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A. Sarracino

Publications and source records attributed to A. Sarracino.

36 records · Page 2Linked to original sources

Self-propulsion against a moving membrane: enhanced accumulation and drag force

Self-propulsion (SP) is a main feature of active particles (AP), such as bacteria or biological micromotors, distinguishing them from passive colloids. A renowned consequence of SP is accumulation at static interfaces, even in the absence of hydrodynamic interactions. Here we address the role of SP in the interaction between AP and a moving semipermeable membrane. In particular, we implement a model of noninteracting AP in a channel crossed by a partially penetrable wall, moving at a constant velocity $c$. With respect to both the cases of passive colloids with $c>0$ and AP with $c=0$, the AP with finite $c$ show enhancement of accumulation in front of the obstacle and experience a largely increased drag force. This effect is understood in terms of an effective potential localised at the interface between particles and membrane, of height proportional to $cτ/ξ$, where $τ$ is the AP's re-orientation time and $ξ$ the width characterising the surface's smoothness ($ξ\to 0$ for hard core obstacles). An approximate analytical scheme is able to reproduce the observed density profiles and the measured drag force, in very good agreement with numerical simulations. The effects discussed here can be exploited for automatic selection and filtering of AP with desired parameters.

cond-mat.soft↗

Heat fluctuations of Brownian oscillators in nonstationary processes: fluctuation theorem and condensation transition

We study analytically the probability distribution of the heat released by an ensemble of harmonic oscillators to the thermal bath, in the nonequilibrium relaxation process following a temperature quench. We focus on the asymmetry properties of the heat distribution in the nonstationary dynamics, in order to study the forms taken by the Fluctuation Theorem as the number of degrees of freedom is varied. After analysing in great detail the cases of one and two oscillators, we consider the limit of a large number of oscillators, where the behavior of fluctuations is enriched by a condensation transition with a nontrivial phase diagram, characterized by reentrant behavior. Numerical simulations confirm our analytical findings. We also discuss and highlight how concepts borrowed from the study of fluctuations in equilibrium under symmetry breaking conditions [Gaspard, J. Stat. Mech. P08021 (2012)] turn out to be quite useful in understanding the deviations from the standard Fluctuation Theorem.

cond-mat.stat-mech↗

Nonlinear response of inertial tracers in steady laminar flows: differential and absolute negative mobility

We study the mobility and the diffusion coefficient of an inertial tracer advected by a two-dimensional incompressible laminar flow, in the presence of thermal noise and under the action of an external force. We show, with extensive numerical simulations, that the force-velocity relation for the tracer, in the nonlinear regime, displays complex and rich behaviors, including negative differential and absolute mobility. These effects rely upon a subtle coupling between inertia and applied force which induce the tracer to persist in particular regions of phase space with a velocity opposite to the force. The relevance of this coupling is revisited in the framework of non-equilibrium response theory, applying a generalized Einstein relation to our system. The possibility of experimental observation of these results is also discussed.

cond-mat.stat-mech↗

Nonlinear response and emerging nonequilibrium micro-structures for biased diffusion in confined crowding environments

We study analytically the dynamics and the micro-structural changes of a host medium caused by a driven tracer particle moving in a confined, quiescent molecular crowding environment. Imitating typical settings of active micro-rheology experiments, we consider here a minimal model comprising a geometrically confined lattice system -- a two-dimensional strip-like or a three-dimensional capillary-like -- populated by two types of hard-core particles with stochastic dynamics -- a tracer particle driven by a constant external force and bath particles moving completely at random. Resorting to a decoupling scheme, which permits us to go beyond the linear-response approximation (Stokes regime) for arbitrary densities of the lattice gas particles, we determine the force-velocity relation for the tracer particle and the stationary density profiles of the host medium particles around it. These results are validated a posteriori by extensive numerical simulations for a wide range of parameters. Our theoretical analysis reveals two striking features: a) We show that, under certain conditions, the terminal velocity of the driven tracer particle is a nonmonotonic function of the force, so that in some parameter range the differential mobility becomes negative, and b) the biased particle drives the whole system into a nonequilibrium steady-state with a stationary particle density profile past the tracer, which decays exponentially, in sharp contrast with the behavior observed for unbounded lattices, where an algebraic decay is known to take place.

cond-mat.stat-mech↗

Diffusion and subdiffusion of interacting particles on comb-like structures

We study the dynamics of a tracer particle (TP) on a comb lattice populated by randomly moving hard-core particles in the dense limit. We first consider the case where the TP is constrained to move on the backbone of the comb only, and, in the limit of high density of particles, we present exact analytical results for the cumulants of the TP position, showing a subdiffusive behavior $\sim t^{3/4}$. At longer times, a second regime is observed, where standard diffusion is recovered, with a surprising non analytical dependence of the diffusion coefficient on the particle density. When the TP is allowed to visit the teeth of the comb, based on a mean-field-like Continuous Time Random Walk description, we unveil a rich and complex scenario, with several successive subdiffusive regimes, resulting from the coupling between the inhomogeneous comb geometry and particle interactions. Remarkably, the presence of hard-core interactions speeds up the TP motion along the backbone of the structure in all regimes.

