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A. Ratkiewicz

Publications and source records attributed to A. Ratkiewicz.

At least 19 recordsLinked to original sources

Statistical properties of $^{133}$Xe and the $^{132}$Xe$(n,\gamma)$ cross section

$^{133}$Xe is an interesting case for plasma physics to explore nuclear excitation by electron capture, as the process can be studied using statistical properties of $^{133}$Xe. In this work we present results on $^{133}$Xe from the inverse-Oslo method where we extract the nuclear level density and the $\gamma$-strength function, which is used to calculate the (n,$\gamma$) cross section on $^{132}$Xe. The $\gamma$-strength function of $^{133}$Xe can constrain the estimated decay rate from nuclear excitation by electron capture. The $\mathrm{d}(^{132}\mathrm{Xe},\mathrm{p})^{132}\mathrm{Xe}$ reaction was used to create the compound nucleus $^{133}$Xe, which was recorded with an annular particle telescope and a scintillator array consisting of \la and BGO-shielded HPGe Clover detectors. With the inverse-Oslo method, it is possible to study nuclei that are impossible or unable to manufacture targets from, short lived isotopes, or as in this work, noble gases. We present the extracted nuclear level density, and $\gamma$-strength function for $^{133}$Xe, along with shell-model calculations of the statistical properties of $^{133}$Xe. These are the first statistical properties extracted below 6 MeV for any xenon isotope. We constrain the $^{132}$Xe(n,$\gamma$) $^{133}$Xe cross section and reaction rate using the TALYS reaction code.

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Abrasion-fission reactions at intermediate energies

The availability of high-intensity, heavy-ion beams coupled to sensitive, large solid-angleacceptance spectrometers has enabled a detailed examination of the fission fragments produced in induced-fission reactions. The abrasion-fission process involves the formation of projectile-like prefragments in violent nuclear collisions at relative energies in excess of 100 MeV/u. At intermediate energies below this threshold, experiments suggest a change in the prefragment kinematic qualities. Information regarding the influence of this transitional phase upon the evolution of nuclei approaching the point of scission is scarce. In this article, data are presented for over 200 nuclei from nickel to palladium produced in abrasion-fission reactions of a 80 MeV/u 238U beam. Cross sections were obtained following yield measurements performed for the principal charge states of the identified fission fragments and a detailed analysis of the ion transmission. A full kinematic analysis of the fission fragments has been performed using the LISE++ software package, where the trajectory of an ion passing through a spectrometer can be reconstructed based upon measurements at the focal plane. The results obtained at the S800 spectrograph are compared with predictions obtained with a three-fission progenitor (3EER) model. Systematic studies of fission-fragment properties continue to provide a valuable experimental benchmark for theoretical efforts directed toward describing this complex decay channel, that is important in the context of planning experiments to explore the neutron-rich region of the nuclear chart at rare-isotope beam facilities.

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Executive Summary of the Topical Program: Nuclear Isomers in the Era of FRIB

We report on the Facility for Rare Isotope Beams (FRIB) Theory Alliance topical program "Nuclear Isomers in the Era of FRIB". We outline the many ways isomers influence and contribute to nuclear science and technology, especially in the four FRIB pillars: properties of rare isotopes, nuclear astrophysics, fundamental symmetries, and applications for the nation and society. We conclude with a resolution stating our recommendation that the nuclear physics community actively pursue isomer research. A white paper is forthcoming.

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Neutron transfer reactions on the ground state and isomeric state of a 130Sn beam

The structure of nuclei around the neutron-rich nucleus 132Sn is of particular interest due to the vicinity of the Z = 50 and N = 82 shell closures and the r-process nucleosynthetic path. Four states in 131Sn with a strong single-particle-like component have previously been studied via the (d,p) reaction, with limited excitation energy resolution. The 130Sn(9Be,8Be)131Sn and 130Sn(13C,12C)131Sn single-neutron transfer reactions were performed in inverse kinematics at the Holifield Radioactive Ion Beam Facility using particle-gamma coincidence spectroscopy. The uncertainties in the energies of the single-particle-like states have been reduced by more than an order of magnitude using the energies of gamma rays. The previous tentative Jpi values have been confirmed. Decays from high-spin states in 131Sn have been observed following transfer on the isomeric component of the 130Sn beam. The improved energies and confirmed spin-parities of the p-wave states important to the r-process lead to direct-semidirect cross-sections for neutron capture on the ground state of 130Sn at 30 keV that are in agreement with previous analyses. A similar assessment of the impact of neutron-transfer on the isomer would require significant nuclear structure and reaction theory input. There are few measurements of transfer reaction on isomers, and this is the first on an isomer in the 132Sn region.

