arXiv subjects

A. Maj

Publications and source records attributed to A. Maj.

At least 19 recordsLinked to original sources

arXiv2026

Level structure of light neutron-rich La isotopes beyond the N=82 shell closure

The high spin excited states of Lanthanum isotopes $^{140-143}$La, above the $N=82$ closed shell, have been populated in fission reactions. The prompt $\gamma$-ray transitions were measured using two complementary methods; a) in coincidence with the isotopically identified fragments produced in the fission of the $^{238}$U+$^{9}$Be system using the VAMOS++ and the AGATA spectrometers and b) high statistics three-fold $\gamma-\gamma-\gamma$ and four-fold $\gamma-\gamma-\gamma-\gamma$ coincidence data from the spontaneous fission of $^{252}$Cf using the Gammasphere. This work reports the first identification of a pair of parity doublet structures in $^{143}$La and the new high spin level structure in $^{140-142}$La from prompt $\gamma$-ray spectroscopy. The level structures are interpreted in terms of the systematics of neighbouring odd-$Z$ nuclei above $Z=50$ shell closure and large-scale shell model calculations. The present results indicate the presence of stable octupole deformation, in $^{143}$La. The excitation energy pattern and their comparison with neighbouring isotones, moving away from the N=82 closed shell, point towards a transition from single particle structures to an alternating parity rotational band structure in the La isotopic chain.

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arXiv2026

Direct transfer to $^{46,48}$K as a survey of the $\pi(s_{1/2})$$-\nu(sdpf)$ interaction

The collapse of the canonical $N=28$ magic number in nuclei with $Z<20$ has drawn significant interest as it relates to the emergence of an island of inversion centered on $^{42}$Si and $^{44}$S. In particular, interactions between the $\pi s_{1/2}$ orbital -- empty in $^{42}$Si and full in $^{44}$S -- and the neutron orbitals just above and below the $N=28$ gap are expected to be critical in this region, but remain relatively unexplored. In this paper, we expand upon the results of our previous study of the direct transfer reaction $^{47}$K(d,p$\gamma$)$^{48}$K [C.\,J.~Paxman \textit{et al.}, Phys. Rev. Lett. 134, 162504 (2025)] with the results of the complementary $^{47}$K(d,t$\gamma$)$^{46}$K reaction. Through this study, we present a comprehensive scan of the interaction between the critical $\pi s_{1/2}$ orbital and a broad range of neutron orbitals spanning nearly two full shells. We identify several discrepancies between the experimental results and state-of-the-art shell model calculations, which suggest a deficiency of the shell model to fully capture the complex proton configuration mixing in this region, highlighting a significant challenge for single-particle descriptions of the island of inversion.

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arXiv2025

First evidence for the J$>$1 components of the pygmy dipole resonance in neutron-rich nuclei

Gamma ($\gamma$) decay shapes the synthesis of heavy elements in neutron-rich nuclear environments of neutron star mergers, supplying the Universe with heavy elements. The low-energy pygmy dipole resonance (PDR) influences nuclear reaction rates of the rapid nucleosynthesis through enhanced $\gamma$ transitions. However, since it is difficult to reproduce astrophysical conditions in laboratories, PDR was previously observed only in $J = 1$ spin states. Here we report the first experimental observation of $J > 1$ components of PDR, identified in the $\beta$-delayed $\gamma$ decay of the J$^{\pi}$ = 3$^{-}$ spin-parity isomer of $^{80}$Ga. The data analysis, combined with decay information and theoretical calculations allows the identification of resonant structures below the neutron emission threshold of the neutron-rich germanium $^{80}$Ge as J$^{\pi} = (2,3)^-$ components of the PDR built on the low-lying J$^{\pi}$ = 2$^+$ quadrupole state. Our findings extend the concept of PDR beyond dipole states, with implications for nuclear structure theory and experiment, as well as the element production in the cosmos.

