to trapped, ultracold atoms whose spectra are not amenable to CW lasers. We laser cool a gas of atoms by driving a two-photon transition with an optical frequency comb, an efficient process to which every comb tooth coherently contributes. We extend this technique to create a magneto-optical trap (MOT), an electromagnetic beaker for accumulating the laser-cooled atoms for further study. Our results suggest that the efficient frequency conversion offered by optical frequency combs could provide a key ingredient for producing trapped, ultracold samples of nature's most abundant building blocks, as well as antihydrogen. As such, the techniques demonstrated here may enable advances in fields as disparate as molecular biology and the search for physics beyond the standard model.

physics.atom-ph↗

arXiv2013

Continuous all-optical deceleration and single-photon cooling of molecular beams

Ultracold molecular gases are promising as an avenue to rich many-body physics, quantum chemistry, quantum information, and precision measurements. This richness, which flows from the complex internal structure of molecules, makes the creation of ultracold molecular gases using traditional methods (laser plus evaporative cooling) a challenge, in particular due to the spontaneous decay of molecules into dark states. We propose a way to circumvent this key bottleneck using an all-optical method for decelerating molecules using stimulated absorption and emission with a single ultrafast laser. We further describe single-photon cooling of the decelerating molecules that exploits their high dark state pumping rates, turning the principal obstacle to molecular laser cooling into an advantage. Cooling and deceleration may be applied simultaneously and continuously to load molecules into a trap. We discuss implementation details including multi-level numerical simulations of strontium monohydride (SrH). These techniques are applicable to a large number of molecular species and atoms with the only requirement being an electric dipole transition that can be accessed with an ultrafast laser.

physics.atom-ph↗

arXiv2012

Fiber-Cavity-Based Optomechanical Device

We describe an optomechanical device consisting of a fiber-based optical cavity containing a silicon nitiride membrane. In comparison with typical free-space cavities, the fiber-cavity's small mode size (10 μm waist, 80 μm length) allows the use of smaller, lighter membranes and increases the cavity-membrane linear coupling to 3 GHz/nm and quadratic coupling to 20 GHz/nm^2. This device is also intrinsically fiber-coupled and uses glass ferrules for passive alignment. These improvements will greatly simplify the use of optomechanical systems, particularly in cryogenic settings. At room temperature, we expect these devices to be able to detect the shot noise of radiation pressure.

physics.optics↗

arXiv2012

Cryogenic Optomechanics with a Si3N4 Membrane and Classical Laser Noise

We demonstrate a cryogenic optomechanical system comprising a flexible Si3N4 membrane placed at the center of a free-space optical cavity in a 400 mK cryogenic environment. We observe a mechanical quality factor Q > 4 x 10^6 for the 261-kHz fundamental drum-head mode of the membrane, and a cavity resonance halfwidth of 60 kHz. The optomechanical system therefore operates in the resolved sideband limit. We monitor the membrane's thermal motion using a heterodyne optical circuit capable of simultaneously measuring both of the mechanical sidebands, and find that the observed optical spring and damping quantitatively agree with theory. The mechanical sidebands exhibit a Fano lineshape, and to explain this we develop a theory describing heterodyne measurements in the presence of correlated classical laser noise. Finally, we discuss the use of a passive filter cavity to remove classical laser noise, and consider the future requirements for laser cooling this relatively large and low-frequency mechanical element to very near its quantum mechanical ground state.

physics.optics↗

arXiv2008

Dispersive optomechanics: a membrane inside a cavity

We present the results of theoretical and experimental studies of dispersively coupled (or "membrane in the middle") optomechanical systems. We calculate the linear optical properties of a high finesse cavity containing a thin dielectric membrane. We focus on the cavity's transmission, reflection, and finesse as a function of the membrane's position along the cavity axis and as a function of its optical loss. We compare these calculations with measurements and find excellent agreement in cavities with empty-cavity finesses in the range 10^4 to 10^5. The imaginary part of the membrane's index of refraction is found to be approximately 10^(-4). We calculate the laser cooling performance of this system, with a particular focus on the less-intuitive regime in which photons "tunnel" through the membrane on a time scale comparable to the membrane's period of oscillation. Lastly, we present calculations of quantum non-demolition measurements of the membrane's phonon number in the low signal-to-noise regime where the phonon lifetime is comparable to the QND readout time.

quant-ph↗