arXiv subjects

A. M. Rucklidge

Publications and source records attributed to A. M. Rucklidge.

At least 19 recordsLinked to original sources

arXiv2026

Tuning polymer architecture for quasicrystal self-assembly

Using computer simulations and theory, we investigate the ultrasoft interactions between dendrimers formed of a central polymer connected by stiff linkers to a corona of flexible polymers, forming `pompoms' at the ends of the linkers. We show that the resulting coarse-grained interaction potential between pairs of dendrimers exhibits tunable lengthscale competition based on properties of the core and corona polymers. We present a simple model for this pair potential, which we confirm using accelerated Monte Carlo methods. We then demonstrate the connection between dendrimer structure and mesoscopic phases by presenting parameter choices that result in stable dodecagonal quasicrystals, and show that the size of the region in the phase diagram where quasicrystals are stable can be controlled by tuning details of the polymer architecture alone. These results pave the way for experimental realization of soft matter quasicrystals by identifying what overall molecular architecture leads to their stability.

cond-mat.soft↗

arXiv2024

Convectons in unbalanced natural doubly diffusive convection

Fluids subject to both thermal and compositional variations can undergo doubly diffusive convection when these properties both affect the fluid density and diffuse at different rates. In natural doubly diffusive convection, the gradients of temperature and salinity are aligned with each other and orthogonal to gravity. The resulting buoyancy-driven flows are known to lead to the formation of a variety of patterns, including spatially localized states of convection surrounded by quiescent fluid, which are known as convectons. Localized pattern formation in natural doubly diffusive convection has been studied under a specific balance where the effects of temperature and salinity changes are opposite but of equal intensity on the fluid density. In this case, a steady conduction state exists and convectons bifurcate from it. The aforementioned buoyancy balance underpins our knowledge of this pattern formation but it is an ideal case that can hardly be met experimentally or in nature. This article addresses how localized pattern formation in natural doubly diffusive convection is affected by departures from the balanced case. In particular, the absence of a conduction state leads to the unfolding of the bifurcations to convectons. In thermally dominated regimes, the background flow promotes localized states with convection rolls attached to the end-walls, known as anticonvectons, and the existence of these states is found to be related to the emergence of convectons. The results presented here shed light on the convecton robustness against changes in the buoyancy ratio and extend the scope of our understanding of localized pattern formation in fluid systems.

physics.flu-dyn↗

arXiv2024

Spirals and heteroclinic cycles in a spatially extended Rock-Paper-Scissors model of cyclic dominance

Spatially extended versions of the cyclic-dominance Rock-Paper-Scissors model have traveling wave (in one dimension) and spiral (in two dimensions) behavior. The far field of the spirals behave like traveling waves, which themselves have profiles reminiscent of heteroclinic cycles. We compute numerically a nonlinear dispersion relation between the wavelength and wavespeed of the traveling waves, and, together with insight from heteroclinic bifurcation theory and further numerical results from 2D simulations, we are able to make predictions about the overall structure and stability of spiral waves in 2D cyclic dominance models.

nlin.PS↗

arXiv2023

Near-onset dynamics in natural doubly diffusive convection

Doubly diffusive convection is considered in a vertical slot where horizontal temperature and solutal variations provide competing effects to the fluid density while allowing the existence of a conduction state. In this configuration, the linear stability of the conductive state is known, but the convection patterns arising from the primary instability have only been studied for specific parameter values. We have extended this by determining the nature of the primary bifurcation for all values of the Lewis and Prandtl numbers using a weakly nonlinear analysis. The resulting convection branches are extended using numerical continuation and we find large-amplitude steady convection states can coexist with the stable conduction state for sub- and supercritical primary bifurcations. The stability of the convection states is investigated and attracting travelling waves and periodic orbits are identified using time-stepping when these steady states are unstable.

physics.flu-dyn↗

arXiv2023

Towards Convectons in the Supercritical Regime: Homoclinic Snaking in Natural Doubly Diffusive Convection

