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A. S. Umar

Publications and source records attributed to A. S. Umar.

At least 73 records · Page 4Linked to original sources

Reduced quasifission competition in fusion reactions forming neutron-rich heavy elements

Measurements of mass-angle distributions (MADs) for Cr + W reactions, providing a wide range in the neutron-to-proton ratio of the compound system, (N/Z)CN, have allowed for the dependence of quasifission on the (N/Z)CN to be determined in a model-independent way. Previous experimental and theoretical studies had produced conflicting conclusions. The experimental MADs reveal an increase in contact time and mass evolution of the quasifission fragments with increasing (N/Z)CN, which is indicative of an increase in the fusion probability. The experimental results are in agreement with microscopic time-dependent Hartree-Fock calculations of the quasifission process. The experimental and theoretical results favor the use of the most neutron-rich projectiles and targets for the production of heavy and superheavy nuclei.

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Quantal description of nucleon exchange in stochastic mean-field approach

Nucleon exchange mechanism is investigated in central collisions of symmetric heavy-ions in the basis of the stochastic mean-field approach. Quantal diffusion coefficients for nucleon exchange are calculated by including non-Markovian effects and shell structure. Variances of fragment mass distributions are calculated in central collisions of ${}^{40}$Ca + ${}^{40}$Ca, ${}^{48}$Ca + ${}^{48}$Ca and ${}^{56}$Ni + ${}^{56}$Ni systems.

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Density constrained TDHF

In this manuscript we provide an outline of the numerical methods used in implementing the density constrained time-dependent Hartree-Fock (DC-TDHF) method and provide a few examples of its application to nuclear fusion. In this approach, dynamic microscopic calculations are carried out on a three-dimensional lattice and there are no adjustable parameters, the only input is the Skyrme effective NN interaction. After a review of the DC-TDHF theory and the numerical methods, we present results for heavy-ion potentials $V(R)$, coordinate-dependent mass parameters $M(R)$, and precompound excitation energies $E^{*}(R)$ for a variety of heavy-ion reactions. Using fusion barrier penetrabilities, we calculate total fusion cross sections $σ(E_\mathrm{c.m.})$ for reactions between both stable and neutron-rich nuclei. We also determine capture cross sections for hot fusion reactions leading to the formation of superheavy elements.

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Time-dependent HF approach to SHE dynamics

We employ the time-dependent Hartree-Fock (TDHF) method to study various aspects of the reactions utilized in searches for superheavy elements. These include capture cross-sections, quasifission, prediction of $P_{\mathrm{CN}}$, and other interesting dynamical quantities. We show that the microscopic TDHF approach provides an important tool to shed some light on the nuclear dynamics leading to the formation of superheavy elements.

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Dissipative dynamics in quasi-fission

Quasi-fission is the primary reaction mechanism that prevents the formation of superheavy elements in heavy-ion fusion experiments. Employing the time-dependent density functional theory approach we study quasi-fission in the systems $^{40,48}$Ca+$^{238}$U. Results show that for $^{48}$Ca projectiles the quasi-fission is substantially reduced in comparison to the $^{40}$Ca case. This partly explains the success of superheavy element formation with $^{48}$Ca beams. For the first time, we also calculate the repartition of excitation energies of the two fragments in a dynamic microscopic theory. The system is found in quasi-thermal equilibrium only for reactions with $^{40}$Ca. The differences between both systems are interpreted in terms of initial neutron to proton asymmetry of the colliding partners.

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Sub-barrier enhancement of fusion as compared to a microscopic method in 18O+12C

Measurement of the energy dependence of the fusion cross-sec on at sub-barrier energies provides an important test for theoretical models of fusion. To extend the measurement of fusion cross-sections in the sub-barrier domain for the 18O+12C system. Use the new experimental data to confront microscopic calculations of fusion. Evaporation residues produced in fusion of 18O ions with 12C target nuclei were detected with good geometric efficiency and identified by measuring their energy and time-of-flight. Theoretical calculations with a density constrained time dependent Hartree-Fock (DC-TDHF) theory include for the first time the effect of pairing on the fusion cross-section. Comparison of the measured fusion excitation function with the predictions of the DC-TDHF calculations reveal that the experimental data exhibits a smaller decrease in cross-section with decreasing energy than is theoretically predicted. The larger cross-sections observed at the lowest energies measured indicate a larger tunneling probability for the fusion process. This larger probability can be associated with a smaller, narrower fusion barrier than presently included in the theoretical calculations.