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Experimental identification of the $T = 1$, $J^{\pi} = 6^+$ state of $^{54}$Co and isospin symmetry in $A = 54$ studied via one-nucleon knockout reactions

New experimental data obtained from $\gamma$-ray tagged one-neutron and one-proton knockout from $^{55}$Co is presented. A candidate for the sought-after $T=1, T_z = 0, J^{\pi} = 6^+$ state in $^{54}$Co is proposed based on a comparison to the new data on $^{54}$Fe, the corresponding observables predicted by large-scale-shell-model (LSSM) calculations in the full $fp$-model space employing charge-dependent contributions, and isospin-symmetry arguments. Furthermore, possible isospin-symmetry breaking in the $A=54$, $T=1$ triplet is studied by calculating the experimental $c$ coefficients of the isobaric mass multiplet equation (IMME) up to the maximum possible spin $J=6$ expected for the $(1f_{7/2})^{-2}$ two-hole configuration relative to the doubly-magic nucleus $^{56}$Ni. The experimental quantities are compared to the theoretically predicted $c$ coefficients from LSSM calculations using two-body matrix elements obtained from a realistic chiral effective field theory potential at next-to-next-to-next-to-leading order (N$^3$LO).

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One-proton and one-neutron knockout reactions from $N = Z = 28$ $^{56}$Ni to the $A = 55$ mirror pair $^{55}$Co and $^{55}$Ni

We present a high-resolution in-beam $\gamma$-ray spectroscopy study of excited states in the mirror nuclei $^{55}$Co and $^{55}$Ni following one-nucleon knockout from a projectile beam of $^{56}$Ni. The newly determined partial cross sections and the $\gamma$-decay properties of excited states provide a test of state-of-the-art nuclear structure models and probe mirror symmetry in unique ways. A mirror asymmetry for the partial cross sections leading to the two lowest $3/2^-$ states in the $A = 55$ mirror pair was identified as well as a significant difference in the $E1$ decays from the $1/2^+_1$ state to the same two $3/2^-$ states. The mirror asymmetry in the partial cross sections cannot be reconciled with the present shell-model picture or small mixing introduced in a two-state model. The observed mirror asymmetry in the $E1$ decay pattern, however, points at stronger mixing between the two lowest $3/2^-$ states in $^{55}$Co than in its mirror $^{55}$Ni.

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New $γ$-ray Transitions Observed in $^{19}$Ne with Implications for the $^{15}$O($α$,$γ$)$^{19}$Ne Reaction Rate

The $^{15}$O($α$,$γ$)$^{19}$Ne reaction is responsible for breakout from the hot CNO cycle in Type I x-ray bursts. Understanding the properties of resonances between $E_x = 4$ and 5 MeV in $^{19}$Ne is crucial in the calculation of this reaction rate. The spins and parities of these states are well known, with the exception of the 4.14- and 4.20-MeV states, which have adopted spin-parities of 9/2$^-$ and 7/2$^-$, respectively. Gamma-ray transitions from these states were studied using triton-$γ$-$γ$ coincidences from the $^{19}$F($^{3}$He,$tγ$)$^{19}$Ne reaction measured with GODDESS (Gammasphere ORRUBA Dual Detectors for Experimental Structure Studies) at Argonne National Laboratory. The observed transitions from the 4.14- and 4.20-MeV states provide strong evidence that the $J^π$ values are actually 7/2$^-$ and 9/2$^-$, respectively. These assignments are consistent with the values in the $^{19}$F mirror nucleus and in contrast to previously accepted assignments.

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Key $^{19}$Ne states identified affecting $γ$-ray emission from $^{18}$F in novae

Detection of nuclear-decay $γ$ rays provides a sensitive thermometer of nova nucleosynthesis. The most intense $γ$-ray flux is thought to be annihilation radiation from the $β^+$ decay of $^{18}$F, which is destroyed prior to decay by the $^{18}$F($p$,$α$)$^{15}$O reaction. Estimates of $^{18}$F production had been uncertain, however, because key near-threshold levels in the compound nucleus, $^{19}$Ne, had yet to be identified. This Letter reports the first measurement of the $^{19}$F($^{3}$He,$tγ$)$^{19}$Ne reaction, in which the placement of two long-sought 3/2$^+$ levels is suggested via triton-$γ$-$γ$ coincidences. The precise determination of their resonance energies reduces the upper limit of the rate by a factor of $1.5-17$ at nova temperatures and reduces the average uncertainty on the nova detection probability by a factor of 2.1.

