arXiv subjects

A. Romanenko

Publications and source records attributed to A. Romanenko.

At least 37 records · Page 2Linked to original sources

arXiv2019

Ultra-Low Surface Resistance via Vacuum Heat Treatment of Superconducting Radiofrequency Cavities

We report on an effort to improve the performance of superconducting radiofrequency cavities by the use of heat treatment in a temperature range sufficient to dissociate the natural surface oxide. We find that the residual resistance is significantly decreased, and we find an unexpected reduction in the BCS resistance. Together these result in extremely high quality factor values at relatively large accelerating fields Eacc ~20 MV/m: Q0 of 3-4x10^11 at <1.5 K and Q0 ~5x10^10 at 2.0 K. In one cavity, measurements of surface resistance versus temperature showed an extremely small residual resistance of just 0.63+/-0.06 nOhms at 16 MV/m. SIMS measurements confirm that the oxide was significantly dissociated, but they also show the presence of nitrogen after heat treatment. We also present studies of surface oxidation via exposure to air and to water, as well as the effects of very light surface removal via HF rinse. The possibilities for applications and the planned future development are discussed.

physics.acc-ph↗

arXiv2019

Achievement of Ultra-High Quality Factor in Prototype Cryomodule for LCLS-II

Quality factor is a primary cost driver for high energy, continuous wave (CW) SRF linacs like the LCLS-II X-ray free electron laser currently under construction. Taking this into account, several innovations were introduced in the LCLS-II cryomodule design to push substantially beyond the previous state-of-the-art quality factor achieved in operation. This includes the first ever implementation of the nitrogen doping cavity treatment, the capability to provide high mass flow cooldown to improve expulsion of magnetic flux based on recent R&D, high performance magnetic shielding, and other critical subcomponents. To evaluate the implementation of these new cryomodule features, two prototype cryomodules were produced. In this paper, we present results from the prototype cryomodule assembled at Fermilab, which achieved unprecedented cavity quality factors of 3.0e10 at a nominal cryomodule voltage. We overview cavity performance, procedures to achieve ambient magnetic field < 5 mG at the cavity wall, and the successful demonstration of high mass flow cooldown in a cryomodule. The cavity performance under various cool down conditions are presented as well to show the impact of flux expulsion on Q0.

physics.acc-ph↗

arXiv2018

Accelerating fields up to 49 MV/m in TESLA-shape superconducting RF niobium cavities via 75C vacuum bake

In this paper we present the discovery of a new surface treatment applied to superconducting radio frequency (SRF) niobium cavities, leading to unprecedented accelerating fields of 49 MV/m in TESLA-shaped cavities, in continuous wave (CW); the corresponding peak magnetic fields are the highest ever measured in CW, about 210 mT. For TESLA-shape cavities the maximum quench field ever achieved was ~45 MV/m - reached very rarely- with most typical values being below 40 MV/m. These values are reached for niobium surfaces treated with electropolishing followed by the so called mild bake, a 120C vacuum bake (for 48 hours for fine grain and 24 hours for large grain surfaces). We discover that the addition during the mild bake of a step at 75C for few hours, before the 120C, increases systematically the quench fields up to unprecedented values of 49 MV/m. The significance of the result lays not only in the relative improvement, but in the proof that niobium surfaces can sustain and exceed CW radio frequency magnetic fields much larger than Hc1, pointing to an extrinsic nature of the current field limitations, and therefore to the potential to reach accelerating fields well beyond the current state of the art.

physics.acc-ph↗

arXiv2018

Insight into bulk niobium superconducting RF cavities performances by tunneling spectroscopy

Point contact tunneling (PCT) spectroscopy measurements are reported over wide areas of cm-sized cut outs from niobium superconducting RF cavities. A comparison is made between a high-quality, conventionally processed (CP) cavity with a high field Q drop for acceleration field E $>$ 20 MV/m and a nitrogen doped (N-doped) cavity that exhibits an increasing Q up to fields approaching 15 MV/m. The CP cavity displays hot spot regions at high RF fields where Q-drop occurs as well as unaffected regions (cold spots). PCT data on cold spots reveals a near ideal BCS density of states (DOS) with gap parameters, $Δ$ as high as 1.62 meV, that are among the highest values ever reported for Nb. Hot spot regions exhibit a wide distribution of gap values down to $Δ\sim$ 1.0 meV and DOS broadening characterized by a relatively large value of pair-breaking rate, $Γ$, indicating surface regions of significantly reduced superconductivity. In addition, hot spots commonly exhibit Kondo tunneling peaks indicative of surface magnetic moments attributed to a defective oxide. N-doped cavities reveal a more homoegeneous gap distribution centered at $Δ\sim$ 1.5 meV and relatively small values of $Γ/Δ$. The absence of regions of significantly reduced superconductivity indicates that the N interstitials are playing an important role in preventing the formation of hydride phases and other macroscopic defects which might otherwise severely affect the local, surface superconductivity that lead to hot spot formation. The N-doped cavities also display a significantly improved surface oxide, i.e., increased thickness and tunnel barrier height, compared to CP cavities. These results help explain the improved performance of N-doped cavities and give insights into the origin of the initial increasing Q with RF amplitude.

