arXiv subjects

A. M. Rey

Publications and source records attributed to A. M. Rey.

At least 19 recordsLinked to original sources

arXiv2024

Entanglement generation in weakly-driven arrays of multilevel atoms via dipolar interactions

We investigate the driven-dissipative dynamics of 1D and 2D arrays of multilevel atoms interacting via dipole-dipole interactions and trapped at subwavelength scales. Here we show that in the weakly driven low excitation regime, multilevel atoms, in contrast to two-level atoms, can become strongly entangled. The entanglement manifests as the growth of collective spin-waves in the ground state manifold, and survives even after turning off the drive. We propose to use the $\sim 2.9~μ$m transition between $\rm ^3{\rm P}_2 \leftrightarrow \, ^3{\rm D}_3$ in $\rm ^{88}Sr$ with $\rm 389~nm$ trapping light as an ideal experimental platform for validating our predictions and as a novel quantum interface for the exploration of complex many-body phenomena emerging from light-matter interactions.

quant-ph↗

arXiv2024

Directional superradiance in a driven ultracold atomic gas in free-space

Ultra-cold atomic systems are among the most promising platforms that have the potential to shed light on the complex behavior of many-body quantum systems. One prominent example is the case of a dense ensemble illuminated by a strong coherent drive while interacting via dipole-dipole interactions. Despite being subjected to intense investigations, this system retains many open questions. A recent experiment carried out in a pencil-shaped geometry reported measurements that seemed consistent with the emergence of strong collective effects in the form of a ``superradiant'' phase transition in free space, when looking at the light emission properties in the forward direction. Motivated by the experimental observations, we carry out a systematic theoretical analysis of the system's steady-state properties as a function of the driving strength and atom number, $N$. We observe signatures of collective effects in the weak drive regime, which disappear with increasing drive strength as the system evolves into a single-particle-like mixed state comprised of randomly aligned dipoles. Although the steady-state features some similarities to the reported superradiant to normal non-equilibrium transition, also known as cooperative resonance fluorescence, we observe significant qualitative and quantitative differences, including a different scaling of the critical drive parameter (from $N$ to $\sqrt{N}$). We validate the applicability of a mean-field treatment to capture the steady-state dynamics under currently accessible conditions. Furthermore, we develop a simple theoretical model that explains the scaling properties by accounting for interaction-induced inhomogeneous effects and spontaneous emission, which are intrinsic features of interacting disordered arrays in free space.

cond-mat.quant-gas↗

arXiv2024

Exploiting nonclassical motion of a trapped ion crystal for quantum-enhanced metrology of global and differential spin rotations

We theoretically investigate prospects for the creation of nonclassical spin states in trapped ion arrays by coupling to a squeezed state of the collective motion of the ions. The correlations of the generated spin states can be tailored for quantum-enhanced sensing of global or differential rotations of sub-ensembles of the spins by working with specific vibrational modes of the ion array. We propose a pair of protocols to utilize the generated states and determine the impact of finite size effects, inhomogeneous couplings between the spin and motional degrees of freedom and technical noise. Our work suggests new opportunities for the preparation of many-body states with tailored correlations for quantum-enhanced metrology in spin-boson systems.

quant-ph↗

arXiv2022

Emergent dark states from superradiant dynamics in multilevel atoms in a cavity

We investigate the collective decay dynamics of atoms with a generic multilevel structure (angular momenta $F\leftrightarrow F'$) coupled to two light modes of different polarization inside a cavity. In contrast to two-level atoms, we find that multilevel atoms can harbour eigenstates that are perfectly dark to cavity decay even within the subspace of permutationally symmetric states (collective Dicke manifold). The dark states arise from destructive interference between different internal transitions and are shown to be entangled. Remarkably, the superradiant decay of multilevel atoms can end up stuck in one of these dark states, where a macroscopic fraction of the atoms remains excited. This opens the door to the preparation of entangled dark states of matter through collective dissipation useful for quantum sensing and quantum simulation. Our predictions should be readily observable in current optical cavity experiments with alkaline-earth atoms or Raman-dressed transitions.

