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A. O. Macchiavelli

Publications and source records attributed to A. O. Macchiavelli.

At least 19 recordsLinked to original sources

Universal Effective Charges in the $sd$ and $fp$ Shells

The 247-keV state in $^{54}$Sc, populated in the $β$ decay of $^{54}$Ca, is reported here as a nanosecond isomer with a half-life of 26.0(22) ns. The state is interpreted as the $1^+$ member of the $πf_{7/2}\otimesνf_{5/2}$ spin-coupled multiplet, which decays to the $3^+,πf_{7/2} \otimes νp_{1/2}$ ground state. The new half-life corresponds to a pure $E2$ transition with a strength of 1.93(16) W.u., providing the most precise, unambiguous $B(E2)$ value in the neutron-rich $fp$ region to date for a nucleus with valence protons above $Z=20$. Notably, it is roughly four times larger than the $B(E2; 1/2^{-} \rightarrow 5/2^{-})$ value in $^{55}$Ca. The results, as compared to semi-empirical and ab initio shell-model calculations, indicate (1) a weak $N=34$ sub-shell gap relative to $N = 32$, (2) a large $E2$ enhancement in Sc as compared to Ca due to $1p-1h$ proton excitations across $Z=28$, and (3) empirical effective proton and neutron charges, $e_π$ = 1.30(8)$e$ and $e_ν$ = 0.452(7)$e$, respectively, that are in contrast to reports of $e_π\approx 1.1-1.15e$ and $e_ν\approx 0.6-0.8e$ for $fp$-shell nuclei near $N = Z$. We demonstrate that these reports are erroneous and that, in fact, a universal set of effective charges can be used across the $sd$ and $fp$ shells.

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Suppressed Electric Quadrupole Collectivity in $^{49}$Ti

Single-step Coulomb excitation of $^{46,48,49,50}$Ti is presented. A complete set of $E2$ matrix elements for the quintuplet of states in $^{49}$Ti, centered on the $2^+$ core excitation, was measured for the first time. A total of nine $E2$ matrix elements are reported, four of which were previously unknown. $^{49}_{22}$Ti$_{27}$ shows a $20\%$ quenching in electric quadrupole transition strength as compared to its semi-magic $^{50}_{22}$Ti$_{28}$ neighbour. This $20\%$ quenching, while empirically unprecedented, can be explained with a remarkably simple two-state mixing model, which is also consistent with other ground-state properties such as the magnetic dipole moment and electric quadrupole moment. A connection to nucleon transfer data and the quenching of single-particle strength is also demonstrated. The simplicity of the $^{49}$Ti-$^{50}$Ti pair (i.e., approximate single-$j$ $0f_{7/2}$ valence space and isolation of yrast states from non-yrast states) provides a unique opportunity to disentangle otherwise competing effects in the ground-state properties of atomic nuclei, the emergence of collectivity, and the role of proton-neutron interactions.

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Microsecond Isomer at the N=20 Island of Shape Inversion Observed at FRIB

Excited-state spectroscopy from the first Facility for Rare Isotope Beams (FRIB) experiment is reported. A 24(2)-$μ$s isomer was observed with the FRIB Decay Station initiator (FDSi) through a cascade of 224- and 401-keV $γ$ rays in coincidence with $^{32}\textrm{Na}$ nuclei. This is the only known microsecond isomer ($1{\text{ }μ\text{s}}\leq T_{1/2} < 1\text{ ms}$) in the region. This nucleus is at the heart of the $N=20$ island of shape inversion and is at the crossroads of spherical shell-model, deformed shell-model, and ab initio theories. It can be represented as the coupling of a proton hole and neutron particle to $^{32}\textrm{Mg}$, $^{32}\textrm{Mg}+π^{-1} + ν^{+1}$. This odd-odd coupling and isomer formation provides a sensitive measure of the underlying shape degrees of freedom of $^{32}\textrm{Mg}$, where the onset of spherical-to-deformed shape inversion begins with a low-lying deformed $2^+$ state at 885 keV and a low-lying shape-coexisting $0_2^+$ state at 1058 keV. We suggest two possible explanations for the 625-keV isomer in $^{32}$Na: a $6^-$ spherical shape isomer that decays by $E2$ or a $0^+$ deformed spin isomer that decays by $M2$. The present results and calculations are most consistent with the latter, indicating that the low-lying states are dominated by deformation.

