arXiv subjects

A. P. Jones

Publications and source records attributed to A. P. Jones.

At least 19 recordsLinked to original sources

arXiv2026

Seeding grain nucleation and dust growth: Ionisation, epoxidation and charge disproportionation effects

This work studies the likely dust seeding processes arising from alkali metal and alkaline earth ionisation, epoxidation (epoxide bond formation via oxygen atom insertion into C=C bonds), and grain charge disproportionation (the existence around the uncharged state of oxidised cationic and reduced anionic states) at (sub-)nanometre size scales. The chemical, physical, and photon-initiated processes leading to dust seeding are explored within the framework of the size-dependent physical, optical, and photoelectric properties of the THEMIS carbonaceous nanoparticles. The critical grain charge states at (sub-)nanometre size scales are derived as a function of the interstellar and circumstellar physical conditions. Photo-initiated low-energy ionisation, epoxide reactions, and disproportionation-driven electrostatic effects could play key roles in seeding dust nucleation and growth. The size-dependent seed cluster and nanograin charge distribution is shown to encompass both positive and negative charges where the ionisation is driven by low ionisation metals or by weak attenuation. Cluster seeding via ionisation and epoxidation could help to explain the co-spatial and contemporaneous nucleation and growth of both carbon-rich and oxygen-rich dust in the same regions. This may be enhanced by electrostatic effects, driven by charge disproportionation, between negatively-charged, nucleation-seeding, polyatomic clusters and positively-charged ions or larger (nano)particles. Such processes could occur in the dust-forming regions in novae, Wolf-Rayet, and Luminous Blue Variable systems and electrostatic effects may also aid the accretion of nanoparticles in the outer regions of molecular clouds.

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arXiv2026

Spatially-resolved interstellar dust properties in the face-on spiral galaxy M 99 as observed by NIKA2

Large dust grains in thermal equilibrium dominate the far-infrared and contribute to the millimetre continuum of star-forming galaxies, but constraining their properties is difficult due to free-free and synchrotron contamination. We study spatial variations in the dust spectral index, mass, and grain properties in the nearby face-on spiral galaxy M 99. We use new 1.15 and 2 mm continuum observations from NIKA2 on the IRAM 30 m telescope (IMEGIN Guaranteed Time Large Programme) combined with multiwavelength data from UV to radio. The infrared-to-radio SED is decomposed into dust, free-free, and synchrotron components using the hierarchical Bayesian code HerBIE. Dust is modelled via a modified blackbody (MBB) with variable millimetre spectral index beta and the THEMIS dust model with fixed beta. We perform spatially-resolved analysis at scales ~1.75 kpc (~25''), covering the centre, spiral arms, and inter-arm regions. MBB fits reveal beta variations from ~1.6-1.7 in diffuse regions to ~2.3-2.5 in dense star-forming areas, likely due to grain coagulation and changes in silicate-to-carbonaceous ratios. Dust masses from variable beta are up to ~4x higher than fixed-beta models, which systematically bias dust-to-stellar and dust-to-gas ratios. The small grain fraction rises from ~10% in the centre to ~15% in the diffuse disc, anti-correlated with the interstellar radiation field; gas-phase metallicity plays a minor role within 8 kpc. Synchrotron spectral index ranges from ~0.6-0.7 in star-forming regions to ~1.2 in the diffuse medium, consistent with cosmic-ray electron ageing.

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arXiv2026

Resolved ISM properties and scaling relations in the barred galaxy NGC 3627: constraints from NIKA2 observations

We investigate the interplay between star formation, interstellar medium (ISM) components, and dust properties in NGC 3627 using new NIKA2 1.15 and 2 mm observations from the IMEGIN Large Program. Our goal is to analyze dust and radio emission, decompose contributions in the millimeter-centimeter regime, and explore ISM properties within the galaxy. We perform spectral energy distribution fitting, at both global and spatial scales, using the THEMIS dust model within the HerBIE code, applied to data from 3.4 $μ$m to 6 cm. We decompose emission into dust, free-free, and synchrotron components, and examine correlations with gas surface density and star formation activity. Additionally, we analyze the small dust grain fraction and its variation across the galaxy. We find $\sim$10% radio emission at 2 mm, peaking at 18% in the southern bar-end, which hosts the highest star formation activity. However, an isolated star-forming region beyond this bar-end is the most efficient, as indicated by its elevated dust production efficiency and effective yield, predicted by our simplistic dust evolution model. The 160 $μ$m emission shows the strongest correlation with molecular gas, while 1.15 mm better traces the dust mass surface density. Small grains, which make up $\sim$13% of dust mass (2 $\times$ 10$^{7}$ M$_{\odot}$), are depleted in intense radiation fields, with a notable deficit in the southern tidal tail. ISM properties and chemical evolution indicate that dynamical processes, such as bar-driven gas flows and tidal interactions, are crucial in shaping the galactic structure, influencing star formation efficiency, and dust distribution.