cond-mat.stat-mech↗

Microscopic theory for negative differential mobility in crowded environments

We study the behavior of the stationary velocity of a driven particle in an environment of mobile hard-core obstacles. Based on a lattice gas model, we demonstrate analytically that the drift velocity can exhibit a nonmonotonic dependence on the applied force, and show quantitatively that such negative differential mobility (NDM), observed in various physical contexts, is controlled by both the density and diffusion time scale of obstacles. Our study unifies recent numerical and analytical results obtained in specific regimes, and makes it possible to determine analytically the region of the full parameter space where NDM occurs. These results suggest that NDM could be a generic feature of biased (or active) transport in crowded environments.

cond-mat.stat-mech↗

Scaling properties of field-induced superdiffusion in Continous Time Random Walks

We consider a broad class of Continuous Time Random Walks with large fluctuations effects in space and time distributions: a random walk with trapping, describing subdiffusion in disordered and glassy materials, and a Lévy walk process, often used to model superdiffusive effects in inhomogeneous materials. We derive the scaling form of the probability distributions and the asymptotic properties of all its moments in the presence of a field by two powerful techniques, based on matching conditions and on the estimate of the contribution of rare events to power-law tails in a field.

cond-mat.stat-mech↗

Nonequilibrium fluctuation-dissipation theorem and heat production

We use a relationship between response and correlation function in nonequilibrium systems to establish a connection between the heat production and the deviations from the equilibrium fluctuation-dissipation theorem. This scheme extends the Harada-Sasa formulation [Phys. Rev. Lett. 95, 130602 (2005)], obtained for Langevin equations in steady states, as it also holds for transient regimes and for discrete jump processes involving small entropic changes. Moreover, a general formulation includes two times and the new concepts of two-time work, kinetic energy, and of a two-time heat exchange that can be related to a nonequilibrium "effective temperature". Numerical simulations of a chain of anharmonic oscillators and of a model for a molecular motor driven by ATP hydrolysis illustrate these points.

cond-mat.stat-mech↗

Fluctuations in partitioning systems with few degrees of freedom

We study the behavior of a moving wall in contact with a particle gas and subjected to an external force. We compare the fluctuations of the system observed in the microcanonical and canonical ensembles, at varying the number of particles. Static and dynamic correlations signal significant differences between the two ensembles. Furthermore, velocity-velocity correlations of the moving wall present a complex two-time relaxation which cannot be reproduced by a standard Langevin-like description. Quite remarkably, increasing the number of gas particles in an elongated geometry, we find a typical timescale, related to the interaction between the partitioning wall and the particles, which grows macroscopically.

cond-mat.stat-mech↗

Time asymmetry of the Kramers equation with nonlinear friction: fluctuation-dissipation relation and ratchet effect

We show by numerical simulations that the presence of nonlinear velocity-dependent friction forces can induce a finite net drift in the stochastic motion of a particle in contact with an equilibrium thermal bath and in an asymmetric periodic spatial potential. In particular, we study the Kramers equation for a particle subjected to Coulomb friction, namely a constant force acting in the direction opposite to the particle's velocity. We characterize the nonequilibrium irreversible dynamics by studying the generalized fluctuation-dissipation relation for this ratchet model driven by Coulomb friction.

cond-mat.stat-mech↗

Rare events and scaling properties in field-induced anomalous dynamics

We show that, in a broad class of continuous time random walks (CTRW), a small external field can turn diffusion from standard into anomalous. We illustrate our findings in a CTRW with trapping, a prototype of subdiffusion in disordered and glassy materials, and in the Lévy walk process, which describes superdiffusion within inhomogeneous media. For both models, in the presence of an external field, rare events induce a singular behavior in the originally Gaussian displacements distribution, giving rise to power-law tails. Remarkably, in the subdiffusive CTRW, the combined effect of highly fluctuating waiting times and of a drift yields a non-Gaussian distribution characterized by long spatial tails and strong anomalous superdiffusion.

cond-mat.dis-nn↗

Ratchet effect driven by Coulomb friction: the asymmetric Rayleigh piston

The effect of Coulomb friction is studied in the framework of collisional ratchets. It turns out that the average drift of these devices can be expressed as the combination of a term related to the lack of equipartition between the probe and the surrounding bath, and a term featuring the average frictional force. We illustrate this general result in the asymmetric Rayleigh piston, showing how Coulomb friction can induce a ratchet effect in a Brownian particle in contact with an equilibrium bath. An explicit analytical expression for the average velocity of the piston is obtained in the rare collision limit. Numerical simulations support the analytical findings.