cond-mat.supr-con↗

arXiv2018

The Effect of Mechanical Cold Work on the Magnetic Flux Expulsion of Niobium

Expulsion of ambient flux has been shown to be crucial to obtain high quality factors in bulk niobium SRF cavities. However, there remain many questions as to what properties of the niobium material determine its flux expulsion behavior. In this paper, we present first results from a new study of two cavities that were specially fabricated to study flux expulsion. Both cavities were made from large grain ingot niobium slices, one of which had its slices rolled prior to fabrication, and none these slices were annealed prior to measurement. Expulsion measurements indicate that a dense network of grain boundaries is not necessary for a cavity to have near-complete flux trapping behavior up to large thermal gradients. The results also contribute to a body of evidence that cold work is a strong determinant of flux expulsion behavior in SRF-grade niobium.

physics.acc-ph↗

arXiv2017

Understanding Quality Factor Degradation in Superconducting Niobium Cavities at Low Microwave Field Amplitudes

In niobium superconducting radio frequency (SRF) accelerating cavities a decrease of the quality factor at lower fields - a so called \emph{low field Q slope or LFQS} - has been a long-standing unexplained effect. By extending the high $Q$ measurement techniques to ultralow fields we discover two previously unknown features of the effect: i) saturation at rf fields lower than $E_\mathrm{acc} \sim 0.1$~MV/m; ii) strong degradation enhancement by growing thicker niobium pentoxide. Our findings suggest that the LFQS may be caused by the two level systems in the natural niobium oxide on the inner cavity surface, thereby identifying a new source of residual resistance and providing guidance for potential non-accelerator low field applications of SRF cavities.

physics.acc-ph↗

arXiv2017

Advancement in the understanding of the field and frequency dependent microwave surface resistance of niobium

The radio-frequency surface resistance of niobium resonators is incredibly reduced when nitrogen impurities are dissolved as interstitial in the material, conferring ultra-high Q-factors at medium values of accelerating field. This effect has been observed in both high and low temperature nitrogen treatments. As a matter of fact, the peculiar anti Q-slope observed in nitrogen doped cavities, i.e. the decreasing of the Q-factor with the increasing of the radio-frequency field, come from the decreasing of the BCS surface resistance component as a function of the field. Such peculiar behavior has been considered consequence of the interstitial nitrogen present in the niobium lattice after the doping treatment. The study here presented show the field dependence of the BCS surface resistance of cavities with different resonant frequencies, such as: 650 MHz, 1.3 GHz, 2.6 GHz and 3.9 GHz, and processed with different state-of-the-art surface treatments. These findings show for the first time that the anti Q-slope might be seen at high frequency even for clean Niobium cavities, revealing useful suggestion on the physics underneath the anti Q-slope effect.

physics.acc-ph↗

arXiv2017

Performance-defining properties of Nb$_3$Sn coating in SRF cavities

Nb$_3$Sn has great potential to become the material of choice for fabrication of SRF cavities. The higher critical temperature of Nb$_3$Sn potentially allows for an increased operational temperature in SRF cavities, which could enable tremendous simplification of cryogenic system, leading to significant cost reduction. We present extended characterization of a Nb$_3$Sn coated Nb cavity prepared at Cornell University. Using combination of thermometry during cavity RF measurements, and structural and analytical characterization of the cavity cutouts, we discover Nb$_3$Sn coating flaws responsible for the poor cavity performance. Our results clearly show degraded material quality in the cavity cutouts which exhibit significant heating during the RF testing. Results of extended comparison of cavity cutouts with different dissipation profiles not only point out the cause of significant Q-slope but also establish figures of merit for material qualities in relation to the quality of SRF performance.

