arXiv subjects

A. Saastamoinen

Publications and source records attributed to A. Saastamoinen.

At least 19 recordsLinked to original sources

arXiv2025

Potential absence of observed $π^2$ linear-chain structures in $^{14}$O via $^{10}$C($α,α$) resonant scattering

Background: The preference for light nuclear systems to coagulate into $α$-particle clusters has been well-studied. The possibility of a linear chain configuration of $α$-particles would allow for a new way to study this phenomenon. Purpose: A rotational band of states in $^{14}$C has been claimed showing a $π^2$ linear chain structure. The mirror system, $^{14}$O, has been studied here to examine how this linear chain structure is affected by replacing the valence neutrons with protons. Method: A beam of $^{10}$C was incident into a chamber filled with He:CO$_2$ gas with the tracks recorded inside the TexAT Time Projection Chamber and the recoil $α$-particles detected by a silicon detector array to measure the $^{10}\mathrm{C}(α,α)$ cross section. Results: The experimental cross section was compared with previous studies and fit using R-Matrix theory with the previously-observed $^{14}$O states being transformed to the $^{14}$C using mirror symmetry. The measured cross section does not replicate the claimed states, with the predicted cross section exceeding that observed at several energies and angles. Conclusion: A series of possibilities are highlighted with the most likely being that the originally-seen $^{14}$C states did not constitute a $π^2$ rotational band with a potentially incorrect spin assignment due to the limitations of the angular correlation method with non-zero spin particles. The work highlights the difficulties in measuring broad resonances corresponding to a linear chain state in a high level density.

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arXiv2025

Quantifying alpha clustering in the ground states of 16-O and 20-Ne

Understanding the role of multi-nucleon correlations in the structure of light nuclei is at the forefront of modern nuclear science. In this letter, we present a quantitative benchmark study of alpha-cluster correlations in the ground states of 16-O and 20-Ne. Experimental data provide direct evidence that the wave functions of the ground states of 16-O and 20-Ne are dominated by alpha-cluster correlations, in agreement with the predictions of sophisticated nuclear structure models. We also provide a new model-independent constraint for the alpha asymptotic normalization coefficient of the 16-O ground state and discuss the implications of these findings on the 12-C(alpha,gamma)16-O reaction, which is of critical importance for nuclear astrophysics.

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arXiv2025

First experimental test of the ratio method for nuclear-reaction analysis

Nuclear halos are very exotic quantal structures observed far from stability. Because of their short lifetime, they are mostly studied through reactions. The ratio method offers a new observable: the ratio of angular differential cross sections for breakup and scattering. It is predicted to be much more sensitive to the projectile structure than individual cross sections thanks to its independence of the reaction process. We test this new observable experimentally for the first time considering the collision of 11Be on C at 22.8 MeV/nucleon. We extend this analysis to similar data recently measured on Pb at 19.1 MeV/nucleon. Both analyses confirm the theoretical predictions, which opens the door to a new era in the study of nuclear structure near the neutron dripline. This should prove invaluable in conjunction with the start of FRIB. The ratio method could also be extended to other fields of quantum physics beyond nuclear reactions.

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arXiv2024

First Experimental Test of the Ratio Method

The ratio is a new reaction observable suggested to extract accurately structure information on halo nuclei. It corresponds to the ratio of differential cross sections for scattering and breakup, which is predicted to remove the uncertainty related to the reaction dynamics. We present here the first experimental test of the method for the 11Be + 12C collision at ELab = 20A MeV performed at Texas A&M University. Differential cross sections for scattering and inclusive one-neutron breakup have been measured with the new detector array BlueSTEAl. The ratio of cross sections is very smooth and independent of the projectile-target interaction, which demonstrates the validity of the ratio method. We extend our analysis to existing 11Be + 208Pb data, confirming that the method works well on any target.

