arXiv subjects

A. M. Kalashnikova

Publications and source records attributed to A. M. Kalashnikova.

At least 19 recordsLinked to original sources

arXiv2026

Switching picosecond magnetoacoustic regimes in a ferromagnetic waveguide

The development of magnonics requires energy-efficient methods for generating spin waves and controlling their parameters. Acoustic waves are known to resonantly excite spin waves through magneto-elastic wave formation or to induce non-resonant forced magnetization oscillations. Short acoustic wavepackets enable another unexplored resonant interaction regime -- the Cherenkov radiation of spin waves. This raises a question regarding the criteria and signatures of these three regimes of picosecond magnetoacoustics and transitions between them in confined magnetic structures. Here, we use a scanning magneto-optical pump-probe technique to directly observe all three regimes of interaction between laser-driven acoustic and magnetostatic wavepackets in a thin permalloy film and a waveguide fabricated on Si substrate. Direct measurements of the phase velocities reveal the transition from a coupled magneto-elastic wavepacket to Cherenkov-like radiation and the non-resonant regime, controlled by the detuning between magnon and phonon group velocities. The acoustic pulse is found to be affected by the excited magnetization dynamics only in the magneto-elastic regime.

cond-mat.mtrl-sci↗

arXiv2026

Propagation of laser-generated GHz surface acoustic wavepackets in FeRh/MgO(001) below and above the antiferromagnetic-ferromagnetic phase transition

Magnetoacoustic devices that harness the strong coupling between acoustic waves and magnons have emerged as a promising platform for energy-efficient spintronics. Laser-generated pulsed surface acoustic waves (SAWs) are particularly attractive for such applications, offering broadband frequency content up to the gigahertz (GHz) range, remote excitation without lithographic patterning, and surface localization for efficient on-chip integration. In this work, we present a comprehensive experimental study of laser-generated SAW pulses in the Fe49Rh51/MgO(001) system. A thin film of the near-equiatomic FeRh alloy serves both as an opto-acoustic transducer and as a mechanical load that modulates SAW propagation. The antiferromagnetic to ferromagnetic phase transition in FeRh, occurring slightly above room temperature, is accompanied by abrupt changes in its elastic properties, enabling controlled modification of the SAW excitation efficiency and dispersion characteristics by tuning the sample temperature and laser fluence. Using 160 fs laser pulses for excitation and time-resolved Sagnac interferometry for detection, we evaluated key SAW parameters, including amplitude, spectral content, phase and group velocities, and their in-plane anisotropy. Particular emphasis is placed on the dispersion relation and its anisotropy, which govern the coherent interaction between phonons and magnons and are determined primarily by the FeRh film.

cond-mat.mtrl-sci↗

arXiv2026

Harnessing magnetic anisotropy for nonlinear magnetization precession and spin waves

The nonlinearity of magnetization precession and spin waves is a cornerstone of contemporary magnonics. We investigate nonlinear magnetization dynamics in a thin epitaxial iron film driven by femtosecond laser pulses in regimes of homogeneous precession and propagating magnetostatic spin wave packets. The magnetization precession anharmonicity, the generation of higher-order harmonics, and the dynamical rectification are experimentally demonstrated. The numerical solution of the non-linearized Landau-Lifshitz-Gilbert equation reveals that these effects stem from the asymmetry in the energy potential and are essentially thresholdless. This asymmetry is readily achievable when an external magnetic field with a strength comparable to the magnetic anisotropy field is applied close to the hard axis. This work establishes a connection between the geometry of the energy profile and nonlinear responses, paving the way for designing magnonic devices with controlled harmonic generation and nonlinear spin wave interaction.

cond-mat.mtrl-sci↗

arXiv2026

Role of magnon-magnon interaction in optical excitation of coherent two-magnon modes

Two-magnon modes are terahertz-frequency magnetic excitations in antiferromagnets, governed by exchange interactions, involving magnons from the entire Brillouin zone and dominated by zone-edge magnons. The ability to couple to light promotes two-magnon modes as contenders for ultrafast optical manipulation of the magnetic state, beyond conventional zone-center magnonics. While magnon-magnon interactions are known to critically shape the two-magnon line in spontaneous Raman scattering spectra, their role in coherent time-domain excitations remains unexplored. We report a detailed experimental and theoretical study of the influence of magnon-magnon interactions on coherent two-magnon modes in a cubic antiferromagnet excited via Impulsive Stimulated Raman scattering. We reveal the nontrivial evolution of coherent magnetic dynamics in the time domain and the corresponding spectrum and compare it with the spontaneous Raman scattering spectrum. By extending the spin-correlations based theory for two-magnon modes, we derive a unified description of their spectra in Raman Scattering and Impulsive Stimulated Raman Scattering and highlight the role of magnon-magnon interactions.

