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A. Nick Vamivakas

Publications and source records attributed to A. Nick Vamivakas.

At least 19 recordsLinked to original sources

Super-phenomena in arbitrary quantum observables

Superoscillations occur when a globally band-limited function locally oscillates faster than its highest Fourier coefficient. We generalize this effect to arbitrary quantum mechanical operators as a weak value, where the preselected state is a superposition of eigenstates of the operator with eigenvalues bounded to a range, and the postselection state is a local position. Superbehavior of this operator occurs whenever the operator's weak value exceeds its eigenvalue bound. We give illustrative examples of this effect for total angular momentum and energy. In the later case, we demonstrate a sequence of harmonic oscillator potentials where a finite energy state converges everywhere on the real line, using only bounded superpositions of states whose asymptotic energy vanishes - "energy out of nothing". This limit requires postselecting the particle in a region whose size diverges in the considered limit. We further show that superenergy behavior implies that the state superoscillates in time with a rate given by the superenergy divided by the reduced Planck's constant. This example demonstrates the possibility of mimicking a high-energy state with coherent superpositions of nearly zero-energy states for as wide a spatial region as desired. We provide numerical evidence of these features to further bolster and elucidate our claims.

quant-ph↗

Experimental realization of supergrowing fields

Supergrowth refers to the local amplitude growth rate of a signal being faster than its fastest Fourier mode. In contrast, superoscillation pertains to the variation of the phase. Compared to the latter, supergrowth can have exponentially higher intensities and promises improvement over superoscillation-based superresolution imaging. Here, we demonstrate the experimental synthesis of controlled supergrowing fields with a maximum growth rate of ~19.1 times the system-bandlimit. Our work is an essential step toward realizing supergrowth-based far-field superresolution imaging.

physics.optics↗

Supergrowth and sub-wavelength object imaging

We further develop the concept of supergrowth [Jordan, Quantum Stud.: Math. Found. $\textbf{7}$, 285-292 (2020)], a phenomenon complementary to superoscillation, defined as the local amplitude growth rate of a function being higher than its largest wavenumber. We identify the superoscillating and supergrowing regions of a canonical oscillatory function and find the maximum values of local growth rate and wavenumber. Next, we provide a quantitative comparison of lengths and relevant intensities between the superoscillating and the supergrowing regions of a canonical oscillatory function. Our analysis shows that the supergrowing regions contain intensities that are exponentially larger in terms of the highest local wavenumber compared to the superoscillating regions. Finally, we prescribe methods to reconstruct a sub-wavelength object from the imaging data using both superoscillatory and supergrowing point spread functions. Our investigation provides an experimentally preferable alternative to the superoscillation based superresolution schemes and is relevant to cutting-edge research in far-field sub-wavelength imaging.

physics.optics↗

Excited-state spin-resonance spectroscopy of V$_\text{B}^-$ defect centers in hexagonal boron nitride

The recently discovered spin-active boron vacancy (V$_\text{B}^-$) defect center in hexagonal boron nitride (hBN) has high contrast optically-detected magnetic resonance (ODMR) at room-temperature, with a spin-triplet ground-state that shows promise as a quantum sensor. Here we report temperature-dependent ODMR spectroscopy to probe spin within the orbital excited-state. Our experiments determine the excited-state spin Hamiltonian, including a room-temperature zero-field splitting of 2.1 GHz and a g-factor similar to that of the ground-state. We confirm that the resonance is associated with spin rotation in the excited-state using pulsed ODMR measurements, and we observe Zeeman-mediated level anti-crossings in both the orbital ground- and excited-state. Our observation of a single set of excited-state spin-triplet resonance from 10 to 300 K is consistent with an orbital-singlet, which has consequences for understanding the symmetry of this defect. Additionally, the excited-state ODMR has strong temperature dependence of both contrast and transverse anisotropy splitting, enabling promising avenues for quantum sensing.

cond-mat.mtrl-sci↗

The Structure and Dispersion of Exciton-Trion-Polaritons in Two-Dimensional Materials: Experiments and Theory