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E2 Rotational Invariants of $0^+_1$ and $2^+_1$ states for $^{106}$Cd: the Emergence of Collective Rotation

The collective structure of $^{106}$Cd is elucidated by multi-step Coulomb excitation of a 3.849 MeV/$A$ beam of $^{106}$Cd on a 1.1 mg/cm$^2$ $^{208}$Pb target using GRETINA-CHICO2 at ATLAS. Fourteen $E2$ matrix elements were obtained. The nucleus $^{106}$Cd is a prime example of emergent collectivity that possesses a simple structure: it is free of complexity caused by shape coexistence and has a small, but collectively active number of valence nucleons. This work follows in a long and currently active quest to answer the fundamental question of the origin of nuclear collectivity and deformation, notably in the cadmium isotopes. The results are discussed in terms of phenomenological models, the shell model, and Kumar-Cline sums of $E2$ matrix elements. The ${\langle 0_2^+ ||E2||2_1^+ \rangle}$ matrix element is determined for the first time, providing a total, converged measure of the electric quadrupole strength, $\langle Q^2 \rangle$, of the first-excited $2_1^+$ level relative to the $0_1^+$ ground state, which does not show an increase as expected of harmonic and anharmonic vibrations. Strong evidence for triaxial shapes in weakly collective nuclei is indicated; collective vibrations are excluded. This is contrary to the only other cadmium result of this kind in $^{114}$Cd by C. Fahlander et al., Nucl. Phys. A485, 327 (1988), which is complicated by low-lying shape coexistence near midshell.

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The Core of $^{25}$F studied by the $^{25}$F(-1p)$^{24}$O reaction

The $^{25}$F($5/2^+) (-1p) ^{24}$O reaction was studied at the NSCL using the S800 spectrometer. The experimental spectroscopic factor for the ground-state to ground-state transition indicates a substantial depletion of the proton $d_{5/2}$ strength compared to shell-model expectations. Our result supports the findings reported by Tang \textit{et al.}, from their study of the $(p,2p)$ reaction at RIBF. The overlap between the $^{25}$F and $^{24}$O ground-states is considerably less than anticipated if $^{24}$O acted as a robust and rigid doubly-magic core in $^{25}$F. We interpret the results within the framework of the Particle-Vibration Coupling (PVC) of a $d_{5/2}$ proton coupled to a quadrupole phonon of an effective core. This approach provides a good description of the experimental data by requiring an effective $^{24}$O* core with a phonon energy of $\hbarω_2$= 3.2 MeV, and a $B(E2) ~ 2.7$ W.u., softer and more collective than a bare $^{24}$O. Both the Nilsson deformed mean field and the PVC models appear to capture the properties of the effective core of $^{25}$F, suggesting that the additional proton tends to polarize the free, doubly magic $^{24}$O in such a way that it becomes either slightly deformed or a quadrupole vibrator.

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Quenching of Single-Particle Strength in A=15 Nuclei

Absolute cross sections for the addition of $s$- and $d$-wave neutrons to $^{14}$C and $^{14}$N have been determined simultaneously via the ($d$,$p$) reaction at 10 MeV/u. The difference between the neutron and proton separation energies, $ΔS$, is around $-20$ MeV for the $^{14}$C$+$$n$ system and $+8$ MeV for $^{14}$N$+$$n$. The population of the $1s_{1/2}$ and $0d_{5/2}$ orbitals for both systems is reduced by a factor of approximately 0.5 compared to the independent single-particle model, or about 0.6 when compared to the shell model. This finding strongly contrasts with results deduced from intermediate-energy knockout reactions between similar nuclei on targets of $^{9}$Be and $^{12}$C. The simultaneous technique used removes many systematic uncertainties.

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Weak binding effects on the structure of $^{40}$Mg

While the phenomenon of one- and two-neutron ground-state halo nuclei is well established, the effects of weak binding on nuclear excitation properties remain largely unexplored. Motivated by this question and by recent data in $^{40}$Mg we investigate the coupling of weakly bound (halo) valence neutrons to a core using the known properties of $^{40}$Mg to explore and illustrate possible particle-core coupling schemes and their impact on the low-lying excitation spectrum.

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Structure of $^{43}$P and $^{42}$Si in a two-level shape-coexistence model

Exclusive cross sections for the $^{43}$P$(-1p)^{42}$Si reaction to the lowest $0^+$ and $2^+$ states, measured at NSCL with GRETINA and the S800, are interpreted in terms of a two-level mixing (collective) model of oblate and prolate co-existing shapes. Using the formalism developed for deformed nuclei we calculate the spectroscopic amplitudes and exclusive cross-sections in the strong coupling limit, where for $^{43}$P the schematic wavefunction includes the coupling of the Nilsson [211]$\frac{1}{2}$ proton orbit. Good agreement with the experimental data is obtained when the amplitude of the oblate configuration is $\gtrsim$ 80\%, suggesting that both nuclei are predominantly oblate, in line with theoretical expectations.

