arXiv subjects

A. Principi

Publications and source records attributed to A. Principi.

34 records · Page 2Linked to original sources

arXiv2020

Control of electron-electron interaction in graphene by proximity screening

Electron-electron interactions play a critical role in many condensed matter phenomena, and it is tempting to find a way to control them by changing the interactions' strength. One possible approach is to place a studied system in proximity of a metal, which induces additional screening and hence suppresses electron interactions. Here, using devices with atomically-thin gate dielectrics and atomically-flat metallic gates, we measure the electron-electron scattering length in graphene and report qualitative deviations from the standard behavior. The changes induced by screening become important only at gate dielectric thicknesses of a few nm, much smaller than a typical separation between electrons. Our theoretical analysis agrees well with the scattering rates extracted from measurements of electron viscosity in monolayer graphene and of umklapp electron-electron scattering in graphene superlattices. The results provide a guidance for future attempts to achieve proximity screening of many-body phenomena in two-dimensional systems.

cond-mat.mes-hall↗

arXiv2019

Magic-angle bilayer graphene nano-calorimeters -- towards broadband, energy-resolving single photon detection

Because of the ultra-low photon energies in the mid-infrared and terahertz frequencies, in these bands photodetectors are notoriously underdeveloped, and broadband single photon detectors (SPDs) are non-existent. Advanced SPDs exploit thermal effects in nano-structured superconductors, and their performance is currently limited to the more energetic near-infrared photons due to their high electronic heat capacity. Here, we demonstrate a superconducting magic-angle twisted bilayer graphene (MAG) device that is capable of detecting single photons of ultra-low energies by utilizing its record-low heat capacity and sharp superconducting transition. We theoretically quantify its calorimetric photoresponse and estimate its detection limits. This device allows the detection of ultra-broad range single photons from the visible to sub-THz with response time around 4 ns and energy resolution better than 1 THz. These attributes position MAG as an excep-tional material for long-wavelength single photon sensing, which could revolutionize such disparate fields as quantum information processing and radio astronomy.

cond-mat.supr-con↗

arXiv2018

Resonant Terahertz Detection Using Graphene Plasmons

Plasmons, collective oscillations of electron systems, can efficiently couple light and electric current, and thus can be used to create sub-wavelength photodetectors, radiation mixers, and on-chip spectrometers. Despite considerable effort, it has proven challenging to implement plasmonic devices operating at terahertz frequencies. The material capable to meet this challenge is graphene as it supports long-lived electrically-tunable plasmons. Here we demonstrate plasmon-assisted resonant detection of terahertz radiation by antenna-coupled graphene transistors that act as both plasmonic Fabry-Perot cavities and rectifying elements. By varying the plasmon velocity using gate voltage, we tune our detectors between multiple resonant modes and exploit this functionality to measure plasmon wavelength and lifetime in bilayer graphene as well as to probe collective modes in its moiré minibands. Our devices offer a convenient tool for further plasmonic research that is often exceedingly difficult under non-ambient conditions (e.g. cryogenic temperatures and strong magnetic fields) and promise a viable route for various photonic applications.

cond-mat.mes-hall↗

arXiv2018

Measuring Hall Viscosity of Graphene's Electron Fluid

Materials subjected to a magnetic field exhibit the Hall effect, a phenomenon studied and understood in fine detail. Here we report a qualitative breach of this classical behavior in electron systems with high viscosity. The viscous fluid in graphene is found to respond to non-quantizing magnetic fields by producing an electric field opposite to that generated by the classical Hall effect. The viscous contribution is large and identified by studying local voltages that arise in the vicinity of current-injecting contacts. We analyze the anomaly over a wide range of temperatures and carrier densities and extract the Hall viscosity, a dissipationless transport coefficient that was long identified theoretically but remained elusive in experiment. Good agreement with theory suggests further opportunities for studying electron magnetohydrodynamics.

cond-mat.mes-hall↗

arXiv2018

Dual Origin of Room Temperature Sub-Terahertz Photoresponse in Graphene Field Effect Transistors

Graphene is considered as a promising platform for detectors of high-frequency radiation up to the terahertz (THz) range due to graphene$'$s superior electron mobility. Previously it has been shown that graphene field effect transistors (FETs) exhibit room temperature broadband photoresponse to incoming THz radiation thanks to the thermoelectric and/or plasma wave rectification. Both effects exhibit similar functional dependences on the gate voltage and therefore it was found to be difficult to disentangle these contributions in the previous studies. In this letter, we report on combined experimental and theoretical studies of sub-THz response in graphene field-effect transistors analyzed at different temperatures. This temperature-dependent study allowed us to reveal the role of photo-thermoelectric effect, p-n junction rectification, and plasmonic rectification in the sub-THz photoresponse of graphene FETs.

cond-mat.mes-hall↗

arXiv2017

Out-of-plane heat transfer in van der Waals stacks: electron-hyperbolic phonon coupling

