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A. Ruocco

Publications and source records attributed to A. Ruocco.

14 recordsLinked to original sources

Towards Low-Energy Electron High-Resolution Spectroscopy with Transition-Edge Sensors

We present a study of the energy resolution of transition-edge sensors (TESs) for the detection of electrons in the 100 eV kinetic energy range. The TES is a Ti-Au bilayer with an active area of $(60 \times 60)$ $\mu \text{m}^2$ and a critical temperature of $\sim$ 80 mK. The electron source is based on vertically-aligned multiwall carbon nanotubes located inside the cryostat, with electrons generated via field emission. For electrons in the (92 - 99) eV kinetic energy range, we obtain a Gaussian energy resolution for fully-absorbed electrons of (0.479 $\pm$ 0.041 $\pm$ 0.055) eV. When considering the full-width at half-maximum of the peak, the corresponding resolution is of (1.44 $\pm$ 0.17 $\pm$ 0.27) eV. The former represents an improvement of (46 - 60)% with respect to previous results, and is mainly attributed to the reduction in the TES active area. The latter is instead an improvement of over a factor of 20, and is mainly due to the reduction in the emitting area of the electron source, which significantly suppresses electron back-scattering in proximity of the TES. These results represent a major milestone toward high-precision spectroscopy on low-energy electrons, which is a key objective for the PTOLEMY experiment.

physics.ins-det

Ultra-high precision high voltage system for PTOLEMY

The PTOLEMY project is prototyping a novel electromagnetic filter for high-precision $\beta$ spectroscopy, with the ultimate and ambitious long-term goal of detecting the cosmic neutrino background through electron capture on tritium bound to graphene. Intermediate small-scale prototypes can achieve competitive sensitivity to the effective neutrino mass, even with reduced energy resolution. To reach an energy resolution better than \SI{500}{meV} at the tritium $\beta$-spectrum endpoint of \SI{18.6}{keV}, and accounting for all uncertainties in the filtering chain, the electrode voltage must be controlled at the level of a few parts per million and monitored in real time. In this work, we present the first results obtained in this effort, using a chain of commercial ultra-high-precision voltage references, read out by precision multimeters and a \emph{field mill} device. The currently available precision on high voltage is, in the conservative case, as low as \SI{0.2}{ppm} per \SI{1}{kV} single board and $\lesssim$ \SI{50}{mV} over the \SI{10}{kV} series, presently limited by field mill read-out noise. However, assuming uncorrelated Gaussian noise extrapolation, the real precision could in principle be as low as \SI{0.05}{ppm} over \SI{20}{kV}.

physics.ins-det

Graphene Electro-Absorption Modulators for Energy-Efficient and High-Speed Optical Transceivers

The increasing demand for energy-efficient hardware for artificial intelligence (AI) and data centres requires integrated photonic solutions delivering optical transceivers with Tbit/s data rates and energy consumption$<$1pJ/bit. Here, we report double single-layer graphene electro-absorption modulators on Si optimized for energy-efficient and ultra-fast operation, demonstrating 67GHz bandwidth and 80Gbit/s data rate, in both O and C bands, using a fabrication tailored for wafer-scale integration. We measure a data rate$\sim$1.6 times larger than previously reported for graphene. We scale the modulator's active area down to 22$\mu$m$^2$, achieving a dynamic power consumption$\sim$58fJ/bit, $\sim$3 times lower than previous graphene modulators and Mach-Zehnder modulators based on Si or lithium niobate. We show devices with$\sim$0.037dB/V$\mu$m modulation efficiency,$\sim$16 times better than previous demonstrations based on graphene. This paves the way to wafer-scale production of graphene modulators on Si useful for Tbit/s optical transceivers and energy-efficient AI

cond-mat.mtrl-sci

A Demonstration of Slowed Electron ${\bf E} \times {\bf B}$ Drift for PTOLEMY

To resolve the effective neutrino mass $m_\beta$ with an energy resolution of 50~meV, the PTOLEMY experiment has proposed a novel transverse electromagnetic filtering process. Substantially reducing the kinetic energy of tritium $\beta$-decay electrons by counteracting motion from ${\bf E}$ $\times$ ${\bf B}$ and $\nabla{\rm B}$ drift, the PTOLEMY filter requires an input of emitted electron kinematic information to generate a tailored, suitable electric field for each candidate. The collaboration proposes to extract these quantities by using antennae to observe the relativistic frequency shift of emitted cyclotron radiation as an electron transits by ${\bf E}$ $\times$ ${\bf B}$ drift through a uniform magnetic field region preceding the filter. Electrons must be contained within this region long enough such that an adequate integrated radiated power signal is received to accurately estimate these kinematics. This necessitates a controlled, slowed drift speed. This paper presents the experimental design to vary ${\bf E}$ $\times$ ${\bf B}$ drift speed of carbon-14 $\beta$-decay electrons using a custom electrode field cage situated between the pole faces of an electromagnet. Matching our results with high-fidelity simulation, we deduce a capacity to increase particle time of flight by a factor of 5 in the field cage's slow drift region. Limited only by the dimensions of our system, we assert drift speed can be arbitrarily slowed to meet the needs of PTOLEMY's future detector. Actualizing such a system is a crucial milestone in developing the detector, enabling future cyclotron radiation measurements, filter implementation, and source injection.

