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A. S. Sefat

Publications and source records attributed to A. S. Sefat.

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Very High Field Two-Band Superconductivity in LaFeAsO_0.89F_0.11

The ongoing search for new superconductors has recently yielded a new family of oxypnictides composed of alternating La_2O_{2-x}F_x and Fe_2As_2 layers [1-4] with transition temperatures T_c of 25-28 K, which can be raised to 40-43 K by replacing La with Ce [5] or Sm [6] or to 52 K by replacing La with Nd and Pr [7, 8]. Recent experiments and band structure calculations have suggested an unconventional multiband superconductivity in the layers of paramagnetic Fe ions, which would normally destroy superconductivity in the traditional mechanism of the s-wave Cooper pairing. Here we report very high-field resistance measurements up to 45T, which show a remarkable enhancement of the upper critical fields B_c2 at low temperatures, as compared to those expected from the already high slopes of dB_c2/dT ~ 2T/K near T_c . The deduced B_c2(0) ~ 63-65 T exceeds the paramagnetic limit, consistent with strong coupling and important two-band effects in LaFeAsO_0.89F_0.11. We argue that oxypnictides are emerging as a new class of high-field superconductors surpassing the B_c2 of Nb_3Sn, MgB_2, and the Chevrel phases and perhaps approaching the 100T field benchmark of the high-T_c cuprates.

cond-mat.supr-con↗

The Anderson-Mott transition induced by hole-doping in Nd1-xTiO3

The insulator/metal transition induced by hole-doping due to neodymium vacancies of the Mott- Hubbard antiferromagnetic insulator, Nd1-xTiO3, is studied over the composition range 0.010(6) < x < 0.243(10). Insulating p-types conduction is found for x < 0.071(10). Anderson localization in the presence of a Mott-Hubbard gap, is the dominant localization mechanism for the range of 0.074(10) < x < 0.089(1) samples. For x < 0.089(1), n-type conduction is observed and the activation energy extrapolates to zero by x < 0.1. The 0.095(8) < x < 0.203(10) samples are Fermi-liquid metals and the effects of strong electronic correlations are evident near the metal-to-insulator boundaries in features such as large Fermi liquid T2 coefficients. For 0.074(9) < x < 0.112(4), a weak negative magnetoresistance is found below ~ 15 K and it is attributed to the interaction of conduction electrons with Nd3+ magnetic moments. Combining information from our companion study of the magnetic properties of Nd1-xTiO3 solid solution, a phase diagram is proposed. The main conclusions are that long range antiferromagnetic order disappears before the onset of metallic behavior and that the Anderson-Mott transition occurs over a finite range of doping levels. Our results differ from conclusions drawn from a similar study on the hole doped Nd1-xCaxTiO3 system which found the co-existence of antiferromagnetic order and metallic behavior and that the Mott transition occurs at a discrete doping level.

cond-mat.str-el↗