quant-ph↗

arXiv2022

Time-of-Flight Quantum Tomography of Single Atom Motion

Time of flight is an intuitive way to determine the velocity of particles and lies at the heart of many capabilities ranging from mass spectrometry to fluid flow measurements. Here we show time-of-flight imaging can realize tomography of a quantum state of motion of a single trapped atom. Tomography of motion requires studying the phase space spanned by both position and momentum. By combining time-of-flight imaging with coherent evolution of the atom in an optical tweezer trap, we are able to access arbitrary quadratures in phase space without relying on coupling to a spin degree of freedom. To create non-classical motional states, we harness quantum tunneling in the versatile potential landscape of optical tweezers, and our tomography both demonstrates Wigner function negativity and assesses coherence of non-stationary states. Our demonstrated tomography concept has wide applicability to a range of particles and will enable characterization of non-classical states of more complex systems or massive dielectric particles.

quant-ph↗

arXiv2021

Characterizing the dynamical phase diagram of the Dicke model via classical and quantum probes

We theoretically study the dynamical phase diagram of the Dicke model in both classical and quantum limits using large, experimentally relevant system sizes. Our analysis elucidates that the model features dynamical critical points that are distinct from previously investigated excited-state equilibrium transitions. Moreover, our numerical calculations demonstrate that mean-field features of the dynamics remain valid in the exact quantum dynamics, but we also find that in regimes where quantum effects dominate signatures of the dynamical phases and chaos can persist in purely quantum metrics such as entanglement and correlations. Our predictions can be verified in current quantum simulators of the Dicke model including arrays of trapped ions.

quant-ph↗

arXiv2021

Dipole-dipole frequency shifts in multilevel atoms

Dipole-dipole interactions lead to frequency shifts that are expected to limit the performance of next-generation atomic clocks. In this work, we compute dipolar frequency shifts accounting for the intrinsic atomic multilevel structure in standard Ramsey spectroscopy. When interrogating the transitions featuring the smallest Clebsch-Gordan coefficients, we find that a simplified two-level treatment becomes inappropriate, even in the presence of large Zeeman shifts. For these cases, we show a net suppression of dipolar frequency shifts and the emergence of dominant non-classical effects for experimentally relevant parameters. Our findings are pertinent to current generations of optical lattice and optical tweezer clocks, opening a way to further increase their current accuracy, and thus their potential to probe fundamental and many-body physics.

cond-mat.quant-gas↗

arXiv2020

Disorder-controlled relaxation in a 3D Hubbard model quantum simulator

Understanding the collective behavior of strongly correlated electrons in materials remains a central problem in many-particle quantum physics. A minimal description of these systems is provided by the disordered Fermi-Hubbard model (DFHM), which incorporates the interplay of motion in a disordered lattice with local inter-particle interactions. Despite its minimal elements, many dynamical properties of the DFHM are not well understood, owing to the complexity of systems combining out-of-equilibrium behavior, interactions, and disorder in higher spatial dimensions. Here, we study the relaxation dynamics of doubly occupied lattice sites in the three-dimensional (3D) DFHM using interaction-quench measurements on a quantum simulator composed of fermionic atoms confined in an optical lattice. In addition to observing the widely studied effect of disorder inhibiting relaxation, we find that the cooperation between strong interactions and disorder also leads to the emergence of a dynamical regime characterized by \textit{disorder-enhanced} relaxation. To support these results, we develop an approximate numerical method and a phenomenological model that each capture the essential physics of the decay dynamics. Our results provide a theoretical framework for a previously inaccessible regime of the DFHM and demonstrate the ability of quantum simulators to enable understanding of complex many-body systems through minimal models.

cond-mat.quant-gas↗

arXiv2019

Single-Particle Decoherence Can Improve Spin-Squeezing Generated In Collective Dynamics

We study the generation of spin-squeezing in arrays of long-lived dipoles subject to collective emission, coherent drive, elastic interactions, and spontaneous emission. Counter-intuitively, it is found that the introduction of spontaneous emission leads to an enhancement of the achievable spin-squeezing, relative to that which emerges in the steady-state of the purely collective dynamics for the same model parameters. This behavior is connected to the dynamical self-tuning of the system through a dissipative phase transition that is present in the collective system alone. Our findings will be applicable to next-generation quantum sensors harnessing correlated quantum matter, including cavity-QED and trapped ion systems.