Fluids subject to both thermal and compositional variations can undergo doubly diffusive convection when these properties both affect the fluid density and diffuse at different rates. A variety of patterns can arise from these buoyancy-driven flows, including spatially localised states known as convectons, which consist of convective fluid motion localised within a background of quiescent fluid. We consider these states in a vertical slot with the horizontal temperature and solutal gradients providing competing effects to the fluid density while allowing the existence of a conduction state. In this configuration, convectons have been studied with specific parameter values where the onset of convection is subcritical, and the states have been found to lie on a pair of secondary branches that undergo homoclinic snaking in a parameter regime below the onset of linear instability. In this paper, we show that convectons persist into parameter regimes in which the primary bifurcation is supercritical and there is no bistability, despite coexistence between the stable conduction state and large-amplitude convection. We detail this transition by considering spatial dynamics and observe how the structure of the secondary branches becomes increasingly complex owing to the increased role of inertia at low Prandtl numbers.

physics.flu-dyn↗

arXiv2019

Which wavenumbers determine the thermodynamic stability of soft matter quasicrystals?

For soft matter to form quasicrystals an important ingredient is to have two characteristic lengthscales in the interparticle interactions. To be more precise, for stable quasicrystals, periodic modulations of the local density distribution with two particular wavenumbers should be favored, and the ratio of these wavenumbers should be close to certain special values. So, for simple models, the answer to the title question is that only these two ingredients are needed. However, for more realistic models, where in principle all wavenumbers can be involved, other wavenumbers are also important, specifically those of the second and higher reciprocal lattice vectors. We identify features in the particle pair interaction potentials which can suppress or encourage density modes with wavenumbers associated with one of the regular crystalline orderings that compete with quasicrystals, enabling either the enhancement or suppression of quasicrystals in a generic class of systems.

cond-mat.soft↗

arXiv2018

Localized Patterns in Periodically Forced Systems: II. Patterns with Non-Zero Wavenumber

In pattern-forming systems, localized patterns are readily found when stable patterns exist at the same parameter values as the stable unpatterned state. Oscillons are spatially localized, time-periodic structures, which have been found experimentally in systems that are driven by a time-periodic force, for example, in the Faraday wave experiment. This paper examines the existence of oscillatory localized states in a PDE model with single frequency time dependent forcing, introduced in [A. M. Rucklidge and M. Silber, SIAM J. Appl. Math., 8 (2009), pp. 298-347, arXiv:0805.0878] as a phenomenological model of the Faraday wave experiment. We choose parameters so that patterns set in with non-zero wavenumber (in contrast to [A. S. Alnahdi, J. Niesen and A. M. Rucklidge, SIAM J. Appl. Dyn. Syst., 13 (2014), pp. 1311-1327, arXiv:1312.2773]). In the limit of weak damping, weak detuning, weak forcing, small group velocity, and small amplitude, we reduce the model PDE to the coupled forced complex Ginzburg-Landau equations. We find localized solutions and snaking behaviour in the coupled forced complex Ginzburg-Landau equations and relate these to oscillons that we find in the model PDE. Close to onset, the agreement is excellent. The periodic forcing for the PDE and the explicit derivation of the amplitude equations make our work relevant to the experimentally observed oscillons.

nlin.PS↗

arXiv2017

Spatially Localized Quasicrystals

We investigate quasicrystal-forming soft matter using a two-scale phase field crystal model. At state points near thermodynamic coexistence between bulk quasicrystals and the liquid phase, we find multiple metastable spatially localized quasicrystals embedded in a background of liquid. In three dimensions we obtain spatially localized icosahedral quasicrystals. In two dimensions, we compute several families of spatially localized quasicrystals with dodecagonal structure and investigate their properties as a function of the system parameters. In both cases the localized quasicrystals are metastable, and so correspond to energetically locally favored structures. The presence of such structures is expected to crucially affect the dynamics of the crystallization process.

nlin.PS↗

arXiv2016

Chaos in the Takens-Bogdanov bifurcation with O(2) symmetry

The Takens-Bogdanov bifurcation is a codimension two bifurcation that provides a key to the presence of complex dynamics in many systems of physical interest. When the system is translation-invariant in one spatial dimension with no left-right preference the imposition of periodic boundary conditions leads to the Takens-Bogdanov bifurcation with O(2) symmetry. This bifurcation, analyzed by G. Dangelmayr and E. Knobloch, Phil. Trans. R. Soc. London A 322, 243 (1987), describes the interaction between steady states and traveling and standing waves in the nonlinear regime and predicts the presence of modulated traveling waves as well. The analysis reveals the presence of several global bifurcations near which the averaging method (used in the original analysis) fails. We show here, using a combination of numerical continuation and the construction of appropriate return maps, that near the global bifurcation that terminates the branch of modulated traveling waves, the normal form for the Takens-Bogdanov bifurcation admits cascades of period-doubling bifurcations as well as chaotic dynamics of Shil'nikov type. Thus chaos is present arbitrarily close to the codimension two point.