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arXiv2025

The essential elements of dust evolution: a-C(:H) nanoparticle sub-structures and photo-fragmentation

Hydrogenated amorphous carbon materials, a-C(:H), are heterogeneous structures consisting of carbon atoms in different hybridisation states and bonding configurations and are thought to constitute a significant and observationally important fraction of the interstellar dust material. This work aims to characterise semi-conducting a-C(:H) nanoparticle structures and, in particular, their property-characterising aromatic domain size distribution and so predict how they will behave in intense UV radiation fields that can fragment them through dissociative and charge effects as a result of carbon-carbon bond-breaking. Using a statistical approach we determine the typical sizes of the aromatic domains, their size distribution, how they are network-bonded, and where they are to be found within the structure. We consider the effects of thermal excitation, photo-dissociation and charging of a-C(:H) nanoparticles, and the products of their fragmentation. The derived UV photon-induced fragmentation lifetimes for nanometre-sized a-C(:H) nanoparticles, with radii ~0.4-0.5nm radius and containing ~40-60 carbon atoms, are of the order of 10^6-10^7yr in the diffuse interstellar medium and likely 10^2-10^4 times shorter in photodissociation regions, depending on the local radiation field intensity. Grains larger than this are stable against photodissociation. In H{\footnotesize II} regions only a-C(:H) nanoparticles with radii greater than 0.7nm (> 150 carbon atoms) are likely to survive. The photon-driven fragmentation of sub-nanometre a-C(:H) particles was determined to be important in the diffuse interstellar medium and also in high excitation regions, such as photodissociation and HII regions. However, in these same regions Coulomb fragmentation is unlikely to be an important dust destruction process.

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arXiv2025

Quantum confinement and carbon nanodots: A conceptual view for the origin of diffuse interstellar bands

The nature of the Diffuse Interstellar Band (DIB) carriers is perhaps the most studied, longest standing, unresolved problem in astronomy. While four bands have been associated with the fullerene cation (C^+_60) the vast majority (> 550) remain unidentified. This works is an attempt to provide a conceptual framework for the typical energy transitions that are central to explaining the origin of DIBs, however, it does not make an association between these transitions and any particular DIBs. The effect of quantum confinement on excitons is used, including charge transfer excitons, to construct a generic basis for the electronic transitions that could, in principle, be coherent with the energies associated with DIBs. In this model the carriers are carbon nanodots (CNDs) modelled as nanodiamonds and a-C(:H) nanoparticles. These preliminary results seem to show that particle size dependent effects in nanodiamond and a-C(:H) CNDs could be consistent with the positions of, and intervals between, some of the DIBs. One particular strength of the model is that predicts single bands from the majority of single-size particles and, at most, two bands from some of these same carriers. In the latter case the two bands come from different transitions and may or may not inter-correlate, depending upon the local environment. This generic framework indicates that the size dependent fundamental transitions in CNDs could provide a viable scenario for the origin of some DIB-type bands. While this work does not identify a single DIB, it furnishes a conceptual view for the DIB origin, and suggests that a more refined exploration of quantum confinement size effects, and exciton physics within the astronomical domain might prove fruitful. This work also hints at the requirement for stable configurations for particular size domains in order to explain DIB wavelength stability.