physics.acc-ph↗

arXiv2017

Unprecedented Quality Factors at Accelerating Gradients up to 45 MV/m in Niobium Superconducting Resonators via Low Temperature Nitrogen Infusion

We report the finding of new surface treatments that permit to manipulate the niobium resonator nitrogen content in the first few nanometers in a controlled way, and the resonator fundamental Mattis-Bardeen surface resistance and residual resistance accordingly. In particular, we find surface infusion conditions that systematically a) increase the quality factor of these 1.3 GHz superconducting radio frequency (SRF) bulk niobium resonators, up to very high gradients; b) increase the achievable accelerating gradient of the cavity compared to its own baseline with state-of-the-art surface processing. Cavities subject to the new surface process have larger than two times the state of the art Q at 2K for accelerating fields > 35 MV/m. Moreover, very high accelerating gradients ~ 45 MV/m are repeatedly reached, which correspond to peak magnetic surface fields of 190 mT, among the highest measured for bulk niobium cavities. These findings open the opportunity to tailor the surface impurity content distribution to maximize performance in Q and gradients, and have therefore very important implications on future performance and cost of SRF based accelerators. They also help deepen the understanding of the physics of the RF niobium cavity surface.

physics.acc-ph↗

arXiv2016

Effect of interstitial impurities on the field dependent microwave surface resistance of niobium

Previous work has demonstrated that the radio frequency surface resistance of niobium resonators is dramatically reduced when nitrogen impurities are dissolved as interstitial in the material. The origin of this effect is attributed to the lowering of the Mattis and Bardeen surface resistance contribution with increasing accelerating field. Meanwhile, an enhancement of the sensitivity to trapped magnetic field is typically observed for such cavities. In this paper we conduct the first systematic study on these different components contributing to the total surface resistance as a function of different levels of dissolved nitrogen, in comparison with standard surface treatments for niobium resonators. Adding these results together we are able to show for the first time which is the optimum surface treatment that maximizes the Q-factor of superconducting niobium resonators as a function of expected trapped magnetic field in the cavity walls. These results also provide new insights on the physics behind the change in the field dependence of the Mattis and Bardeen surface resistance, and of the trapped magnetic vortex induced losses in superconducting niobium resonators.

physics.acc-ph↗

arXiv2016

Quench-Induced Degradation of the Quality Factor in Superconducting Resonators

Quench of superconducting radio-frequency cavities frequently leads to the lowered quality factor Q0, which had been attributed to the additional trapped magnetic flux. Here we demonstrate that the origin of this magnetic flux is purely extrinsic to the cavity by showing no extra dissipation (unchanged Q0) after quenching in zero magnetic field, which allows us to rule out intrinsic mechanisms of flux trapping such as generation of thermal currents or trapping of the rf field. We also show the clear relation of dissipation introduced by quenching to the orientation of the applied magnetic field and the possibility to fully recover the quality factor by requenching in the compensated field. We discover that for larger values of the ambient field, the Q-factor degradation may become irreversible by this technique, likely due to the outward flux migration beyond the normal zone opening during quench. Our findings are of special practical importance for accelerators based on low- and medium-beta accelerating structures residing close to focusing magnets, as well as for all high-Q cavity-based accelerators.

physics.acc-ph↗

arXiv2016

Efficient expulsion of magnetic flux in superconducting RF cavities for high $Q_0$ applications

Even when cooled through its transition temperature in the presence of an external magnetic field, a superconductor can expel nearly all external magnetic flux. This Letter presents an experimental study to identify the parameters that most strongly influence flux trapping in high purity niobium during cooldown. This is critical to the operation of superconducting radiofrequency cavities, in which trapped flux degrades the quality factor and therefore cryogenic efficiency. Flux expulsion was measured on a large survey of 1.3 GHz cavities prepared in various ways. It is shown that both spatial thermal gradient and high temperature treatment are critical to expelling external magnetic fields, while surface treatment has minimal effect. For the first time, it is shown that a cavity can be converted from poor expulsion behavior to strong expulsion behavior after furnace treatment, resulting in a substantial improvement in quality factor. Future plans are described to build on this result in order to optimize treatment for future cavities.

physics.acc-ph↗

arXiv2015

Accelerator physics and technology research toward future multi-MW proton accelerators