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arXiv2025

Data sorting modes of phoswich detector array

The different data-sorting modes of the phoswich detector array PARIS used for detecting high-energy (4$-$10 MeV) $\gamma$ rays are investigated. The characteristics including time resolution, energy resolution and detection efficiency under various modes are studied. The present study shows that PARIS has capabilities of rejecting escape and pileup events when used for decay spectroscopy. Notably, the methods presented in this work refer specifically to the $\beta$-decay experiment of $^{80g+m}$Ga conducted with three PARIS clusters comprising 27 phoswich detectors, rather than to a general report on the PARIS array or its overall performance for in-beam spectroscopy. Compared with the 2"$\times$2"$\times$2" LaBr$_3$(Ce) detector (Ciema{\l}a et al., 2009), even in individual mode, PARIS provides significant suppression of single- and double-escape peaks and reduces background via vetoing function of the outer-volume NaI(Tl) crystals. In contrast to the common approach of adding back the energies in LaBr$_3$(Ce) and NaI(Tl) to increase the detection efficiency of the full-energy peak, using NaI(Tl) as a veto shield provides a superior trade-off for applications where spectral purity is essential. Employing add-back analysis within each cluster of nine phoswiches or between all phoswiches could enhance full-energy peak efficiency and further suppress escape peaks and background. Applying a multiplicity condition provides a further suppression but simultaneously lowers the statistics of full-energy peaks.

physics.ins-det↗

arXiv2024

Probing exotic cross-shell interactions at N=28 with single-neutron transfer on 47K

We present the first measurement of the $^{47}$K($d,p\gamma$)$^{48}$K transfer reaction, performed in inverse kinematics using a reaccelerated beam of $^{47}$K. The level scheme of $^{48}$K has been greatly extended with nine new bound excited states identified and spectroscopic factors deduced. Detailed comparisons with SDPF-U and SDPF-MU shell-model calculations reveal a number of discrepancies with these results, and a preference for SDPF-MU is found. Intriguingly, an apparent systematic overestimation of spectroscopic factors and a poor reproduction of the energies for 1$^-$ states suggests that the mixing between the $\pi s^{\,\,\,1}_{1/2} d^{\,\,\,4}_{3/2}$ and $\pi s^{\,\,\,2}_{1/2} d^{\,\,\,3}_{3/2}$ proton configurations in $^{48}$K is not correctly described using current interactions, challenging our descriptions of light $N=28$ nuclei.

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arXiv2024

High-precision spectroscopy of $^{20}$O benchmarking ab-initio calculations in light nuclei

The excited states of unstable $^{20}$O were investigated via $\gamma$-ray spectroscopy following the $^{19}$O$(d,p)^{20}$O reaction at 8 $A$MeV. By exploiting the Doppler Shift Attenuation Method, the lifetime of the 2$^+_2$ and 3$^+_1$ states were firmly established. From the $\gamma$-ray branching and E2/M1 mixing ratios for transitions deexciting the 2$^+_2$ and 3$^+_1$ states, the B(E2) and B(M1) were determined. Various chiral effective field theory Hamiltonians, describing the nuclear properties beyond ground states, along with a standard USDB interaction, were compared with the experimentally obtained data. Such a comparison for a large set of $\gamma$-ray transition probabilities with the valence space in medium similarity renormalization group ab-initio calculations was performed for the first time in a nucleus far from stability. It was shown that the ab-initio approaches using chiral EFT forces are challenged by detailed high-precision spectroscopic properties of nuclei. The reduced transition probabilities were found to be a very constraining test of the performance of the ab-initio models.