quant-ph↗

arXiv2019

Subradiance of multilevel fermionic atoms in arrays with filling $n \geq 2$

We investigate the subradiance properties of $n\geq 2$ multilevel fermionic atoms loaded into the lowest motional level of a single trap (e.g.~a single optical lattice site or an optical tweezer). As pointed out in our previous work [arXiv:1907.05541], perfectly dark subradiant states emerge from the interplay between fermionic statistics and dipolar interactions. While in [arXiv:1907.05541] we focused on the $n=2$ case, here we provide an in-depth analysis of the single-site dark states for generic filling $n$, and show a tight connection between generic dark states and total angular momentum eigenstates. We show how the latter can also be used to understand the full eigenstate structure of the single-site problem, which we analyze numerically. Apart from this, we discuss two possible schemes to coherently prepare dark states using either a Raman transition or an external magnetic field to lift the Zeeman degeneracy. Although the analysis focuses on the single-site problem, we show that multi-site dark states can be trivially constructed in any geometry out of product states of single-site dark states. Finally, we discuss some possible implementations with alkaline-earth(-like) atoms such as $^{171}$Yb or $^{87}$Sr loaded into optical lattices, where they could be used for potential applications in quantum metrology and quantum information.

quant-ph↗

arXiv2019

Unifying fast scrambling, thermalization and entanglement through the measurement of FOTOCs in the Dicke model

Scrambling of quantum information is the process by which information initially stored in the local degrees of freedom of a quantum many-body system spreads over its many-body degrees of freedom, becoming inaccessible to local probes and thus apparently lost. Scrambling and entanglement are key concepts reconciling seemingly unrelated behaviors including thermalization of isolated quantum systems and information loss in black holes, and have revolutionized our understanding of non-equilibrium phenomena. Here, we demonstrate that a family of fidelity out-of-time-order correlators (FOTOCs), recently measured in a trapped-ion quantum simulator via time reversal of the many-body dynamics followed by a fidelity measurement, can serve as a unifying diagnostic tool that elucidates the intrinsic connection between fast scrambling, volume law entanglement, ergodicity, quantum chaos, and the associated butterfly effect in the semiclassical dynamics of the system. We demonstrate the utility of FOTOCs by computing them in the Dicke model, an iconic model in quantum optics, recently implemented in atomic and trapped-ion setups. This model describes the coupling of a large spin to an oscillator and features rich behaviors, including a quantum phase transition and chaos. Here, we show that FOTOCs provide a direct measure of the spin-phonon Renyi entropy and quantum thermalization. Moreover, we connect the FOTOCs to the variance of simple operators, allowing us to observe fast scrambling in the parameter regime where the system's classical trajectories are chaotic, and to explicitly relate the quantum and classical Lyapunov exponents in a truly quantum many-body system. Our results open a path for the experimental use of FOTOCs to quantify fast scrambling, determine bounds on quantum information processing and to identify possible candidates of black hole analogs in controllable quantum systems.

quant-ph↗

arXiv2019

Dynamics of quantum information

The ability to harness the dynamics of quantum information and entanglement is necessary for the development of quantum technologies and the study of complex quantum systems. On the theoretical side the dynamics of quantum information is a topic that is helping us unify and confront common problems in otherwise disparate fields in physics, such as quantum statistical mechanics and cosmology. On the experimental side the impressive developments on the manipulation of neutral atoms and trapped ions are providing new capabilities to probe their quantum dynamics. Here, we overview and discuss progress in characterizing and understanding the dynamics of quantum entanglement and information scrambling in quantum many-body systems. The level of control attainable over both the internal and external degrees of freedom of individual particles in these systems provides great insight into the intrinsic connection between entanglement and thermodynamics, bounds on information transport and computational complexity of interacting systems. In turn this understanding should enable the realization of quantum technologies.

quant-ph↗

arXiv2019

Dark states of multilevel fermionic atoms in doubly-filled optical lattices

We propose to use fermionic atoms with degenerate ground and excited internal levels ($F_g\rightarrow F_e$), loaded into the motional ground state of an optical lattice with two atoms per lattice site, to realize dark states with no radiative decay. The physical mechanism behind the dark states is an interplay of Pauli blocking and multilevel dipolar interactions. The dark states are independent of lattice geometry, can support an extensive number of excitations and can be coherently prepared using a Raman scheme taking advantage of the quantum Zeno effect. These attributes make them appealing for atomic clocks, quantum memories, and quantum information on decoherence free subspaces.

quant-ph↗

arXiv2019

A cavity-QED simulator of slow and fast scrambling

We study information scrambling, as diagnosed by the out-of-time order correlations (OTOCs), in a system of large spins collectively interacting via spatially inhomogeneous and incommensurate exchange couplings. The model is realisable in a cavity QED system in the dispersive regime. Fast scrambling, signalled by an exponential growth of the OTOCs, is observed when the couplings do not factorise into the product of a pair of local interaction terms, and at the same time the state of the spins points initially coplanar to the equator of the Bloch sphere. When one of these conditions is not realised, OTOCs grow algebraically with an exponent sensitive to the orientation of the spins in the initial state. The impact of initial conditions on the scrambling dynamics is attributed to the presence of a global conserved quantity, which critically slows down the evolution for initial states close to the poles of the Bloch sphere.