physics.ins-det

Graphene phase modulators operating in the transparency regime

Next-generation data networks need to support Tb/s rates. In-phase and quadrature (IQ) modulation combine phase and intensity information to increase the density of encoded data, reduce overall power consumption by minimising the number of channels, and increase noise tolerance. To reduce errors when decoding the received signal, intersymbol interference must be minimised. This is achieved with pure phase modulation, where the phase of the optical signal is controlled without changing its intensity. Phase modulators are characterised by the voltage required to achieve a $\pi$ phase shift V$_{\pi}$, the device length L, and their product V$_{\pi}$L. To reduce power consumption, IQ modulators are needed with$<$1V drive voltages and compact (sub-cm) dimensions, which translate in V$_\pi$L$<$1Vcm. Si and LiNbO$_3$ (LN) IQ modulators do not currently meet these requirements, because V$_{\pi}$L$>$1Vcm. Here, we report a double single-layer graphene (SLG) Mach-Zehnder modulator (MZM) with pure phase modulation in the transparent regime, where optical losses are minimised and remain constant with increasing voltage. Our device has $V_{\pi}L\sim$0.3Vcm, matching state-of-the-art SLG-based MZMs and plasmonic LN MZMs, but with pure phase modulation and low insertion loss ($\sim$5dB), essential for IQ modulation. Our $V_\pi L$ is$\sim$5 times lower than the lowest thin-film LN MZMs, and$\sim$3 times lower than the lowest Si MZMs. This enables devices with complementary metal-oxide semiconductor compatible V$_\pi$L ($<$1Vcm) and smaller footprint than LN or Si MZMs, improving circuit density and reducing power consumption by one order of magnitude.

physics.ins-det

Graphene-perovskite fibre photodetectors

The integration of optoelectronic devices, such as transistors and photodetectors (PDs), into wearables and textiles is of great interest for applications such as healthcare and physiological monitoring. These require flexible/wearable systems adaptable to body motions, thus materials conformable to non-planar surfaces, and able to maintain performance under mechanical distortions. Here, we prepare fibre PDs combining rolled graphene layers and photoactive perovskites. Conductive fibres ($\sim$500$\Omega$/cm) are made by rolling single layer graphene (SLG) around silica fibres, followed by deposition of a dielectric layer (Al$_{2}$O$_{3}$ and parylene C), another rolled SLG as channel, and perovskite as photoactive component. The resulting gate-tunable PDs have response time$\sim$5ms, with an external responsivity$\sim$22kA/W at 488nm for 1V bias. The external responsivity is two orders of magnitude higher and the response time one order of magnitude faster than state-of-the-art wearable fibre based PDs. Under bending at 4mm radius, up to$\sim$80\% photocurrent is maintained. Washability tests show$\sim$72\% of initial photocurrent after 30 cycles, promising for wearable applications.

physics.app-ph

Absolute efficiency of a two-stage microchannel plate for electrons in the 30 - 900 eV energy range

We report on an apparatus able to measure the absolute detection efficiency of a detector for electrons in the 30 - 900 eV range. In particular, we discuss the characterisation of a two-stage chevron microchannel plate (MCP). The measurements have been performed in the LASEC laboratory at Roma Tre University, whit a custom-made electron gun. The very good stability of the beam current in the fA range, together with the picoammeter nominal resolution of 0.01 fA, allowed the measurement of the MCP absolute efficiency $\epsilon$. We found an $\epsilon$ = (0.489 $\pm$ 0.003) with no evident energy dependence. We fully characterised the MCP pulse shape distribution, which is quasi-Gaussian with a well visible peak above the noise level. We measured a 68% variation of the average pulse height between 30 and 500 eV. Furthermore, with a deeper analysis of the pulse shape, and in particular of the correlation between pulse height, area and width, we found a method to discriminate single- and multi- electron events occurring within a 10 ns time window.

physics.ins-det

Heisenberg's uncertainty principle in the PTOLEMY project: a theory update

We discuss the consequences of the quantum uncertainty on the spectrum of the electron emitted by the $\beta$-processes of a tritium atom bound to a graphene sheet. We analyze quantitatively the issue recently raised in [Cheipesh et al., Phys. Rev. D 104, 116004 (2021)], and discuss the relevant time scales and the degrees of freedom that can contribute to the intrinsic spread in the electron energy. We perform careful calculations of the potential between tritium and graphene with different coverages and geometries. With this at hand, we propose possible avenues to mitigate the effect of the quantum uncertainty.

hep-ph

Implementation and Optimization of the PTOLEMY Transverse Drift Electromagnetic Filter