nlin.CD↗

arXiv2016

Three-dimensional Phase Field Quasicrystals

We investigate the formation and stability of icosahedral quasicrytalline structures using a dynamic phase field crystal model. Nonlinear interactions between density waves at two length scales stabilize three-dimensional quasicrystals. We determine the phase diagram and parameter values required for the quasicrystal to be the global minimum free energy state. We demonstrate that traits that promote the formation of two-dimensional quasicrystals are extant in three dimensions, and highlight the characteristics required for 3D soft matter quasicrystal formation.

nlin.PS↗

arXiv2015

Soft-core particles freezing to form a quasicrystal and a crystal-liquid phase

Systems of soft-core particles interacting via a two-scale potential are studied. The potential is responsible for peaks in the structure factor of the liquid state at two different but comparable length scales, and a similar bimodal structure is evident in the dispersion relation. Dynamical density functional theory in two dimensions is used to identify two novel states of this system, the crystal-liquid state, in which the majority of the particles are located on lattice sites but a minority remains free and so behaves like a liquid, and a 12-fold quasicrystalline state. Both are present even for deeply quenched liquids and are found in a regime in which the liquid is unstable with respect to modulations on the smaller scale only. As a result the system initially evolves towards a small scale crystal state; this state is not a minimum of the free energy, however, and so the system subsequently attempts to reorganize to generate the lower energy larger scale crystals. This dynamical process generates a disordered state with quasicrystalline domains, and takes place even when this large scale is linearly stable, i.e., it is a nonlinear process. With controlled initial conditions a perfect quasicrystal can form. The results are corroborated using Brownian dynamics simulations.

cond-mat.soft↗

arXiv2015

Can weakly nonlinear theory explain Faraday wave patterns near onset?

The Faraday problem is an important pattern-forming system that provides some middle ground between systems where the initial instability involves just a single mode and in which complexity then results from mode interactions or secondary bifurcations, and cases where a system is highly turbulent and many spatial and temporal modes are excited. It has been a rich source of novel patterns and of theoretical work aimed at understanding how and why such patterns occur. Yet it is particularly challenging to tie theory to experiment: the experiments are difficult to perform; the parameter regime of interest (large box, moderate viscosity) along with the technical difficulties of solving the free boundary Navier--Stokes equations make numerical solution of the problem hard; and the fact that the instabilities result in an entire circle of unstable wavevectors presents considerable theoretical difficulties. In principle, weakly nonlinear theory should be able to predict which patterns are stable near pattern onset. In this paper we present the first quantitative comparison between weakly nonlinear theory of the full Navier-Stokes equations and (previously published) experimental results for the Faraday problem with multiple frequency forcing. We confirm that three-wave interactions sit at the heart of why complex patterns are stablised but also highlight some discrepancies between theory and experiment. These suggest the need for further experimental and theoretical work to fully investigate the issues of pattern bistability and the role of bicritical/tricritical points in determining bifurcation structure.

nlin.PS↗

arXiv2013

Quasicrystalline order and a crystal-liquid state in a soft-core fluid

A two-dimensional system of soft particles interacting via a two-length-scale potential is studied. Density functional theory and Brownian dynamics simulations reveal a fluid phase and two crystalline phases with different lattice spacing. Of these the larger lattice spacing phase can form an exotic periodic state with a fraction of highly mobile particles: a crystal liquid. Near the transition between this phase and the smaller lattice spacing phase, quasicrystalline structures may be created by a competition between linear instability at one scale and nonlinear selection of the other.

cond-mat.soft↗

arXiv2011

Skew-Varicose Instability in Two Dimensional Generalized Swift-Hohenberg Equations