Recent P5 report indicated the accelerator-based neutrino and rare decay physics research as a centrepiece of the US domestic HEP program. Operation, upgrade and development of the accelerators for the near-term and longer-term particle physics program at the Intensity Frontier face formidable challenges. Here we discuss accelerator physics and technology research toward future multi-MW proton accelerators.

physics.acc-ph↗

arXiv2015

Cooling Dynamics Through Transition Temperature of Niobium SRF Cavities Captured by Temperature Mapping

Cool-down dynamics of superconducting accelerating cavities became particularly important for obtaining very high quality factors in SRF cavities. Previous studies proved that when cavity is cooled fast, the quality factor is higher than when cavity is cooled slowly. This has been discovered to derive from the fact that a fast cool-down allows better magnetic field expulsion during the superconducting transition. In this paper we describe the first experiment where the temperature all around the cavity was mapped during the cavity cool-down through transition temperature, proving the existence of two different transition dynamics: a sharp superconducting-normal conducting transition during fast cool-down which favors flux expulsion and nucleation phase transition during slow cool-down, which leads to full flux trapping.

physics.acc-ph↗

arXiv2015

Magnetic Flux Dynamics in Horizontally Cooled Superconducting Cavities

Previous studies on magnetic flux expulsion as a function of cooling details have been performed for superconducting niobium cavities with the cavity beam axis placed parallel respect to the helium cooling flow, and findings showed that for sufficient cooling thermogradients all magnetic flux could be expelled and very low residual resistance could be achieved. In this paper we investigate the flux trapping and its impact on radio frequency surface resistance when the resonators are positioned perpendicularly to the helium cooling flow, which is representative of how superconducting radio-frequency (SRF) cavities are cooled in an accelerator. We also extend the studies to different directions of applied magnetic field surrounding the resonator. Results show that in the cavity horizontal configuration there is a different impact of the various field components on the final surface resistance, and that several parameters have to be considered to understand flux dynamics. A newly discovered phenomenon of concentration of flux lines at the cavity top leading to cavity equator temperature rise is presented.

physics.acc-ph↗

arXiv2015

Nanostructural features degrading the performance of superconducting radio frequency niobium cavities revealed by TEM and EELS

Nanoscale defect structure within the magnetic penetration depth of ~100nm is key to the performance limitations of niobium superconducting radio frequency (SRF) cavities. Using a unique combination of advanced thermometry during cavity RF measurements, and TEM structural and compositional characterization of the samples extracted from cavity walls, we discover the existence of nanoscale hydrides in electropolished cavities limited by the high field Q slope, and show the decreased hydride formation in the electropolished cavity after 120C baking. Furthermore, we demonstrate that adding 800C hydrogen degassing followed by light buffered chemical polishing restores the hydride formation to the pre-120C bake level. We also show absence of niobium oxides along the grain boundaries and the modifications of the surface oxide upon 120C bake.

physics.acc-ph↗

arXiv2014

Ultra-high quality factors in superconducting niobium cavities in ambient magnetic fields up to 190 mG

Ambient magnetic field, if trapped in the penetration depth, leads to the residual resistance and therefore sets the limit for the achievable quality factors in superconducting niobium resonators for particle accelerators. Here we show that a complete expulsion of the magnetic flux can be performed and leads to: 1) record quality factors $Q > 2\times10^{11}$ up to accelerating gradient of 22 MV/m; 2) $Q\sim3\times10^{10}$ at 2 K and 16 MV/m in up to 190 mG magnetic fields. This is achieved by large thermal gradients at the normal/superconducting phase front during the cooldown. Our findings open up a way to ultra-high quality factors at low temperatures and show an alternative to the sophisticated magnetic shielding implemented in modern superconducting accelerators.

physics.acc-ph↗

arXiv2014

Comment on the "Decrease of the surface resistance in superconducting niobium resonator cavities by the microwave field"

In a recent publication [Appl. Phys. Lett. 104, 092601 (2014)] Ciovati et al. claim that: 1) thermal effects were disregarded in our original work [*]; 2) increase of $Q$ at $T=2$ K up to about $B\sim$100 mT in nitrogen doped cavities is just an extended low field $Q$ slope observed in non-doped cavities, which is furthermore attributed to the decrease of the "BCS" component of surface resistance. Here we show that both claims are wrong and the conclusions of Ciovati et al. are incorrect. [*] A. Romanenko and A. Grassellino, Appl. Phys. Lett. 102, 252603 (2013)

physics.acc-ph↗