The PTOLEMY transverse drift filter is a new concept to enable precision analysis of the energy spectrum of electrons near the tritium beta-decay endpoint. This paper details the implementation and optimization methods for successful operation of the filter. We present the first demonstrator that produces the required magnetic field properties with an iron return-flux magnet. Two methods for the setting of filter electrode voltages are detailed. The challenges of low-energy electron transport in cases of low field are discussed, such as the growth of the cyclotron radius with decreasing magnetic field, which puts a ceiling on filter performance relative to fixed filter dimensions. Additionally, low pitch angle trajectories are dominated by motion parallel to the magnetic field lines and introduce non-adiabatic conditions and curvature drift. To minimize these effects and maximize electron acceptance into the filter, we present a three-potential-well design to simultaneously drain the parallel and transverse kinetic energies throughout the length of the filter. These optimizations are shown, in simulation, to achieve low-energy electron transport from a 1 T iron core (or 3 T superconducting) starting field with initial kinetic energy of 18.6 keV drained to <10 eV (<1 eV) in about 80 cm. This result for low field operation paves the way for the first demonstrator of the PTOLEMY spectrometer for measurement of electrons near the tritium endpoint to be constructed at the Gran Sasso National Laboratary (LNGS) in Italy.

physics.ins-det

Unexpectedly large electron correlation measured in Auger spectra of ferromagnetic iron thin films: orbital-selected Coulomb and exchange contributions

A set of electron-correlation energies as large as 10 eV have been measured for a magnetic 2ML Fefilm deposited on Ag(001). By exploiting the spin selectivity in angle-resolved Auger-photoelectroncoincidence spectroscopy and the Cini-Sawatzky theory, the core-valence-valence Auger spectrumof a spin-polarized system have been resolved: correlation energies have been determined for eachindividual combination of the two holes created in the four sub-bands involved in the decay: majorityand minority spin, as well asegandt2g. The energy difference between final states with paralleland antiparallel spin of the two emitted electrons is ascribed to the spin-flip energy for the final ionstate, thus disentangling the contributions of Coulomb and exchange interactions.

cond-mat.str-el

Driving with temperature the synthesis of graphene films on Ge(110)

We systematically investigate the chemical vapor deposition growth of graphene on Ge(110) as a function of the deposition temperature close to the Ge melting point. By merging spectroscopic and morphological information, we find that the quality of graphene films depends critically on the growth temperature improving significantly by increasing this temperature in the 910-930 °C range. We correlate the abrupt improvement of the graphene quality to the formation of a quasi-liquid Ge surface occurring in the same temperature range, which determines increased atom diffusivity and sublimation rate. Being observed for diverse Ge orientations, this process is of general relevance for graphene synthesis on Ge.

cond-mat.mes-hall

Waveguide-integrated, plasmonic enhanced graphene photodetectors

We present a micrometer scale, on-chip integrated, plasmonic enhanced graphene photodetector (GPD) for telecom wavelengths operating at zero dark current. The GPD is designed and optimized to directly generate a photovoltage and has an external responsivity~12.2V/W with a 3dB bandwidth~42GHz. We utilize Au split-gates with a$\sim$100nm gap to electrostatically create a p-n-junction and simultaneously guide a surface plasmon polariton gap-mode. This increases light-graphene interaction and optical absorption and results in an increased electronic temperature and steeper temperature gradient across the GPD channel. This paves the way to compact, on-chip integrated, power-efficient graphene based photodetectors for receivers in tele and datacom modules

physics.app-ph

CuPc molecules adsorbed on Au(110)-(1x2): growth morphology and evolution of valence band states

We present the growth morphology, the long range ordering, and the evolution of the valence band electronic states of ultra-thin films of copper phthalocyanine (CuPc) deposited on the Au(110)-(1x2) reconstructed surface, as a function of the organic molecule coverage. The Low Energy Electron Diffraction (LEED) patterns present a (5x3) reconstruction from the early adsorption stages. High-Resolution UV photoelectron spectroscopy (HR-UPS) data show the disappearance of the Au surface states related to the (1x2) reconstruction, and the presence of new electronic features related to the molecule-substrate interaction and to the CuPc molecular states. The CuPc highest occupied molecular orbital (HOMO) gradually emerges in the valence band, while the interface electronic states are quenched, upon increasing the coverage.

cond-mat.mtrl-sci

Relevance of the EEL spectroscopy for in-situ studies of the growth mechanism of copper-phthalocyanine molecules on metal surfaces: Al(100)

Reflection electron energy loss spectroscopy (EELS) in specular and off specular geometry has been employed to study the early stage of the copper phthalocyanine (CuPc) growth on Al (100) substrate. EEL spectroscopy has been a useful tool in order to study electronic structure of molecular films also in the submonolayer regime. The electronic structure of the first deposited layer of CuPc is strongly influenced by charge transfer from the Al substrate to the lowest unoccupied molecular orbital (LUMO). The strong molecule-substrate interaction gives rise to a coverage dependent frequency shift of the Al surface plasmon. Successive layers have essentially the electronic structure of the molecular solid. Momentum resolved EELS measurements reveal that, in the case of the thicker film investigated (22 Å), the plane of the molecule is almost perpendicular to the surface of the substrate.

cond-mat.mtrl-sci