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arXiv2024

Interpreting Millimeter Emission from IMEGIN galaxies NGC 2146 and NGC 2976

The millimeter continuum emission from galaxies provides important information about cold dust, its distribution, heating, and role in their InterStellar Medium (ISM). This emission also carries an unknown portion of the free-free and synchrotron radiation. The IRAM 30m Guaranteed Time Large Project, Interpreting Millimeter Emission of Galaxies with IRAM and NIKA2 (IMEGIN) provides a unique opportunity to study the origin of the millimeter emission on angular resolutions of <18" in a sample of nearby galaxies. As a pilot study, we present millimeter observations of two IMEGIN galaxies, NGC 2146 (starburst) and NGC 2976 (peculiar dwarf) at 1.15 mm and 2 mm. Combined with the data taken with Spitzer, Herschel, Plank, WSRT, and the 100m Effelsberg telescopes, we model the infrared-to-radio Spectral Energy Distribution (SED) of these galaxies, both globally and at resolved scales, using a Bayesian approach to 1) dissect different components of the millimeter emission, 2) investigate the physical properties of dust, and 3) explore correlations between millimeter emission, gas, and Star Formation Rate (SFR). We find that cold dust is responsible for most of the 1.15 mm emission in both galaxies and at 2 mm in NGC 2976. The free-free emission emits more importantly in NGC 2146 at 2 mm. The cold dust emissivity index is flatter in the dwarf galaxy ($β= 1.3\pm 0.1$) compared to the starburst galaxy ($β= 1.7\pm 0.1$). Mapping the dust-to-gas ratio, we find that it changes between 0.004 and 0.01 with a mean of $0.006\pm0.001$ in the dwarf galaxy. In addition, no global balance holds between the formation and dissociation of H$_2$ in this galaxy. We find tight correlations between the millimeter emission and both the SFR and molecular gas mass in both galaxies.

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arXiv2023

IAS/CEA Evolution of Dust in Nearby Galaxies (ICED): the spatially-resolved dust properties of NGC4254

We present the first preliminary results of the project \textit{ICED}, focusing on the face-on galaxy NGC4254. We use the millimetre maps observed with NIKA2 at IRAM-30m, as part of the IMEGIN Guaranteed Time Large Program, and of a wide collection of ancillary data (multi-wavelength photometry and gas phase spectral lines) that are publicly available. We derive the global and local properties of interstellar dust grains through infrared-to-radio spectral energy distribution fitting, using the hierarchical Bayesian code HerBIE, which includes the grain properties of the state-of-the-art dust model, THEMIS. Our method allows us to get the following dust parameters: dust mass, average interstellar radiation field, and fraction of small grains. Also, it is effective in retrieving the intrinsic correlations between dust parameters and interstellar medium properties. We find an evident anti-correlation between the interstellar radiation field and the fraction of small grains in the centre of NGC4254, meaning that, at strong radiation field intensities, very small amorphous carbon grains are efficiently destroyed by the ultra-violet photons coming from newly formed stars, through photo-desorption and sublimation. We observe a flattening of the anti-correlation at larger radial distances, which may be driven by the steep metallicity gradient measured in NGC4254.

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arXiv2023

Exploring the interstellar medium of NGC 891 at millimeter wavelengths using the NIKA2 camera

In the framework of the IMEGIN Large Program, we used the NIKA2 camera on the IRAM 30-m telescope to observe the edge-on galaxy NGC 891 at 1.15 mm and 2 mm and at a FWHM of 11.1" and 17.6", respectively. Multiwavelength data enriched with the new NIKA2 observations fitted by the HerBIE SED code (coupled with the THEMIS dust model) were used to constrain the physical properties of the ISM. Emission originating from the diffuse dust disk is detected at all wavelengths from mid-IR to mm, while mid-IR observations reveal warm dust emission from compact HII regions. Indications of mm excess emission have also been found in the outer parts of the galactic disk. Furthermore, our SED fitting analysis constrained the mass fraction of the small (< 15 Angstrom) dust grains. We found that small grains constitute 9.5% of the total dust mass in the galactic plane, but this fraction increases up to ~ 20% at large distances (|z| > 3 kpc) from the galactic plane.