Van der Waals heterostructures have emerged as promising building blocks that offer access to new physics, novel device functionalities, and superior electrical and optoelectronic properties. Applications such as thermal management, photodetection, light emission, data communication, high-speed electronics and light harvesting require a thorough understanding of (nanoscale) heat flow. Here, using time-resolved photocurrent measurements we identify an efficient out-of-plane energy transfer channel, where charge carriers in graphene couple to hyperbolic phonon polaritons in the encapsulating layered material. This hyperbolic cooling is particularly efficient, giving picosecond cooling times, for hexagonal BN, where the high-momentum hyperbolic phonon polaritons enable efficient near-field energy transfer. We study this heat transfer mechanism through distinct control knobs to vary carrier density and lattice temperature, and find excellent agreement with theory without any adjustable parameters. These insights may lead to the ability to control heat flow in van der Waals heterostructures.

cond-mat.mes-hall↗

arXiv2017

Superballistic flow of viscous electron fluid through graphene constrictions

Electron-electron (e-e) collisions can impact transport in a variety of surprising and sometimes counterintuitive ways. Despite strong interest, experiments on the subject proved challenging because of the simultaneous presence of different scattering mechanisms that suppress or obscure consequences of e-e scattering. Only recently, sufficiently clean electron systems with transport dominated by e-e collisions have become available, showing behavior characteristic of highly viscous fluids. Here we study electron transport through graphene constrictions and show that their conductance below 150 K increases with increasing temperature, in stark contrast to the metallic character of doped graphene. Notably, the measured conductance exceeds the maximum conductance possible for free electrons. This anomalous behavior is attributed to collective movement of interacting electrons, which 'shields' individual carriers from momentum loss at sample boundaries. The measurements allow us to identify the conductance contribution arising due to electron viscosity and determine its temperature dependence. Besides fundamental interest, our work shows that viscous effects can facilitate high-mobility transport at elevated temperatures, a potentially useful behavior for designing graphene-based devices.

cond-mat.mes-hall↗

arXiv2016

Negative local resistance caused by viscous electron backflow in graphene

Graphene hosts a unique electron system in which electron-phonon scattering is extremely weak but electron-electron collisions are sufficiently frequent to provide local equilibrium above liquid nitrogen temperature. Under these conditions, electrons can behave as a viscous liquid and exhibit hydrodynamic phenomena similar to classical liquids. Here we report strong evidence for this transport regime. We find that doped graphene exhibits an anomalous (negative) voltage drop near current injection contacts, which is attributed to the formation of submicrometer-size whirlpools in the electron flow. The viscosity of graphene's electron liquid is found to be ~0.1 m$^2$ /s, an order of magnitude larger than that of honey, in agreement with many-body theory. Our work shows a possibility to study electron hydrodynamics using high quality graphene.

cond-mat.str-el↗

arXiv2014

Luttinger-field approach to thermoelectric transport in nanoscale conductors

Thermoelectric transport in nanoscale conductors is analyzed in terms of the response of the system to a thermo-mechanical field, first introduced by Luttinger, which couples to the electronic energy density. While in this approach the temperature remains spatially uniform, we show that a spatially varying thermo-mechanical field effectively simulates a temperature gradient across the system and allows us to calculate the electric and thermal currents that flow due to the thermo-mechanical field. In particular, we show that, in the long-time limit, the currents thus calculated reduce to those that one obtains from the Landauer-Büttiker formula, suitably generalized to allow for different temperatures in the reservoirs, if the thermo-mechanical field is applied to prepare the system, and subsequently turned off at ${t=0}$. Alternatively, we can drive the system out of equilibrium by switching the thermo-mechanical field after the initial preparation. We compare these two scenarios, employing a model noninteracting Hamiltonian, in the linear regime, in which they coincide, and in the nonlinear regime in which they show marked differences. We also show how an operationally defined local effective temperature can be computed within this formalism.

cond-mat.mes-hall↗

arXiv2014

Violation of the Wiedemann-Franz law in clean graphene layers

The Wiedemann-Franz law, connecting the electronic thermal conductivity to the electrical conductivity of a disordered metal, is generally found to be well satisfied even when electron-electron (e-e) interactions are strong. In ultra-clean conductors, however, large deviations from the standard form of the law are expected, due to the fact that e-e interactions affect the two conductivities in radically different ways. Thus, the standard Wiedemann-Franz ratio between the thermal and the electric conductivity is reduced by a factor $1+τ/τ_{\rm th}^{\rm ee}$, where $1/τ$ is the momentum relaxation rate, and $1/τ_{\rm th}^{\rm ee}$ is the relaxation time of the thermal current due to e-e collisions. Here we study the density and temperature dependence of $1/τ_{\rm th}^{\rm ee}$ in the important case of doped, clean single layers of graphene, which exhibit record-high thermal conductivities. We show that at low temperature $1/τ_{\rm th}^{\rm ee}$ is $8/5$ of the quasiparticle decay rate. We also show that the many-body renormalization of the thermal Drude weight coincides with that of the Fermi velocity.