We apply analytical and numerical methods to study the linear stability of stripe patterns in two generalizations of the two-dimensional Swift-Hohenberg equation that include coupling to a mean flow. A projection operator is included in our models to allow exact stripe solutions. In the generalized models, stripes become unstable to the skew-varicose, oscillatory skew-varicose and cross-roll instabilities, in addition to the usual Eckhaus and zigzag instabilities. We analytically derive stability boundaries for the skew-varicose instability in various cases, including several asymptotic limits. We also use numerical techniques to determine eigenvalues and hence stability boundaries of other instabilities. We extend our analysis to both stress-free and no-slip boundary conditions and we note a cross over from the behaviour characteristic of no-slip to that of stress-free boundaries as the coupling to the mean flow increases or as the Prandtl number decreases. Close to the critical value of the bifurcation parameter, the skew varicose instability has the same curvature as the Eckhaus instability provided the coupling to the mean flow is greater than a critical value. The region of stable stripes is completely eliminated by the cross-roll instability for large coupling to the mean flow.

math.DS↗

arXiv2009

On the existence of quasipattern solutions of the Swift-Hohenberg equation

Quasipatterns (two-dimensional patterns that are quasiperiodic in any spatial direction) remain one of the outstanding problems of pattern formation. As with problems involving quasiperiodicity, there is a small divisor problem. In this paper, we consider 8-fold, 10-fold, 12-fold, and higher order quasipattern solutions of the Swift-Hohenberg equation. We prove that a formal solution, given by a divergent series, may be used to build a smooth quasiperiodic function which is an approximate solution of the pattern-forming PDE up to an exponentially small error.

nlin.PS↗

arXiv2008

Design of parametrically forced patterns and quasipatterns

The Faraday wave experiment is a classic example of a system driven by parametric forcing, and it produces a wide range of complex patterns, including superlattice patterns and quasipatterns. Nonlinear three-wave interactions between driven and weakly damped modes play a key role in determining which patterns are favoured. We use this idea to design single and multi-frequency forcing functions that produce examples of superlattice patterns and quasipatterns in a new model PDE with parametric forcing. We make quantitative comparisons between the predicted patterns and the solutions of the PDE. Unexpectedly, the agreement is good only for parameter values very close to onset. The reason that the range of validity is limited is that the theory requires strong damping of all modes apart from the driven pattern-forming modes. This is in conflict with the requirement for weak damping if three-wave coupling is to influence pattern selection effectively. We distinguish the two different ways that three-wave interactions can be used to stabilise quasipatterns, and present examples of 12-, 14- and 20-fold approximate quasipatterns. We identify which computational domains provide the most accurate approximations to 12-fold quasipatterns, and systematically investigate the Fourier spectra of the most accurate approximations.

nlin.PS↗

arXiv2008

Numerical simulations of rotating axisymmetric sunspots

A numerical model of axisymmetric convection in the presence of a vertical magnetic flux bundle and rotation about the axis is presented. The model contains a compressible plasma described by the nonlinear MHD equations, with density and temperature gradients simulating the upper layer of the sun's convection zone. The solutions exhibit a central magnetic flux tube in a cylindrical numerical domain, with convection cells forming collar flows around the tube. When the numerical domain is rotated with a constant angular velocity, the plasma forms a Rankine vortex, with the plasma rotating as a rigid body where the magnetic field is strong, as in the flux tube, while experiencing sheared azimuthal flow in the surrounding convection cells, forming a free vortex. As a result, the azimuthal velocity component has its maximum value close to the outer edge of the flux tube. The azimuthal flow inside the magnetic flux tube and the vortex flow are prograde relative to the rotating cylindrical reference frame. A retrograde flow appears at the outer wall. The most significant convection cell outside the flux tube is the location for the maximum value of the azimuthal magnetic field component. The azimuthal flow and magnetic structure are not generated spontaneously, but decay exponentially in the absence of any imposed rotation of the cylindrical domain.

astro-ph↗

arXiv2006

Quasipatterns in parametrically forced systems

We examine two mechanisms that have been put forward to explain the selection of quasipatterns in single and multi-frequency forced Faraday wave experiments. Both mechanisms can be used to generate stable quasipatterns in a parametrically forced partial differential equation that shares some characteristics of the Faraday wave experiment. One mechanism, which is robust and works with single-frequency forcing, does not select a specific quasipattern: we find, for two different forcing strengths, a 12-fold quasipattern and the first known example of a spontaneously formed 14-fold quasipattern. The second mechanism, which requires more delicate tuning, can be used to select particular angles between wavevectors in the quasipattern.

nlin.PS↗