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arXiv2023

Constraining Millimeter Dust Emission in Nearby Galaxies with NIKA2: the case of NGC2146 and NGC2976

This study presents the first millimeter continuum mapping observations of two nearby galaxies, the starburst spiral galaxy NGC2146 and the dwarf galaxy NGC2976, at 1.15 mm and 2 mm using the NIKA2 camera on the IRAM 30m telescope, as part of the Guaranteed Time Large Project IMEGIN. These observations provide robust resolved information about the physical properties of dust in nearby galaxies by constraining their FIR-radio SED in the millimeter domain. After subtracting the contribution from the CO line emission, the SEDs are modeled spatially using a Bayesian approach. Maps of dust mass surface density, temperature, emissivity index, and thermal radio component of the galaxies are presented, allowing for a study of the relations between the dust properties and star formation activity (using observations at 24$μ$m as a tracer). We report that dust temperature is correlated with star formation rate in both galaxies. The effect of star formation activity on dust temperature is stronger in NGC2976, an indication of the thinner interstellar medium of dwarf galaxies. Moreover, an anti-correlation trend is reported between the dust emissivity index and temperature in both galaxies.

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arXiv2023

The stratification of ISM properties in the edge-on galaxy NGC 891 revealed by NIKA2

As the millimeter wavelength range remains a largely unexplored spectral region for galaxies, the IMEGIN large program aims to map the millimeter continuum emission of 22 nearby galaxies at 1.15 and 2 mm. Using the high-resolution maps produced by the NIKA2 camera, we explore the existence of very cold dust and take possible contamination by free-free and synchrotron emission into account. We study the IR-to-radio emission coming from different regions along the galactic plane and at large vertical distances. New observations of NGC 891, using the NIKA2 camera on the IRAM 30m telescope, along with a suite of observations at other wavelengths were used to perform a multiwavelength study of the spectral energy distribution in the interstellar medium in this galaxy. This analysis was performed globally and locally, using the advanced hierarchical Bayesian fitting code, HerBIE, coupled with the THEMIS dust model. Our dust modeling is able to reproduce the near-IR to millimeter emission of NGC 891, with the exception of an excess at a level of 25% obtained by the NIKA2 observations in the outermost parts of the disk. The radio continuum and thermal dust emission are distributed differently in the disk and galaxy halo. Different dusty environments are also revealed by a multiwavelength investigation of the emission features. Our detailed decomposition at millimeter and centimeter wavelengths shows that emission at 1 mm is purely originated by dust. Radio components become progressively important with increasing wavelengths. Finally, we find that emission arising from small dust grains accounts for ~ 9.5% of the total dust mass, reaching up to 20% at large galactic latitudes. Shock waves in the outflows that shatter the dust grains might explain this higher fraction of small grains in the halo.

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arXiv2022

Low-temperature optical constants of amorphous silicate dust analogues

Cosmic dust models are key ingredients in advancing our understanding of astronomical environments as diverse as interstellar clouds in galaxies, circumstellar envelopes around evolved and young stars, and protoplanetary disks. Such models consist of several dust populations, each with different compositions and size distributions. They may also consider different grain shapes, although most models assume spherical grains. All include a component of silicate dust. The absorption and emission properties of these dust components are calculated from the optical constants of each dust material which have various experimental, phenomenological, and theoretical origins depending on the model. We aim to provide the community with new sets of optical constants for amorphous silicate dust analogues at low temperatures. The analogues consist of four Mg-rich silicate samples of stoichiometry ranging from enstatite to olivine, and of eight samples of Mg and Fe rich silicates with a pyroxene stoichiometry and differing magnesium and iron content. We calculated the optical constants from transmission measurements using the Kramers-Kronig relations, assuming that the grains are small compared to the wavelength and prolate in shape with axis ratios of 1.5 and 2 for the Mg and Fe rich samples, respectively. New optical constants for silicate dust analogues were calculated over the wavelength range from 5 to 800-1000 microns, depending on the sample, and at temperatures of 10, 30, 100, 200, and 300 K.We determined the uncertainties on the derived optical constants based on the assumptions used to calculate them. To facilitate the use of these data in cosmic dust models, we provide optical constants extrapolated outside the measured spectral range into the UV-NIR and mm-cm wavelength ranges, as well as formulae that can be used to interpolate them at any temperature in the range 10 - 300 K.