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arXiv2023

Characterization of a novel proton-CT scanner based on Silicon and LaBr$_3$(Ce) detectors

Treatment planning systems at proton-therapy centres generally use X-ray computed tomography (CT) as primary imaging technique to infer the proton treatment doses to tumour and healthy tissues. However, proton stopping powers in the body, as derived from X-ray images, suffer from important proton-range uncertainties. In order to reduce this uncertainty in range, one could use proton-CT images instead. The main goal of this work is to test the capabilities of a newly-developed proton-CT scanner, based on the use of a set of tracking detectors and a high energy resolution scintillator for the residual energy of the protons. Different custom-made phantoms were positioned at the field of view of the scanner and were irradiated with protons at the CCB proton-therapy center in Krakow. We measured with the phantoms at different angles and produced sinograms that were used to obtain reconstructed images by Filtered Back-Projection (FBP). The obtained images were used to determine the capabilities of our scanner in terms of spatial resolution and proton Relative Stopping Power mapping and validate its use as proton-CT scanner. The results show that the scanner can produce medium-high quality images, with spatial resolution better than 2 mm in radiography, below 3 mm in tomography and resolving power in the RSP comparable to other state of the art pCT cameras.

physics.med-ph↗

arXiv2021

Narrow resonances in the continuum of the unbound nucleus $^{15}$F

The structure of the unbound $^{15}$F nucleus is investigated using the inverse kinematics resonant scattering of a radioactive $^{14}$O beam impinging on a CH$_2$ target. The analysis of $^{1}$H($^{14}$O,p)$^{14}$O and $^{1}$H($^{14}$O,2p)$^{13}$N reactions allowed the confirmation of the previously observed narrow $1/2^{-}$ resonance, near the two-proton decay threshold, and the identification of two new narrow 5/2$^{-}$ and 3/2$^{-}$ resonances. The newly observed levels decay by 1p emission to the ground of $^{14}$O, and by sequential 2p emission to the ground state (g.s.) of $^{13}$N via the $1^-$ resonance of $^{14}$O. Gamow shell model (GSM) analysis of the experimental data suggests that the wave functions of the 5/2$^{-}$ and 3/2$^{-}$ resonances may be collectivized by the continuum coupling to nearby 2p- and 1p- decay channels. The observed excitation function $^{1}$H($^{14}$O,p)$^{14}$O and resonance spectrum in $^{15}$F are well reproduced in the unified framework of the GSM.

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arXiv2021

Proton radiographs using position-sensitive silicon detectors and high-resolution scintillators

Proton therapy is a cancer treatment technique currently in growth worldwide. It offers advantages with respect to conventional X-ray and $\gamma$-ray radiotherapy, in particular, a better control of the dose deposition allowing to reach a higher conformity in the treatments. Therefore, it causes less damage to the surrounding healthy tissue and less secondary effects. However, in order to take full advantage of its potential, improvements in treatment planning and dose verification are required. A new prototype of proton Computed Tomography scanner is proposed to design more accurate and precise treatment plans for proton therapy. Here, results obtained from an experiment performed using a 100-MeV proton beam at the CCB facility in Krakow (Poland) are presented. Proton radiographs of PMMA samples of 50-mm thickness with spatial patterns in aluminum were taken. Their properties were studied, including reproduction of the dimensions, spatial resolution and sensitivity to different materials. They demonstrate the capabilities of the system to produce images with protons. Structures of up to 2 mm are nicely resolved and the sensitivity of the system was enough to distinguish thicknesses of 10 mm of aluminum or PMMA. This constitutes a first step to validate the device as a proton radiography scanner previous to the future tests as a proton CT scanner.

physics.med-ph↗

arXiv2021

Coulomb and nuclear excitations of $^{70}$Zn and $^{68}$Ni at intermediate energy