cond-mat.quant-gas↗

arXiv2019

Controlling Dipolar Exchange Interactions in a Dense 3D Array of Large Spin Fermions

Dipolar interactions are ubiquitous in nature and rule the behavior of a broad range of systems spanning from energy transfer in biological systems to quantum magnetism. Here, we study magnetization-conserving dipolar induced spin-exchange dynamics in dense arrays of fermionic erbium atoms confined in a deep three-dimensional lattice. Harnessing the special atomic properties of erbium, we demonstrate control over the spin dynamics by tuning the dipole orientation and changing the initial spin state within the large 20 spin hyperfine manifold. Furthermore, we demonstrate the capability to quickly turn on and off the dipolar exchange dynamics via optical control. The experimental observations are in excellent quantitative agreement with numerical calculations based on discrete phase-space methods, which capture entanglement and beyond-mean field effects. Our experiment sets the stage for future explorations of rich magnetic behaviors in long-range interacting dipoles, including exotic phases of matter and applications for quantum information processing.

cond-mat.quant-gas↗

arXiv2019

Bang-bang shortcut to adiabaticity in the Dicke model as realized in a Penning trap experiment

We introduce a bang-bang shortcut to adiabaticity for the Dicke model, which we implement via a 2-D array of trapped ions in a Penning trap with a spin-dependent force detuned close to the center-of-mass drumhead mode. Our focus is on employing this shortcut to create highly entangled states that can be used in high-precision metrology. We highlight that the performance of the bang-bang approach is comparable to standard preparation methods, but can be applied over a much shorter time frame. We compare these theoretical ideas with experimental data which serve as a first step towards realizing this theoretical procedure for generating multi-partite entanglement.

quant-ph↗

arXiv2018

Exploring out-of-equilibrium quantum magnetism and thermalization in a spin-3 many-body dipolar lattice system

Understanding quantum thermalization through entanglement build-up in isolated quantum systems addresses fundamental questions on how unitary dynamics connects to statistical physics. Here, we study the spin dynamics and approach towards local thermal equilibrium of a macroscopic ensemble of S = 3 spins prepared in a pure coherent spin state, tilted compared to the magnetic field, under the effect of magnetic dipole-dipole interactions. The experiment uses a unit filled array of 104 chromium atoms in a three dimensional optical lattice, realizing the spin-3 XXZ Heisenberg model. The buildup of quantum correlation during the dynamics, especially as the angle approaches pi/2, is supported by comparison with an improved numerical quantum phase-space method and further confirmed by the observation that our isolated system thermalizes under its own dynamics, reaching a steady state consistent with the one extracted from a thermal ensemble with a temperature dictated from the system's energy. This indicates a scenario of quantum thermalization which is tied to the growth of entanglement entropy. Although direct experimental measurements of the Renyi entropy in our macroscopic system are unfeasible, the excellent agreement with the theory, which can compute this entropy, does indicate entanglement build-up.

cond-mat.quant-gas↗

arXiv2018

The Hong-Ou-Mandel effect with atoms

Controlling light at the level of individual photons has led to advances in fields ranging from quantum information and precision sensing to fundamental tests of quantum mechanics. A central development that followed the advent of single photon sources was the observation of the Hong-Ou- Mandel (HOM) effect, a novel two-photon path interference phenomenon experienced by indistinguishable photons. The effect is now a central technique in the field of quantum optics, harnessed for a variety of applications such as diagnosing single photon sources and creating probabilistic entanglement in linear quantum computing. Recently, several distinct experiments using atomic sources have realized the requisite control to observe and exploit Hong-Ou-Mandel interference of atoms. This article provides a summary of this phenomenon and discusses some of its implications for atomic systems. Transitioning from the domain of photons to atoms opens new perspectives on fundamental concepts, such as the classification of entanglement of identical particles. It aids in the design of novel probes of quantities such as entanglement entropy by combining well established tools of AMO physics - unity single-atom detection, tunable interactions, and scalability - with the Hong-Ou-Mandel interference. Furthermore, it is now possible for established protocols in the photon community, such as measurement-induced entanglement, to be employed in atomic experiments that possess deterministic single-particle production and detection. Hence, the realization of the HOM effect with atoms represents a productive union of central ideas in quantum control of atoms and photons.

quant-ph↗