The nature of trions and their interaction with light has remained a puzzle. The composition and dispersion of polaritons involving trions provide insights into this puzzle. Trions and excitons in doped two-dimensional (2D) materials are not independent excitations but are strongly coupled as a result of Coulomb interactions. When excitons in doped 2D materials are also strongly coupled with light inside an optical waveguide, the resulting polariton states are coherent superpositions of exciton, trion, and photon states. We realize these exciton-trion-polaritons by coupling an electron-doped monolayer of two-dimensional material MoSe2 to the optical mode in a photonic crystal waveguide. Our theoretical model, based on a many-body description of these polaritons, reproduces the measured polariton energy band dispersion and Rabi splittings with excellent accuracy. Our work sheds light on the structure of trion states in 2D matrials and also on the indirect mechanism by which they interact with light.

cond-mat.mes-hall↗

Injection locking of a levitated optomechanical oscillator for precision force sensing

We report on the injection locking of an optically levitated nanomechanical oscillator (a silica nanosphere) to resonant intensity modulations of an external optical signal. We explore the characteristic features of injection locking in this system, e.g. the phase pull-in effect and the injection-induced reduction of the oscillation linewidth. Our measurements are in good agreement with theoretical predictions and deepen the analogy of injection locking in levitated optomechanical systems to that in optical systems (lasers). By measuring the force noise of our feedback cooled free-running oscillator, we attain a force sensitivity of $\sim23~\rm{zN}/\sqrt{\rm{Hz}}$. This can readily allow, in fairly short integration times, for tests of violations of Newtonian gravity and searching for new small-scale forces. As a proof of concept, we show that the injection locking can be exploited to measure the forces optically induced on levitated nanoparticles, with potential applications in explorations of optical binding and entanglement between optically coupled nanomechanical oscillators.

physics.optics↗

Exciton-Trion-Polaritons in Two-Dimensional Materials

We present a many-body theory for exciton-trion-polaritons in doped two-dimensional materials. Exciton-trion-polaritons are robust coherent hybrid excitations involving excitons, trions, and photons. Signatures of these polaritons have been recently seen in experiments. In these polaritons, the 2-body exciton states are coupled to the material ground state via exciton-photon interaction and the 4-body trion states are coupled to the exciton states via Coulomb interaction. The trion states are not directly optically coupled to the material ground state. The energy-momentum dispersion of these polaritons exhibit three bands. We calculate the energy band dispersions and the compositions of polaritons at different doping densities using Green's functions. The energy splittings between the polariton bands, as well as the spectral weights of the polariton bands, depend on the strength of the Coulomb coupling between the excitons and the trions and which in turn depends on the doping density. The excitons are Coulomb coupled to both bound and unbound trion states. The latter are exciton-electron scattering states and their inclusion is necessary to capture the spectral weight transfer among the polariton bands as a function of the doping density.

cond-mat.mes-hall↗

Achieving a quantum smart workforce

Interest in building dedicated Quantum Information Science and Engineering (QISE) education programs has greatly expanded in recent years. These programs are inherently convergent, complex, often resource intensive and likely require collaboration with a broad variety of stakeholders. In order to address this combination of challenges, we have captured ideas from many members in the community. This manuscript not only addresses policy makers and funding agencies (both public and private and from the regional to the international level) but also contains needs identified by industry leaders and discusses the difficulties inherent in creating an inclusive QISE curriculum. We report on the status of eighteen post-secondary education programs in QISE and provide guidance for building new programs. Lastly, we encourage the development of a comprehensive strategic plan for quantum education and workforce development as a means to make the most of the ongoing substantial investments being made in QISE.