cond-mat.stat-mech↗

Brownian ratchet in a thermal bath driven by Coulomb friction

The rectification of unbiased fluctuations, also known as the ratchet effect, is normally obtained under statistical non-equilibrium conditions. Here we propose a new ratchet mechanism where a thermal bath solicits the random rotation of an asymmetric wheel, which is also subject to Coulomb friction due to solid-on-solid contacts. Numerical simulations and analytical calculations demonstrate a net drift induced by friction. If the thermal bath is replaced by a granular gas, the well known granular ratchet effect also intervenes, becoming dominant at high collision rates. For our chosen wheel shape the granular effect acts in the opposite direction with respect to the friction-induced torque, resulting in the inversion of the ratchet direction as the collision rate increases. We have realized a new granular ratchet experiment where both these ratchet effects are observed, as well as the predicted inversion at their crossover. Our discovery paves the way to the realization of micro and sub-micrometer Brownian motors in an equilibrium fluid, based purely upon nano-friction.

cond-mat.soft↗

Non-equilibrium fluctuations in a driven stochastic Lorentz gas

We study the stationary state of a one-dimensional kinetic model where a probe particle is driven by an external field E and collides, elastically or inelastically, with a bath of particles at temperature T. We focus on the stationary distribution of the velocity of the particle, and of two estimates of the total entropy production Δs_tot. One is the entropy production of the medium Δs_m, which is equal to the energy exchanged with the scatterers, divided by a parameter θ, coinciding with the particle temperature at E=0. The other is the work W done by the external field, again rescaled by θ. At small E, a good collapse of the two distributions is found: in this case the two quantities also verify the Fluctuation Relation (FR), indicating that both are good approximations of Δs_tot. Differently, for large values of E, the fluctuations of W violate the FR, while Δs_m still verifies it.

cond-mat.stat-mech↗

Dynamics of a massive intruder in a homogeneously driven granular fluid

A massive intruder in a homogeneously driven granular fluid, in dilute configurations, performs a memory-less Brownian motion with drag and temperature simply related to the average density and temperature of the fluid. At volume fraction $\sim 10-50%$ the intruder's velocity correlates with the local fluid velocity field: such situation is approximately described by a system of coupled linear Langevin equations equivalent to a generalized Brownian motion with memory. Here one may verify the breakdown of the Fluctuation-Dissipation relation and the presence of a net entropy flux - from the fluid to the intruder - whose fluctuations satisfy the Fluctuation Relation.

cond-mat.soft↗

Structure factors in granular experiments with homogeneous fluidization

Velocity and density structure factors are measured over a hydrodynamic range of scales in a horizontal quasi-2d fluidized granular experiment, with packing fractions $ϕ\in[10%,40%]$. The fluidization is realized by vertically vibrating a rough plate, on top of which particles perform a Brownian-like horizontal motion in addition to inelastic collisions. On one hand, the density structure factor is equal to that of elastic hard spheres, except in the limit of large length-scales, as it occurs in the presence of an effective interaction. On the other hand, the velocity field shows a more complex structure which is a genuine expression of a non-equilibrium steady state and which can be compared to a recent fluctuating hydrodynamic theory with non-equilibrium noise. The temporal decay of velocity modes autocorrelations is compatible with linear hydrodynamic equations with rates dictated by viscous momentum diffusion, corrected by a typical interaction time with the thermostat. Equal-time velocity structure factors display a peculiar shape with a plateau at large length-scales and another one at small scales, marking two different temperatures: the "bath" temperature $T_b$, depending on shaking parameters, and the "granular" temperature $T_g<T_b$, which is affected by collisions. The two ranges of scales are separated by a correlation length which grows with $ϕ$, after proper rescaling with the mean free path.

cond-mat.soft↗

Estimate of temperature and its uncertainty in small systems

The energy of a finite system thermally connected to a thermal reservoir may fluctuate, while the temperature is a constant representing a thermodynamic property of the reservoir. The finite system can also be used as a thermometer for the reservoir. From such a perspective the temperature has an uncertainty, which can be treated within the framework of estimation theory. We review the main results of this theory, and clarify some controversial issues regarding temperature fluctuations. We also offer a simple example of a thermometer with a small number of particles. We discuss the relevance of the total observation time, which must be much longer than the decorrelation time.

cond-mat.stat-mech↗

Nonlinear susceptibilities and the measurement of a cooperative length

We derive the exact beyond-linear fluctuation dissipation relation, connecting the response of a generic observable to the appropriate correlation functions, for Markov systems. The relation, which takes a similar form for systems governed by a master equation or by a Langevin equation, can be derived to every order, in large generality with respect to the considered model, in equilibrium and out of equilibrium as well. On the basis of the fluctuation dissipation relation we propose a particular response function, namely the second order susceptibility of the two-particle correlation function, as an effective quantity to detect and quantify cooperative effects in glasses and disordered systems. We test this idea by numerical simulations of the Edwards-Anderson model in one and two dimensions.

cond-mat.stat-mech↗