cond-mat.mtrl-sci↗

arXiv2026

Role of spatiotemporal nonuniformities in laser-induced magnetization precession damping

Laser-induced magnetization precession measurements in ferromagnets often reveal an anomalous decrease in the damping time near a field-induced second-order spin-orientation transition, a behavior that cannot be described by the linearized Landau-Lifshitz-Gilbert equation. Here we demonstrate that this anomaly is not a material property but results from interference of precessing local magnetizations within the inhomogeneously excited region. By combining pump-probe experiments, analytical modeling that accounts for the finite sizes of the pump and probe spots, and micromagnetic simulations, we show that the standard macrospin approach fails to capture the observed dynamics. The inhomogeneous relaxation of magnetic parameters within the excitation area distorts the measured precession envelope, while dipole fields give rise to a temporally non-monotonic term in its frequency. Our results highlight the critical role of excitation locality in a vicinity of critical fields.

cond-mat.mtrl-sci↗

arXiv2026

Laser-generated GHz surface acoustic waves with tunable amplitude during the magnetostructural phase transition in FeRh thin films

Laser-generated surface acoustic waves (SAW) facilitate efficient information processing in modern spintronics and magnonics. The ability to tune the SAW parameters such as amplitude is crucial to achieve acoustic control over magnonic properties. Such tunability can be achieved in phasechanging magnetic materials that accommodate both spin waves and SAWs. A promising material is the FeRh alloy, a metallic antiferromagnet at room temperature that undergoes a phase transition to the ferromagnetic state accompanied by a crystal lattice expansion at 370 K. This transition can also be induced by femtosecond laser pulses. In this paper, we use the phase transition in a 60 nm Fe49Rh51 film to optically generate pulses of Gigahertz quasi-Rayleigh SAWs. We detect them via the photoelastic effect and show that the lattice transformation during the phase transition is a dominant strain-generation mechanism for above-threshold excitation. The weight of this contribution rises as the sample is heated closer to the AFM-FM transition temperature and 'switches off' when heated above it, allowing for control of the SAW amplitude. A model based on thermodynamic parameters of Fe49Rh51 shows that the lattice transformation occurring within 95 ps effectively contributes to SAW generation happening on a comparable timescale, while non-equilibrium fast kinetics of the phase transition does not.

cond-mat.mtrl-sci↗

arXiv2025

Switching of an antiferromagnet controlled by spin canting in a laser-induced hidden phase

During laser-induced phase transitions, fast transformations of electronic, atomic, and spin configurations often involve emergence of hidden and metastable phases. Being inaccessible under any other stimuli, such phases are indispensable for unveiling mechanisms and controlling the transitions. We experimentally explore spin kinetics during ultrafast first-order 90$^{\circ}$ spin-reorientation (SR) transition in a canted antiferromagnet Fe$_3$BO$_6$, and reveal that the transition is controlled by the canting between the magnetic sublattices. Laser-induced perturbation of the Dzyaloshinskii-Moriya interaction results in a change of the intersublattice canting within first picoseconds, bringing Fe$_3$BO$_6$ to a hidden phase. Once this phase emerges, laser-induced heating activates precessional 90$^\circ$ spin switching. Combination of the spin canting and heating controls the final spin configuration comprising coexisting initial and switched phases. Extended phase coexistence range is in a striking contrast to the narrow SR transition in Fe$_3$BO$_6$ induced by conventional heating.

cond-mat.str-el↗

arXiv2025

Spin and lattice dynamics at the spin-reorientation transitions in the rare-earth orthoferrite Sm$_{0.55}$Tb$_{0.45}$FeO$_{3}$