physics.ed-ph↗

Solid-state laser refrigeration of nanodiamond quantum sensors

The negatively-charged nitrogen vacancy (NV$^-$) centre in diamond is a remarkable optical quantum sensor for a range of applications including, nanoscale thermometry, magnetometry, single photon generation, quantum computing, and communication. However, to date the performance of these techniques using NV$^-$ centres has been limited by the thermally-induced spectral wandering of NV$^-$ centre photoluminescence due to detrimental photothermal heating. Here we demonstrate that solid-state laser refrigeration can be used to enable rapid (ms) optical temperature control of nitrogen vacancy doped nanodiamond (NV$^-$:ND) quantum sensors in both atmospheric and \textit{in vacuo} conditions. Nanodiamonds are attached to ceramic microcrystals including 10\% ytterbium doped yttrium lithium fluoride (Yb:LiYF$_4$) and sodium yttrium fluoride (Yb:NaYF$_4$) by van der Waals bonding. The fluoride crystals were cooled through the efficient emission of upconverted infrared photons excited by a focused 1020 nm laser beam. Heat transfer to the ceramic microcrystals cooled the adjacent NV$^-$:NDs by 10 and 27 K at atmospheric pressure and $\sim$10$^{-3}$ Torr, respectively. The temperature of the NV$^-$:NDs was measured using both Debye-Waller factor (DWF) thermometry and optically detected magnetic resonance (ODMR), which agree with the temperature of the laser cooled ceramic microcrystal. Stabilization of thermally-induced spectral wandering of the NV$^{-}$ zero-phonon-line (ZPL) is achieved by modulating the 1020 nm laser irradiance. The demonstrated cooling of NV$^-$:NDs using an optically cooled microcrystal opens up new possibilities for rapid feedback-controlled cooling of a wide range of nanoscale quantum materials.

cond-mat.mtrl-sci↗

Spectral and spatial isolation of single WSe$_2$ quantum emitters using hexagonal boron nitride wrinkles

Monolayer WSe$_2$ hosts bright single-photon emitters. Because of its compliance, monolayer WSe$_2$ conforms to patterned substrates without breaking, thus creating the potential for large local strain, which is one activation mechanism of its intrinsic quantum emitters. Here, we report an approach to creating spatially and spectrally isolated quantum emitters from WSe$_2$ monolayers with few or no detrimental sources of emission. We show that a bilayer of hexagonal boron nitride (hBN) and WSe$_2$ placed on a nanostructured substrate can be used to create and shape wrinkles that communicate local strain to the WSe$_2$, thus creating quantum emitters that are isolated from substrate features. We compare quantum emitters created directly on top of substrate features with quantum emitters forming along wrinkles and find that the spectra of the latter consist of mainly a single peak and a low background fluorescence. We also discuss possible approaches to controlling emitter position along hBN wrinkles.

cond-mat.mes-hall↗

Optomechanics with Levitated Particles

Optomechanics is concerned with the use of light to control mechanical objects. As a field, it has been hugely successful in the production of precise and novel sensors, the development of low-dissipation nanomechanical devices, and the manipulation of quantum signals. Micro- and nano-particles levitated in optical fields act as nanoscale oscillators, making them excellent low-dissipation optomechanical objects, with minimal thermal contact to the environment when operating in vacuum. Levitated optomechanics is seen as the most promising route for studying high-mass quantum physics, with the promise of creating macroscopically separated superposition states at masses of $10^6$ amu and above. Optical feedback, both using active monitoring or the passive interaction with an optical cavity, can be used to cool the centre-of-mass of levitated nanoparticles well below 1 mK, paving the way to operation in the quantum regime. In addition, trapped mesoscopic particles are the paradigmatic system for studying nanoscale stochastic processes, and have already demonstrated their utility in state-of-the-art force sensing.

physics.optics↗

Quantum-limited estimation of the axial separation of two incoherent point sources

Improving axial resolution is crucial for three-dimensional optical imaging systems. Here we present a scheme of axial superresolution for two incoherent point sources based on spatial mode demultiplexing. A radial mode sorter is used to losslessly decompose the optical fields into a radial mode basis set to extract the phase information associated with the axial positions of the point sources. We show theoretically and experimentally that, in the limit of a zero axial separation, our scheme allows for reaching the quantum Cramér-Rao lower bound and thus can be considered as one of the optimal measurement methods. Unlike other superresolution schemes, this scheme does not require neither activation of fluorophores nor sophisticated stabilization control. Moreover, it is applicable to the localization of a single point source in the axial direction. Our demonstration can be useful to a variety of applications such as far-field fluorescence microscopy.