The reduced transition probabilities $B(E2; 0^+_{g.s.}\rightarrow2_1^+,2^+_2)$ in $^{70}$Zn and the full $B(E2; 0^+_{g.s.}\rightarrow2^+)$ strength up to S$_n$=7.79 MeV in $^{68}$Ni have been determined at the LISE/GANIL facility using the Coulomb-excitation technique at intermediate beam energy on a $^{208}$Pb target. The $\gamma$ rays emitted in-flight were detected with an array of 46 BaF$_2$ crystals. The angles of the deflected nuclei were determined in order to disentangle and extract the Coulomb and nuclear contributions to the excitation of the 2$^+$ states. The measured $B(E2; 0^+_{g.s.}\rightarrow2_1^+)$ of 1432(124) e$^2$fm$^4$ for $^{70}$Zn falls in the lower part of the published values which clustered either around 1600 or above 2000 e$^2$fm$^4$, while the $B(E2; 0^+_{g.s.}\rightarrow2^+_2)$ of 53(7) e$^2$fm$^4$ agrees very well with the two published values. The relatively low $B(E2; 0^+_{g.s.}\rightarrow2_1^+)$ of 301(38) e$^2$fm$^4$ for $^{68}$Ni agrees with previous studies and confirms a local magicity at $Z=28, N=40$. Combining the results of the low-energy spectra of $^{68}$Ni and $^{70}$Zn and their shell-model interpretations, it is interesting to notice that four different shapes (spherical, oblate, prolate and triaxial) are present. Finally, a summed $E2$ strength of only about 150 e$^2$fm$^4$ has been found experimentally at high excitation energy, likely due to proton excitations across the $Z=28$ gap. The experimental distribution of this high-energy $E2$ excitation agrees with SM calculations, but its strength is about two times weaker.

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arXiv2021

Evidence for enhanced neutron-proton correlations from the level structure of the $N=Z+1$ nucleus $^{87}_{43}$Tc$^{\ }_{44}$

The low-lying excited states in the neutron-deficient $N=Z+1$ nucleus $^{87}_{43}$Tc$^{\ }_{44}$ have been studied via the fusion-evaporation reaction $^{54}$Fe($^{36}$Ar, $2n1p$)$^{87}$Tc at the Grand Acc\'el\'erateur National d'Ions Lourds (GANIL), France. The AGATA spectrometer was used in conjunction with the auxiliary NEDA, Neutron Wall, and DIAMANT detector arrays to measure coincident prompt $\gamma$-rays, neutrons, and charged particles emitted in the reaction. A level scheme of $^{87}$Tc from the (9/2$^{+}_{g.s.}$) state to the (33/2$^{+}_{1}$) state was established based on 6 mutually coincident $\gamma$-ray transitions. The constructed level structure exhibits a rotational behavior with a sharp backbending at $\hbar\omega\approx 0.50$ MeV. A decrease in alignment frequency and increase in alignment sharpness in the odd-mass isotonic chains around $N=44$ is proposed as an effect of the enhanced isoscalar neutron-proton interactions in odd-mass nuclei when approaching the $N=Z$ line.

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arXiv2021

Complete set of bound negative-parity states in the neutron-rich 18N nucleus

High-resolution gamma-ray spectroscopy of 18N is performed with the Advanced GAmma Tracking Array AGATA, following deep-inelastic processes induced by an 18O beam on a 181Ta target. Six states are newly identified, which together with the three known excitations exhaust all negative-parity excited states expected in 18N below the neutron threshold. Spin and parities are proposed for all located states on the basis of decay branchings and comparison with large-scale shell-model calculations performed in the p-sd space, with the YSOX interaction. Of particular interest is the location of the 0^-_1 and 1^-_2 excitations, which provide strong constrains for cross-shell p-sd matrix elements based on realistic interactions, and help to simultaneously reproduce the ground and first-excited states in 16N and 18N, for the first time. Understanding the 18N structure may also have significant impact on neutron-capture cross-section calculations in r-process modeling including light neutron-rich nuclei.

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arXiv2020

Accessing tens-to-hundreds femtoseconds nuclear state lifetimes with low-energy binary heavy-ion reactions

A novel Monte Carlo technique has been developed to determine lifetimes of excited states in the tens-to-hundreds femtoseconds range. The method is applied to low-energy heavy-ion binary reactions populating nuclei with complex velocity distributions. Its relevance is demonstrated in connection with the $^{18}$O(7.0 MeV/u) + $^{181}$Ta experiment, performed at GANIL with the AGATA+VAMOS+PARIS setup, to study neutron-rich O, C, N, ... nuclei. Excited states in $^{17}$O and $^{19}$O, with known lifetimes, are used to validate the method over the $\sim$20-400 fs lifetime-sensitivity range. Emphasis is given to the unprecedented position resolution provided by $\gamma$-tracking arrays, which turns out to be essential for reaching the required accuracy in Doppler-shift correction, at the basis of the detailed analysis of $\gamma$-ray lineshape and resulting state lifetime determination. The technique is anticipated to be an important tool for lifetime investigations in exotic neutron-rich nuclei, produced with intense ISOL-type beams.