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arXiv2022

Nano-grain depletion in photon-dominated regions

Context. Carbonaceous nano-grains play a fundamental role in the physico-chemistry of the interstellar medium (ISM) and especially of photon-dominated regions (PDRs). Their properties vary with the local physical conditions and affect the local chemistry and dynamics. Aims. We aim to highlight the evolution of carbonaceous nano-grains in three different PDRs and propose a scenario of dust evolution as a response to the physical conditions. Methods. We used Spitzer/IRAC (3.6, 4.5, 5.8, and 8 $μ$m) and Spitzer/MIPS (24 $μ$m) together with Herschel/PACS (70 $μ$m) to map dust emission in IC63 and the Orion Bar. To assess the dust properties, we modelled the dust emission in these regions using the radiative transfer code SOC together with the THEMIS dust model. Results. Regardless of the PDR, we find that nano-grains are depleted and that their minimum size is larger than in the diffuse ISM (DISM), which suggests that the mechanisms that lead nano-grains to be photo-destroyed are very efficient below a given critical size limit. The evolution of the nano-grain dust-to-gas mass ratio with both G0 and the effective temperature of the illuminating star indicates a competition between the nano-grain formation through the fragmentation of larger grains and nano-grain photo-destruction. We modelled dust collisions driven by radiative pressure with a classical 1D approach to show that this is a viable scenario for explaining nano-grain formation through fragmentation and, thus, the variations observed in nano-grain dust-to-gas mass ratios from one PDR to another. Conclusions. We find a broad variation in the nano-grain dust properties from one PDR to another, along with a general trend of nano-grain depletion in these regions. We propose a viable scenario of nano-grain formation through fragmentation of large grains due to radiative pressure-induced collisions.

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arXiv2022

The Interstellar dust properties of nearby galaxies

This article gives an overview of the constitution, physical conditions and observables of dust in the interstellar medium of nearby galaxies. We first review the macroscopic, spatial distribution of dust in these objects, and its consequence on our ability to study grain physics. We also discuss the possibility to use dust tracers as diagnostic tools. We then survey our current understanding of the microscopic, intrinsic properties of dust in different environments, derived from different observables: emission, extinction, polarization, depletions, over the whole electromagnetic spectrum. Finally, we summarize the clues of grain evolution, evidenced either on local scales or over cosmic time. We put in perspective the different evolution scenarios. We attempt a comprehensive presentation of the main observational constraints, analysis methods and modelling frameworks of the distinct processes. We do not cover the dust properties of the Milky Way and distant galaxies, nor circumstellar or active galactic nucleus torus dust.

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arXiv2022

Dust emissivity in resolved spiral galaxies

Context: The far-infrared (FIR) and sub-millimeter (submm) emissivity of the Milky Way (MW) cirrus is an important benchmark for dust grain models. Dust masses in other galaxies are generally derived from the FIR/submm using the emission properties of these MW-calibrated models. Aims: We seek to derive the FIR/submm emissivity in nine nearby spiral galaxies to check its compatibility with MW cirrus measurements. Methods: We obtained values of the emissivity at 70 to 500 um, using maps of dust emission from the Herschel satellite and of gas surface density from the THINGS and HERACLES surveys on a scale generally corresponding to 440 pc. We studied the variation of the emissivity with the surface brightness ratio I(250um)/I(500um), a proxy for the intensity of the interstellar radiation field heating the dust. Results: We find that the average value of the emissivity agrees with MW estimates for pixels sharing the same color as the cirrus, namely, for I(250um)/I(500um) = 4.5. For I(250um)/I(500um) > 5, the measured emissivity is instead up to a factor ~2 lower than predicted from MW dust models heated by stronger radiation fields. Regions with higher I(250um)/I(500um) are preferentially closer to the galactic center and have a higher overall (stellar+gas) surface density and molecular fraction. The results do not depend strongly on the adopted CO-to-molecular conversion factor and do not appear to be affected by the mixing of heating conditions. Conclusions: Our results confirm the validity of MW dust models at low density, but are at odds with predictions for grain evolution in higher density environments. If the lower-than-expected emissivity at high I(250um)/I(500um) is the result of intrinsic variations in the dust properties, it would imply an underestimation of the dust mass surface density of up to a factor ~2 when using current dust models.