Linear and non-linear couplings of magnetic and lattice excitations are at the heart of many fascinating magnetophononic phenomena observed in rare-earth orthoferrites, the distinctive feature of which is the tendency to spin-reorientation transitions. Here we report the results of the experimental study of the spin and lattice dynamics in the Brillouin zone center of the rare-earth orthoferrite Sm$_{0.55}$Tb$_{0.45}$FeO$_{3}$ by using polarized infrared reflectivity and Raman scattering spectroscopic techniques. The obtained results were supported by the first-principles calculations, which allowed us to reliably identify the parameters of most infrared- and Raman-active phonons. We reveal the spin-reorientation transitions $Γ_{4}(G_{a}F_{c}) \overset{T_{1}}\longleftrightarrow Γ_{24}(G_{ac}F_{ac}) \overset{T_{2}}\longleftrightarrow Γ_{2}(G_{c}F_{a})$ at $T_{1} \simeq 220$ K and $T_{2} \simeq 130$ K and carefully studied the following evolution of Raman scattering on magnetic excitations at these transitions. Notably, the intermediate magnetic structure $Γ_{24}$ displays an exceptionally broad temperature range $Δ{T} = T_{1} - T_{2} \simeq 90$ K in mixed Sm$_{0.55}$Tb$_{0.45}$FeO$_{3}$ compared to pure rare-earth orthoferrites. We attribute this broadening of the intermediate phase to the modification of the magnetocrystalline anisotropy as a result of the inhomogeneous magnetic structure caused by the random distribution of rare-earth $\mathrm{Sm}^{3+}$ and $\mathrm{Tb}^{3+}$ ions. We found neither change in the parameters of Raman-active $B_{1g}$ phonons nor the appearance of new phonons induced by spin-reorientation transitions, which have been reported in $\mathrm{SmFeO}_{3}$. We assume that our results provide a solid basis for more deeper understanding of magnetophononic phenomena in rare-earth orthoferrites.

cond-mat.mtrl-sci↗

arXiv2024

Enhanced laser-induced single-cycle terahertz generation in a spintronic emitter with a gradient interface

The development of spintronic emitters of broadband THz pulses relies on designing heterostructures where processes of laser-driven spin current generation and subsequent spin-to-charge current conversion are the most efficient. An interface between ferromagnetic and nonmagnetic layers in the emitter is one of the critical elements. Here, we study experimentally single-cycle THz pulse generation from a laser-pulse excited Pt/Co emitter with a composition gradient interface between Pt and Co and compare it with the emission from a conventional Pt/Co structure with an abrupt interface. We find that the gradient interface enhances the efficiency of optics-to-THz conversion by a factor of two in a wide range of optical fluences up to 3 mJ cm$^{-2}$. We reveal that this enhancement is caused by a pronounced increase in transmittance of the laser-driven spin-polarized current through the gradient interface compared to the abrupt one. Furthermore, we find that such a transmission deteriorates with laser fluence due to the spin accumulation effect.

physics.app-ph↗

arXiv2024

Lattice dynamics and mixing of polar phonons in the rare-earth orthoferrite TbFeO$_{3}$

Rare-earth orthoferrites are a promising platform for antiferromagnetic spintronics with a rich variety of terahertz spin and lattice dynamics phenomena. For instance, it has been experimentally demonstrated that the light-driven optical phonons can coherently manipulate macroscopic magnetic states via nonlinear magnetophononic effects. Here using TbFeO$_{3}$ as an example, we reveal the origin of the mode mixing between the LO and TO phonons, which is important for understanding of nonlinear phononics. We performed a comprehensive study of the lattice dynamics of the TbFeO$_{3}$ single crystal by polarized infrared and Raman scattering spectroscopic techniques, and experimentally obtained and carefully analyzed the spectra of anisotropic complex dielectric functions in the far-infrared spectral range. This allowed us to reliably identify the symmetries and parameters of most infrared- and Raman-active phonons. Next, the experimental studies were supplemented by the lattice dynamics calculations which allowed us to propose the normal mode assignments. We reveal that the relation between LO and TO polar phonons is complex and does not strictly follow the ``LO-TO rule'' due to the strong mode mixing. We further analyze how displacements of different ions contribute to phonon modes and reveal that magnetic Fe ions are not involved in Raman-active phonons, thus shedding light on a lack of spin phonon coupling for such phonons. The obtained results establish a solid basis for further in-depth experimental research in the field of nonlinear phononics and magnetophononics in rare-earth orthoferrites.