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arXiv2020

Prompt-delayed $γ$-ray spectroscopy of neutron-rich $^{119,121}$In isotopes

The fusion and transfer induced fission reaction $^{9}$Be($^{238}$U,~f) with 6.2 MeV/u beam energy, using a unique setup consisting of AGATA, VAMOS++ and EXOGAM detectors, was used to populate through the fission process and study the neutron-rich $^{119,121}$In isotopes. This setup enabled the prompt-delayed $γ$-ray spectroscopy of isotopes in the time range of $100~\rm{ns} - 200~μ\rm{s}$. In the odd-$A$ $^{119,121}$In isotopes, indications of a short half-life $19/2^{-}$ isomeric state, in addition to the previously known $25/2^{+}$ isomeric state, were observed from the present data. Further, new prompt transitions above the $25/2^{+}$ isomer in $^{121}$In were identified along with reevaluation of its half-life. The experimental data were compared with the theoretical results obtained in the framework of large-scale shell-model calculations in a restricted model space. The $\langle πg_{9/2} νh_{11/2};I \arrowvert \hat{\mathcal{H}}\arrowvert πg_{9/2} νh_{11/2};I\rangle$ two-body matrix elements of residual interaction were modified to explain the excitation energies and the $B(E2)$ transition probabilities in the neutron-rich In isotopes. The (i) decreasing trend of $E(29/2^{+}) - E(25/2^{+})$ in odd-In (with dominant configuration $πg_{9/2}^{-1}νh_{11/2}^{-2}$ and maximum aligned spin of $29/2^{+}$) and (ii) increasing trend of $E(27/2^{+}) - E(23/2^{+})$ in odd-Sb (with dominant configuration $πg_{7/2}^{+1}νh_{11/2}^{-2}$ and maximum aligned spin of $27/2^{+}$) with increasing neutron number could be understood as a consequence of hole-hole and particle-hole interactions, respectively.

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arXiv2020

Testing ab initio nuclear structure in neutron-rich nuclei: lifetime measurements of second 2+ states in 16C and 20O

To test the predictive power of ab initio nuclear structure theory, the lifetime of the second 2+ state in neutron-rich 20O, tau(2+_2 ) = 150(+80-30) fs, and an estimate for the lifetime of the second 2+ state in 16C have been obtained, for the first time. The results were achieved via a novel Monte Carlo technique that allowed us to measure nuclear state lifetimes in the tens-to-hundreds femtoseconds range, by analyzing the Doppler-shifted gamma-transition line shapes of products of low-energy transfer and deep-inelastic processes in the reaction 18O (7.0 MeV/u) + 181Ta. The requested sensitivity could only be reached owing to the excellent performances of the AGATA gamma-tracking array, coupled to the PARIS scintillator array and to the VAMOS++ magnetic spectrometer. The experimental lifetimes agree with predictions of ab initio calculations using two- and three-nucleon interactions, obtained with the valence-space in-medium similarity renormalization group for 20O, and with the no-core shell model for 16C. The present measurement shows the power of electromagnetic observables, determined with high-precision gamma spectroscopy, to assess the quality of first-principles nuclear structure calculations, complementing common benchmarks based on nuclear energies. The proposed experimental approach will be essential for short lifetimes measurements in unexplored regions of the nuclear chart, including r-process nuclei, when intense ISOL-type beams become available.