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arXiv2022

Searching for Anomalous Microwave Emission in nearby galaxies. K-band observations with the Sardinia Radio Telescope

We observed four nearby spiral galaxies (NGC 3627, NGC 4254, NGC 4736 and NGC 5055) in the K band with the 64-m Sardinia Radio Telescope, with the aim of detecting the Anomalous Microwave Emission (AME), a radiation component presumably due to spinning dust grains, observed so far in the Milky Way and in a handful of other galaxies only (most notably, M 31). We mapped the galaxies at 18.6 and 24.6 GHz and studied their global photometry together with other radio-continuum data from the literature, in order to find AME as emission in excess of the synchrotron and thermal components. We only find upper limits for AME. These non-detections, and other upper limits in the literature, are nevertheless consistent with the average AME emissivity from the few detections: it is $ε^\mathrm{AME}_{\mathrm{30~GHz}} = 2.4\pm0.4 \times 10^{-2}$ MJy sr$^{-1}$ (M$_\odot$ pc$^{-2}$)$^{-1}$ in units of dust surface density (equivalently, $1.4\pm0.2 \times 10^{-18}$ Jy sr$^{-1}$ (H cm$^{-2}$)$^{-1}$ in units of H column density). We finally suggest to search for AME in quiescent spirals with relatively low radio luminosity, such as M~31.

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arXiv2021

Dust evolution, a global view: I. Nano-particles, nascence, nitrogen and natural selection . . . joining the dots

The role and importance of nano-particles for interstellar chemistry and beyond is explored within the framework of The Heterogeneous dust Evolution Model at the IaS (THEMIS), focussing on their active surface chemistry (nascence), the effects of nitrogen doping and the natural selection of interesting nano-particle sub-structures. Nano-particle driven chemistry, and in particular the role of intrinsic epoxide-type structures could provide a viable route to the observed gas phase OH in tenuous interstellar clouds en route to becoming molecular clouds. The aromatic-rich moieties present in asphaltenes likely provide a viable model for the structures present within aromatic-rich interstellar carbonaceous grains. The observed doping of such nano-particle structures with nitrogen, if also prevalent in interstellar dust, is likely to have important and observable consequences for surface chemistry and the formation of pre-cursor pre-biotic species.

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arXiv2021

Dust evolution, a global view: II. Top-down branching, nano-particle fragmentation and the mystery of the diffuse interstellar band carriers

The origin of the diffuse interstellar bands is one of the longest-standing mysteries of the interstellar medium is explored within the framework of The Heterogeneous dust Evolution Model at the IaS (THEMIS). The likely nature of the diffuse interstellar band carriers and their evolution is here explored within the framework of the structures and sub-structures inherent to doped hydrogenated amorphous carbon grains in the interstellar medium. Based on the natural aromatic-rich moieties (ashphaltenes) recovered from coal and oil the likely structure of their interstellar analogues is investigated within the context of the diffuse band problem. It is here proposed that the top- down evolution of interstellar carbonaceous grains, and in particular a-C(:H) nano-particles, is at the heart of the formation and evolution of the diffuse interstellar band carriers and their associations with small molecules and radicals such as C2, C3, CH and CN. It is most likely that the diffuse interstellar bands are carried by dehydrogenated, ionised, hetero- cyclic, aromatic rich moieties that form an integral part of the contiguous structure of hetero-atom doped hydrogenated amorphous carbon nano-particles and their daughter fragmentation products.

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arXiv2021

Dust evolution, a global view: III. Core/mantle grains, organic nano-globules, comets and surface chemistry

Within the framework of The Heterogeneous dust Evolution Model at the IaS (THEMIS) this work investigates in detail the surface processes and chemistry relating to core/mantle interstellar and cometary grain structures and its influence on the nature of these fascinating particles. It appears that a realistic consideration of the nature and chemical reactivity of interstellar grain surfaces could self-consistently and within a coherent framework explain: the anomalous oxygen depletion, the nature of the CO dark gas, the formation of 'polar ice' mantles, the red wing on the 3 um water ice band, the basis for the O-rich chemistry observed in hot cores, the origin of organic nano-globules and the \sim 3.2 um 'carbonyl' absorption band observed in comet reflectance spectra. It is proposed that the reaction of gas phase species with carbonaceous a- C(:H) grain surfaces in the interstellar medium, in particular the incorporation of atomic oxygen into grain surfaces in epoxide functional groups, is the key to explaining these observations. Thus, the chemistry of cosmic dust is much more intimately related with that of the interstellar gas than has previously been considered. The current models for interstellar gas and dust chemistry will therefore most likely need to be fundamentally modified to include these new grain surface processes.

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