cond-mat.mes-hall↗

arXiv2012

Theory of Coulomb drag for massless Dirac fermions

Coulomb drag between two unhybridized graphene sheets separated by a dielectric spacer has recently attracted considerable theoretical interest. We first review, for the sake of completeness, the main analytical results which have been obtained by other authors. We then illustrate pedagogically the minimal theory of Coulomb drag between two spatially-separated two-dimensional systems of massless Dirac fermions which are both away from the charge-neutrality point. This relies on second-order perturbation theory in the screened interlayer interaction and on Boltzmann transport theory. In this theoretical framework and in the low-temperature limit, we demonstrate that, to leading (i.e. quadratic) order in temperature, the drag transresistivity is completely insensitive to the precise intralayer momentum-relaxation mechanism (i.e. to the functional dependence of the scattering time on energy). We also provide analytical results for the low-temperature drag transresistivity for both cases of "thick" and "thin" spacers and for arbitrary values of the dielectric constants of the media surrounding the two Dirac-fermion layers. Finally, we present numerical results for the low-temperature drag transresistivity in the case in which one of the media surrounding the Dirac-fermion layers has a frequency-dependent dielectric constant. We conclude by suggesting an experiment that can potentially allow for the observation of departures from the canonical Fermi-liquid quadratic-in-temperature behavior of the transresistivity.

cond-mat.str-el↗

arXiv2011

The tunneling density-of-states of interacting massless Dirac fermions

We calculate the tunneling density-of-states (DOS) of a disorder-free two-dimensional interacting electron system with a massless-Dirac band Hamiltonian. The DOS exhibits two main features: i) linear growth at large energies with a slope that is suppressed by quasiparticle velocity enhancement, and ii) a rich structure of plasmaron peaks which appear at negative bias voltages in an n-doped sample and at positive bias voltages in a p-doped sample. We predict that the DOS at the Dirac point is non-zero even in the absence of disorder because of electron-electron interactions, and that it is then accurately proportional to the Fermi energy. The finite background DOS observed at the Dirac point of graphene sheets and topological insulator surfaces can therefore be an interaction effect rather than a disorder effect.

cond-mat.mes-hall↗

arXiv2011

Acoustic plasmons and "soundarons" in graphene on a metal gate

We demonstrate that single-layer graphene in the presence of a metal gate displays a gapless collective (plasmon) mode that has a linear dispersion at long wavelengths. We calculate exactly the acoustic-plasmon group velocity at the level of the random phase approximation and carry out microscopic calculations of the one-body spectral function of such system. Despite screening exerted by the metal, we find that graphene's quasiparticle spectrum displays a very rich structure characterized by composite hole-acoustic plasmon satellite bands (that we term for brevity "soundarons"), which can be observed by e.g. angle-resolved photoemission spectroscopy.

cond-mat.mes-hall↗

arXiv2011

Drude weight, plasmon dispersion, and a.c. conductivity in doped graphene sheets

We demonstrate that the plasmon frequency and Drude weight of the electron liquid in a doped graphene sheet are strongly renormalized by electron-electron interactions even in the long-wavelength limit. This effect is not captured by the Random Phase Approximation (RPA), commonly used to describe electron fluids and is due to coupling between the center of mass motion and the pseudospin degree of freedom of the graphene's massless Dirac fermions. Making use of diagrammatic perturbation theory to first order in the electron-electron interaction, we show that this coupling enhances both the plasmon frequency and the Drude weight relative to the RPA value. We also show that interactions are responsible for a significant enhancement of the optical conductivity at frequencies just above the absorption threshold. Our predictions can be checked by far-infrared spectroscopy or inelastic light scattering.

cond-mat.mes-hall↗

arXiv2010

Many-body orbital paramagnetism in doped graphene sheets

The orbital magnetic susceptibility (OMS) of a gas of noninteracting massless Dirac fermions is zero when the Fermi energy is away from the Dirac point. Making use of diagrammatic perturbation theory, we calculate exactly the OMS of massless Dirac fermions to first order in the Coulomb interaction demonstrating that it is finite and positive. Doped graphene sheets are thus unique systems in which the OMS is completely controlled by many-body effects.

cond-mat.mes-hall↗

arXiv2009

Linear response of doped graphene sheets to vector potentials

A two-dimensional gas of massless Dirac fermions (MDFs) is a very useful model to describe low-energy electrons in monolayer graphene. Because the MDF current operator is directly proportional to the (sublattice) pseudospin operator, the MDF current-current response function, which describes the response to a vector potential, happens to coincide with the pseudospin-pseudospin response function. In this work we present analytical results for the wavevector- and frequency-dependent longitudinal and transverse pseudospin-pseudospin response functions of noninteracting MDFs. The transverse response in the static limit is then used to calculate the noninteracting orbital magnetic susceptibility. These results are a starting point for the construction of approximate pseudospin-pseudospin response functions that would take into account electron-electron interactions (for example at the random-phase-approximation level). They also constitute a very useful input for future applications of current-density-functional theory to graphene sheets subjected to time- and spatially-varying vector potentials.

cond-mat.str-el↗