arXiv subjects

A. Rulmont

Publications and source records attributed to A. Rulmont.

3 recordsLinked to original sources

arXiv2003

AC magnetic behavior of large grain magneto-resistive La0.78Ca0.22Mn0.90Ox materials

We report a detailed set of AC magnetic measurements carried out on bulk large grain La-Ca-Mn-O samples extracted from a floating zone method-grown rod. Three samples with $La_{0.78}Ca_{0.22}Mn_{0.90}O_{x}$ stoichiometry but differing in their microstructure were investigated by electrical resistivity and AC susceptibility measurements: (i) a single grain sample, (ii) a sample containing two grains and (iii) a polycrystalline sample. We show that the superimposition of DC magnetic fields during AC magnetic susceptibility measurements is an efficient way for characterizing the magnetic transition of samples with different microstructures. Whereas both single grain and polycrystalline samples display a single susceptibility peak, an additional kink structure is observed in the case of the double grain sample. The temperature dependence of the AC susceptibility measured with superimposed DC magnetic fields is analyzed in the framework of second-order phase transition ideas. The relations between the critical exponents ($β+ γ$ ~ 1.5, $δ$ ~ 2.5) are found to be close to those of the mean-field model for all samples. This is attributed to the disordering caused by unoccupied Mn sites.

cond-mat.supr-con↗

arXiv2003

The contribution of 211 particles to the mechanical reinforcement mechanism of 123 superconducting single domains

Hardness and fracture toughness of Dy-123 single-domains were studied by Vickers micro-indentation. A significant anisotropy of the mechanical properties was observed. Hardness tests give higher values when performed in (001) planes rather than in planes parallel to the c-axis. Moreover cracks pattern around the indentation follows preferential orientation in planes parallel to the c-axis whereas a classical ''four-cracks'' pattern is observed in the (001) planes. It has been possible to show the crucial role played by the 211-particles in the deviating mechanism of cracks and the relevance of the 211-particle distribution high homogeneity in the material.

cond-mat.supr-con↗

arXiv1999

Anomalous temperature behavior of resistivity in lightly doped manganites around a metal-insulator phase transition

An unusual temperature and concentration behavior of resistivity in $La_{0.7}Ca_{0.3}Mn_{1-x}Cu_xO_3$ has been observed at slight $Cu$ doping ($0\leq x \leq 0.05$). Namely, introduction of copper results in a splitting of the resistivity maximum around a metal-insulator transition temperature $T_0(x)$ into two differently evolving peaks. Unlike the original $Cu$-free maximum which steadily increases with doping, the second (satellite) peak remains virtually unchanged for $x<x_c$, increases for $x\ge x_c$ and finally disappears at $x_m\simeq 2x_c$ with $x_c\simeq 0.03$. The observed phenomenon is thought to arise from competition between substitution induced strengthening of potential barriers (which hamper the charge hopping between neighboring $Mn$ sites) and weakening of carrier's kinetic energy. The data are well fitted assuming a nonthermal tunneling conductivity theory with randomly distributed hopping sites.

cond-mat.str-el↗