cond-mat.mtrl-sci↗

arXiv2024

Tunable quasi-discrete spectrum of spin waves excited by periodic laser patterns

We present a concept for selective excitation of magnetostatic surface waves with quasi-discrete spectrum using spatially patterned femtosecond laser pulses inducing either ultrafast change of magnetic anisotropy or inverse Faraday effect. We micromagnetically simulate excitation of the waves with periodically patterned uni- or bipolar laser impact. Such excitation yields multiple wavepackets propagating with different group velocities, whose dispersion corresponds to the set of quasi-discrete points. In addition, we show that the frequency of the spectral peaks can be controlled by the polarity of the periodic impact and its spatial period. Presented consideration of multiple spatially periodic magnetostatic surface wave sources as a whole enables implementation of a comprehensive toolkit of spatio-temporal optical methods for tunable excitation and control of spin wave parameters

physics.optics↗

arXiv2024

Giant intrinsic nonlinear phonon-magnon coupling in the antiferromagnet CoF$_2$

The observation of strongly coupled lattice and spin dynamics in altermagnet CoF$_2$ is reported. On the background of the expected spin-phonon interaction leading to renormalization of all phonons at the Neel temperature an additional strong coupling between one-magnon excitation and the lowest frequency Raman-active phonon of B1g symmetry was observed and manifested an anomaly in its energy, full width, and intensity at temperature T*=23 K precisely where the frequency of the phonon becomes exactly twice the frequency of the magnon. We assigned this effect to unique magnon-phonon coupling in the form of a two-magnons-one-phonon interaction. The consistent experimental data clearly demonstrate that there is an intrinsic coupling that does not require coherent excitation.

cond-mat.mtrl-sci↗

arXiv2024

Laser-induced Demagnetization in van der Waals $XY$- and Ising-like Antiferromagnets NiPS$_3$ and FePS$_3$

The critical behaviour of laser-induced changes in magnetic ordering is studied experimentally in two-dimensional zigzag antiferromagnets $XY$-like NiPS$_3$ and Ising-like FePS$_3$. To examine laser-induced dynamics in flakes of these compounds, we employ time-resolved exchange linear dichroism effect sensitive to zigzag magnetic ordering and independent of the orientation of the antiferromagnetic vector. In both compounds laser excitation in the vicinity of the absorption edge induces partial quenching of the antiferromagnetic ordering manifested by exchange linear dichroism reduction. The amplitude of the effect varies with temperature as the derivative of the antiferromagnetic vector and exhibits a critical behaviour with the exponents corresponding to $XY$- and Ising-models for NiPS$_3$ and FePS$_3$, respectively. Critical slowing down of the demagnetization in the vicinity of Néel temperature is found, however, only in FePS$_3$. In contrast, the increase of the demagnetization time near the ordering temperature in NiPS$_3$ is minor. We show that the difference in the demagnetization times correlates well with the spin specific heat in both compounds. Beyond the range of slowing down, the demagnetization times in NiPS$_3$ and FePS$_3$ are comparable, about 5 - 10 ps, and are longer than those reported earlier for CoPS$_3$ and considerably shorter than for MnPS$_3$. This points to the importance of the unquenched angular momentum of transition-metal ions in laser-induced demagnetization process.

cond-mat.mes-hall↗

arXiv2023

Coherent THz Spin Dynamics in Antiferromagnets Beyond the Approximation of the Néel vector

Controlled generation of coherent spin waves with highest possible frequencies and the shortest possible wavelengths is a cornerstone of spintronics and magnonics. Here, using the Heisenberg antiferromagnet RbMF$_3$, we demonstrate that laser-induced THz spin dynamics corresponding to pairs of mutually coherent counter propagating spin waves with the wavevectors up to the edge of the Brillouin zone cannot be understood in terms of magnetization and antiferromagnetic (Néel) vectors, conventionally used to describe spin waves. Instead, we propose to model such spin dynamics using the spin correlation function. We derive a quantum-mechanical equation of motion for the latter and emphasize that, unlike the magnetization and antiferromagnetic vectors the spin correlations in antiferromagnets do not exhibit inertia.

cond-mat.str-el↗

arXiv2023

Spatial asymmetry of optically excited spin waves in anisotropic ferromagnetic film