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Weisskopf units for neutron-proton pair transfers

We introduce the concept of neutron-proton two-particle units ($np$-Weisskopf units) to be used in the analysis of the ($^3$He,$p)$ and $(p,^3$He) \added{reactions on nuclei} along the N=Z line. These are presented for the conditions relevant to the $(n,j,\ell$) orbits expected from $^{16}$O to $^{100}$Sn. As is the case of the Weisskopf units for electromagnetic transitions, the $np$-WU's will provide a simple, yet robust, measure of isoscalar and isovector $np$ pairing collective effects.

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Shell model analysis of the $ B(E2,2^+ \rightarrow 0^+)$'s in the A=70 T=1 triplet

he $B(E2,2^+ \rightarrow 0^+)$ transition strengths of the T=1 isobaric triplet $^{70}$Kr, $^{70}$Br, $^{70}$Se, recently measured at RIKEN/RIBF, are discussed in terms of state of the art large scale shell model calculations using the JUN45 and JUN45+LNPS plus Coulomb interactions. In this letter we argue that, depending on the effective charges used, the calculations are either in line with the experimental data within statistical uncertainties, or the anomaly happens in $^{70}$Br, rather than $^{70}$Kr. In the latter case, we suggest that it can be due to the presence of a hitherto undetected 1$^+$ T=0 state below the yrast 2$^+$ T=1 state. Our results do not support a shape change of $^{70}$Kr with respect to the other members of the isobaric multiplet.

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Neutron--proton spin--spin correlations in the ground states of N=Z nuclei

We present expressions for the matrix elements of the spin--spin operator $\vec S_{\rm n}\cdot\vec S_{\rm p}$ in a variety of coupling schemes. These results are then applied to calculate the expectation value $\langle\vec S_{\rm n}\cdot\vec S_{\rm p}\rangle$ in eigenstates of a schematic Hamiltonian describing neutrons and protons interacting in a single-$l$ shell through a Surface Delta Interaction. The model allows us to trace $\langle\vec S_{\rm n}\cdot\vec S_{\rm p}\rangle$ as a function of the competition between the isovector and isoscalar interaction strengths and the spin--orbit splitting of the $j=l\pm \frac{1}{2}$ shells. We find negative $\langle\vec S_{\rm n}\cdot\vec S_{\rm p}\rangle$ values in the ground state of all even--even $N=Z$ nuclei, contrary to what has been observed in hadronic inelastic scattering at medium energies. We discuss the possible origin of this discrepancy and indicate directions for future theoretical and experimental studies related to neutron--proton spin--spin correlations.

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Neutron-proton pairing in the N=Z radioactive fp-shell nuclei 56Ni and 52Fe probed by pair transfer

The isovector and isoscalar components of neutron-proton pairing are investigated in the N=Z unstable nuclei of the \textit{fp}-shell through the two-nucleon transfer reaction (p,$^3$He) in inverse kinematics. The combination of particle and gamma-ray detection with radioactive beams of $^{56}$Ni and $^{52}$Fe, produced by fragmentation at the GANIL/LISE facility, made it possible to carry out this study for the first time in a closed and an open-shell nucleus in the \textit{fp}-shell. The transfer cross-sections for ground-state to ground-state (J=0$^+$,T=1) and to the first (J=1$^+$,T=0) state were extracted for both cases together with the transfer cross-section ratios $σ$(0$^+$,T=1) /$σ$(1$^+$,T=0). They are compared with second-order distorted-wave born approximation (DWBA) calculations. The enhancement of the ground-state to ground-state pair transfer cross-section close to mid-shell, in $^{52}$Fe, points towards a superfluid phase in the isovector channel. For the "deuteron-like" transfer, very low cross-sections to the first (J=1$^+$,T=0) state were observed both for \Ni\phe\, and \Fe\phe\, and are related to a strong hindrance of this channel due to spin-orbit effect. No evidence for an isoscalar deuteron-like condensate is observed.

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Search for the $1/2^+$ intruder state in $^{35}$P

The excitation energy of deformed intruder states (specifically the 2p2h bandhead) as a function of proton number $Z$ along $N=20$ is of interest both in terms of better understanding the evolution of nuclear structure between spherical $^{40}$Ca and the Island of Inversion nuclei, and for benchmarking theoretical descriptions in this region. At the center of the $N=20$ Island of Inversion, the npnh (where n=2,4,6) neutron excitations across a diminished $N=20$ gap result in deformed and collective ground states, as observed in $^{32}$Mg. In heavier isotones, npnh excitations do not dominate in the ground states, but are present in the relatively low-lying level schemes. With the aim of identifying the expected 2p2h$\otimes\mathrm{s}_{1/2^+}$ state in $^{35}$P, the only $N=20$ isotone for which the neutron 2p2h excitation bandhead has not yet been identified, the $^{36}$S(d,$^3$He)$^{35}$P reaction has been revisited in inverse kinematics with the HELical Orbit Spectrometer (HELIOS) at the Argonne Tandem Linac Accelerator System (ATLAS). While a candidate state has not been located, an upper limit for the transfer reaction cross-section to populate such a configuration within a 2.5 to 3.6\,MeV energy range, provides a stringent constraint on the wavefunction compositions in both $^{36}$S and $^{35}$P.