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Towards Neutron Capture on Exotic Nuclei: Demonstrating $(d,pγ)$ as a Surrogate Reaction for $(n,γ)$

The neutron-capture reaction plays a critical role in the synthesis of the elements in stars and is important for societal applications including nuclear power generation and stockpile-stewardship science. However, it is difficult - if not impossible - to directly measure neutron capture cross sections for the exotic, short-lived nuclei that participate in these processes. In this Letter we demonstrate a new technique which can be used to indirectly determine neutron-capture cross sections for exotic systems. This technique makes use of the $(d,p)$ transfer reaction, which has long been used as a tool to study the structure of nuclei. Recent advances in reaction theory, together with data collected using this reaction, enable the determination of neutron-capture cross sections for short-lived nuclei. A benchmark study of the $^{95}$Mo$(d,p)$ reaction is presented, which illustrates the approach and provides guidance for future applications of the method with short-lived isotopes produced at rare isotope accelerators.

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Recent direct reaction experimental studies with radioactive tin beams

Direct reaction techniques are powerful tools to study the single-particle nature of nuclei. Performing direct reactions on short-lived nuclei requires radioactive ion beams produced either via fragmentation or the Isotope Separation OnLine (ISOL) method. Some of the most interesting regions to study with direct reactions are close to the magic numbers where changes in shell structure can be tracked. These changes can impact the final abundances of explosive nucleosynthesis. The structure of the chain of tin isotopes is strongly influenced by the Z=50 proton shell closure, as well as the neutron shell closures lying in the neutron-rich, N=82, and neutron-deficient, N=50, regions. Here we present two examples of direct reactions on exotic tin isotopes. The first uses a one-neutron transfer reaction and a low-energy reaccelerated ISOL beam to study states in 131Sn from across the N=82 shell closure. The second example utilizes a one-neutron knockout reaction on fragmentation beams of neutron-deficient 106,108Sn. In both cases, measurements of gamma rays in coincidence with charged particles proved to be invaluable.

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$^{24}$Mg($p$, $\alpha$)$^{21}$Na reaction study for spectroscopy of $^{21}$Na

The $^{24}$Mg($p$, $\alpha$)$^{21}$Na reaction was measured at the Holifield Radioactive Ion Beam Facility at Oak Ridge National Laboratory in order to better constrain spins and parities of energy levels in $^{21}$Na for the astrophysically important $^{17}$F($\alpha, p$)$^{20}$Ne reaction rate calculation. 31 MeV proton beams from the 25-MV tandem accelerator and enriched $^{24}$Mg solid targets were used. Recoiling $^{4}$He particles from the $^{24}$Mg($p$, $\alpha$)$^{21}$Na reaction were detected by a highly segmented silicon detector array which measured the yields of $^{4}$He particles over a range of angles simultaneously. A new level at 6661 $\pm$ 5 keV was observed in the present work. The extracted angular distributions for the first four levels of $^{21}$Na and Distorted Wave Born Approximation (DWBA) calculations were compared to verify and extract angular momentum transfer.

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Elastic breakup cross sections of well-bound nucleons

The 9Be(28Mg,27Na) one-proton removal reaction with a large proton separation energy of Sp(28Mg)=16.79 MeV is studied at intermediate beam energy. Coincidences of the bound 27Na residues with protons and other light charged particles are measured. These data are analyzed to determine the percentage contributions to the proton removal cross section from the elastic and inelastic nucleon removal mechanisms. These deduced contributions are compared with the eikonal reaction model predictions and with the previously measured data for reactions involving the re- moval of more weakly-bound protons from lighter nuclei. The role of transitions of the proton between different bound single-particle configurations upon the elastic breakup cross section is also quantified in this well-bound case. The measured and calculated elastic breakup fractions are found to be in good agreement.

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Mirror Energy Differences at Large Isospin Studied through Direct Two-Nucleon Knockout

The first spectroscopy of excited states in 52Ni (Tz=2) and 51Co (Tz=-3/2) has been obtained using the highly selective two-neutron knockout reaction. Mirror energy differences between isobaric analogue states in these nuclei and their mirror partners are interpreted in terms of isospin nonconserving effects. A comparison between large scale shell-model calculations and data provides the most compelling evidence to date that both electromagnetic and an additional isospin nonconserving interactions for J=2 couplings, of unknown origin, are required to obtain good agreement.