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arXiv2024

Cluster structure of 3$α$+p states in $^{13}$N

Background: Cluster states in $^{13}$N are extremely difficult to measure due to the unavailability of $^{9}$B+$α$ elastic scattering data. Purpose: Using $β$-delayed charged-particle spectroscopy of $^{13}$O, clustered states in $^{13}$N can be populated and measured in the 3$α$+p decay channel. Method: One-at-a-time implantation/decay of $^{13}$O was performed with the Texas Active Target Time Projection Chamber (TexAT TPC). 149 $β3αp$ decay events were observed and the excitation function in $^{13}$N reconstructed. Results: Four previously unknown $α$-decaying excited states were observed in $^{13}$N at an excitation energy of 11.3 MeV, 12.4 MeV, 13.1 MeV and 13.7 MeV decaying via the 3$α$+p channel. Conclusion: These states are seen to have a [$^{9}\mathrm{B}(\mathrm{g.s}) \bigotimes α$/ $p+^{12}\mathrm{C}(0_{2}^{+})$], [$^{9}\mathrm{B}(\frac{1}{2}^{+}) \bigotimes α$], [$^{9}\mathrm{B}(\frac{5}{2}^{+}) \bigotimes α$] and [$^{9}\mathrm{B}(\frac{5}{2}^{+}) \bigotimes α$] structure respectively. A previously-seen state at 11.8 MeV was also determined to have a [$p+^{12}\mathrm{C}(\mathrm{g.s.})$/ $p+^{12}\mathrm{C}(0_{2}^{+})$] structure. The overall magnitude of the clustering is not able to be extracted however due to the lack of a total width measurement. Clustered states in $^{13}$N (with unknown magnitude) seem to persist from the addition of a proton to the highly $α$-clustered $^{12}$C. Evidence of the $\frac{1}{2}^{+}$ state in $^{9}$B was also seen to be populated by decays from $^{13}$N$^{\star}$.

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arXiv2024

Radiative decay branching ratio of the Hoyle state

Background: The triple-alpha process is a vital reaction in nuclear astrophysics, characterized by two consecutive reactions [$2α\leftrightarrows{^{8}\rm{Be}}(α,γ){^{12}\rm{C}}$] that drive carbon formation. The second reaction occurs through the Hoyle state, a 7.65 MeV excited state in ${^{12}\rm{C}}$ with $J^π=0^{+}$. The rate of the process depends on the radiative width, which can be determined by measuring the branching ratio for electromagnetic decay. Recent measurements by Kibédi et al. conflicted with the adopted value and resulted in a significant increase of nearly 50\% in this branching ratio, directly affecting the triple-alpha reaction. Purpose: This work aims to utilize charged-particle spectroscopy with magnetic selection as a means to accurately measure the total radiative branching ratio ($Γ_{\rm{rad}}/Γ$) of the Hoyle state in $^{12}{\rm C}$. Methods: The Hoyle state in $^{12}{\rm C}$ was populated via $^{12}\rm{C}(α, α')^{12}\rm{C^{*}}$ inelastic scattering. The scattered $α$ particles were detected using a $Δ$E-E telescope, while the recoiled $^{12}{\rm C}$ ions were identified in a magnetic spectrometer. Results: A radiative branching ratio value of $Γ_{\rm{rad}}/Γ\times10^{4}=4.0\pm0.3({\rm stat.})\pm0.16({\rm syst.})$ was obtained. Conclusions: The radiative branching ratio for the Hoyle state obtained in this work is in agreement with the original adopted value. Our result suggests that the proton-$γ$-$γ$ spectroscopy result reported by Kibédi et al. may be excluded.

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arXiv2023

Silicon tracker array for RIB experiments at SAMURAI

This work describes a silicon tracker system developed for experiments with proton-rich radioactive ion beams at the SAMURAI superconducting spectrometer of RIBF at RIKEN. The system is designed for accurate angular reconstruction and atomic number identification of relativistic heavy ions and protons which are simultaneously produced in reactions motivated by studies of proton capture reactions of interest for nuclear astrophysics. The technical characteristics of the tracking array are described in detail as are its performance in two pilot experiments. The physics justification for such a system is also presented.

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arXiv2023

First observation of the $β$3$α$p decay of $^{13}\mathrm{O}$ via $β$-delayed charged-particle spectroscopy

Background: The $β$-delayed proton-decay of $^{13}\mathrm{O}$ has previously been studied, but the direct observation of $β$-delayed $α$+$α$+$α$+p decay has not been reported. Purpose: Observing rare 3$α$+p events from the decay of excited states in $^{13}\mathrm{N}^{\star}$ allows for a sensitive probe of exotic highly-clustered configurations in $^{13}$N. Method: To measure the low-energy products following $β$-delayed 3$α$p-decay, the TexAT Time Projection Chamber was employed using the one-at-a-time $β$-delayed charged-particle spectroscopy technique at the Cyclotron Institute, Texas A&M University. Results: A total of $1.9 \times 10^{5}$ $^{13}\mathrm{O}$ implantations were made inside the TexAT Time Projection Chamber. 149 3$α$+p events were observed yielding a $β$-delayed 3$α+p$ branching ratio of 0.078(6)%. Conclusion: Four previously unknown $α$-decaying states were observed, one with a strong $^{9}\mathrm{B(g.s)}+α$ characteristic at 11.3 MeV, one with a $^{9}\mathrm{B}(\frac{1}{2}^{+})+α$ nature at 12.4 MeV, and another two that are dominated by $^{9}\mathrm{B}({\frac{5}{2}}^{+})+α$ at 13.1 and 13.7 MeV. Population of the $\frac{1}{2}^{+}$ state in $^{9}\mathrm{B}$ has been unambiguously seen, cementing the predicted existence of the mirror-state based on the states observed in $^{9}\mathrm{Be}$.