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Microscopic study of the effect of intrinsic degrees of freedom on fusion

Fusion cross-sections are computed for the $^{40}$Ca$+^{40}$Ca system over a wide energy range with two microscopic approaches where the only phenomenological input is the Skyrme energy density functional. The first method is based on the coupled-channels formalism, using the bare nucleus-nucleus potential calculated with the frozen Hartree-Fock technique and the deformation parameters of vibrational states computed with the time-dependent Hartree-Fock (TDHF) approach. The second method is based on the density-constrained TDHF method to generate nucleus-nucleus potentials from TDHF evolution. Both approaches incorporate the effect of couplings to internal degrees of freedoms in different ways. The predictions are in relatively good agreement with experimental data.

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Formation and dynamics of fission fragments

Although the overall time-scale for nuclear fission is long, suggesting a slow process, rapid shape evolution occurs in its later stages near scission. Theoretical prediction of the fission fragments and their characteristics are often based on the assumption that the internal degrees of freedom are equilibrated along the fission path. However, this adiabatic approximation may break down near scission. This is studied for the symmetric fission of $^{258,264}$Fm. The non-adiabatic evolution is computed using the time-dependent Hartree-Fock method, starting from an adiabatic configuration where the fragments have acquired their identity. It is shown that dynamics has an important effect on the kinetic and excitation energies of the fragments. The vibrational modes of the fragments in the post-scission evolution are also analyzed.

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Eulerian Rotations of Deformed Nuclei for TDDFT Calculations

We discuss three practical methods for performing Eulerian rotations of Slater determinants in a three-dimensional Cartesian geometry. In addition to the straightforward application of the active form of the quantum mechanical rotation operator, we introduce two methods using a passive position-space rotation followed by an active spin-space rotation, one after variation and the other before variation. These methods can be used to initialize reactions involving deformed nuclei where a particular alignment of the deformed nuclei with respect to the collision axis is desired. We show that doing the rotation before the variation is the most efficient way of generating such initial states.

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Fusion using time-dependent density-constrained DFT

We present results for calculating fusion cross-sections using a new microscopic approach based on a time-dependent density-constrained DFT calculations. The theory is implemented by using densities and other information obtained from TDDFT time-evolution of the nuclear system as constraint on the density for DFT calculations.

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Energy dependence of potential barriers and its effect on fusion cross-sections

Couplings between relative motion and internal structures are known to affect fusion barriers by dynamically modifying the densities of the colliding nuclei. The effect is expected to be stronger at energies near the barrier top, where changes in density have longer time to develop than at higher energies. Quantitatively, modern TDHF calculations are able to predict realistic fusion thresholds. However, the evolution of the potential barrier with bombarding energy remains to be confronted with the experimental data. The aim is to find signatures of the energy dependence of the barrier by comparing fusion cross-sections calculated from potentials obtained at different bombarding energies with the experimental data. This comparison is made for the $^{40}$Ca+$^{40}$Ca and $^{16}$O+$^{208}$Pb systems. Fusion cross-sections are computed from potentials calculated with the density-constrained TDHF method. The couplings decrease the barrier at low-energy in both cases. A deviation from the Woods-Saxon nuclear potential is also observed at the lowest energies. In general, fusion cross-sections around a given energy are better reproduced by the potential calculated at this energy. The coordinate-dependent mass plays a crucial role for the reproduction of sub-barrier fusion cross-sections. Effects of the energy dependence of the potential can be found in experimental barrier distributions only if the variation of the barrier is significant in the energy-range spanned by the distribution. It appears to be the case for $^{16}$O+$^{208}$Pb but not for $^{40}$Ca+$^{40}$Ca. These results show that the energy dependence of the barrier predicted in TDHF calculations is realistic. This confirms that the TDHF approach can be used to study the couplings between relative motion and internal degrees of freedom in heavy-ion collisions.