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Correlations in intermediate-energy two-proton removal reactions

We report final-state-exclusive measurements of the light charged fragments in coincidence with 26Ne residual nuclei following the direct two-proton removal from a neutron-rich 28Mg secondary beam. A Dalitz-plot analysis and comparisons with simulations show that a majority of the triple- coincidence events with two protons display phase-space correlations consistent with the (two-body) kinematics of a spatially-correlated pair-removal mechanism. The fraction of such correlated events, 56(12) %, is consistent with the fraction of the calculated cross section, 64 %, arising from spin S = 0 two-proton configurations in the entrance-channel (shell-model) 28Mg ground state wave function. This result promises access to an additional and more specific probe of the spin and spatial correlations of valence nucleon pairs in exotic nuclei produced as fast secondary beams.

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Probing elastic and inelastic breakup contributions to intermediate-energy two-proton removal reactions

The two-proton removal reaction from 28Mg projectiles has been studied at 93 MeV/u at the NSCL. First coincidence measurements of the heavy 26Ne projectile residues, the removed protons and other light charged particles enabled the relative cross sections from each of the three possible elastic and inelastic proton removal mechanisms to be determined. These more final-state-exclusive measurements are key for further interrogation of these reaction mechanisms and use of the reaction channel for quantitative spectroscopy of very neutron-rich nuclei. The relative and absolute yields of the three contributing mechanisms are compared to reaction model expectations - based on the use of eikonal dynamics and sd-shell-model structure amplitudes.

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Observation of mutually enhanced collectivity in self-conjugate $^{76}_{38}$Sr$_{38}$

The lifetimes of the first 2$^{+}$ states in the neutron-deficient $^{76,78}$Sr isotopes were measured using a unique combination of the $γ$-ray line-shape method and two-step nucleon exchange reactions at intermediate energies. The transition rates for the 2$^{+}$ states were determined to be $B$(E2;2$^{+}$$\to 0^{+}$) = 2220(270) e$^{2}$fm$^{4}$ for $^{76}$Sr and 1800(250) e$^{2}$fm$^{4}$ for $^{78}$Sr, corresponding to large deformation of $β_2$ = 0.45(3) for $^{76}$Sr and 0.40(3) for $^{78}$Sr. The present data provide experimental evidence for mutually enhanced collectivity that occurs at $N$ = $Z$ = 38. The systematic behavior of the excitation energies and $B$(E2) values indicates a signature of shape coexistence in $^{76}$Sr, characterizing $^{76}$Sr as one of most deformed nuclei with an unusually reduced $E$(4$^{+}$)/$E$(2$^{+}$) ratio.

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Quadrupole collectivity beyond N=28: Intermediate-energy Coulomb excitation of 47,48Ar

We report on the first experimental study of quadrupole collectivity in the very neutron-rich nuclei \nuc{47,48}{Ar} using intermediate-energy Coulomb excitation. These nuclei are located along the path from doubly-magic Ca to collective S and Si isotopes, a critical region of shell evolution and structural change. The deduced $B(E2)$ transition strengths are confronted with large-scale shell-model calculations in the $sdpf$ shell using the state-of-the-art SDPF-U and EPQQM effective interactions. The comparison between experiment and theory indicates that a shell-model description of Ar isotopes around N=28 remains a challenge.

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Intermediate-energy inverse-kinematics one-proton pickup reactions on neutron-deficient $fp$-shell nuclei

Background: Thick-target-induced nucleon-adding transfer reactions onto energetic rare-isotope beams are an emerging spectroscopic tool. Their sensitivity to single-particle structure complements one-nucleon removal reaction capabilities in the quest to reveal the evolution of nuclear shell structure in very exotic nuclei. Purpose: To add intermediate-energy, carbon-target-induced one-proton pickup reactions to the arsenal of $γ$-ray tagged direct reactions applicable in the regime of low beam intensities and to apply these for the first time to $fp$-shell nuclei. Methods: Inclusive and partial cross sections were measured for the $\nuc{12}{C}(\nuc{48}{Cr},\nuc{49}{Mn}+γ)$X and $\nuc{12}{C}(\nuc{50}{Fe},\nuc{51}{Co}+γ)$X proton pickup reactions at 56.7 and 61.2 MeV/nucleon, respectively, using coincident particle-$γ$ spectroscopy at the NSCL. The results are compared to reaction theory calculations using $fp$-shell-model nuclear structure input. For comparison with our previous work, the same reactions were measured on \nuc{9}{Be} targets. Results: The measured partial cross sections confirm the specific population pattern predicted by theory, with pickup into high-$\ell$ orbitals being strongly favored; driven by linear and angular momentum matching. Conclusion: Carbon target-induced pickup reactions are well-suited, in the regime of modest beam intensity, to study the evolution of nuclear structure, with specific sensitivities that are well described by theory.

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