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arXiv2022

alpha-cluster structure of 18Ne

In this work we study alpha-clustering in 18Ne and compare it with what is known about clustering in the mirror nucleus 18O. The excitation function of 18Ne was measured in inverse kinematics from the resonant elastic scattering reaction of 14O on 4He in the excitation energy range from 8 to 17 MeV, using the active target TexAT. The analysis was performed using a multi-channel R-matrix approach. Detailed spectroscopic information is obtained from the R-matrix analysis: excitation energy of the states, spin and parity as well as partial alpha and total widths. This information is compared with theoretical models and previous data. Clustering structures appear to be robust and mostly isospin symmetric. A good correspondence was found between the levels in 18O and 18Ne. We carried out an extensive shell model analysis of the experimental data. This comparison suggests that strongly clustered states remain organized in relation to the corresponding reaction channel identified by the number of nodes in the relative alpha plus core wave function. The agreement between theory and experiment is very good and especially useful when it comes to understanding the clustering strength distribution. The comparison of the experimental data with theory shows that certain states, especially at high excitation energies, are significantly more clustered than predicted. This indicates that the structure of these states is collective and is aligned towards the corresponding alpha reaction channel.

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arXiv2021

Study of ($^6$Li, $d$) and ($^6$Li, $t$) reactions on $^{22}$Ne and implications for $s$-process nucleosynthesis

We studied $α$ cluster states in $^{26}$Mg via the $^{22}$Ne($^{6}$Li,$dγ$)$^{26}$Mg reaction in inverse kinematics at an energy of $7$ MeV/nucleon. States between $E_x$ = 4 - 12 MeV in $^{26}$Mg were populated and relative $α$ spectroscopic factors were determined. Some of these states correspond to resonances in the Gamow window of the $^{22}$Ne($α$,n)$^{25}$Mg reaction, which is one of the main neutron sources in the astrophysical $s$-process. We show that $α$-cluster strength of the states analyzed in this work have critical impact on s-process abundances. Using our new $^{22}$Ne($α$,n)$^{25}$Mg and $^{22}$Ne($α$,$γ$)$^{26}$Mg reaction rates, we performed new s-process calculations for massive stars and Asymptotic Giant Branch stars and compared the resulting yields with the yields obtained using other $^{22}$Ne+$α$ rates from the literature. We observe an impact on the s-process abundances up to a factor of three for intermediate-mass AGB stars and up to a factor of ten for massive stars. Additionally, states in $^{25}$Mg at $E_x$ $<$ 5 MeV are identified via the $^{22}$Ne($^{6}$Li,$t$)$^{25}$Mg reaction for the first time. We present the ($^6$Li, $t$) spectroscopic factors of these states and note similarities to the $(d,p$) reaction in terms of reaction selectivity.

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arXiv2021

Evidence against the Efimov effect in $^{12}\mathrm{C}$ from spectroscopy and astrophysics