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Coriolis coupling effects in proton-pickup spectroscopic factors from $^{12}$B

Spectroscopic factors to low-lying negative-parity states in $^{11}$Be extracted from the $^{12}$B($d$,$^3$He)$^{11}$Be proton-removal reaction are interpreted within the rotational model. Earlier predictions of the $p$-wave proton removal strengths in the strong coupling limit of the Nilsson model underestimated the spectroscopic factors to the $3/2^-_1$ and $5/2^-_1$ states and suggested that deviations in the $1^+$ ground state of the odd-odd $^{12}$B due to Coriolis coupling should be further explored. In this work we use the Particle Rotor Model to take into account these effects and obtain a good description of the level scheme in $^{11}$B, with a moderate $K$-mixing of the proton Nilsson levels [110]1/2 and [101]3/2. This mixing, present in the $1^+$ bandhead of $^{12}$B, is key to explaining the proton pickup data.

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Effects of Magnetic Fields on HPGe Tracking Detectors

We present a study of magnetic fields effects on the position resolution and energy response of hyper-pure germanium detectors. Our results provide realistic estimates of the potential impact on the resolving power of tracking-arrays from (fringe) magnetic fields present when operating together with large spectrometers. By solving the equations of motion for the electron and holes in the presence of both electric and magnetic fields, we analyzed the drift trajectories of the charge carriers to determine the deviations in the positions at the end point of the trajectories, as well as changes in drift lengths affecting the energy resolution and peak shift due to trapping. Our results show that the major effect is in the deviation of the transverse (to the electric field direction) position and suggest that, if no corrective action is taken in the pulse-shape and tracking data analysis procedures, a field strength $\gtrsim$ 0.1 T will start to impact the intrinsic position resolution of 2 mm (RMS). At fields above $\sim$1 T, the degradation of the energy response becomes observable.

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Probing the Z = 6 spin-orbit shell gap with (p,2p) quasi-free scattering reactions

The evolution of the traditional nuclear magic numbers away from the valley of stability is an active field of research. Experimental efforts focus on providing key spectroscopic information that will shed light into the structure of exotic nuclei and understanding the driving mechanism behind the shell evolution. In this work, we investigate the Z = 6 spin-orbit shell gap towards the neutron dripline. To do so, we employed $^{A}$N(p,2p)$^{A-1}$C quasi-free scattering reactions to measure the proton component of the 2$^+_1$ state of $^{16,18,20}$C. The experimental findings support the notion of a moderate reduction of the proton 1p$_{1/2}$-1p$_{3/2}$ spin-orbit splitting, at variance to recent claims for a prevalent Z = 6 magic number towards the neutron dripline.

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Nucleon-nucleon correlations and the single-particle strength in atomic nuclei

We propose a phenomenological approach to examine the role of short- and long-range nucleon-nucleon correlations in the quenching of single-particle strength in atomic nuclei and their evolution in asymmetric nuclei and neutron matter. These correlations are thought to be the reason for the quenching of spectroscopic factors observed in $\rm (e,e'p)$, $\rm (p,2p)$ and transfer reactions. We show that the recently observed increase of the high-momentum component of the protons in neutron-rich nuclei is consistent with the reduced proton spectroscopic factors. Our approach connects recent results on short-range correlations from high-energy electron scattering experiments with the quenching of spectroscopic factors and addresses for the first time quantitatively this intriguing question in nuclear physics, in particular regarding its isospin dependence. We also speculate about the nature of a {\sl quasi-proton} (nuclear polaron) in neutron matter and its kinetic energy, an important quantity for the properties of neutron stars.

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Global trends of nuclear $d_{5/2}^{2,3,4}$ configurations: Application of a simple effective-interaction model

With new experimental information on nuclei far from stability being available, a systematic investigation of excitation energies and electromagnetic properties along the $N=10, 11, 12$ isotones and $Z=10, 11, 12$ isotopes is presented. The experimental data are discussed in the context of the appearance and disappearance of shell closures at $N=Z=8,14,16,20$, and compared to an effective-interaction approach applied to neutrons and protons in $d_{5/2}^{2,3,4}$ configurations. In spite of its simplicity the model is able to explain the observed properties.

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