We analytically discuss and micromagnetically prove the ways to tune the spatial asymmetry of the initial phase, amplitude, and wavevectors of magnetostatic waves driven by ultrafast laser excitation. We consider that the optical pulse heats a thin ferromagnetic metallic film and abruptly decreases the saturation magnetization and the parameter of uniaxial anisotropy. The two corresponding terms of laser-induced torque have different azimuthal symmetries, with the 4-fold symmetry of the demagnetization-related term, and the isotropic distribution of the anisotropy-related term. As a result, the initial phase and amplitude of excited magnetostatic waves have a non-trivial azimuthal distribution tunable with the angle between the external magnetic field and anisotropy axis, and the laser spot diameter. Moreover, the variation of these parameters tunes the distribution of wavevectors, resulting in additional asymmetry between the spectral components of the waves propagating in different directions.

cond-mat.str-el↗

arXiv2023

Nonreciprocal collective magnetostatic wave modes in geometrically asymmetric bilayer structure with nonmagnetic spacer

Nonreciprocity, i.e. inequivalence in amplitudes and frequencies of spin waves propagating in opposite directions, is a key property underlying functionality in prospective magnonic devices. Here we demonstrate experimentally and theoretically a simple approach to induce frequency nonreciprocity in a magnetostatically coupled ferromagnetic bilayer structure with a nonmagnetic spacer by its geometrical asymmetry. Using Brillouin light scattering, we show the formation of two collective spin wave modes in Fe$_{81}$Ga$_{19}$/Cu/Fe$_{81}$Ga$_{19}$ structure with different thicknesses of ferromagnetic layers. Experimental reconstruction and theoretical modeling of the dispersions of acoustic and optical collective spin wave modes reveal that both possess nonreciprocity reaching several percent at the wavenumber of $22~\cdot~10^4$ rad cm$^{-1}$. The analysis demonstrates that the shift of the amplitudes of counter-propagating coupled modes towards either of the layers is responsible for the nonreciprocity because of the pronounced dependence of spin wave frequency on the layers thickness. The proposed approach enables the design of multilayered ferromagnetic structures with a given spin wave dispersion for magnonic logic gates.

cond-mat.mtrl-sci↗

arXiv2023

Unidirectional propagation of spin waves excited by femtosecond laser pulses in a planar waveguide

Low-energy magnonic logic circuits are an actively developing field of modern magnetism. The potential benefits of magnonics for data processing are vitally dependent on units based on non-reciprocal propagation of spin waves in analogy to semiconductor diodes and transistors in electronics. In this article, we suggest the approach to realize non-reciprocal propagation of spin waves in a ferromagnetic metallic waveguide by exciting them with femtosecond laser pulse. Using micromagnetic modeling, we show that the combination of an external magnetic field and the position of the excitation laser spot across the waveguide leads to unidirectional propagation of the excited spin-wave packet. The results are crucial for the design of hybrid magnonic-photonic circuits in future generations of data processing devices.

cond-mat.mtrl-sci↗

arXiv2022

Laser-driven first-order spin reorientation and Verwey phase transitions in the magnetite Fe$_3$O$_4$ beyond the range of thermodynamic equilibrium

Ultrafast photo-induced phase transitions occurring under the impact of femtosecond laser pulses provide versatile opport unities for switching solids between distinctly-different crystalline, electronic, and magnetic states and thus modify their functional properties in a significant way. In this paper, we report on the laser-induced spin reorientation and Verwey phase transitions in a single crystalline ferrimagnetic magnetite Fe$_3$O$_4$. Using femtosecond optical and magneto-optical pump-probe techniques, we define the range of the initial sample temperatures and laser fluences when partialor complete photo-induced phase transitions occur from a monoclinic insulating to a cubic metallic state with concomitant switching of magnetic anisotropy from the uniaxial to the cubic one. We thus reveal a connection between these phase transitions when driven by femtosecond laser pulses.Using transient linear and quadratic magneto-optical effects, we examine magnetization dynamics launched the switching of the magnetic anisotropy axis. We unveil the presence of the domains under going the laser-induced phase transitions even below the established threshold fluence for the transitions, as well as when the material is initially in the cubic phase. This is the manifestation of the first-order of these both laser-induced phase transitions beyond the range of thermodynamic equilibrium.

cond-mat.mtrl-sci↗