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The TDHF Code Sky3D

The nuclear mean-field model based on Skyrme forces or related density functionals has found wide-spread application to the description of nuclear ground states, collective vibrational excitations, and heavy-ion collisions. The code Sky3D solves the static or dynamic equations in a three-dimensional Cartesian mesh with isolated or periodic boundary conditions and no further symmetry assumptions. Pairing can be included in the BCS approximation. The code is implemented with a view to allow easy modifications for including additional physics or special analysis of the results.

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Microscopic Calculation of Fusion: Light to Heavy Systems

The density-constrained time-dependent Hartree-Fock (DC-TDHF) theory is a fully microscopic approach for calculating heavy-ion interaction potentials and fusion cross sections below and above the fusion barrier. We discuss recent applications of DC-TDHF method to fusion of light and heavy neutron-rich systems.

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Microscopic study of $^{16}$O+$^{16}$O fusion

We perform a study of $^{16}$O+$^{16}$O fusion at above and below the interaction barrier energies using three-dimensional time-dependent Hartree-Fock (TDHF) calculations at above barrier energies and density-constrained TDHF calculations for the entire energy range. We discuss the variations of the experimental data at above the barrier energies. Calculations reasonably reproduce the observed energy-dependent broad oscillations in the fusion excitation functions. These oscillations result from overcoming $L$-dependent fusion barriers. The role of the coupling to low-lying octupole states is also discussed.

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Confronting measured near and sub-barrier fusion cross-sections for 20O+12C with a microscopic method

Recently measured fusion cross-sections for the neutron-rich system 20O+12C are compared to dynamic, microscopic calculations using time-dependent density functional theory. The calculations are carried out on a three-dimensional lattice and performed both with and without a constraint on the density. The method has no adjustable parameters, and its only input is the Skyrme effective NN interaction. While the microscopic DC-TDHF calculations lie closer to the experimental data than standard fusion systematics they underpredict the experimental data significantly.

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Microscopic analysis of sub-barrier fusion enhancement in $^{132}$Sn+$^{40}$Ca vs. $^{132}$Sn+$^{48}$Ca}

We provide a theoretical analysis of recently measured fusion cross sections which show a surprising enhancement at low $E_\mathrm{c.m.}$ energies for the system $^{132}$Sn+$^{40}$Ca as compared to the more neutron-rich system $^{132}$Sn+$^{48}$Ca. Dynamic microscopic calculations are carried out on a three-dimensional lattice with a time-dependent density-constrained density functional theory. There are no adjustable parameters, the only input is the Skyrme effective NN interaction. Heavy-ion potentials $V(R)$, coordinate-dependent mass parameters $M(R)$, and total fusion cross sections $σ(E_\mathrm{c.m.})$ are calculated for both systems. We are able to explain the measured fusion enhancement in terms of the {\it narrower width} of the ion-ion potential for $^{132}$Sn+$^{40}$Ca, while the barrier heights and positions are approximately the same in both systems.

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Single-particle dissipation in TDHF studied from a phase-space perspective

We study dissipation and relaxation processes within the time-dependent Hartree-Fock approach using the Wigner distribution function. On the technical side we present a geometrically unrestricted framework which allows us to calculate the full six-dimensional Wigner distribution function. With the removal of geometrical constraints, we are now able to extend our previous phase-space analysis of heavy-ion collisions in the reaction plane to unrestricted mean-field simulations of nuclear matter on a three-dimensional Cartesian lattice. From the physical point of view we provide a quantitative analysis on the stopping power in TDHF. This is linked to the effect of transparency. For the medium-heavy $^{40}$Ca+$^{40}$Ca system we examine the impact of different parametrizations of the Skyrme force, energy-dependence, and the significance of extra time-odd terms in the Skyrme functional.

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Dynamic Microscopic Theory of Fusion Using DC-TDHF

The density-constrained time-dependent Hartree-Fock (DC-TDHF) theory is a fully microscopic approach for calculating heavy-ion interaction potentials and fusion cross sections below and above the fusion barrier. We discuss recent applications of DC-TDHF method to fusion of light and heavy systems.

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