physics.optics↗

Influence of Vacuum modes on Photodetection

Photodetection is a process in which an incident field induces a polarization current in the detector. The interaction of the field with this induced current excites an electron in the detector from a localized bound state to a state in which the electron freely propagates and can be classically amplified and detected. The induced current can interact not only with the applied field, but also with all of the initially unpopulated vacuum modes. This interaction with the vacuum modes is assumed to be small and is neglected in conventional photodetection theory. We show that this interaction contributes to the quantum efficiency of the detector. We also show that in the Purcell enhancement regime, shot noise in the photocurrent depends on the bandwidth of the the vacuum modes interacting with the detector. Our theory allows design of sensitive detectors to probe the properties of the vacuum modes.

quant-ph↗

Emerging Connections: Quantum and Classical Optics

Quantum optics and classical optics have coexisted for nearly a century as two distinct, self-consistent descriptions of light. What influences there were between the two domains all tended to go in one direction, as concepts from classical optics were incorporated into quantum theory's early development. But it's becoming increasingly clear that a significant quantum presence exists in classical territory-and, in particular, that the quintessential quantum attribute, entanglement, can be seen, studied and exploited in classical optics. This blurring of the classical-quantum boundary has opened up a potential new direction for frontier work in optics.

physics.optics↗

Basis-neutral Hilbert-space analyzers

Interferometry is one of the central organizing principles of optics. Key to interferometry is the concept of optical delay, which facilitates spectral analysis in terms of time-harmonics. In contrast, when analyzing a beam in a Hilbert space spanned by spatial modes -- a critical task for spatial-mode multiplexing and quantum communication -- basis-specific principles are invoked that are altogether distinct from that of `delay.' Here, we extend the traditional concept of temporal delay to the spatial domain, thereby enabling the analysis of a beam in an arbitrary spatial-mode basis -- exemplified using Hermite-Gaussian and radial Laguerre-Gaussian modes. Such generalized delays correspond to optical implementations of fractional transforms; for example, the fractional Hankel transform is the generalized delay associated with the space of Laguerre-Gaussian modes, and an interferometer incorporating such a `delay' obtains modal weights in the associated Hilbert space. By implementing an inherently stable, reconfigurable spatial-light-modulator-based polarization- interferometer, we have constructed a `Hilbert-space analyzer' capable of projecting optical beams onto any modal basis.

physics.optics↗

Coherence Constraints and the Last Hidden Optical Coherence

We have discovered a new domain of optical coherence, and show that it is the third and last member of a previously unreported fundamental triad of coherences. These are unified by our derivation of a parallel triad of coherence constraints that take the form of complementarity relations. We have been able to enter this new coherence domain experimentally and we describe the novel tomographic approach devised for that purpose.

quant-ph↗

Integrated nanophotonics based on wire plasmons and atomically-thin material

Photonic integrated circuits are an enabling technology in modern communications systems. The continually increasing demands for higher-speed and lower operating power devices have resulted in the continued impetus to shrink photonic components. In this work, we demonstrate a primitive nanophotonic integrated circuit element composed of a single silver nanowire and single-layer molybdenum disulfide (MoS2) flake. We show that nanowire plasmons can excite MoS2 photoluminescence via direct plasmon-to-exciton conversion along the wire and plasmon-to-photon-to-exciton conversion at the MoS2-covered wire end. We also find that the reverse process is possible: MoS2 excitons can decay into nanowire plasmons that can then be routed via the nanowire on-chip. Finally, we demonstrate that the nanowire may serve the dual purpose of both exciting MoS2 photoluminescence via plasmons and recollecting the decaying excitons.

cond-mat.mes-hall↗

Observation of nitrogen vacancy photoluminescence from an optically levitated nanodiamond

We present the first evidence of nitrogen vacancy (NV) photoluminescence from a nanodiamond suspended in a free-space optical dipole trap at atmospheric pressure. The photoluminescence rates are shown to decrease with increasing trap laser power, but are inconsistent with a thermal quenching process. For a continuous-wave trap, the neutral charge state (NV$^0$) appears to be suppressed. Chopping the trap laser yields higher total count rates and results in a mixture of both NV$^0$ and the negative charge state (NV$^-$).

physics.optics↗