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arXiv2019

Effects of one valence proton on seniority and angular momentum of neutrons in neutron-rich $^{122-131}$Sb$_{51}$ isotopes

The neutron-rich $^{122-131}$Sb isotopes were produced as fission fragments in the reaction $^{9}$Be($^{238}$U,~f) with 6.2 MeV/u beam energy. An unique setup, consisting of AGATA, VAMOS++ and EXOGAM detectors, was used which enabled the prompt-delayed gamma-ray ($γ$) spectroscopy of fission fragments in the time range of 100 ns - 200 $μ$s. New isomers, prompt and delayed transitions were established in the even-A $^{122-130}$Sb isotopes. In the odd-A $^{123-131}$Sb isotopes, new prompt and delayed $γ$-ray transitions were identified, in addition to the confirmation of the previously known isomers. The half-lives of the isomeric states and the $B(E2)$ transition probabilities of the observed transitions depopulating these isomers were extracted. The experimental data was compared with the theoretical results obtained in the framework of Large-Scale Shell-Model (LSSM) calculations in a restricted model space. Modifications of several components of the shell model interaction were introduced to obtain a consistent agreement with the excitation energies and the $B(E2)$ transition probabilities in neutron-rich Sn and Sb isotopes. The isomeric configurations in Sn and Sb were found to be relatively pure. Further, the calculations revealed that the presence of a single valence proton, mainly in the $g_{7/2}$ orbital in Sb isotopes, leads to significant mixing (due to the $νπ$ interaction) of: (i) the neutron seniorities ($\upsilon_ν$) and (ii) the neutron angular momentum ($I_ν$). The above features have a weak impact on the excitation energies, but have an important impact on the $B(E2)$ transition probabilities. In addition, a constancy of the relative excitation energies irrespective of neutron seniority and neutron number in Sn and Sb was observed.

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arXiv2019

Pairing-quadrupole interplay in the neutron-deficient tin nuclei: first lifetime measurements of low-lying states in $^{106,108}$Sn

The lifetimes of the low-lying excited states $2^+$ and $4^+$ have been directly measured in the neutron-deficient $^{106,108}$Sn isotopes. The nuclei were populated via a deep-inelastic reaction and the lifetime measurement was performed employing a differential plunger device. The emitted $γ$ rays were detected by the AGATA array, while the reaction products were uniquely identified by the VAMOS++ magnetic spectrometer. Large-Scale Shell-Model calculations with realistic forces indicate that, independently of the pairing content of the interaction, the quadrupole force is dominant in the $B(E2; 2_1^+ \to 0_{g.s.}^+)$ values and it describes well the experimental pattern for $^{104-114}$Sn; the $B(E2; 4_1^+ \to 2_1^+)$ values, measured here for the first time, depend critically on a delicate pairing-quadrupole balance, disclosed by the very precise results in $^{108}$Sn. This result provides insight in the hitherto unexplained $B(E2; 4_1^+ \to 2_1^+)/B(E2; 2_1^+ \to 0_{g.s.}^+) < 1$ anomaly.

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arXiv2017

Pre-equilibrium effects of the hot nuclei de-excitation via GDR emission - theoretical approach

The hot rotating nuclei could be formed in the complete and incomplete fusion reaction of two heavy ions. At low bombarding energies the reaction goes via compound nucleus formation and subsequent evaporation of charged particles, neutrons and $γ$-rays. However, with increasing the energy of the projectile, the emission of particles during the equilibration process becomes more and more probable. This effect can be estimated by the Heavy-Ion Phase-Space Exploration (HIPSE) code which describes the production of clusters of various size from nucleons initially in the target or projectile. This dynamic evolution finalizes with the compound nuclei, quasi-fission or multi-fragmentation products. The hot rotating nuclei produced in fusion reaction can de-excitate by evaporation of particles and emission of $γ$-rays from the Giant Dipole Resonance, or by fission into two fragments. These processes, evaporation and fission, are described within statistical codes such as GEMINI++ or in dynamical approaches by solving the transport equations of Langevin type. In the present article we will concentrate on the possible effect of the pre-equilibrium emission on the strength function of the effective Giant Dipole Resonance, which can be described within Thermal Shape Fluctuation Model (TSFM) approach.

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