Background: The Efimov effect is a universal phenomenon in physics whereby three-body systems are stabilized via the interaction of an unbound two-body sub-systems. A hypothetical state in $^{12}\mathrm{C}$ at 7.458 MeV excitation energy, comprising of a loose structure of three $α$-particles in mutual two-body resonance, has been suggested in the literature to correspond to an Efimov state in nuclear physics. The existence of such a state has not been demonstrated experimentally. Method: Using the combined data sets from two recent experiments, one with the TexAT TPC to measure $α$-decay and the other with Gammasphere to measure $γ$-decay of states in $^{12}\mathrm{C}$ populated by $^{12}\mathrm{N}$ and $^{12}\mathrm{B}$ $β$-decay respectively, we achieve high sensitivity to states in close-proximity to the $α$-threshold in $^{12}\mathrm{C}$. Results: No evidence of a state at 7.458 MeV is seen in either data set. Using a likelihood method, the 95\% C.L. $γ$-decay branching ratio is determined as a function of the $β$-decay feeding strength relative to the Hoyle state. In parallel, calculations of the triple-alpha reaction rate show the inclusion of the Efimov corresponds to a large increase in the reaction rate around $5 \times 10^{7}$ K. Conclusion: From decay spectroscopy - at the 95\% C.L., the Efimov state cannot exist at 7.458 MeV with any $γ$-decay branching ratio unless the $β$-strength is less than 0.7\% of the Hoyle state. This limit is evaluated for a range of different excitation energies and the results are not favorable for existence of the hypothetical Efimov state in $^{12}\mathrm{C}$. Furthermore, the triple-alpha reaction rate with the inclusion of a state between 7.43 and 7.53 MeV exceeds the rate required for stars to undergo the red giant phase.

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arXiv2020

Almost medium-free measurement of the Hoyle state direct-decay component with a TPC

Background: The structure of the Hoyle state, a highly $α$-clustered state at 7.65 MeV in $^{12}\mathrm{C}$, has long been the subject of debate. Understanding if the system comprises of three weakly-interacting $α$-particles in the 0s orbital, known as an $α$-condensate state, is possible by studying the decay branches of the Hoyle state. Purpose: The direct decay of the Hoyle state into three $α$-particles, rather than through the $^{8}\mathrm{Be}$ ground state, can be identified by studying the energy partition of the 3 $α$-particles arising from the decay. This paper provides details on the break-up mechanism of the Hoyle stating using a new experimental technique. Method: By using beta-delayed charged-particle spectroscopy of $^{12}\mathrm{N}$ using the TexAT (Texas Active Target) TPC, a high-sensitivity measurement of the direct 3 $α$ decay ratio can be performed without contributions from pile-up events. Results: A Bayesian approach to understanding the contribution of the direct components via a likelihood function shows that the direct component is $<0.043\%$ at the 95\% confidence level (C.L.). This value is in agreement with several other studies and here we can demonstrate that a small non-sequential component with a decay fraction of about $10^{-4}$ is most likely. Conclusion: The measurement of the non-sequential component of the Hoyle state decay is performed in an almost medium-free reaction for the first time. The derived upper-limit is in agreement with previous studies and demonstrates sensitivity to the absolute branching ratio. Further experimental studies would need to be combined with robust microscopic theoretical understanding of the decay dynamics to provide additional insight into the idea of the Hoyle state as an $α$-condensate.

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arXiv2020

Texas Active Target (TexAT) detector for experiments with rare isotope beams

The TexAT (Texas Active Target) detector is a new active-target time projection chamber (TPC) that was built at the Cyclotron Institute Texas A$\&$M University. The detector is designed to be of general use for nuclear structure and nuclear astrophysics experiments with rare isotope beams. TexAT combines a highly segmented Time Projection Chamber (TPC) with two layers of solid state detectors. It provides high efficiency and flexibility for experiments with low intensity exotic beams, allowing for the 3D track reconstruction of the incoming and outgoing particles involved in nuclear reactions and decays.

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arXiv2020

Constraining the $^{22}$Ne($α$,$γ$)$^{26}$Mg and $^{22}$Ne($α$,n)$^{25}$Mg reaction rates using sub-Coulomb $α$-transfer reactions

The $^{22}$Ne($α$,$γ$)$^{26}$Mg and $^{22}$Ne($α$,n)$^{25}$Mg reactions play an important role in astrophysics because they have significant influence on the neutron flux during the weak branch of the s-process. We constrain the astrophysical rates for these reactions by measuring partial $α$-widths of resonances in $^{26}$Mg located in the Gamow window for the $^{22}$Ne+$α$ capture. These resonances were populated using $^{22}$Ne($^6$Li,d)$^{26}$Mg and $^{22}$Ne($^7$Li,t)$^{26}$Mg reactions at energies near the Coulomb barrier. At these low energies $α$-transfer reactions favor population of low spin states and the extracted partial $α$-widths for the observed resonances exhibit only minor dependence on the model parameters. The astrophysical rates for both the $^{22}$Ne($α$,$γ$)$^{26}$Mg and the $^{22}$Ne($α$,n)$^{25}$Mg reactions are shown to be significantly different than the previously suggested values.

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arXiv2020

Decay properties of $^{22}\mathrm{Ne} + α$ resonances and their impact on $s$-process nucleosynthesis

The astrophysical $s$-process is one of the two main processes forming elements heavier than iron. A key outstanding uncertainty surrounding $s$-process nucleosynthesis is the neutron flux generated by the ${}^{22}\mathrm{Ne}(α, n){}^{25}\mathrm{Mg}$ reaction during the He-core and C-shell burning phases of massive stars. This reaction, as well as the competing ${}^{22}\mathrm{Ne}(α, γ){}^{26}\mathrm{Mg}$ reaction, is not well constrained in the important temperature regime from ${\sim} 0.2$--$0.4$~GK, owing to uncertainties in the nuclear properties of resonances lying within the Gamow window. To address these uncertainties, we have performed a new measurement of the ${}^{22}\mathrm{Ne}({}^{6}\mathrm{Li}, d){}^{26}\mathrm{Mg}$ reaction in inverse kinematics, detecting the outgoing deuterons and ${}^{25,26}\mathrm{Mg}$ recoils in coincidence. We have established a new $n / γ$ decay branching ratio of $1.14(26)$ for the key $E_x = 11.32$ MeV resonance in $^{26}\mathrm{Mg}$, which results in a new $(α, n)$ strength for this resonance of $42(11)~μ$eV when combined with the well-established $(α, γ)$ strength of this resonance. We have also determined new upper limits on the $α$ partial widths of neutron-unbound resonances at $E_x = 11.112,$ $11.163$, $11.169$, and $11.171$ MeV. Monte-Carlo calculations of the stellar ${}^{22}\mathrm{Ne}(α, n){}^{25}\mathrm{Mg}$ and ${}^{22}\mathrm{Ne}(α, γ){}^{26}\mathrm{Mg}$ rates, which incorporate these results, indicate that both rates are substantially lower than previously thought in the temperature range from ${\sim} 0.2$--$0.4$~GK.

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arXiv2019

Structure of 9C through proton resonance scattering with Texas Active Target detector

Background: Level structure of the most neutron deficient nucleon-bound carbon isotope, 9C, is not well known. Definitive spin-parity assignments are only available for two excited states. No positive parity states have been conclusively identified so far and the location of the sd-shell in A=9 T=3/2 isospin quadruplet is not known. Purpose: We have studied the level structure of exotic nucleus 9C at excitation energies below 6.4 MeV. Methods: Excited states in 9C were populated in 8B+p resonance elastic scattering and excitation functions were measured using active target approach. Results: Two excited states in 9C were conclusively observed, and R-matrix analysis of the excitation functions was performed to make the spin-parity assignments. The first positive parity state in A=9 T=3/2 nuclear system, the 5/2+ resonance at 4.3 MeV, has been identified. Conclusions: The new 5/2+ state at 4.3 MeV in 9C is a single-particle L=0 broad resonance and it determines the energy of the 2s shell. The 2s shell in this exotic nucleus appears well within the region dominated by the p-shell states.

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arXiv2019

Determining the average prompt-fission-neutron multiplicity for $^{239}$Pu($n$,$f$) via a $^{240}$Pu($α$,$α^{\prime}f$) surrogate reaction

The average prompt-fission-neutron multiplicity $\barν$ is of significance in the areas of nuclear theory, nuclear nonproliferation, and nuclear energy. In this work, the surrogate-reaction method has been used for the first time to indirectly determine $\barν$ for $^{239}$Pu($n$,$f$) via $^{240}$Pu($α$,$α^{\prime}f$) reactions. A $^{240}$Pu target was bombarded with a beam of 53.9-MeV $α$ particles. Scattered $α$ particles, fission products, and neutrons were measured with the NeutronSTARS detector array. Values of $\barν$ were obtained for a continuous range of equivalent incident neutron energies between 0.25--26.25~MeV, and the results agree well with direct neutron measurements.

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arXiv2019

Nuclear level densities and gamma-ray strength functions in samarium isotopes

The gamma-strength functions and level densities in the quasi-continuum of 147;149Sm isotopes have been extracted from particle-coincidences using the Oslo method. The nuclei of interest were populated via (p,d) reactions on pure 148;150Sm targets and the reaction products were recorded by the Hyperion array. An upbend in the low-energy region of the gSF has been observed. The systematic analysis of the gSF for a range of Sm isotopes highlights the interplay between scissors mode and the upbend. Shell-model calculations show reasonable agreement with the experimental gSFs and confirm the correspondence between the upbend and scissors mode.

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